Boron hybridized phthalonitrile based phenolic resin and preparation method and application thereof

Boron hybrid resin is prepared through the nucleophilic substitution reaction between nitrophthalonitrile and boron hybrid phenolic resin, which solves the problems of poor oxidation resistance and high curing temperature of phenolic resin, and realizes the preparation of high-performance composite materials. Suitable for ablative heat protection and refractory materials.

CN109942767AActive Publication Date: 2019-06-28INST OF CHEM CHINESE ACAD OF SCI
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Patent Information

Application Number
CN201910251241.6
Authority / Receiving Office
CN · China
Patent Type
Applications(China)
Current Assignee / Owner
Filing Date
2019-03-29
Publication Date
2019-06-28
Estimated Expiration
2039-03-29

AI Technical Summary

Technical Problem

The antioxidant properties of phenolic resin are poor, and the release of small molecule by-products during the curing process results in high porosity, poor quality, and high curing temperature of composite materials, which limits its application scope.

Method used

Through the nucleophilic substitution reaction between boron hybridized thermoplastic phenolic resin and nitrophthalonitrile, an addition-curing boron hybridized phthalonitrile-based phenolic resin is prepared, and boron element is introduced to improve the antioxidant performance, and Reduce the curing temperature through thermal polymerization to avoid the release of small molecules.

Benefits of technology

It improves the oxidation resistance and thermal stability of the resin, reduces the curing temperature, improves the molding process performance, and enhances the high temperature resistance and ablation resistance of composite materials. It is suitable for ablation heat protection, refractory materials and other fields.

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Abstract

The invention discloses an addition curing type boron hybridized phthalonitrile based phenolic resin and a preparation method and application thereof. The phenolic resin is a addition curing type boron hybridized phthalonitrile based phenolic resin prepared by nucleophilic substitution reaction of thermoplastic boron hybridized phenolic resin (denoted as BN) prepared by condensation reaction of boron hybridized aryl phenol shown in the following formula I and formaldehyde, and a nitro-substituted phthalonitrile monomer shown in the following formula II. The resin has excellent molding and curing process performance, heat resistance and carbon residue performance, and can be applied to the field of high-performance composite material matrix resin with high temperature resistance, oxidationresistance and easy molding.
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