A method for calibrating the binding energy scale of surface indeterminate carbon peaks based on work function

By combining XPS and UPS, the binding energy of surface indeterminate carbon peaks was calibrated using the work function, which solved the problem of inaccurate binding energy scaling caused by exogenous indeterminate carbon, and enabled accurate chemical state and bonding structure analysis of unknown materials.

CN117007626BActive Publication Date: 2026-05-26TAICANG SIDIKE NEW MATERIALS SCI & TECH CO LTD +1
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Patent Information

Application Number
CN202310473911.5
Authority / Receiving Office
CN · China
Patent Type
Patents(China)
Current Assignee / Owner
Filing Date
2023-04-28
Publication Date
2026-05-26
Estimated Expiration
2043-04-28

AI Technical Summary

Technical Problem

In existing technologies, the binding energies of the C/CH peaks of exogenous indeterminate carbon are arbitrarily set, resulting in inaccurate elemental binding energy scaling and affecting the correct interpretation of chemical bonds. This is especially problematic in materials with unknown structures or unknown standard band gaps, where calibration becomes difficult.

Method used

The method of combining XPS and UPS was used to determine the C 1s binding energy of the indeterminate carbon on the sample surface by full-spectrum scanning and narrow-spectrum scanning. The binding energy of the CC/CH peak was calibrated using the work function, and its sum with the work function of the sample was defined as 289.50 eV. The drift value was calculated and the binding energy of other elements was calibrated.

Benefits of technology

It enables accurate analysis of the chemical state and bonding structure of sample surfaces, and is applicable to materials with unknown structures or unknown standard band gaps, thus improving the accuracy of binding energy scaling.

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Abstract

This invention discloses a method for calibrating the binding energy scale of indeterminate carbon peaks on a surface based on work function, comprising the following steps: obtaining the binding energy scale distribution spectrum of all elements on the sample surface through XPS full-spectrum scanning; further performing narrow-spectrum scanning on the elements on the sample surface, wherein the binding energy of the C-C / C-H peak of the indeterminate carbon C 1s on the sample surface is labeled as E. 1 BE The work function of the sample was tested using UPS, and the peak value of the C-C / C-H peak binding energy of the indeterminate carbon on the sample surface was obtained after calibration. This invention employs a combined XPS and UPS characterization method to calibrate the C 1s binding energy of the indeterminate carbon on the sample surface. This method is highly applicable to materials with unknown structures or unknown standard band gaps, and can be further extended to all systems where charge transfer at the indeterminate carbon / substrate interface is negligible.
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