Dual XRF Raman Spectroscopy for Light Element Analysis

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Solution Overview

Problem

X-ray fluorescence (XRF) analyzers struggle to directly measure light elements such as oxygen, nitrogen, and carbon, which limits the accuracy of elemental analysis in samples like minerals and plastics, as these elements interfere with the detection of other elements and are often present in mixtures like oxides of aluminum and silicon.

Innovation Solution

A dual-analyzing system combining XRF and Raman spectroscopy, where XRF provides elemental data and Raman spectroscopy characterizes molecules, with a processor integrating both signals to identify compounds and reduce interference from optical fluorescence using time-gating techniques, allowing for more accurate analysis of samples containing light elements.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Measurement precision

If XRF is used for elemental analysis, then heavy elements can be detected, but light elements (oxygen, nitrogen, carbon) cannot be directly measured

Engineering Contradiction:
Improvedetection accuracy of light elementsVSAvoidinability to detect light elements below 2.5 keV
Core Design Contradiction:
Measurement precisionVSDifficulty of detecting and measuring

Solution Approach 1:

The patent combines XRF and Raman spectroscopy into a single analytical system. XRF provides elemental composition data for heavier elements, while Raman spectroscopy detects molecular vibrations characteristic of light elements (C, H, O, N). The processor integrates both datasets to achieve comprehensive analysis of all elements including those undetectable by XRF alone.

Inventive Principle:
Principle #5Merging (Combining)

Solution Approach 2:

Raman spectroscopy acts as an intermediary technique to detect light elements that XRF cannot measure directly. By measuring molecular vibrations rather than atomic fluorescence, Raman provides indirect detection of light elements, which the processor then combines with direct XRF measurements of heavier elements.

Inventive Principle:
Principle #24Intermediary (Mediator)

2Measurement precision

If XRF analyzes samples with light elements, then heavy element detection is provided, but accuracy is reduced due to interference from light elements

Engineering Contradiction:
Improveaccuracy of elemental analysisVSAvoidinterference from light elements
Core Design Contradiction:
Measurement precisionVSObject-generated harmful factors

Solution Approach 1:

The processor uses Raman spectral data as feedback to correct and refine the XRF analysis results. By detecting the presence and concentration of light elements through Raman spectroscopy, the system can compensate for their interfering effects on XRF measurements of heavy elements, thereby improving overall analytical accuracy.

Inventive Principle:
Principle #23Feedback

Solution Approach 2:

Raman spectroscopy serves as an intermediary measurement technique that indirectly detects light elements causing interference. This intermediary data allows the system to account for and correct the harmful interference effects on heavy element detection without requiring direct XRF measurement of the interfering light elements.

Inventive Principle:
Principle #24Intermediary (Mediator)

3Loss of information

If a dual-analyzing system combining XRF and Raman spectroscopy is used, then comprehensive chemical information is obtained, but device complexity increases

Engineering Contradiction:
Improvecompleteness of chemical analysisVSAvoidcomplexity of dual-analyzing system
Core Design Contradiction:
Loss of informationVSDevice complexity

Solution Approach 1:

The analytical system is designed with multi-functionality, where a single integrated device performs both XRF and Raman spectroscopy measurements. The processor universally handles both types of spectral data, and the system can adaptively select which technique to use or combine based on the analytical requirements, reducing the need for separate specialized devices.

Inventive Principle:
Principle #6Universality (Multi-functionality)

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

This approach enhances the accuracy of elemental analysis by effectively identifying and quantifying light elements, improving the analysis of samples containing mixtures like minerals and plastics, by utilizing both XRF and Raman spectroscopy to provide comprehensive and precise chemical information.

Implementation Method 1

X-ray fluorescence ("XRF") is a technique which has been used for elemental analysis of various samples, including minerals. An XRF analyzer determines the chemistry of a sample by illuminating a spot on the sample with x-rays and measuring the spectrum of characteristic x-rays emitted by the different elements in the sample.

Methodology Applied
Scientific EffectX-ray fluorescence: Fluorescence

Implementation Method 2

Raman spectral data obtained from a sample in response to illuminating the sample with light

Methodology Applied
Scientific EffectRaman scattering: Scattering

Implementation Method 3

separating the Raman spectral data from an interfering optical fluorescence signal when present

Methodology Applied
Scientific EffectTime-gating:

Data Source

PatentEP2856125B1Sample analysis using combined x-ray fluorescence and raman spectroscopy
Publication Date: 2020.07.01 THERMO SCIENTIFIC PORTABLE ANALYTICAL INSTRUMENTS INC
  • EP2856125B1 patent drawingFigure 1
  • EP2856125B1 patent drawingFigure 2A~2B
  • EP2856125B1 patent drawingFigure 3

AI summary

An analyzer for analyzing a composition of a sample, and methods of operating an analyzer. The analyzer may include an optical illuminator and a Raman spectrometer to produce Raman spectral data representative of Raman radiation emitted from the sample in response to the illuminating light. Features to reduce background fluorescence are optionally provided. An x-ray illuminator may be provided to illuminate the sample with x-rays, and also an x-ray spectrometer may be present to produce x-ray spectral data representative of fluorescence radiation emitted from the sample in response to the illuminating x-rays. A processor receives the Raman spectral data and any x-ray spectral data and provides an analysis of a compound in the sample.