High-temperature-resistant fluorescent dye and preparation method thereof

By reacting modified fluorescent dyes with transparent polyimide porous microspheres and hydrogen-containing silicone oil, a three-layer core-shell structure was constructed, which solved the problem of easy decomposition and migration of fluorescent dyes at high temperatures and achieved a synergistic improvement in high temperature resistance and high fluorescence efficiency.

CN122213719APending Publication Date: 2026-06-16RAINBOW PLASTIC COLOURS CO LTD
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Patent Information

Application Number
CN202610473170.4
Authority / Receiving Office
CN · China
Patent Type
Applications(China)
Current Assignee / Owner
Filing Date
2026-04-10
Publication Date
2026-06-16

AI Technical Summary

Technical Problem

Existing fluorescent dyes are prone to thermal decomposition or fluorescence quenching during high-temperature processing, and they are also prone to diffusion and migration within materials, leading to problems such as color difference and precipitation on the surface of products, which limits their development in high-reliability application fields.

Method used

A modified fluorescent dye was prepared by reacting 4-bromo-1,8-naphthalenedicarboxylic anhydride with allylamine and 4-(N,N-dimethylaminosulfonyl)phenylboronic acid pinacol ester. The dye was then reacted with transparent polyimide porous microspheres and hydrogen-containing silicone oil to construct a three-layer core-shell structure of rigid polyimide microspheres-flexible silicone oil segments-fluorescent dye. The fluorescent dye was fixed by hydrosilylation reaction, which enhanced its high-temperature resistance and migration resistance.

Benefits of technology

This study achieves the stability and efficient luminescence of fluorescent dyes under high-temperature conditions, avoids dye migration and quenching, and improves the durability and fluorescence efficiency of the material.

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Abstract

This invention discloses a high-temperature resistant fluorescent dye and its preparation method, relating to the field of dyes. In preparing the high-temperature resistant fluorescent dye, 4-bromo-1,8-naphthalenedicarboxylic anhydride is reacted sequentially with allylamine and 4-(N,N-dimethylaminosulfonyl)phenylboronic acid pinacol ester to obtain a modified fluorescent dye. 2,2'-bis(trifluoromethyl)-4,4'-diaminobiphenyl and 3,3',4,4'-biphenyltetracarboxylic dianhydride are polymerized using silica as a template, followed by grafting of an epoxy compound containing double bonds. The silica is then etched with hydrofluoric acid to obtain transparent polyimide porous microspheres. The transparent polyimide porous microspheres, the modified fluorescent dye, and hydrogen-containing silicone oil are reacted to obtain the high-temperature resistant fluorescent dye. The high-temperature resistant fluorescent dye prepared by this invention exhibits excellent migration resistance and high-temperature resistance.
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