Active compound combinations

Abstract

The present invention relates to a combination of active compounds, in particular included in a fungicide composition, comprising a compound of formula (I) as compound (A) and a further fungicidal compound as specified below as compound (B). Furthermore, the present invention relates to a composition comprising such a combination of compounds, and to the use of said combination of compounds and fungicide compositions as bioactive agents, in particular for the control of phytopathogenic fungi in crop protection and industrial material protection, and as plant growth regulators.

Description

Technical field

[0001] The present invention relates to combinations of active compounds, especially included in fungicidal compositions, comprising a compound of formula (I) as compound (A) and a further fungicidal active compound specified below as compound (B). Furthermore, the present invention relates to compositions comprising such combinations of compounds and compounds as bioactive agents, especially for the control of phytopathogenic fungi in crop protection and industrial material protection, and as plant growth regulators. It relates to the use of said compound combinations and fungicidal compositions.

[0002] Throughout this application, the terms "composition" and "formulation" are used synonymously and refer to a mixture of the combination of compounds according to the invention and at least one agriculturally suitable adjuvant. [Background technology]

[0003] US Patent Application Publication No. 2009 / 0143355 discloses 6-chloropyridazine-4-carboxamides as intermediates in the preparation of substituted arylamine derivatives useful in treating cancer. International Patent Publication No. WO2011 / 117254 discloses pyridazine-4-carboxamides as potential modulators of the ghrelin receptor useful in the treatment of diabetes and obesity. US Patent Application Publication No. 2011 / 0108767 mentions 6-chloropyridazine-4-carboxamide as a component of compositions that can be used to prepare light emitting devices. [Outline of the Invention]

[0004] Although the compounds of formula (I) provide an excellent means of protecting plants from diseases caused by fungi, there is a growing environmental and economic demand for agents and compositions for crop protection in modern times. There is a need to improve those tools in order to meet the demands of the public sector. This includes, for example, improving the spectrum of action, safety profile, selectivity, application rate, residue formation, and favorable preparative capacity, as well as developing new compositions to address potential problems such as tolerance. included.

[0005] According to the present invention there are provided combinations of active compounds and compositions containing said combinations which in at least some aspects achieve the stated objectives.

[0006] Therefore, according to the invention: (A) at least one compound of formula (I) [formation] [In the formula, T is O or S; n is 0 or 1; m is 0 or 1; However, if n is 1, then m is 1; R. 1 are hydrogen, hydroxyl, cyano, C 1 -C 6 Alkyl, C 1 -C 6 Alkoxy, C 1 -C 6 Alkoxy-C 1 -C 6 Alkyl, -C(=O)R a1 , -C(=O)(OR a1 ), -S(=O)R a1 , -S(=O) 2 R. a1 , -C(=O)N(R a2 ) 2 and S(=O) 2 N(R a2 ) 2 is selected from the group consisting of R a1 is C 1 -C 6 Alkyl, C 1 -C 6 haloalkyl, C 3 -C 8 cycloalkyl and C 2 -C 6 is selected from the group consisting of alkenyl; a2 is hydrogen, C 1 -C 6 Alkyl, C 1 -C 6 haloalkyl, C 3 -C 8 cycloalkyl and C 2 -C 6 selected from the group consisting of alkenyl; R. 2 and R 3 are hydrogen, halogen, cyano, hydroxyl, carboxyl, C 1 -C 6 Alkyl, C 1 -C 6 haloalkyl, C 1 -C 6 Alkoxy, C 1 -C 6 Alkoxycarbonyl and C 3 -C 8 is independently selected from the group consisting of cycloalkyl, or R 2 and R 3 are C together with the carbon atom to which they are attached 3 -C 8 forming a cycloalkyl or a 3- to 7-membered non-aromatic monocyclic heterocycle; R. 4 and R 5 are hydrogen, halogen, cyano, hydroxyl, carboxyl, C 1 -C 6 Alkyl, C 1 -C 6 haloalkyl, C 1 -C 6 Alkoxy, C 1 -C 6 Alkoxycarbonyl and C 3 -C 8 is independently selected from the group consisting of cycloalkyl, or R 4 and R 5 , together with the carbon atoms to which they are attached, C 3 -C 8 forming a cycloalkyl or non-aromatic 3- to 7-membered monocyclic heterocycle; or R. 2 and R 4 together with the carbon atoms to which they are attached, C 3 -C 8 forming a cycloalkyl or non-aromatic 3- to 7-membered monocyclic heterocyclic ring, and 3 and R 5 is independently hydrogen or halogen; or R. 2 and R 4 together form a covalent bond, and R 3 and R 5 is independently hydrogen or C 1 -C 6 is an alkyl; R. 6 is the non-aromatic C 3 -C 12 carbocyclic, aromatic C 6 -C 14 carbocyclic ring, non-aromatic 3-14 membered heterocyclic ring, aromatic 5-14 membered heterocyclic ring, non-aromatic C 3 -C 12 carbocyclyloxy, aromatic C 6 -C 14 carbocyclyloxy, aromatic 5-14 membered heterocyclyloxy, non-aromatic 3-14 membered heterocyclyloxy, non-aromatic C 3 -C 12 carbocyclic substituted C 1 -C 3 alkoxy, aromatic C 6 -C 14 carbocyclic substituted C 1 -C 3 alkoxy, non-aromatic 3-14 membered heterocyclic substituted C 1 -C 3 Alkoxy, C substituted with aromatic 5-14 membered heterocyclic ring 1 -C 3 alkoxy, non-aromatic C 3 -C 12 carbocyclic substituted C 1 -C 3 haloalkoxy, aromatic C 6 -C 14 carbocyclic substituted C 1 -C 3 haloalkoxy, non-aromatic 3-14 membered heterocyclic substituted C 1 -C 3 C substituted with haloalkoxy and aromatic 5-14 membered heterocycle 1 -C 3 is selected from the group consisting of haloalkoxy and R 6 A ring or cyclic portion of a substituent may be the same or different one or more R 6S optionally substituted with a substituent, R. 6S is halogen, cyano, isocyano, nitro, hydroxyl, mercapto, pentafluorosulfanyl, oxo, methylidene, halomethylidene, C 1 -C 6 Alkyl, C 1 -C 6 haloalkyl, C 1 -C 6 Alkoxy, C 1 -C 6 haloalkoxy, C 2 -C 6 alkenyl, C 2 -C 6 haloalkenyl, C 2 -C 6 alkynyl, C 2 -C 6 haloalkynyl, C 2 -C 6 alkenyloxy, C 2 -C 6 haloalkenyloxy, C1 -C 6 Alkylsulfanyl, C 1 -C 6 haloalkylsulfanyl, C 3 -C 8 Cycloalkylsulfanyl, C 1 -C 6 Alkylsulfinyl, C 1 -C 6 haloalkylsulfinyl, C 3 -C 8 cycloalkylsulfinyl, C 1 -C 6 alkylsulfonyl, C 1 -C 6 haloalkylsulfonyl, C 3 -C 8 Cycloalkylsulfonyl, C 3 -C 8 Cycloalkyl, C 3 -C 8 Cycloalkyloxy, C 3 -C 8 cycloalkenyl, aromatic C 6 -C 14 carbocyclic ring, aromatic 5- or 6-membered monocyclic heterocyclic ring, non-aromatic 3- to 7-membered monocyclic heterocyclic ring, -N(R c ) 2 , -C(=O)R d , -C(=O)(OR d ), -C(=O)N(R d ) 2 , -S(=O) 2 N(R d ) 2 , -O-Si(C 1 -C 6 alkyl) 3 and -Si(C 1 -C 6 alkyl) 3 or two R 6S Substituents together with the carbon atom to which they are attached are C 3 -C 8 forming a cycloalkyl, R. c are independently hydrogen, C 1 -C 6 Alkyl and C 3 -C 8 is selected from the group consisting of cycloalkyl; R. d are independently hydrogen, C 1 -C 6 Alkyl and C 1 -C 6 is selected from the group consisting of haloalkyl; Aliphatic R 6S , R c and R d The substituents are independently cyano, hydroxyl, C 1 -C 6 Alkoxy, C 1 -C 6 Haloalkoxy, -O-Si(C 1 -C 6 alkyl) 3 , -Si(C 1 -C 6 alkyl) 3 , C 3 -C 8 Cycloalkyl, C 3 -C 8 optionally substituted with one or more substituents selected from the group consisting of halocycloalkyl and non-aromatic 3- to 7-membered monocyclic heterocycles; R. 6S the ring or cyclic portion of and cyclic R c Substituents are independently halogen, cyano, nitro, hydroxyl, formyl, carboxyl, oxo, methylidene, halomethylidene, C 1 -C 6 Alkyl, C 1 -C 6 haloalkyl, C 1 -C 6 Alkoxy, C 1 -C 6 haloalkoxy, C 1 -C 6 Alkoxycarbonyl, C 1 -C 6 haloalkoxycarbonyl, C 2 -C 6 alkenyl, C 3 -C 8 cycloalkyl and C 3 -C 8 optionally substituted with one or more substituents selected from the group consisting of halocycloalkyl and / or R 6S Rings or cyclic moieties of substituents are C with the carbon atom to which they are attached. 3 -C 8 optionally substituted with two substituents to form a cycloalkyl; R. 7 is hydrogen, halogen, cyano, isocyano, hydroxyl, mercapto, nitro, amino, formyl, C 1 -C 6 Alkyl, C 1 -C 6 haloalkyl, C 1 -C 6 hydroxyalkyl, C 1 -C 6 alkylcarbonyl, C 1 -C 6 haloalkylcarbonyl, C 1 -C 6 Alkoxy, C 1 -C 6 haloalkoxy, C 2 -C 6 alkenyl, C 2 -C 6 haloalkenyl, C 2 -C 6 alkynyl, C 2 -C 6 haloalkynyl, C 2 -C 6 alkenyloxy, C 2 -C 6 haloalkenyloxy, C 2 -C 6 alkynyloxy, C 2 -C 6 haloalkynyloxy, C 1 -C 6 Alkylsulfanyl, C 1 -C 6 haloalkylsulfanyl, C 3 -C 8 Cycloalkylsulfanyl, C 1 -C 6 Alkylsulfinyl, C 1 -C 6 haloalkylsulfinyl, C 3 -C 8 cycloalkylsulfinyl, C 1 -C 6 alkylsulfonyl, C 1 -C 6 haloalkylsulfonyl, C 3 -C 8 Cycloalkylsulfonyl, C 3 -C 8 Cycloalkyl, C 3 -C 6 cycloalkenyl, aromatic C 6 -C 14 carbocyclic ring, aromatic 5- or 6-membered monocyclic heterocyclic ring, non-aromatic 3- to 7-membered monocyclic heterocyclic ring, C 3 -C 8 cycloalkyloxy, aromatic C 6 -C 14 carbocyclyloxy, aromatic 5- or 6-membered monocyclic heterocyclyloxy, non-aromatic 3- to 7-membered monocyclic heterocyclyloxy, -O-Si(C 1 -C 6 alkyl) 3 , -Si(C 1 -C 6 alkyl) 3 , -N(R e ) 2 , -C(=NR f )R f , -NR g C(=O)R g , -C(=O)(OR g ), -C(=O)N(R g ) 2 , -S(=O) 2 N(R g ) 2 and -S(=O)(=NR g )R g is selected from the group consisting of R. e are independently hydrogen, C 1 -C 6 Alkyl, C 1 -C 6 haloalkyl, C 1 -C 6 Alkoxy, C 2 -C 6 alkenyl, C 2 -C 6 haloalkenyl, C 2 -C 6 alkynyl, C 2 -C 6 haloalkynyl, C 3 -C 8 Cycloalkyl, C 3 -C 8 halocycloalkyl, aromatic C 6 -C 14 selected from the group consisting of carbocycle, aromatic 5- or 6-membered monocyclic heterocycle and non-aromatic 3- to 7-membered monocyclic heterocycle, R. f are independently hydroxyl, amino, cyano, C 1 -C 6 Alkyl, C 1 -C 6 haloalkyl, C 1 -C 6 Alkoxy, C 1 -C 6 alkylamino and di(C 1 -C 6 alkyl)amino, R. gare independently hydrogen, C 1 -C 6 Alkyl, C 1 -C 6 haloalkyl and C 3 -C 8 is selected from the group consisting of cycloalkyl; Aliphatic R 7 , R e , R f and R g Substituents may be the same or different one or more R 7Sa optionally substituted with a substituent, R. 7 The ring or cyclic portion of the cyclic R e and cyclic R g Substituents may be the same or different one or more R 7Sc optionally substituted with a substituent, R. 7Sa are cyano, hydroxyl, carboxyl, C 1 -C 6 Alkoxy, C 1 -C 6 haloalkoxy, C 3 -C 8 Cycloalkyl, C 3 -C 8 halocycloalkyl, C 1 -C 6 Alkoxycarbonyl, -O-Si(C 1 -C 6 alkyl) 3 , -Si(C 1 -C 6 alkyl) 3 , aromatic C 6 -C 14 selected from the group consisting of carbocycles and non-aromatic 3- to 7-membered monocyclic heterocycles, R. 7Sc is halogen, cyano, nitro, hydroxyl, formyl, oxo, methylidene, halomethylidene, C 1 -C 6 Alkyl, C 1 -C 6 haloalkyl, C 1 -C 6 Alkoxy, C 1 -C 6 haloalkoxy, C 2 -C 6 alkenyl, C 3 -C 8 Cycloalkyl, C 3 -C 8 Halocycloalkyl, -O-Si(C 1 -C 6 alkyl) 3 and a non-aromatic 3- to 7-membered monocyclic heterocycle, or two R 7Sc Substituents together with the carbon atom to which they are attached are C 3 -C 8 forming a cycloalkyl, R. 8 is hydrogen, halogen, cyano, isocyano, amino, nitro, hydroxyl, mercapto, carboxyl, C 1 -C 6 Alkoxycarbonyl, C 1 -C 6 Alkyl, C 1 -C 6 haloalkyl, C 1 -C 6 hydroxyalkyl, C 1 -C 6 Alkoxy, C 1 -C 6 haloalkoxy, C 2 -C 6 alkenyl, C 2 -C 6 haloalkenyl, C 2 -C 6 alkynyl, C 2 -C 6 haloalkynyl, C 2 -C 6 alkenyloxy, C 2 -C 6 haloalkenyloxy, C 2 -C 6 alkynyloxy, C 2 -C 6 haloalkynyloxy, C 1 -C 6 Alkylsulfanyl, C 1 -C 6 haloalkylsulfanyl, C 1 -C 6 Alkylsulfinyl, C 1 -C 6 haloalkylsulfinyl, C 1 -C 6 alkylsulfonyl, C 1 -C 6 haloalkylsulfonyl, C 3 -C 8 Cycloalkyl, C 3 -C 6 cycloalkenyl, aromatic C 6 -C 14 carbocyclic ring, non-aromatic 3-14 membered heterocyclic ring, aromatic 5-14 membered heterocyclic ring, C 3 -C 8 cycloalkyloxy, aromatic C 6 -C 14 carbocyclyloxy, non-aromatic 3-14 membered heterocyclyloxy, aromatic 5-14 membered heterocyclyloxy, -O-Si(C 1 -C 6 alkyl) 3 , -Si(C 1 -C 6 alkyl) 3 , -N(R h ) 2 , -SR i , -S(=O)R i and -S(=O) 2 R. i is selected from the group consisting of R. h are independently hydrogen, C 1 -C 6 Alkyl, C 1 -C 6 haloalkyl, C 1 -C 6 Alkoxy, C 2 -C 6 alkenyl, C 2 -C 6 haloalkenyl, C 2 -C 6 alkynyl, C 2 -C 6 haloalkynyl, C 3 -C 8 Cycloalkyl, C 3 -C 8 halocycloalkyl, aromatic C 6 -C 14 selected from the group consisting of a carbocyclic ring, an aromatic 5- to 14-membered heterocyclic ring and a non-aromatic 3- to 7-membered monocyclic heterocyclic ring; R. i is C 2 -C 6 alkenyl, C 2 -C 6 haloalkenyl, C 2 -C 6 alkynyl, C 2 -C 6 haloalkynyl, C 3 -C 8 Cycloalkyl, C 3 -C 8 halocycloalkyl, aromatic C 6 -C 14 selected from the group consisting of a carbocyclic ring, an aromatic 5- to 14-membered heterocyclic ring and a non-aromatic 3- to 7-membered monocyclic heterocyclic ring; Aliphatic R 8 , R h and R i Substituents may be the same or different one or more R 8Sa optionally substituted with a substituent, R. 8 The ring or cyclic portion of the cyclic R h and cyclic R i Substituents may be the same or different one or more R 8Sc optionally substituted with a substituent, R. 8Sa are cyano, amino, nitro, hydroxyl, formyl, carboxyl, C 1 -C 6 Alkoxy, C 1 -C 6 haloalkoxy, C 1 -C 6 Alkoxy-C 1 -C 6 Alkoxy, C 1 -C 6 Alkoxycarbonyl, C 1 -C 6 haloalkoxycarbonyl, C 1 -C 6 alkylcarbonyl, C 1 -C 6 haloalkylcarbonyl, C 3 -C 8 Cycloalkyl, C 3 -C 8 halocycloalkyl, C 1 -C 6 Alkylsulfanyl, C 1 -C 6 haloalkylsulfanyl, C 1 -C 6 Alkylsulfinyl, C 1 -C 6 haloalkylsulfinyl, C 1 -C 6 alkylsulfonyl, C 1 -C 6 Haloalkylsulfonyl, -O-Si(C 1 -C 6 alkyl) 3 , -Si(C 1 -C 6 alkyl) 3 , non-aromatic 3- to 7-membered monocyclic heterocycles and -N(Ra') 2 is selected from the group consisting of, and Ra' is independently hydrogen, formyl, C 1 -C 6 Alkyl, C 1 -C6 haloalkyl, C 3 -C 8 cycloalkyl and C 1 -C 6 The non-aromatic 3- to 7-membered monocyclic heterocycle R is selected from the group consisting of alkylcarbonyl 8Sa is one or more identical or different C 1 -C 6 optionally substituted with an alkyl substituent, R. 8Sc is halogen, cyano, amino, nitro, hydroxyl, formyl, carboxyl, oxo, methylidene, halomethylidene, C 1 -C 6 Alkyl, C 1 -C 6 haloalkyl, C 1 -C 6 Alkoxy, C 1 -C 6 haloalkoxy, C 1 -C 6 Alkoxycarbonyl, C 1 -C 6 haloalkoxycarbonyl, C 2 -C 6 alkenyl, C 1 -C 6 Alkylsulfanyl, C 1 -C 6 Alkylsulfinyl, C 1 -C 6 alkylsulfonyl, C 3 -C 8 Cycloalkyl, C 3 -C 8 Halocycloalkyl, -O-Si(C 1 -C 6 alkyl) 3 and one or more Cs that are the same or different 1 -C 6 is selected from the group consisting of non-aromatic 3- to 7-membered monocyclic heterocycles optionally substituted with alkyl substituents, or two R 8Sc Substituents together with the carbon atom to which they are attached are C 3 -C 8 to form a cycloalkyl or non-aromatic 3- to 7-membered monocyclic heterocyclic ring, wherein the non-aromatic 3- to 7-membered monocyclic heterocyclic ring is composed of one or more C 1 -C 6 optionally substituted with an alkyl substituent, Q is aromatic C 6 -C 14 carbocyclic, non-aromatic C 3 -C 12 one or more Q selected from the group consisting of carbocycles, non-aromatic 3- to 14-membered heterocycles and aromatic 5- to 14-membered heterocycles, wherein any of said carbocyclic groups or heterocyclic groups are the same or different; S optionally substituted with a substituent, Q. S is halogen, cyano, isocyano, nitro, hydroxyl, mercapto, formyl, carboxyl, C 1 -C 6 Alkyl, C 1 -C 6 haloalkyl, C 1 -C 6 alkylcarbonyl, C 1 -C 6 haloalkylcarbonyl, C 1 -C 6 Alkoxy, C 1 -C 6 haloalkoxy, C 1 -C 6 Alkoxy-C 1 -C 6 Alkyl, C 1 -C 6 Alkoxycarbonyl, C 1 -C 6 haloalkoxycarbonyl, C 2 -C 6 alkenyl, C 2 -C 6 haloalkenyl, C 2 -C 6 alkynyl, C 2 -C 6 haloalkynyl, C 2 -C 6 alkenyloxy, C 2 -C 6 haloalkenyloxy, C 1 -C 6 Alkylsulfanyl, C 1 -C 6 haloalkylsulfanyl, C 1 -C 6 Alkylsulfinyl, C 1 -C 6 haloalkylsulfinyl, C 1 -C 6 alkylsulfonyl, C 1 -C 6 haloalkylsulfonyl, C 3 -C 8 Cycloalkyl, C 3 -C 8 Cycloalkyloxy, C 3 -C 6 Cycloalkenyl, non-aromatic 3- to 7-membered monocyclic heterocycle, aromatic 5- to 14-membered heterocycle, -O-Si(C 1 -C 6 alkyl) 3 , -Si(C 1 -C 6 alkyl) 3 , -OC(=O)R j , -NR j C(=O)R j , -C(=O)N(R j ) 2 , -C(=S)R j , -C(=S)N(R j ) 2 , -C(=NR j )R j and -C(=NOR j )R j and -N(R k ) 2 is selected from the group consisting of R. j are independently hydrogen, C 1 -C 6 Alkyl, C 1 -C 6 haloalkyl and C 1 -C 6 is selected from the group consisting of alkoxy; R. k are independently hydrogen, hydroxyl, C 1 -C 6 Alkyl, C 1 -C 6 haloalkyl, C 1 -C 6 Alkoxy, C 2 -C 6 alkenyl, C 2 -C 6 haloalkenyl and C 3 -C 8 is selected from the group consisting of cycloalkyl; Aliphatic Q S , R j and R k Substituents are independently cyano, amino, nitro, hydroxyl, C 1 -C 6 Alkoxy, C 1 -C 6 haloalkoxy, C 1 -C 6 Alkoxycarbonyl, C 1 -C 6 haloalkoxycarbonyl, C 3 -C 8 Cycloalkyl, C 3 -C 8 Halocycloalkyl, -Si(C 1 -C 6 alkyl) 3 and optionally substituted with one or more substituents selected from the group consisting of non-aromatic 3- to 7-membered monocyclic heterocycles, Q. S the ring or cyclic portion of and cyclic R k Substituents are independently halogen, cyano, amino, nitro, hydroxyl, formyl, carboxyl, oxo, methylidene, halomethylidene, C 1 -C 6 Alkyl, C 1 -C 6 haloalkyl, C 1 -C 6 Alkoxy, C 1 -C 6 haloalkoxy, C 1 -C 6 Alkoxycarbonyl, C 1 -C 6 haloalkoxycarbonyl, C 3 -C 8 Cycloalkyl, C 3 -C 8 halocycloalkyl, C 2 -C 6 one or more R selected from the group consisting of alkenyl and non-aromatic 3- to 7-membered monocyclic heterocycles Qs optionally substituted with a substituent, the cyclic R Qs Substituents are C together with the carbon atom to which they are attached. 3 -C 8 optionally substituted with two substituents to form cycloalkyl, provided that the compound of formula (I) is (a) 3-(1H-benzotriazol-1-yloxy)-N-(4-tert-butylphenyl)-6-chloropyridazine-4-carboxamide ([561297-99-2]), (b) 3-(cyclopentyloxy)-6-(4-fluorophenoxy)-N-{[(3R)-1-isopropylpiperidin-3-yl]methyl}pyridazine-4-carboxamide ([1336909-91-1 ]), (c) 6-(4-fluorophenoxy)-N-{[(3R)-1-isopropylpiperidin-3-yl]methyl}-3-(tetrahydro-2H-pyran-4-yloxy)pyridazine-4-carboxamide ([1336909-90-0]), (d) 6-chloro-N-{[(3R)-1-isopropylpiperidin-3-yl]methyl}-3-(tetrahydro-2H-pyran-4-yloxy)pyridazine-4-carboxamide ([1336910-48 -Five]), (e) 6-chloro-3-(cyclopentyloxy)-N-{[(3R)-1-isopropylpiperidin-3-yl]methyl}pyridazine-4-carboxamide ([1336910-49-6]), (f) 3-(1H-benzotriazol-1-yloxy)-6-chloro-N-(cyclohexylmethyl)pyridazine-4-carboxamide ([1202404-84-9)] isn't it, and (B) at least one further active compound selected from (1) inhibitors of ergosterol synthesis, (2) inhibitors of the respiratory chain at complex I or II, (3) inhibitors of the respiratory chain at complex III, (4) inhibitors of mitosis and cell division; (5) compounds with multisite action, (6) compounds capable of inducing host defenses; (7) inhibitors of amino acid and / or protein biosynthesis; (8) inhibitors of ATP production; (9) inhibitors of cell wall synthesis; (10) inhibitors of lipid and membrane synthesis, (11) inhibitors of melanin biosynthesis, (12) inhibitors of nucleic acid synthesis; (13) signaling inhibitors; (14) compounds capable of acting as uncouplers; (15) other fungicides, (16) an antibacterial agent; (17) biological fungicides; (18) Fatty acids or derivatives thereof There is provided a combination of active compounds comprising:

[0007] Compound (A) The active compound combinations according to the invention comprise as compound (A) at least one compound of formula (I) or a salt or N-oxide thereof.

[0008] In a more preferred embodiment, the compound of the invention is a compound of formula (I) T is O; n is 0 or 1; m is 0 or 1; But if n is 1 then m is 1 and R. 1 is hydrogen, hydroxyl, C 1 -C alkyl and -C(=O)(OR a1 ) and R a1 is C 1 -C 4 Alkyl and C 2 -C 4 is selected from the group consisting of alkenyl, R. 2 and R 3 is hydrogen or R 2 and R 3 are C together with the carbon atom to which they are attached 3 -C 6 forming a cycloalkyl, R. 4 and R 5 are independently hydrogen, fluorine, chlorine and C 1 -C 4 is selected from the group consisting of alkyl, or R 4 and R 5 are C together with the carbon atom to which they are attached 3 -C 6 form a cycloalkyl, or R. 2 and R 4 are C together with the carbon atom to which they are attached 3 -C 6 to form a cycloalkyl and R 3 and R 5 is independently hydrogen or halogen, or R. 6 is a 4- to 6-membered monocyclic non- Aromatic heterocycle, monocyclic C 3 -C 8 5- or 6-membered monocyclic heteroaryl fused with cycloalkyl, aromatic 5- or 6-membered monocyclic heterocycle, aryl, phenoxy, benzyloxy or -OCF 2 - is selected from the group consisting of 5- or 6-membered monocyclic aromatic heterocycles fused with phenyl, and R 6 The rings or cyclic moieties of the substituents are fluorine, chlorine, cyano, C 1 -C 4 Alkyl, C 1 -C 4 haloalkyl, C 1 -C 4 Alkoxy, C 1 -C 4 haloalkoxy, C 2 -C 6 alkenyl, C 2 -C 6 alkynyl, C 1 -C 4 haloalkylsulfanyl, C 3 -C 6 1 to 3 R selected from the group consisting of cycloalkyl, phenyl, pyridyl, pyrazolyl, imidazolyl, triazolyl, oxetanyl and tetrahydrofuranyl 6S optionally substituted with a substituent, R. 6S The rings or cyclic moieties of the substituents are independently fluorine, chlorine, C 1 -C 4 Alkyl, C 1 -C 4 haloalkyl and C 1 -C 4 optionally substituted with 1 to 3 substituents selected from the group consisting of alkoxycarbonyl, R. 7 is hydrogen, chlorine, C 1 -C 4 Alkyl, C 1 -C 4 haloalkyl, C 1 -C 4 hydroxyalkyl, C 1 -C 4 alkylcarbonyl, C 1 -C 4 Alkoxy, C 2 -C 6 alkenyl, C 2 -C 6 alkynyl, C 3 -C 6 Cycloalkyl, pyridinyl, imidazolyl, pyrazolyl, oxetanyl, tetrahydrofuranyl, tetrahydropyranyl, pyrrolidinyl, azetidinyl and -N(R e ) 2 is selected from the group consisting of R. e are independently hydrogen, C 1 -C 4 Alkyl and C 3 -C 6 is selected from the group consisting of cycloalkyl; Aliphatic R 7 and R e The substituents are independently C 1 -C 4 Alkoxy, C 3 -C 6 Cycloalkyl, C 1 -C 2 1 or 2 R selected from the group consisting of alkoxycarbonyl and phenyl 7Sa optionally substituted with a substituent, R. 7 the ring or cyclic portion of and cyclic R e are independently fluorine, chlorine, hydroxyl, C 1 -C 4 Alkyl and C 1 -C 4 1 or 2 R selected from the group consisting of alkoxy 7Sc optionally substituted with a substituent, R. 8 are hydrogen, halogen, hydroxyl, C 1 -C 4 Alkyl, C 1 -C 4 haloalkyl, C 1 -C 4 Alkoxy, C 2 -C 6 alkenyl, C 2 -C 6 alkenyloxy, C 2 -C 6 haloalkenyloxy, C 1 -C 4 Alkylsulfanyl, C 1 -C 4 haloalkylsulfanyl, C 1 -C 4 Alkylsulfinyl, C 1 -C 4 alkylsulfonyl, C 3 -C 6 Cycloalkyl, phenyl, non-aromatic 3- to 7-membered heterocyclic ring, aromatic 5- or 6-membered heterocyclic ring, non-aromatic 3- to 7-membered heterocyclyloxy and -N(R h ) 2 is selected from the group consisting of R. h are independently hydrogen, C 1 -C 4 Alkyl, C 2 -C 6 alkenyl, C 3 -C 6selected from the group consisting of cycloalkyl, phenyl and non-aromatic 3- to 7-membered monocyclic heterocycles; Aliphatic R 8 and R h Substituents are independently hydroxyl, carboxyl, C 1 -C 4 Alkoxy, C 1 -C 4 Alkoxy-C 1 -C 4 Alkoxy, C 1 -C 4 Alkoxycarbonyl, C 3 -C 6 Cycloalkyl, non-aromatic 3- to 7-membered monocyclic heterocycle and -N(Ra’) 2 is selected from the group consisting of Ra' is independently hydrogen, C 1 -C 4 Alkyl and C 1 -C 2 independently selected from the group consisting of alkylcarbonyl, R. 8 the ring or cyclic portion of and cyclic R h Substituents are independently chlorine, cyano, hydroxyl, C 1 -C 4 Alkyl, C 1 -C 4 haloalkyl, C 1 -C 4 Alkoxy, C-C 4 Alkoxycarbonyl, C 3 -C 6 is selected from the group consisting of cycloalkyl, oxolanyl, oxetanyl and tetrahydrofuranyl, or two R 8Sc substituents form oxetanyl or oxiranyl with the carbon atom to which they are attached; Q is phenyl, naphth-2-yl, bicyclo[4.2.0]octa-1(6), 2,4-trienyl, indanyl, 1,2,3,4-tetrahydronaphthalenyl, indenyl, dihydronaphthalene nyl, bicyclo[4.2.0]octa-1(6), 2,4-trienyl, 2,3-dihydrobenzofuranyl, 1,3-dihydroisobenzofuranyl, indolinyl, 1,3-benzodioxolyl , chromanyl, 2,3-dihydro-1,4-benzodioxinyl, [1,3]dioxolo[4,5-b]pyridinyl, 5,6,7,8-tetrahydroquinolinyl, 6,7- Dihydro-5H cyclopenta[b]pyridinyl, 1,3-benzodioxolyl, 2,3-dihydrobenzofuranyl, pyrrolyl, furanyl, thienyl, imidazolyl, triazolyl, oxazolyl, thiazolyl, pyridinyl, pyridazinyl and pyrimidinyl, indolyl, benzmadazolyl , indazolyl, benzofuranyl, benzothiophenyl, benzothiazolyl, benzoxazolyl, quinolinyl, furo[3,2-b]pyridinyl, thieno[3,2-b]thiophenyl and thieno[2,3-d]thiazolyl is selected from Any of the above carbocyclic or heterocyclic groups are independently halogen, C 1 -C 4 Alkyl, C 1 -C 4 haloalkyl, C 1 -C 4 Alkoxy, C 1 -C 4 haloalkoxy, C 2 -C 4 alkenyl, C 2 -C 4 alkynyl, C 1 -C 4 Alkylsulfanyl, C 1 -C 4 haloalkylsulfanyl, C 3 -C 6 Cycloalkyl, oxiranyl, oxetanyl and -N(R k ) 2 1 to 3 Qs selected from the group consisting of S optionally substituted with a substituent, R. k is hydrogen and Q. S The ring or cyclic portion of the substituent is independently 1 or 2 R selected from the group consisting of fluorine and chlorine. Qs It may be substituted with a substituent.

[0009] In an even more preferred embodiment, the compound of the invention is a compound of formula (I) T is O, R. 1 is hydrogen and R. 2 and R 3 exists (that is, n=1), then R 2 and R 3 is hydrogen or R 2 and R 3 form cyclopropyl or cyclobutyl with the carbon atom to which they are attached, R. 4 and R 5 exists (i.e. m=1), then R 4 and R 5 is independently selected from the group consisting of hydrogen and halogen; R. 6 is indanyl, 1,2,3,4-tetrahydronaphthalenyl, spiro[cyclopropan-1,2'-indan]-1-yl, phenyl, 2,3-dihydrobenzofuranyl, 1,3-benzodi oxolyl, 2,3-dihydro-1,4-benzodioxinyl, 4,5,6,7-tetrahydrobenzothiophenyl, thienyl, pyridinyl, indolyl, benzoxazolyl, quinolinyl or isoquinolinyl; The indanyl is 1,2,3,4-tetrahydronaphthalenyl, spiro[cyclopropan-1,2′-indan]-1-yl, phenyl, 2,3-dihydrobenzofuranyl, 1,3-benzo Dioxolyl, 2,3-dihydro-1,4-benzodioxinyl, 4,5,6,7-tetrahydrobenzothiophenyl, thienyl, pyridinylindolyl, benzoxazolyl, quinolinyl or isoquinolinyl are independently and halogen, cyano, C 1 -C 6 Alkyl, C 1 -C 6 haloalkyl, C 1 -C 6 Alkoxy, C 1 -C 6 haloalkoxy, C 2 -C 6 alkenyl, C 2 -C 6 1 to 3 R selected from the group consisting of alkynyl and cyclopropyl 6S optionally substituted with a substituent, R. 7 is hydrogen, halogen, cyano, C 1 -C 4 Alkyl, C 1 -C 4 haloalkyl, C 1 -C 4 hydroxyalkyl, C 1 -C 4 alkylcarbonyl, C 1 -C 4 Alkoxy, C 2 -C 6 alkenyl, C 2 -C 6 alkynyl or cyclopropyl, Aliphatic R 7 is one or two R 7Sa optionally substituted with a substituent, R. 8 is hydrogen, halogen, C 1 -C 4 Alkyl, C 1 -C 4 Alkoxy, C 2 -C 4 alkenyl, C 1 -C 4 alkylsulfanyl, pyrazolyl, imidazolyl, thiazolyl, pyridinyl or -N(R h ) 2 and R. h are independently hydrogen, C 1 -C 4 selected from the group consisting of alkyl and cyclopropyl; The aliphatic R 8 The substituents are independently C 1 -C 4 haloalkyl, C 1 -C 4 Alkoxy, C 1 -C 4 Alkoxy-C 1 -C 2 1 or 2 R selected from the group consisting of alkoxy, cyclopropyl and cyclobutyl 8Sa optionally substituted with a substituent, The cyclic R 8 Substituents are 1 or 2 R independently selected from the group consisting of halogen 8Sc optionally substituted with a substituent, Q is phenyl, thienyl or pyridinyl, Said phenyl, thienyl and pyridinyl are independently halogen, C 1 -C 4 Alkyl, C 1 -C 4 haloalkyl, C 1 -C 4 Alkoxy, C 1 -C 4 haloalkoxy, C 2 -C 4 alkenyl, C 2 -C 4 alkynyl, C 1 -C 4 Alkylsulfanyl, C 1 -C 4 1-3 Q selected from the group consisting of haloalkylsulfanyl, cyclopropyl, cyclobutyl, oxiranyl and oxetanyl SIt may be substituted with a substituent.

[0010] A more preferred combination of compounds of the invention is (A)(I-655)6-chloro-3-(3-cyclopropyl-2-fluorophenoxy)-N-[2-(2,4-dimethylphenyl) -2,2-difluoroethyl]-5-methylpyridazine-4-carboxamide, (I-667) 3-(3-bromo-2-fluorophenoxy)-6-chloro-N-[2-(2-chloro- 4-methylphenyl)-2,2-difluoroethyl]-5-methylpyridazine-4-carboxamide, (I-746) 6-chloro-N-[2-(2-chloro-4-methylphenyl))-2 ,2-difluoroethyl]-3-(3-cyclopropyl-2-fluorophenoxy)-5-methylpyridazine-4-carboxamide, (I-749) 6-chloro-3-(3-cyclopropyl-2-fluoro phenoxy)-N-[2-(3,4-dimethylphenyl)-2,2-difluoroethyl]-5-methylpyridazine-4-carboxamide, (I-784) 6-chloro-3-(3-chloro- 2-fluorophenoxy)-N-[2-(2,4-dimethylphenyl)-2,2-difluoroethyl]-5-methylpyridazine-4-carboxamide, (I-840)N-[2-(2- a formula selected from the group consisting of bromo-4-methylphenyl)-2,2-difluoroethyl]-6-chloro-3-(3-cyclopropyl-2-fluorophenoxy)-5-methylpyridazine-4-carboxamide Including compounds of (I).

[0011] An even more preferred combination of compounds of the invention is (A)(I-655)6-chloro-3-(3-cyclopropyl-2-fluorophenoxy)-N-[2-(2,4-dimethylphenyl )-2,2-difluoroethyl]-5-methylpyridazine-4-carboxamide, (I-746)6-chloro-N-[2-(2-chloro-4-methylphenyl))-2,2-difluoro Ethyl]-3-(3-cyclopropyl-2-fluorophenoxy)-5-methylpyridazine-4-carboxamide, (I-749) 6-chloro-3-(3-cyclopropyl-2-fluorophenoxy)-N -[2-(3,4-dimethylphenyl)-2,2-difluoroethyl]-5-methylpyridazine-4-carboxamides.

[0012] definition The term "halogen" as used herein refers to a fluorine, chlorine, bromine or iodine atom.

[0013] The term "methylidene" as used herein refers to a CH attached to a carbon atom through a double bond. 2 point to the base.

[0014] The term "halomethylidene" as used herein refers to a CX 2 refers to a group, where X is halogen.

[0015] The term "oxo" as used herein refers to an oxygen atom bonded through a double bond to a carbon or sulfur atom.

[0016] As used herein, "C 1 -C 6 The term "alkyl" refers to a saturated branched or straight hydrocarbon chain having 1, 2, 3, 4, 5 or 6 carbon atoms. C. 1 -C 6 Examples of alkyl include, but are not limited to, methyl, ethyl, propyl (n-propyl), 1-methylethyl (isopropyl), butyl (n-butyl), 1-methylpropyl (sec-butyl), 2-methylpropyl (isobutyl), 1,1-dimethylethyl (tert-butyl), pentyl, 1-methylbutyl, 2-methylbutyl, 3-methylbutyl, 2,2-dimethylpropyl, 1-ethylpropyl, 1,1-dimethylpropyl, 1 ,2-dimethylpropyl, hexyl, 1-methylpentyl, 2-methylpentyl, 3-methylpentyl, 4-methylpentyl, 1,1-dimethylbutyl, 1,2-dimethylbutyl, 1,3-dimethylbutyl, 2 ,2-dimethylbutyl, 2,3-dimethylbutyl, 3,3-dimethylbutyl, 1-ethylbutyl, 2-ethylbutyl, 1,1,2-trimethylpropyl, 1,2,2-trimethylpropyl, 1-ethyl- 1-methylpropyl and 1-ethyl-2-methylpropyl are included. In particular, the hydrocarbon chain has 1, 2, 3 or 4 carbon atoms ("C 1 -C 4 alkyl"), for example methyl, ethyl, propyl, isopropyl, butyl, sec-butyl, isobutyl or tert-butyl.

[0017] As used herein, "C 2 -C 6 The term "alkenyl" means an unsaturated branched or straight chain hydrocarbon having 2, 3, 4, 5 or 6 carbon atoms and containing at least one double bond. Point to the chain. C. 2 -C 6 Examples of alkenyl include, but are not limited to, ethenyl (or "vinyl"), prop-2-en-1-yl (or "allyl"), prop-1-en-1-yl, but-3-enyl, but-2-enyl, but-1-enyl, pent-4-enyl, pent-3-enyl, pent-2-enyl, pent-1-enyl, hex-5-enyl, hex-4-enyl, hexa- 3-enyl, hex-2-enyl, hex-1-enyl, prop-1-en-2-yl (or "isopropenyl"), 2-methylprop-2-enyl, 1-methylprop-2-enyl, 2 -methylprop-1-enyl, 1-methylprop-1-enyl, 3-methylbut-3-enyl, 2-methylbut-3-enyl, 1-methylbut-3-enyl, 3-methylbut-2-enyl, 2-methylbuta -2-enyl, 1-methylbut-2-enyl, 3-methylbut-1-enyl, 2-methylbut-1-enyl, 1-methylbut-1-enyl, 1,1-dimethylprop-2-enyl, 1- Ethylprop-1-enyl, 1-propylvinyl, 1-isopropylvinyl, 4-methylpent-4-enyl, 3-methylpent-4-enyl, 2-methylpent-4-enyl, 1-methylpent-4-enyl, 4- Methylpent-3-enyl, 3-methylpent-3-enyl, 2-methylpent-3-enyl, 1-methylpent-3-enyl, 4-methylpent-2-enyl, 3-methylpent-2-enyl, 2-methylpent- 2-enyl, 1-methylpent-2-enyl, 4-methylpent-1-enyl, 3-methylpent-1-enyl, 2-methylpent-1-enyl, 1-methylpent-1-enyl, 3-ethylbut-3- enyl, 2-ethylbut-3-enyl, 1-ethylbut-3-enyl, 3-ethylbut-2-enyl, 2-ethylbut-2-enyl, 1-ethylbut-2-enyl, 3-ethylbut-1-enyl, 2-ethylbut-1-enyl, 1-ethylbut-1-enyl, 2-propylprop-2-enyl, 1-propylprop-2-enyl, 2-isopropylprop-2-enyl, 1-isopropylprop-2- enyl, 2-propylprop-1-enyl, 1-propylprop-1-enyl, 2-isopropylprop-1-enyl, 1-isopropylprop-1-enyl, 3,3-dimethylprop-1-enyl, 1 -(1,1-dimethylethyl)ethenyl, buta-1,3-dienyl, penta-1,4-dienyl, hexa-1,5-dienyl or methylhexadienyl groups.

[0018] As used herein, "C 2 -C 6 The term "alkynyl" refers to a branched or straight hydrocarbon chain having 2, 3, 4, 5 or 6 carbon atoms and containing at least one triple bond. C. 2 -C 6 Examples of alkynyl include, but are not limited to, ethynyl, prop-1-ynyl, prop-2-ynyl (or "propargyl"), but-1-ynyl, but-2-ynyl, but-3-ynyl, penta- 1-ynyl, pent-2-ynyl, pent-3-ynyl, pent-4-ynyl, hex-1-ynyl, hex-2-ynyl, hex-3-ynyl, hex-4-ynyl, hex-5- inyl, 1-methylprop-2-ynyl, 2-methylbut-3-ynyl, 1-methylbut-3-ynyl, 1-methylbut-2-ynyl, 3-methylbut-1-ynyl, 1-ethylprop-2-ynyl, 3-methylpent-4-ynyl, 2-methylpent-4-ynyl, 1-methylpent-4-ynyl, 2-methylpent-3-ynyl, 1-methylpent-3-ynyl, 4-methylpent-2-ynyl, 1- Methylpent-2-ynyl, 4-methylpent-1-ynyl, 3-methylpent-1-ynyl, 2-ethylbut-3-ynyl, 1-ethylbut-3-ynyl, 1-ethylbut-2-ynyl, 1-propylpropane -2-ynyl, 1-isopropylprop-2-ynyl, 2,2-dimethylbut-3-ynyl, 1,1-dimethylbut-3-ynyl, 1,1-dimethylbut-2-ynyl or 3,3 -dimethylbut-1-ynyl group.

[0019] As used herein, "C 1 -C 6 The term "haloalkyl" means C as defined above in which one or more hydrogen atoms have been replaced with one or more halogen atoms which may be the same or different. 1 -C 6 Refers to an alkyl group.

[0020] As used herein, "C 2 -C 6 The term "haloalkenyl" means C as defined above in which one or more hydrogen atoms have been replaced with one or more halogen atoms which may be the same or different.2 -C 6 Refers to an alkenyl group.

[0021] As used herein, "C 2 -C 6 The term "haloalkynyl" means C as defined above in which one or more hydrogen atoms are replaced with one or more halogen atoms which may be the same or different. 2 -C 6 Refers to an alkynyl group.

[0022] As used herein, "C 1 -C 6 The term "alkoxy" refers to the formula (C 1 -C 6 alkyl)-O- group, the term "C 1 -C 6 "Alkyl" is as defined herein. C. 1 -C 6 Examples of alkoxy include, but are not limited to, methoxy, ethoxy, n-propoxy, 1-methylethoxy, n-butoxy, 1-methylpropoxy, 2-methylpropoxy, 1,1-dimethylethoxy, n-pentoxy, 1- methylbutoxy, 2-methylbutoxy, 3-methylbutoxy, 2,2-dimethylpropoxy, 1-ethylpropoxy, 1,1-dimethylpropoxy, 1,2-dimethylpropoxy, n-hexyloxy, 1-methylpentoxy, 2-methylpentoxy, 3-methylpentoxy, 4-methylpentoxy, 1,1-dimethylbutoxy, 1,2-dimethylbutoxy, 1,3-dimethylbutoxy, 2,2-dimethylbutoxy, 2,3- dimethylbutoxy, 3,3-dimethylbutoxy, 1-ethylbutoxy, 2-ethylbutoxy, 1,1,2-trimethylpropoxy, 1,2,2-trimethylpropoxy, 1-ethyl-1-methylpropoxy and 1-ethyl -2-methylpropoxy.

[0023] As used herein, "C 1 -C 6 The term "haloalkoxy" means C as defined above wherein one or more hydrogen atoms are replaced with one or more halogen atoms which may be the same or different. 1 -C 6 It refers to alkoxy groups. C. 1 -C 6 Examples of haloalkoxy include, but are not limited to, chloromethoxy, bromomethoxy, dichloromethoxy, trichloromethoxy, fluoromethoxy, difluoromethoxy, trifluoromethoxy, chlorofluoromethoxy, dichlorofluoromethoxy, chlorodifluoromethoxy, 1-chloroethoxy, 1-bromoethoxy, 1-fluoroethoxy, 2-fluoroethoxy, 2,2-difluoroethoxy, 2,2,2-trifluoroethoxy, 2-chloro-2-fluoroethoxy, 2-chloro-2,2-difluoro Ethoxy, 2,2-dichloro-2-fluoroethoxy, 2,2,2-trichloroethoxy, pentafluoroethoxy and 1,1,1-trifluoroprop-2-oxy.

[0024] As used herein, "C 1 -C 6 The term "haloalkoxy" means C as defined above wherein one or more hydrogen atoms are replaced with one or more halogen atoms which may be the same or different. 1 -C 6 It refers to alkoxy groups.

[0025] As used herein, "C 1 -C 6 The term hydroxyalkyl" means C as defined above in which at least one hydrogen atom is replaced with a hydroxyl group. 1 -C 6 Refers to an alkyl group. C. 1 -C 6 Examples of hydroxyalkyl include, but are not limited to, hydroxymethyl, 1-hydroxyethyl, 2-hydroxyethyl, 1,2-dihydroxyethyl, 3-hydroxypropyl, 2-hydroxypropyl, 1-hydroxypropyl, 1-hydroxypropane -2-yl, 2-hydroxypropan-2-yl, 2,3-dihydroxypropyl and 1,3-dihydroxypropan-2-yl.

[0026] As used herein, "C 1 -C 6 The term "alkylsulfanyl" refers to the formula (C 1 -C 6 Alkyl)-S-saturated straight or branched chain groups, the term "C 1 -C 6 "Alkyl" is as defined herein. C. 1 -C 6 Examples of alkylsulfanyl include, but are not limited to, methylsulfanyl, ethylsulfanyl, propylsulfanyl, isopropylsulfanyl, butylsulfanyl, sec-butylsulfanyl, isobutylsulfanyl, tert-butylsulfanyl, pentylsulfanyl, isopentylsulfanyl, hexylsulfanyl groups. mentioned.

[0027] As used herein, "C 1 -C 6 The term "haloalkylsulfanyl" means a C 1 -C 6 It refers to alkylsulfanyl.

[0028] As used herein, "C 1 -C 6 The term "alkylsulfinyl" refers to the formula (C 1 -C 6 Alkyl)-S(=O)-saturated straight or branched chain group, the term “C 1 -C 6 "Alkyl" is as defined herein. C. 1 -C 6 Examples of alkylsulfinyl include, but are not limited to, saturated linear or branched alkylsulfinyl radicals having 1 to 8, preferably 1 to 6, more preferably 1 to 4 carbon atoms, such as (without limitation), methylsulfinyl, ethylsulfinyl, propylsulfinyl, 1-methylethylsulfinyl, butylsulfinyl, 1-methylpropylsulfinyl, 2-methylpropylsulfinyl, 1,1-dimethylethylsulfinyl, pentylsulfinyl, 1-methyl Butylsulfinyl, 2-methylbutylsulfinyl, 3-methylbutylsulfinyl, 2,2-dimethylpropylsulfinyl, 1-ethylpropylsulfinyl, 1,1-dimethylpropylsulfinyl, 1,2-dimethylpropylsulfinyl, hexylsulfinyl, 1- methylpentylsulfinyl, 2-methylpentylsulfinyl, 3-methylpentylsulfinyl, 4-methylpentylsulfinyl, 1,1-dimethylbutylsulfinyl, 1,2-dimethylbutylsulfinyl, 1,3-dimethylbutylsulfinyl, 2,2- Dimethylbutylsulfinyl, 2,3-dimethylbutylsulfinyl, 3,3-dimethylbutylsulfinyl, 1-ethylbutylsulfinyl, 2-ethylbutylsulfinyl, 1,1,2-trimethylpropylsulfinyl, 1,2,2-trimethylpropyl C such as sulfinyl, 1-ethyl-1-methylpropylsulfinyl and 1-ethyl-2-methylpropylsulfinyl 1 -C 6 Alkylsulfinyl can be mentioned.

[0029] As used herein, "C 1 -C 6 The term "haloalkylsulfinyl" means C as defined above wherein one or more hydrogen atoms are replaced with one or more halogen atoms which may be the same or different 1 -C 6 It refers to alkylsulfinyl.

[0030] As used herein, "C 1 -C 6 The term "alkylsulfonyl" refers to the formula (C 1 -C 6 alkyl)-S(=O) 2 - refers to a saturated straight or branched chain group, the term “C 1 -C 6 "Alkyl" is as defined herein. C. 1 -C 6 Examples of alkylsulfonyl include, but are not limited to, methylsulfonyl, ethylsulfonyl, propylsulfonyl, 1-methylethylsulfonyl, butylsulfonyl, 1-methylpropylsulfonyl, 2-methylpropylsulfonyl, 1,1-dimethylethylsulfonyl, pentyl sulfonyl, 1-methylbutylsulfonyl, 2-methylbutylsulfonyl, 3-methylbutylsulfonyl, 2,2-dimethylpropylsulfonyl, 1-ethylpropylsulfonyl, 1,1-dimethylpropylsulfonyl, 1,2-dimethylpropylsulfonyl, Hexylsulfonyl, 1-methylpentylsulfonyl, 2-methylpentylsulfonyl, 3-methylpentylsulfonyl, 4-methylpentylsulfonyl, 1,1-dimethylbutylsulfonyl, 1,2-dimethylbutylsulfonyl, 1,3-dimethylbutylsulfonyl , 2,2-dimethylbutylsulfonyl, 2,3-dimethylbutylsulfonyl, 3,3-dimethylbutylsulfonyl, 1-ethylbutylsulfonyl, 2-ethylbutylsulfonyl, 1,1,2-trimethylpropylsulfonyl, 1,2 ,2-trimethylpropylsulfonyl, 1-ethyl-1-methylpropylsulfonyl and 1-ethyl-2-methylpropylsulfonyl.

[0031] As used herein, "C 1 -C 6 The term "haloalkylsulfonyl" means C 1 -C 6 It refers to alkylsulfonyl.

[0032] As used herein, "C 1 -C 6 The term "alkylcarbonyl" refers to the formula (C 1 -C 6 Alkyl)-C(=O)-saturated straight or branched chain group, the term "C 1 -C 6 "Alkyl" is as defined herein.

[0033] As used herein, "C 1 -C 6 The term "haloalkylcarbonyl" means a C 1 -C 6 It refers to alkylcarbonyl.

[0034] As used herein, "C 1 -C 6 The term "alkoxycarbonyl" refers to the formula (C 1 -C 6 alkoxy)-C(=O)-, the term "C 1 -C 6 Alkoxy" is as defined herein.

[0035] As used herein, "C 1 -C 6 The term "haloalkoxycarbonyl" means C as defined above wherein one or more hydrogen atoms are replaced with one or more halogen atoms which may be the same or different. 1 -C 6 It refers to alkoxycarbonyl.

[0036] As used herein, "C 1 -C 6 The term "dialkylamino" refers to two independently selected C 1 -C 6 It refers to an amino radical with an alkyl group. C. 1 -C 6 Examples of dialkylamino include, but are not limited to, N,N-dimethylamino, N,N-diethylamino, N,N-diisopropylamino, N-ethyl-N-methylamino, N-methyl-N-n-propylamino, N -isopropyl-N-n-propylamino and N-tert-butyl-N-methylamino.

[0037] As used herein, "non-aromatic C 3 -C 12 The term "carbocycle" refers to a non-aromatic, saturated or unsaturated hydrocarbon ring system in which the ring members, which vary from 3 to 12, are all carbon atoms. Ring systems can be monocyclic or polycyclic (fused, spiro or bridged). non-aromatic C 3 -C 12 Carbocycles include, but are not limited to, C 3 -C 12 Cycloalkyl (monocyclic or bicyclic), C 3 -C 12 Cycloalkenyl (monocyclic or bicyclic), monocyclic C 3 -C 8 Bicyclic (e.g. tetrahydronaphthalenyl, indanyl) containing aryl (e.g. phenyl) fused to cycloalkyl, monocyclic C 3 -C 8 Bicyclic ring systems (e.g. indenyl, dihydronaphthalenyl) containing aryl (e.g. phenyl) fused to cycloalkenyl, and monocyclic C 3 -C 8 cycloalkyl or monocyclic C 3 -C 8 Tricyclic ring systems containing cyclopropyl linked via one carbon atom to a bicyclic ring system containing an aryl (eg, phenyl) fused to a cycloalkenyl are included. non-aromatic C 3 -C 12 The carbocycle can be attached to the parent molecular moiety through any carbon atom.

[0038] As used herein, "C 3 -C 12 The term cycloalkyl" means a saturated monovalent, monocyclic or Refers to a bicyclic hydrocarbon ring. Monocyclic C 3 -C 8 Examples of cycloalkyl include, but are not limited to, cyclopropyl, cyclobutyl, cyclopentyl, cyclohexyl, cycloheptyl or cyclooctyl. Bicyclic C 6 -C 12 Examples of cycloalkyl include, but are not limited to, bicyclo[3.1.1]heptane, bicyclo[2.2.1]heptane, bicyclo[2.2.2]octane, bicyclo[3.2.2]nonane, bicyclo[3.3.1]nonane , bicyclo[4.2.0]octyl, octahydropentalenyl and bicyclo[4.2.1]nonane.

[0039] As used herein, "C 3 -C 12 The term "cycloalkenyl" means an unsaturated monovalent, monocyclic ring containing 3, 4, 5, 6, 7, 8, 9, 10, 11 or 12 carbon atoms or refers to a bicyclic hydrocarbon ring. Monocyclic C 3 -C 8 Examples of cycloalkenyl groups include, but are not limited to, cyclobutenyl, cyclopentenyl, cyclohexenyl, cycloheptenyl and cyclooctenyl groups. Bicyclic C 6 -C 12 Examples of cycloalkenyl groups include, but are not limited to, bicyclo[2.2.1]hept-2-enyl or bicyclo[2.2.2]oct-2-enyl.

[0040] As used herein, "aromatic C 6 -C 14 The term "carbocycle" or "aryl" refers to an aromatic hydrocarbon ring system in which the ring members, which vary from 6 to 14, preferably from 6 to 10, are all carbon atoms. Ring systems can be monocyclic or fused polycyclic (eg, bicyclic or tricyclic). Examples of aryl include, but are not limited to, phenyl, azulenyl and naphthyl. The aryl can be attached to the parent molecular moiety through any carbon atom. It is further understood that when said aryl group is substituted with one or more substituents, the substituents may be at any position on the aryl ring. In particular, when aryl is a phenyl group, said substituents may occupy one or both ortho-positions, one or both meta-positions, or para-positions, or any combination of these positions.

[0041] As used herein, the term "non-aromatic 3- to 14-membered heterocyclic ring" refers to a saturated or unsaturated ring containing 1-4 heteroatoms independently selected from the group consisting of oxygen, nitrogen and sulfur. Refers to non-aromatic ring systems. When the ring system contains multiple oxygen atoms, they are not directly adjacent. Non-aromatic heterocycles include, but are not limited to, 3- to 7-membered monocyclic non-aromatic heterocycles and 6- to 14-membered polycyclic (eg, bicyclic or tricyclic) non-aromatic heterocycles. be done. A non-aromatic 3- to 14-membered heterocycle can be attached to the parent molecular moiety through any carbon or nitrogen atom contained within the heterocycle.

[0042] The term "non-aromatic 3- to 7-membered monocyclic heterocycle" as used herein means 1, 2 or 3 heteroatoms independently selected from the group consisting of oxygen, nitrogen and sulfur. refers to a 3-, 4-, 5-, 6- or 7-membered monocyclic ring system containing a , which is saturated or unsaturated but not aromatic. For example, a heterocyclic ring has 1 to 3 nitrogen atoms, or 1 or 2 oxygen atoms, or 1 or 2 sulfur atoms, or 1 to 3 nitrogen atoms and 1 oxygen atom, or It may contain 1-3 nitrogen atoms and 1 sulfur atom, or 1 sulfur atom and 1 oxygen atom. Examples of saturated non-aromatic heterocycles include, but are not limited to, 3-membered rings such as oxiranyl and aziridinyl, 4-membered rings such as azetidinyl, oxetanyl, thietanyl, tetrahydrofuranyl, 1,3-dioxolanyl, tetrahydrothienyl, pyrrolidinyl, pyrazolidinyl. , imidazolidinyl, triazolidinyl, isoxazolidinyl, oxazolidinyl, oxadiazolidinyl, thiazolidinyl, isothiazolidinyl, thiadiazolidinyl and other five-membered rings, piperidinyl, hexahydropyridazinyl, hexahydropyrimidinyl, piperazinyl, 6-membered rings such as triazinanyl, hexahydrotriazinyl, tetrahydropyranyl, dioxanyl, tetrahydrothiopyranyl, dithianyl, morpholinyl, 1,2-oxazinanyl, oxathianyl, thiomorpholinyl, or oxepanyl, azepanyl, 1,4-diazepanyl and 1 and 7-membered rings such as ,4-oxazepanyl. Examples of unsaturated non-aromatic heterocycles include, but are not limited to, dihydrofuranyl, 1,3-dioxolyl, dihydrothienyl, pyrrolinyl, dihydroimidazolyl, dihydropyrazolyl, isoxazolinyl, dihydrooxazolyl, dihydrothiazolyl, and the like. 5-membered rings or 6-membered rings such as pyranyl, thiopyranyl, thiazinyl and thiadiazinyl are included.

[0043] The term "non-aromatic 6- to 14-membered polycyclic heterocycle" as used herein includes 1, 2 or 3 heteroatoms independently selected from the group consisting of oxygen, nitrogen and sulfur. refers to a 6-, 7-, 8-, 9-, 10-, 11-, 12-, 13- or 14-membered polycyclic (e.g., bicyclic or tricyclic) ring system comprising the ring The system can be saturated or unsaturated but not aromatic. Non-aromatic bicyclic heterocycles are monocyclic C 3 -C 8 cycloalkyl, monocyclic C 3 -C 8 may consist of a monocyclic heteroaryl as defined herein fused to a cycloalkenyl or monocyclic non-aromatic heterocycle, or an aryl (e.g., phenyl), monocyclic C 3 -C 8 cycloalkyl, monocyclic C 3 -C 8 It may consist of a monocyclic non-aromatic heterocycle fused to either a cycloalkenyl or a monocyclic non-aromatic heterocycle. When two monocyclic heterocycles (aromatic or non-aromatic) containing a nitrogen atom are fused, the nitrogen atom may be a bridgehead (e.g., 4,5,6,7- Tetrahydropyrazolo[1,5-a]pyridinyl, 5,6,7,8-tetrahydro-[1,2,4]triazolo[1,5-a]pyridinyl, 5,6,7,8-tetrahydroimidazo[ 1,2-a]pyridinyl). A non-aromatic tricyclic heterocycle may consist of a monocyclic cycloalkyl linked through one common atom to a non-aromatic bicyclic heterocycle.

[0044] The term "5- to 14-membered heteroaromatic ring" or "heteroaryl" as used herein refers to an aromatic ring containing 1-4 heteroatoms independently selected from the group consisting of oxygen, nitrogen and sulfur. refers to a tricyclic ring system. When the ring system contains more than one oxygen atom, they are not directly adjacent. Aromatic heterocycles include aromatic 5- or 6-membered monocyclic heterocycles and 6- to 14-membered polycyclic (eg, bicyclic or tricyclic) aromatic heterocycles. The 5- to 14-membered aromatic heterocycles can be attached to the parent molecular moiety through any carbon or nitrogen atom contained within the heterocycle.

[0045] The term "aromatic 5- or 6-membered monocyclic heterocycle" or "monocyclic heteroaryl" as used herein means one independently selected from the group consisting of oxygen, nitrogen and sulfur, It refers to a 5- or 6-membered monocyclic ring system containing 2, 3 or 4 heteroatoms. Examples of 5-membered monocyclic heteroaryl include, but are not limited to, furyl (furanyl), thienyl, pyrrolyl, pyrazolyl, imidazolyl, triazolyl, tetrazolyl, isoxazolyl, oxazolyl, oxadiazolyl, oxatriazolyl, isothiazolyl, thiazolyl, thiadiazolyl and thiatriazolyl. Examples of 6-membered monocyclic heteroaryls include, but are not limited to, pyridinyl, pyridazinyl, pyrimidinyl, pyrazinyl, triazinyl, tetrazinyl.

[0046] The term "6- to 14-membered polycyclic heteroaromatic ring" or "polycyclic heteroaryl" as used herein means one, two, independently selected from the group consisting of oxygen, nitrogen and sulfur. 6-, 7-, 8-, 9-, 10-, 11-, 12-, 13- or 14-membered polycyclic (e.g. bicyclic or tricyclic) rings containing one or three heteroatoms refers to the system. An aromatic bicyclic heterocycle may consist of a monocyclic heteroaryl as defined herein fused to an aryl (eg, phenyl) or a monocyclic heteroaryl. Examples of bicyclic heteroaromatic rings include, but are not limited to, indolyl, indolizinyl, isoindolyl, benzimadazolyl, imidazopyridinyl, indazolyl, benzotriazolyl, purinyl, benzofuranyl, benzothiophenyl, benzothiazolyl, benzoxazolyl and 9-membered rings such as benzisoxazolyl, or 10-membered rings such as quinolinyl, isoquinolinyl, cinnolinyl, quinazolinyl, quinoxalinyl, phthalazinyl, naphthyridinyl, pteridinal and benzodioxinyl. In 9- or 10-membered aromatic bicyclic heterocycles, including two fused 5- or 6-membered monocyclic aromatic heterocycles, the nitrogen atoms may be bridgeheads (e.g., imidazo[1,2 -a]pyridinyl, [1,2,4]triazolo[4,3-a]pyridinyl, imidazo[1,2-a]pyridinyl, imidazo[2,1-b]oxazolyl, furo[2,3-d] isoxazolyl). Examples of tricyclic heteroaromatic rings include, but are not limited to, carbazolyl, acridinyl and phenazinyl.

[0047] As used herein, "non-aromatic C 3 -C 12 carbocyclyloxy”, “C 3 -C 8 cycloalkyloxy”, “aromatic C 6 -C 14 The terms "carbocyclyloxy", "aromatic 5-14 membered heterocyclyloxy", "non-aromatic 3-14 membered heterocyclyloxy" refer to groups of the formula -O-R, where R is each defined herein. non-aromatic C 3 -C 12 Carbocyclyl, C 3 -C 8 cycloalkyl, aromatic C 6 -C 14 It is carbocyclyl, aromatic 5- to 14-membered heterocyclyl or non-aromatic 3- to 14-membered heterocyclyl group.

[0048] As used herein, when a group is said to be "substituted," that group may be substituted with one or more substituents. The phrase "one or more substituents" refers to the maximum number of possible substituents based on the number of available binding sites from one, provided that conditions of stability and chemical feasibility are met. Refers to the number of substituents ranging up to number.

[0049] As used herein, the term "leaving group" refers to a group that is removed from a compound in a substitution or elimination reaction, such as halogen atoms, trifluoromethanesulfonate ("triflate") groups, alkoxy, methanesulfonate, p- It is understood to mean toluenesulfonate and the like.

[0050] Varying Q, T, R 1 , R 2 , R 3 , R 4 , R 5 , R 6 , R 7 , R 8 The term "as described herein" when referring to , n and m encompasses by reference the broad definition of the variation, as well as the preferred, more preferred and even more preferred definitions, if any. .

[0051] Compounds resulting from combinations that are contrary to the laws of nature and therefore would be ruled out by a person skilled in the art based on his expertise are not covered herein. For example, ring structures with 3 or more adjacent oxygen atoms are excluded.

[0052] The compounds of formula (I) may suitably be in their free, salt, N-oxide or solvate form (eg hydrates).

[0053] Depending on the nature of the substituents, the compounds of formula (I) can exist in different stereoisomeric forms. These stereoisomers are for example enantiomers, diastereomers, atropisomers or geometric isomers. Accordingly, the present invention includes both the pure stereoisomers and any mixtures of those isomers. Where a compound can exist in two or more tautomeric forms at equilibrium, a reference to a compound by describing a single tautomer shall encompass all tautomeric forms. It is regarded.

[0054] Any of the compounds of the present invention can also exist in one or more geometric isomeric forms, depending on the number of double bonds in the compound. Geometric isomers due to the nature of substituents on double bonds or rings can exist in cis (=Z-) or trans (=E-) forms. Accordingly, the invention equally relates to all geometric isomers and all possible mixtures in all proportions.

[0055] Depending on the nature of the substituents, the compounds of formula (I) may exist in the form of free compounds and / or their salts, such as pesticidally active salts.

[0056] Agrochemically active salts include acid addition salts of inorganic and organic acids and salts of conventional bases. Examples of inorganic acids are hydrohalic acids such as hydrogen fluoride, hydrogen chloride, hydrogen bromide and hydrogen iodide, sulfuric acid, phosphoric acid and nitric acid, and acidic salts such as sodium and potassium bisulfate. Useful organic acids include, for example, formic acid, carbonic acid, and alkanoic acids such as acetic acid, trifluoroacetic acid, trichloroacetic acid and propionic acid, as well as glycolic, thiocyanic, lactic, succinic, citric, benzoic, cinnamic acids. , oxalic acid, saturated or monounsaturated or diunsaturated fatty acids having 6 to 20 carbon atoms, alkylsulfuric acid monoesters, alkylsulfonic acids (linear or branched chain having 1 to 20 carbon atoms) sulfonic acids with alkyl radicals), arylsulfonic acids or aryldisulfonic acids (aromatic radicals such as phenyl and naphthyl with 1 or 2 sulfonic acid groups), alkylphosphonic acids (having 1 to 20 carbon atoms phosphonic acids with linear or branched alkyl radicals), arylphosphonic acids or aryldiphosphonic acids (aromatic groups such as phenyl and naphthyl with 1 or 2 phosphonic acid radicals); Radicals and aryl radicals may have further substituents such as p-toluenesulfonic acid, salicylic acid, p-aminosalicylic acid, 2-phenoxybenzoic acid, 2-acetoxybenzoic acid and the like.

[0057] A solvate of a compound of the invention or a salt thereof is a stoichiometric composition of the compound and a solvent.

[0058] The compounds of the present invention may exist in multiple crystalline and / or amorphous forms. Crystalline forms include unsolvated crystal forms, solvates and hydrates.

[0059] As used herein, "aliphatic R 6S , R c and R d Aliphatic R in the phrase "a substituent may be substituted with one or more substituents" 6S Substituents are C 1 -C 6 Alkyl, C 1 -C 6 haloalkyl, C 1 -C 6 Alkoxy, C 1 -C 6 haloalkoxy, C 2 -C 6 alkenyl, C 2 -C 6 haloalkenyl, C 2 -C 6 alkynyl, C 2 -C 6 haloalkynyl, C 2 -C 6 alkenyloxy, C 2 -C 6 haloalkenyloxy, C 1 -C 6 Alkylsulfanyl, C 1 -C 6 haloalkylsulfanyl, C 1 -C 6 Alkylsulfinyl, C 1 -C 6 haloalkylsulfinyl, C 1 -C 6 alkylsulfonyl, C 1 -C 6 haloalkylsulfonyl, and -Si(C 1 -C 6 alkyl) 3 and -O-Si(C 1 -C 6 alkyl) 3 C of 1 -C 6 refers to the alkyl moiety.

[0060] As used herein, "aliphatic R 6S , R c and R d Aliphatic R in the phrase "a substituent may be substituted with one or more substituents" c Substituents are C 1 -C 6 refers to alkyl.

[0061] As used herein, "aliphatic R 6S , R c and R d Aliphatic R in the phrase "a substituent may be substituted with one or more substituents" d Substituents are C 1 -C 6 Alkyl and C 1 -C 6 Refers to haloalkyl.

[0062] As used herein, "aliphatic R 7 , R e , R f and R g Substituents are one or more R 7Sa Aliphatic R in the expression "optionally substituted with a substituent 7 Substituents are C 1 -C 6 Alkyl, C 1 -C 6 haloalkyl, C 1 -C 6 hydroxyalkyl, C 1 -C 6 alkylcarbonyl, C 1 -C 6 haloalkylcarbonyl, C 1 -C 6 Alkoxy, C 1 -C 6 haloalkoxy, C 1 -C 6 Alkoxycarbonyl, C 1 -C 6 haloalkoxycarbonyl, C 2 -C 6 alkenyl, C 2 -C 6 haloalkenyl, C 2 -C 6 alkynyl, C 2 -C 6 haloalkynyl, C 2 -C 6 alkenyloxy, C 2 -C 6 haloalkenyloxy, C 2 -C 6 alkynyloxy, C 2 -C 6 haloalkynyloxy, C 1 -C 6 Alkylsulfanyl, C 1 -C 6 haloalkylsulfanyl, C 1 -C 6 Alkylsulfinyl, C 1 -C 6 haloalkylsulfinyl, C 1 -C 6 alkylsulfonyl, C 1 -C 6 haloalkylsulfonyl, and -Si(C 1 -C 6 alkyl) 3 and -O-Si(C 1 -C 6 alkyl) 3 C of 1 -C 6 refers to the alkyl moiety.

[0063] As used herein, "aliphatic R 7 , R e , R f and R g Substituents are one or more R 7Sa Aliphatic R in the expression "optionally substituted with a substituent e Substituents are C 1 -C 6 Alkyl, C 1 -C 6 haloalkyl, C 1 -C 6 Alkoxy, C 2 -C 6 alkenyl, C 2 -C 6 haloalkenyl, C 2 -C 6 alkynyl and C 2 -C 6 Refers to haloalkynyl.

[0064] As used herein, "aliphatic R 7 , R e , R f and R g Substituents are one or more R 7Sa Aliphatic R in the expression "optionally substituted with a substituent f Substituents are C 1 -C 6 Alkyl, C 1 -C 6 haloalkyl, C 1 -C 6 alkoxy, as well as C 1 -C 6 alkylamino and di(C 1 -C 6 Alkyl)amino C 1 -C 6 refers to the alkyl moiety.

[0065] As used herein, "aliphatic R 7 , R e , R f and R g Substituents are one or more R 7Sa Aliphatic R in the expression "optionally substituted with a substituent g Substituents are C 1 -C 6 Alkyl and C 1 -C 6 Refers to haloalkyl.

[0066] As used herein, "aliphatic R 8 , R h and R i Substituents are one or more R 8Sa Aliphatic R in the expression "optionally substituted with a substituent 8 Substituents are C 1 -C 6 Alkyl, C 1 -C 6 haloalkyl, C 1 -C 6 hydroxyalkyl, C 1 -C 6 Alkoxy, C 1 -C 6 haloalkoxy, C 2 -C 6 alkenyl, C 2 -C 6 haloalkenyl, C 2 -C 6 alkynyl, C 2 -C 6 haloalkynyl, C 2 -C 6 alkenyloxy, C 2 -C 6 haloalkenyloxy, C 2 -C 6 alkynyloxy, C 2 -C 6 haloalkynyloxy, C1 -C 6 Alkylsulfanyl, C 1 -C 6 haloalkylsulfanyl, C 1 -C 6 Alkylsulfinyl, C 1 -C 6 haloalkylsulfinyl, C 1 -C 6 alkylsulfonyl, C 1 -C 6 Haloalkylsulfonyl, and -Si(C 1 -C 6 alkyl) 3 and -O-Si(C 1 -C 6 alkyl) 3 C of 1 -C 6 refers to the alkyl moiety.

[0067] As used herein, "aliphatic R 8 , R h and R i Substituents are one or more R 8Sa Aliphatic R in the expression "optionally substituted with a substituent h Substituents are C 1 -C 6 Alkyl, C 1 -C 6 haloalkyl, C 1 -C 6 Alkoxy, C 2 -C 6 alkenyl, C 2 -C 6 haloalkenyl, C 2 -C 6 alkynyl and C 2 -C 6 Refers to haloalkynyl.

[0068] As used herein, "aliphatic R 8 , R h and R i Substituents are one or more R 8Sa Aliphatic R in the expression "optionally substituted with a substituent i Substituents are C 2 -C 6 alkenyl, C 2 -C 6 haloalkenyl, C 2 -C 6 alkynyl and C 2 -C 6 Refers to haloalkynyl.

[0069] As used herein, "aliphatic Q S , R j and R k Aliphatic Q in the phrase "a substituent may be optionally substituted with one or more substituents" S Substituents are C 1 -C 6 Alkyl, C 1 -C 6 haloalkyl, C 1 -C 6 alkylcarbonyl, C 1 -C 6 haloalkylcarbonyl, C 1 -C 6 Alkoxy, C 1 -C 6 haloalkoxy, C 1 -C 6 Alkoxy-C 1 -C 6 Alkyl, C 1 -C 6 Alkoxycarbonyl, C 1 -C 6 haloalkoxycarbonyl, C 2 -C 6 alkenyl, C 2 -C 6 haloalkenyl, C 2 -C 6 alkynyl, C 2 -C 6 haloalkynyl, C 2 -C 6 alkenyloxy, C 2 -C 6 haloalkenyloxy, C 1 -C 6 Alkylsulfanyl, C 1 -C 6 haloalkylsulfanyl, C 1 -C 6 Alkylsulfinyl, C 1 -C 6 haloalkylsulfinyl, C 1 -C 6 alkylsulfonyl, C 1 -C 6 haloalkylsulfonyl, and -Si(C 1 -C 6 alkyl) 3 and -O-Si(C 1 -C 6 alkyl) 3 C of 1 -C 6 refers to the alkyl moiety.

[0070] As used herein, "aliphatic Q S , R j and R k The aliphatic R in the expression "a substituent may be optionally substituted with one or more substituents j Substituents are C 1 -C 6 Alkyl, C 1 -C 6 haloalkyl and C 1 -C 6 indicates alkoxy.

[0071] As used herein, "aliphatic Q S , R j and R k The aliphatic R in the expression "a substituent may be optionally substituted with one or more substituents k Substituents are C 1 -C 6 Alkyl, C 1 -C 6 haloalkyl, C 1 -C 6 Alkoxy, C 2 -C 6 alkenyl and C 2 -C 6 Refers to haloalkenyl.

[0072] As used herein, "R 6 A ring or cyclic portion of a substituent may be one or more R 6S cyclic R in the expression "optionally substituted with a substituent 6 Substituents are non-aromatic C 3 -C 12 carbocyclic, aromatic C 6 -C 14 It refers to carbocycles, non-aromatic 3- to 14-membered heterocycles and aromatic 5- to 14-membered heterocycles.

[0073] As used herein, "R 6 A ring or cyclic portion of a substituent may be one or more R 6S R in the expression "may be substituted with a substituent 6 The cyclic portion of the substituent is a non-aromatic C 3 -C 12 non-aromatic C of carbocyclyloxy 3 -C 12 carbocyclic, aromatic C 6 -C 14 carbocyclyloxy aromatic C 6 -C 14 carbocyclyl, aromatic 5-14 membered heterocyclic ring of aromatic 5-14 membered heterocyclyloxy, non-aromatic 3-14 membered heterocyclic ring of non-aromatic 3-14 membered heterocyclyloxy, non-aromatic C 3 -C 12 carbocyclic substituted C 1 -C 3 non-aromatic C of alkoxy 3 -C 12 carbocyclic, aromatic C 6 -C 14 carbocyclic substituted C 1 -C 3 alkoxy aromatic C 6 -C 14 C substituted with carbocyclic, non-aromatic 3-14 membered heterocyclic ring 1 -C 3 non-aromatic 3- to 14-membered heterocyclic ring of alkoxy, C substituted with aromatic 5- to 14-membered heterocyclic ring 1 -C 3 Alkoxy aromatic 5-14 membered heterocycle, non-aromatic C 3 -C 12 carbocyclic substituted C 1 -C 3 haloalkoxy aromatic C 3 -C 12 carbocyclic, aromatic C 6 -C 14 carbocyclic substituted C 1 -C 3 haloalkoxy aromatic C 6 -C 14 C substituted with carbocyclic, non-aromatic 3-14 membered heterocyclic ring 1 -C 3 haloalkoxy non-aromatic 3- to 14-membered heterocyclic ring and C substituted with aromatic 5- to 14-membered heterocyclic ring 1 -C 3 Refers to a haloalkoxy aromatic 5- to 14-membered heterocyclic ring.

[0074] As used herein, "cyclic R 6S Substituents and R c A cyclic R in the expression "a substituent may be optionally substituted with one or more substituents 6S Substituents are C 3 -C 8 Cycloalkyl, C 3 -C 8 cycloalkenyl, aromatic C 6 -C 14It refers to carbocycles, aromatic 5- or 6-membered monocyclic heterocycles and non-aromatic 3- to 7-membered monocyclic heterocycles.

[0075] As used herein, "R 6S the ring or cyclic portion of and cyclic R c A substituent may be substituted with one or more substituents" in the expression 6S The cyclic portion of the substituent is C 3 -C 8 Cycloalkyloxy, C 3 -C 8 Cycloalkylsulfanyl, C 3 -C 8 cycloalkylsulfinyl and C 3 -C 8 C of cycloalkylsulfonyl 3 -C 8 Refers to cycloalkyl.

[0076] As used herein, "R 6S the ring or cyclic portion of and cyclic R c A cyclic R in the expression "a substituent may be optionally substituted with one or more substituents c Substituents are C 3 -C 8 Refers to cycloalkyl.

[0077] As used herein, "R 7 , R e and R g Substituents are one or more R 7Sc cyclic R in the expression "optionally substituted with a substituent 7 Substituents are C 3 -C 8 Cycloalkyl, C 3 -C 6 cycloalkenyl, aromatic C 6 -C 14 It refers to carbocycles, aromatic 5- or 6-membered monocyclic heterocycles and non-aromatic 3- to 7-membered monocyclic heterocycles.

[0078] As used herein, "R 7 The ring or cyclic portion of the cyclic R e and cyclic R g Substituents are one or more R 7Sc R in the expression "may be substituted with a substituent 7 The cyclic portion of the substituent is C 3 -C 8 Cycloalkyloxy, C 3 -C 8 Cycloalkylsulfanyl, C 3 -C 8 cycloalkylsulfinyl and C 3 -C 8 C of cycloalkylsulfonyl 3 -C 8 cycloalkyl, aromatic C 6 -C 14 carbocyclyloxy aromatic C 6 -C 14 Carbocyclic, aromatic 5- or 6-membered monocyclic heterocycle of aromatic 5- or 6-membered monocyclic heterocyclyloxy, and non-aromatic 3- to 7-membered of non-aromatic 3- to 7-membered monocyclic heterocyclyloxy It refers to monocyclic heterocycles.

[0079] As used herein, "R 7 , R e and R g Substituents are one or more R 7Sc cyclic R in the expression "optionally substituted with a substituent e Substituents are C 3 -C 8 Cycloalkyl, C 3 -C 8 halocycloalkyl, aromatic C 6 -C 14 It refers to carbocycles, aromatic 5- or 6-membered monocyclic heterocycles and non-aromatic 3- to 7-membered monocyclic heterocycles.

[0080] As used herein, "R 7 , R e and R g Substituents are one or more R 7Sc cyclic R in the expression "optionally substituted with a substituent g Substituents are C 3 -C 8 Refers to cycloalkyl.

[0081] As used herein, "R 8 , R h and R i Substituents are one or more R 8Sc cyclic R in the expression "optionally substituted with a substituent 8 Substituents are C 3 -C 8 Cycloalkyl, C 3 -C 6 cycloalkenyl, aromatic C 6 -C 14 It refers to carbocycles, non-aromatic 3- to 14-membered heterocycles and aromatic 5- to 14-membered heterocycles.

[0082] As used herein, "R 8 The ring or cyclic portion of the cyclic R h and cyclic R i Substituents are one or more R 8Sc R in the expression "may be substituted with a substituent 8 The cyclic portion of the substituent is C 3 -C 8 C of cycloalkyloxy 3 -C 8 cycloalkyl, aromatic C 6 -C 14 carbocyclyloxy aromatic C 6 -C 14 It refers to a carbocyclic ring, a non-aromatic 3- to 14-membered heterocyclic ring of a non-aromatic 3- to 14-membered heterocyclyloxy, and an aromatic 5- to 14-membered heterocyclic ring of an aromatic 5- to 14-membered heterocyclyloxy.

[0083] As used herein, "R 8 The ring or cyclic portion of the cyclic R h and cyclic R i Substituents are one or more R 8Sc cyclic R in the expression "optionally substituted with a substituent h Substituents are C 3 -C 8 Cycloalkyl, C 3 -C 8 halocycloalkyl, aromatic C 6 -C 14 It refers to carbocycles, aromatic 5- to 14-membered heterocycles and non-aromatic 3- to 7-membered monocyclic heterocycles.

[0084] As used herein, "R 8 , R h and R i Substituents are one or more R 8Sc cyclic R in the expression "optionally substituted with a substituent i Substituents are C 3 -C 8 Cycloalkyl, C 3 -C 8 halocycloalkyl, aromatic C 6 -C 14 It refers to carbocyclic rings, aromatic 5- to 14-membered heterocyclic rings, and non-aromatic 3- to 7-membered monocyclic heterocyclic rings.

[0085] As used herein, "Q S the ring or cyclic portion of and cyclic R k Substituents are one or more R Qs cyclic Q in the expression "optionally substituted with a substituent S Substituents are C 3 -C 8 Cycloalkyl, C 3 -C 6 It refers to cycloalkenyl, non-aromatic 3- to 7-membered monocyclic heterocycles and aromatic 5- to 14-membered heterocycles.

[0086] As used herein, "Q S the ring or cyclic portion of and cyclic R k Substituents are one or more R Qs Q in the expression "may be substituted with substituents" S The cyclic portion of the substituent is C 3 -C 8 C of cycloalkyloxy 3 -C 8 Refers to cycloalkyl.

[0087] As used herein, "annular Q S and R k Substituents are one or more R Qs cyclic R in the expression "optionally substituted with a substituent k Substituents are C 3 -C 8 Refers to cycloalkyl.

[0088] In this specification R 2 and R 4 are said to form a covalent bond together, the following groups are obtained: -CR 3 = CR 5 -.

[0089] In formula (I) above, n is 0 or 1 and m is 0 or 1, provided that when n is 1, m is 1. The present invention relates to compounds wherein n is 1 and m is 1, or n is 0 and m is 1, or n is 0 and m is 0.

[0090] Methods for the preparation of compounds of formula (I) and intermediates The present invention relates to processes for the preparation of compounds of formula (I) and intermediates thereof. The groups Q, T, R unless otherwise indicated 1 , R 2 , R 3 , R 4 , R 5, R 6 , R 7 , R 8 , m and n have the meanings given above for the compounds of formula (I). These definitions apply not only to the final product of formula (I), but also to all intermediates.

[0091] Compounds of formulas (I-a) through (I-g) are various subsets of formula (I). Compounds of formulas (I-a-1) through (I-a-8) are various subsets of formula (I-a). All substituents in formulas (I-a) through (I-g) and (I-a-1) through (I-a-8) are as defined above for formula (I) unless otherwise specified.

[0092] Compounds of general formula (I) can be prepared by a variety of routes analogous to known methods (see, eg, and references therein). Non-limiting examples of suitable methods are described herein.

[0093] A compound of formula (I) may be obtained directly by performing methods A or B, or by transformation or derivatization of another compound of formula (I) prepared according to the methods described herein. Obtainable. For example, a compound of formula (I) can be converted to another compound of formula (I) by replacing one or more substituents of the starting compound of formula (I) with another substituent. Non-limiting examples of such transformations or derivatizations are described below (Methods C-H).

[0094] The methods described herein may suitably be carried out using one or more inert organic solvents customary for the reactions under consideration. Suitable inert organic solvents can be selected from: aliphatic, cycloaliphatic or aromatic hydrocarbons (e.g. petroleum ether, pentane, hexane, heptane, cyclohexane, methylcyclohexane, ligroin, benzene, toluene, xylene or decalin), halogenated aliphatic, alicyclic or aromatic hydrocarbons (e.g. chlorobenzene, dichlorobenzene, dichloromethane, chloroform, carbon tetrachloride, 1,2-dichloroethane or trichloroethane), ethers (e.g. diethyl ether, diisopropyl ether, methyl t-butyl ether, methyl t-amyl ether, dioxane, tetrahydrofuran, 2-methyltetrahydrofuran, 1,2-dimethoxyethane, 1,2-diethoxyethane or anisole), ketones (e.g. acetone, methyl ethyl ketone, methyl isopropyl ketone and methyl isobutyl ketone), esters (e.g. methyl acetate, ethyl acetate or butyl acetate), alcohols (e.g. methanol, ethanol, propanol, isopropanol, butanol, tert-butanol), nitriles (e.g. acetonitrile) , propionitrile, n- or i-butyronitrile or benzonitrile), amides (e.g. N,N-dimethylformamide, N,N-dimethylacetamide, N-methylformanilide, N-methylpyrrolidone or hexamethylphosphoric triamide ), sulfoxides (e.g. dimethylsulfoxide) or sulfones (e.g. sulfolane), urea (e.g. 1,3-dimethyl-3,4,5,6-tetrahydro-2(1H)-pyrimidinone) or any thereof a mixture of

[0095] Some methods described herein require or can optionally use one or more inorganic or organic bases commonly used in such reactions. Examples of suitable inorganic and organic bases include, but are not limited to, alkaline earth metal or alkali metal carbonates (such as sodium carbonate, potassium carbonate, potassium bicarbonate, sodium bicarbonate or cesium carbonate), alkali metal hydrides. (e.g. sodium hydride), alkaline earth metals or alkali metal hydroxides (e.g. sodium hydroxide, calcium hydroxide, potassium hydroxide or other ammonium hydroxide derivatives), alkaline earth metals, alkali metals or ammonium Fluorides (e.g. potassium fluoride, cesium fluoride or tetrabutylammonium fluoride), alkali metal or alkaline earth metal acetates (e.g. sodium acetate, lithium acetate, potassium acetate or calcium acetate), alkali metal alcoholates (e.g. potassium tert-butoxide or sodium tert-butoxide), alkali metal phosphates (e.g. tripotassium phosphate), tertiary amines (e.g. trimethylamine, triethylamine, tributylamine, N,N-dimethylaniline, N ,N-dicyclohexylmethylamine, N,N-diisopropylethylamine, N-methylpiperidine, N,N-dimethylaminopyridine, diazabicyclooctane (DABCO), diazabicyclononene (DBN), diazabicycloundecene (DBU ), quinuclidine, 3-acetoxyquinuclidine, guanidine or aromatic bases such as pyridine, picoline, lutidine or collidine.

[0096] Some of the methods described herein are optionally carried out in the presence of a transition metal catalyst such as a salt or complex of a metal (e.g., copper or palladium) and, where appropriate, a ligand. can be done with

[0097] Suitable copper salts or complexes and hydrates thereof include, but are not limited to, copper metal, copper(I) iodide, copper(I) chloride, copper(I) bromide, copper(II) chloride, Copper(II) chloride, Copper(II) oxide, Copper(I) oxide, Copper(II) acetate, Copper(I) acetate, Copper(I) thiophene-2-carboxylate, Copper(I) cyanide, Copper sulfate (II), copper (II) bis(2,2,6,6-tetramethyl-3,5-heptanedionate), copper (II) trifluoromethanesulfonate, tetrakis(acetonitrile) copper (I) hexafluorophosphate, Tetrakis(acetonitrile)copper(I) tetrafluoroborate.

[0098] Copper salts and ethylenediamine, N,N'-dimethylethylenediamine, N,N'-dimethylethylenediamine, rac-trans-1,2-diaminocyclohexane, rac-trans-N,N'-dimethylcyclohexane-1,2- Diamine, 1,1'-binaphthyl-2,2'-diamine, N,N,N',N'-tetramethylethylenediamine, proline, N,N-dimethylglycine, quinolin-8-ol, pyridine, 2-amino pyridine, 4-(dimethylamino)pyridine, 2,2'-bipyridyl, 2,6-di(2-pyridyl)pyridine, 2-picolinic acid, 2-(dimethylaminomethyl)-3-hydroxypyridine, 1,10 -phenanthroline, 3,4,7,8-tetramethyl-1,10-phenanthroline, 2,9-dimethyl-1,10-phenanthroline, 4,7-dimethoxy-1,10-phenanthroline, N,N'-bis [(E)-pyridin-2-ylmethylidene]cyclohexane-1,2-diamine, N-[(E)-phenylmethylidene], N-[(E)-phenylmethylidene]cyclohexanamine, 1,1,1 -tris(hydroxymethyl)ethane, ethylene glycol, 2,2,6,6-tetramethylheptane-3,5-dione, 2-(2,2-dimethylpropanoyl)cyclohexanone, acetylacetone, dibenzoylmethane, 2- (2-methylpropanoyl)cyclohexanone, biphenyl-2-yl(di-tert-butyl)phosphane, ethylenebis-(diphenylphosphine), N,N-diethylsalicylamide, 2-hydroxybenzaldehyde oxime, oxo[(2, Formation of suitable copper complexes in situ in the reaction mixture by separately adding ligands or salts such as 4,6-trimethylphenyl)amino]acetic acid or 1H-pyrrole-2-carboxylic acid to the reaction You can also

[0099] Suitable palladium salts or complexes include, but are not limited to, palladium chloride, palladium acetate, tetrakis(triphenylphosphine)palladium(0), bis(dibenzylideneacetone)palladium(0), tris(dibenzylideneacetone)dipalladium (0), bis(triphenylphosphine) palladium(II) dichloride, [1,1'-bis(diphenylphosphino)ferrocene]dichloropalladium(II), bis(cinnamyl)dichlorodipalladium(II), bis( allyl)-dichlorodipalladium(II) or [1,1′-bis(di-tert-butylphosphino)ferrocene]dichloropalladium(II).

[0100] Palladium salts, triethylphosphine, tri-tert-butylphosphine, tri-tert-butylphosphonium tetrafluoroborate, tricyclohexylphosphine, 2-(dicyclohexylphosphino)biphenyl, 2-(di-tert-butylphosphino)biphenyl , 2-(dicyclohexylphosphino)-2'-(N,N-dimethylamino)biphenyl, 2-(tert-butylphosphino)-2'-(N,N-dimethylamino)biphenyl, 2-di-tert -Butylphosphino-2',4',6'-triisopropylbiphenyl, 2-dicyclohexylphosphino-2',4',6'-triisopropylbiphenyl, 2-dicyclohexylphosphino-2,6'-dimethoxybiphenyl , 2-dicyclohexylphosphino-2',6'-diisopropoxybiphenyl, triphenylphosphine, tris-(o-tolyl)phosphine, sodium 3-(diphenylphosphino)benzenesulfonate, tris-(2-methoxy- Phenyl)phosphine, 2,2'-bis(diphenylphosphino)-1,1'-binaphthyl, 1,4-bis(diphenylphosphino)butane, 1,2-bis(diphenylphosphino)ethane, 1,4 -bis(dicyclohexylphosphino)butane, 1,2-bis(dicyclohexylphosphino)-ethane, 2-(dicyclohexylphosphino)-2'-(N,N-dimethylamino)-biphenyl, 1,1'-bis (Diphenylphosphino)-ferrocene, (R)-(-)-1-[(S)-2-diphenylphosphino)ferrocenyl]ethyldicyclohexylphosphine, tris-(2,4-tert-butyl-phenyl)phosphite , di(1-adamantyl)-2-morpholinophenylphosphine or 1,3-bis(2,4,6-trimethylphenyl)imidazolium chloride, and a ligand or salt, such as, separately added to the reaction. It is also possible to form palladium complexes in the reaction mixture.

[0101] Suitable catalysts and / or ligands can be obtained from commercial catalogs such as Strem Chemicals' Metal Catalysts for Organic Synthesis or from reviews (Chemical Society Reviews (2014), 43, 3525, Coordination Chemistry Reviews (2004), 248, 2337 and citations thereof).

[0102] Some of the methods described herein are described in Nature chemistry review, (2017) 0052 and references therein; Science (2016) 352, 6291, 1304; Org. Lett. 2016, 18, 4012, J. Org. Chem 2016, 81, 6898; J. Am. Chem. Soc. 2016, 138, 12715, J. Am. Chem. Soc. 2016, 138, 13862; J. Am. J. Org. Chem. 2016, 81, 12525, J. Org. Chem. 2015, 80, 7642) by Metallaphotoredox catalysis. The method is then carried out in the presence of photosensitizers such as Ir and Ru complexes or organic dyes, and metal catalysts such as Ni complexes. The reaction can be carried out in the presence of a ligand, if appropriate in the presence of a base, under irradiation with blue or white light.

[0103] Suitable photosensitizers include, but are not limited to, [Ir(dFCF 3 ppy) 2 (bpy)]PF 6 (dFCF 3 ppy=2-(2,4-difluorophenyl)-5-trifluoromethylpyridine, bpy=2,2'-bipyridine), [Ir(dFCF 3 ppy) 2 (dtbbpy)]PF 6 (dtbbpy=4,4'-di-tert-butyl-2,2'-bipyridine), Ir(ppy) 2 (dtbbpy)PF 6 (ppy=2-phenylpyridine), Ir(ppy) 2 (bpy)PF 6 , Ir(dFppy) 3 PF 6 (dFCF 3 ppy=2-(2,4-difluorophenyl)pyridine), fac-Ir(ppy) 3 , (Ir[diF(5-Me)ppy] 2 (tetraMePhen)PF 6 Ir(III) such as (diF(5-Me)ppy=2-(2,4-difluorophenyl)-5-methylpyridine, tetraMePheN=3,4,7,8-tetramethyl-1,10-phenanthroline) Photocatalyst, Ru(bpy) 3 Cl 2 or Ru(bpy) 3 (PF 6 ) 2 or organic dyes such as 9-mesityl-10-acridinium, salts such as perchlorate or tetrafluoroborate, or 2,4,5,6-tetra-9H-carbazole-9- yl-1,3-benzenedicarbonitrile, 9-fluorenone and 9,10-phenanthrenequinone, and the like.

[0104] Suitable nickel catalysts include, but are not limited to, bis(1,5cyclooctadiene)nickel(0), nickel(II) chloride, nickel(II) bromide, in anhydrous or hydrated form or as a dimethoxyetha complex ), nickel (II) iodide such as nickel (II) acetylacetonate and nickel (II) nitrate hexahydrate. These nickel catalysts are 2,2'-bipyridine, 4,4'-di-tert-butyl-2,2'-bipyridine, 4,4'-dimethoxy-2,2'-bipyridine, 4,4'- Dimethyl-2,2'-bipyridine, or phenanthroline such as 1,10-phenanthroline, 4,7-dimethyl-1,10-phenanthroline, 4,7-dimethoxy-1,10-phenanthroline, or N,N,N' It can be used in combination with a ligand such as a diamine such as ,N'-tetramethylethylenediamine or a dione such as tetramethylheptanedione.

[0105] The methods described herein can be carried out at temperatures ranging from -105°C to 250°C, preferably from -78°C to 185°C.

[0106] Reaction times vary as a function of reaction scale and reaction temperature, but are generally between a few minutes and 48 hours.

[0107] The methods described herein are generally carried out under standard pressure. However, it is also possible to work under elevated or reduced pressure.

[0108] In the methods described herein, the starting materials are generally used in approximately equimolar amounts. However, it is also possible to use a relatively excess amount of one of the starting materials.

[0109] Methods for the preparation of compounds of formula (I) Method A Compounds of formula (I-a) (i.e., T is O and R 1 Formula (I)), wherein is defined in Scheme 1, is prepared by a process comprising reacting a compound of Formula (1) with an amine of Formula (2) or one of its salts shown in Scheme 1. can do.

[0110] [formation]

[0111] U 1 A compound of formula (1) wherein is a hydroxyl group can be reacted with an amine of formula (2) in the presence of a condensing reagent by methods described in the literature (e.g. Tetrahedron 2005, 61, 10827-10852). can. Examples of suitable condensing reagents include, but are not limited to, halogenating reagents (e.g., phosgene, phosphorus tribromide, phosphorus trichloride, phosphorus pentachloride, phosphorous trichloride, oxalyl chloride or thionyl chloride), dehydrating reagents ( ethyl chloroformate, methyl chloroformate, isopropyl chloroformate, isobutyl chloroformate or methanesulfonyl chloride), carbodiimides (eg N,N'-dicyclohexylcarbodiimide (DCC)) or other conventional condensation (or peptide coupling) ) reagents (e.g. phosphorus pentoxide, polyphosphoric acid, bis(2-oxo-3-oxazolidinyl)phosphinic acid chloride, 1-[bis(dimethylamino)methylene]-1H-1,2,3-triazolo[4,5 -b]pyridinium 3-oxide hexafluorophosphate (HATU), N,N'-carbonyldiimidazole, 2-ethoxy-N-ethoxycarbonyl-1,2-dihydroquinoline (EEDQ), triphenylphosphine / tetrachloromethane, 4-(4,6-dimethoxy[1.3.5]-triazin-2-yl)-4-methylmorpholinium chloride hydrate, bromo-tripyrrolidinophosphonium hexafluorophosphate or propanephosphonic anhydride (T3P) are mentioned.

[0112] U 1 A compound of formula (1) wherein is a halogen atom can be reacted with an amine of formula (2) in the presence of an acid scavenger by known methods. Suitable acid scavengers include any inorganic and organic bases commonly used in such reactions, as described herein. Preferred are alkali metal carbonates, alkaline earth metal acetates, tertiary amines or aromatic bases.

[0113] U 1 is C 1 -C 6 A compound of formula (1) that is an alkoxy group can be reacted with an excess of an amine of formula (2), optionally in the presence of a Lewis acid such as trimethylaluminum.

[0114] Compounds of formula (1) can be prepared by one or more of the methods described herein (see Methods I, J and K).

[0115] Amines of formula (2) may be commercially available or may be obtained from the literature (e.g. 07629). good too.

[0116] Method B Compounds of formula (I-a-1) (i.e., T is O and R 1 is hydrogen, cyano, hydroxyl, C 1 -C 6 alkyl or C 1 -C 6 is alkoxy and R 7 and R 8 is as defined in Scheme 2) is a compound of formula (3) and a compound of formula (4) in the presence of a base (e.g., an organic or inorganic base) as shown in Scheme 2. It can be produced by a method including the step of reacting with.

[0117] [formation]

[0118] In scheme 2, R e is as disclosed herein, and R 7 , R 8 and R e may be substituted as disclosed herein.

[0119] Method B can be carried out in the presence of a transition metal catalyst such as a copper salt or complex and, if appropriate, in the presence of a ligand.

[0120] Compounds of formula (3) can be prepared by Method L described herein.

[0121] Compounds of formula (4) are either commercially available or can be obtained by transforming or derivatizing another compound of formula (4) according to known methods.

[0122] Method C. Compounds of formula (I-b) (i.e., T is S and R 1 is hydrogen) can be converted to compounds of formula (I-a-2) (i.e., T is O and R 1 is hydrogen) with a thionating agent.

[0123] [formation]

[0124] Suitable thionating agents for carrying out Method C include, but are not limited to, sulfur (S), hydrosulfate (H 2 S), sodium sulfide (Na 2 S), sodium hydrosulfide (NaHS), boron trisulfide (B 2 S. 3 ), bis(diethylaluminum) sulfide ((AlEt 2 ) 2 S), ammonium sulfide ((NH 4 ) 2 S), phosphorus pentasulfide (P) 2 S. 5 ), Lawesson's reagent (2,4-bis(4-methoxyphenyl)-1,2,3,4-dithiadiphosphetane 2,4-disulfide), or Journal of the Chemical Society, Perkin 1 (2001), 358, and polymer-supported thionating reagents.

[0125] The process is optionally carried out in the presence of catalytic or stoichiometric or excess amounts of bases (inorganic and organic bases). Preferably alkali metal carbonates (e.g. sodium carbonate, potassium carbonate, potassium bicarbonate, sodium bicarbonate), heterocyclic aromatic bases (e.g. pyridine, picoline, lutidine, collidine) and tertiary amines (e.g. trimethylamine , triethylamine, tributylamine, N,N-dimethylaniline, N,N-dimethylpyridin-4-amine or N-methyl-piperidine).

[0126] Compounds of formula (I-a-2) can be prepared by one or more methods described herein.

[0127] Process D Compounds of formula (I-c) (i.e., R 1 is -C(=O)R a1 , -C(=O)(OR a1 ) and R a1 Formula (I) as described herein is a compound of Formula (I-a-2) (i.e., T is O and R 1 is hydrogen (i.e., T is S and R 1 is hydrogen) with a compound of formula (5).

[0128] [formation]

[0129] Method D can be performed by methods described in literature (e.g., Tetrahedron Lett. 1995, 36, 8949; Greene's Protective Groups in organic Synthesis; Peter G. M. Wuts; Wiley; Fifth Edition; 2014; 1174-1175).

[0130] Compounds of formula (5) are commercially available.

[0131] Compounds of formula (I-a-2) or (I-b) can be prepared by one or more methods described herein.

[0132] Process E Compounds of formula (I-a-3) (i.e. R 1 is H, T is O, and R 7 is R 7a (I)) can be obtained by one or more steps by methods described in the literature, as shown in Scheme 5, to the corresponding compound (I-a-4) (i.e., as shown in Scheme 5 R. 1 is H, T is O, and R 7 is R 7b (I) or (I-a-5) (i.e., R 1 is H, T is O, and R 7 is R 7c can be converted into formula (I)).

[0133] [formation]

[0134] In scheme 5, R e , R f , R g are as disclosed herein, and aliphatic and cyclic substituents R 7b , R 7c , R e , R f , R g can be substituted as disclosed herein.

[0135] Non-limiting examples of transformations performed according to Scheme 5 are shown below.

[0136] R. 7a Compounds of formula (I-a-3), wherein is a chlorine atom, can be prepared by methods described in the literature (e.g. WO2016185342, WO2007022937). 7b is a bromine or iodine atom.

[0137] R. 7a Compounds of formula (I-a-3), wherein is a halogen atom, can react with R 7b is a hydrogen atom to compounds of formula (I-a-4).

[0138] R. 7aA compound of formula (I-a-3) wherein is a hydrogen atom or a halogen atom can be converted to R 7b is cyano, C 1 -C 6 Alkyl, C 1 -C 6 haloalkyl, C 2 -C 6 alkenyl, C 2 -C 6 haloalkenyl, C 2 -C 6 alkynyl, C 2 -C 6 haloalkynyl, C 1 -C 6 Alkylsulfanyl, C 1 -C 6 haloalkylsulfanyl, C 3 -C 8 Cycloalkyl, C 3 -C 6 cycloalkenyl, aromatic C 6 -C 14 carbocyclic ring, aromatic 5- or 6-membered monocyclic heterocyclic ring, non-aromatic 3- to 7-membered monocyclic heterocyclic ring, -N(R e ) 2 or -C(=O)(OR g ) to compounds of formula (I-a-4).

[0139] R. 7b is C 1 -C 3 C substituted by alkoxy 2 -C 6 Compounds of formula (I-a-4), which are alkenyl groups, can be prepared by methods described in the literature (e.g. J. Org. Chem. 1993, 55, 3114) to form R 7c is C 1 -C 6 It can be converted to a compound of formula (I-a-5) which is an alkylcarbonyl group.

[0140] R. 7c is C 1 -C 6 Compounds of formula (I-a-5), which are alkylcarbonyl groups, can be prepared by methods described in the literature (e.g. Greene's Protective Groups in organic Synthesis; Peter G. M. Wuts; Wiley; Fifth Edition; 2014; 655, 661, 667). R. 7c is -C(=NR f )-C 1 -C 6 It can be further transformed into compounds of formula (I-a-5) which are alkyl groups.

[0141] R. 7c is C 1 -C 6 A compound of formula (I-a-5), which is an alkylcarbonyl group, can be converted to NaBH 4 Classical functional group interconversions such as the reduction of ketones to alcohols in the presence of R 7c is C 1 -C 6 It can be further transformed into compounds of formula (I-a-5) which are hydroxyalkyl groups.

[0142] R. 7c is C 1 -C 6 A compound of formula (I-a-5), which is a hydroxyalkyl group, is treated with R 7c is C 1 -C 6 It can be further transformed into compound (I-a-5) which is -fluoroalkyl. Non-limiting examples of fluorinating agents include sulfur tetrafluoride, diethylaminosulfur trifluoride, morpholino sulfur trifluoride, bis(2-methoxyethyl)aminosulfur trifluoride, 2,2-difluoro-1, sulfur fluorides such as 3-dimethylimidazolidine or 4-tert-butyl-2,6-dimethylphenyl sulfur trifluoride;

[0143] Compounds of formula (I-a-3) can be prepared by one or more methods described herein.

[0144] Method F. Compounds of formula (I-a-6) (i.e., R 1 is H, T is O, and R 7 is a halogen and R 8 is hydrogen) can be converted in one or more steps by methods described in the literature to the corresponding compound of formula (I-a-7) (i.e., R 1 is H, T is O, and R 7 is a halogen and R 8 is R shown in Scheme 6 8a (i.e., R 1 is H, T is O, and R 7 is a halogen and R 8 is R shown in Scheme 6 8b can be converted into formula (I)).

[0145] [formation]

[0146] In scheme 6, R h and R i are as disclosed herein, and the aliphatic and cyclic substituents R 8a and R 8b can be substituted as disclosed herein.

[0147] Non-limiting examples of transformations performed according to Scheme 6 are shown below.

[0148] Compounds of formula (I-a-6) can be converted to bases and electrophiles such as NCS, NBS, NIS, hexachloroethane, bromine or iodine by methods described in the literature (e.g. Org.Lett. 2009, 11, 1837). in the presence of R 8a is a halogen atom to compounds of formula (I-a-7). Suitable bases for carrying out this method are lithium-diisopropylamide, lithium 2,2,6,6-tetramethylpiperidide, n-butyllithium, methyllithium, TMPZnCl.LiCl(2,2,6,6 -tetramethylpiperidinylzinc chloride-lithium chloride complex), TMP 2 Zn 2MgCl 2 2LiCl (bis(2,2,6,6-tetramethylpiperidinyl)magnesium chloride-lithium chloride complex), see for example Dissertation Albrecht Metzer 2010 by the University of Munich.

[0149] Compounds of formula (I-a-6) can be prepared as described herein or by methods described in the literature (Heterocycles 1976, 4(8), 1331) optionally in the presence of a base. In the presence of a transition metal catalyst and ligand, such as a metal salt or complex, R 8a is C 1 -C 6 Alkyl, C 1 -C 6 haloalkyl, C 1 -C 6 hydroxyalkyl, C 3 -C 8 Cycloalkyl, C 3 -C 8 halocycloalkyl, C 3 -C 6 cycloalkenyl, aromatic C 6 -C 14 It can be converted to a compound of formula (I-a-7) which is a carbocyclic ring, a 5- to 14-membered aromatic heterocyclic ring, or a 3- to 14-membered non-aromatic heterocyclic ring.

[0150] R. 8a is a halogen atom, in the presence of a base, optionally in the presence of a transition metal catalyst such as a metal salt or complex, and if appropriate in the presence of a ligand , R 8b are cyano, nitro, amino, mercapto, hydroxyl, C 2 -C 6 alkenyl, C 2 -C 6 haloalkenyl, C 2 -C 6 alkynyl, C 2 -C 6 haloalkynyl, C 1 -C 6 Alkoxy, C 1 -C 6 haloalkoxy, C 2 -C 6 alkenyloxy, C 2 -C 6 haloalkenyloxy, C 3 -C 8 Cycloalkyl, C 3 -C 6 cycloalkenyl, aromatic 5-14 membered heterocycle, C 3 -C 8 cycloalkyloxy, aromatic C 6 -C 14 carbocyclyloxy, non-aromatic 3-14 membered heterocyclyloxy, aromatic 5-14 membered heterocyclyloxy, -N(R h ) 2 or S.R. i can be converted to a compound of formula (I-a-8) representing

[0151] R. 8b is C 2 -C 6A compound of formula (I-a-8) that is an alkenyl group can be converted to R 8b but C 1 -C 6 Alkoxy, C 1 -C 6 haloalkoxy, C 1 -C 6 Alkoxy-C 1 -C 6 Alkoxy, C 1 -C 6 Alkylsulfanyl, C 1 -C 6 haloalkylsulfanyl, non-aromatic 3- to 7-membered monocyclic heterocycle, and Ra’ is independently hydrogen, C 1 -C 6 Alkyl, C 1 -C 6 haloalkyl and C 3 -C 8 -N(Ra') independently selected from the group consisting of cycloalkyl 2 is further converted to a compound of formula (I-a-8) substituted with

[0152] R. 8b is SR i The compound of formula (I-a-8), which is a group, can be converted to R by reacting the starting compound of formula (I-a-8) with an oxidizing agent such as hydrogen peroxide 8b is -S(=O)R i or -S(=O) 2 R. i It can be further transformed into compounds of formula (I-a-8) which are radicals.

[0153] Compounds of formula (I-a-6) can be prepared by one or more methods described herein.

[0154] Method G. Compounds of formula (I-d) (i.e., R 6S is a halogen compound of formula (I)) or formula (6) is reacted with a compound of formula (7) as shown in Scheme 7 to give a compound of formula (I-e) (i.e., R 6S is as shown in Scheme 7, formula (I)) can be obtained.

[0155] [formation]

[0156] In Scheme 7, aliphatic and cyclic R 6S Substituents may be substituted as disclosed herein.

[0157] Method G can be performed by metal catalysis as described herein.

[0158] Alternatively, Method G can be performed by Metallophotoredox catalysis. More specifically, G 1 Compounds of formula (I-d) wherein is preferably Br or I are carried out in the presence of photosensitizers such as Ir and Ru complexes or organic dyes and metal catalysts such as Ni complexes. The reaction can be carried out in the presence of a ligand, if appropriate in the presence of a base, under irradiation with blue or white light.

[0159] Compounds of formula (I-d) can be prepared by one or more of the methods described herein.

[0160] Compounds of formula (6) can be prepared by known methods.

[0161] Compounds of formula (7) are commercially available.

[0162] Process H Compounds of formula (I-f) (i.e., Q S is a halogen) or a compound of Formula 8 is reacted with a compound of Formula 9 as shown in Scheme 8 to give a compound of Formula (I-g) (i.e., Q S is as shown in Scheme 8). [formation]

[0163] In Scheme 8, aliphatic and cyclic Q S Substituents may be substituted as disclosed herein.

[0164] Method H can be performed by transition metal catalysis.

[0165] Alternatively, Method H can be performed by Metallophotoredox catalysis. More specifically, G 1 Compounds of formula (I-f) where is preferably Br or I are carried out in the presence of photosensitizers such as Ir and Ru complexes or organic dyes, and metal catalysts such as Ni complexes. The reaction can be carried out in the presence of a ligand, if appropriate in the presence of a base, under irradiation with blue or white light.

[0166] Compounds of formula (I-f) can be prepared by one or more of the methods described herein.

[0167] Compounds of formula (8) can be prepared by known methods.

[0168] Compounds of formula (9) are commercially available.

[0169] Process for producing compounds of formula (1) Compounds of formula (1) are obtained directly by performing Method I below or by transformation or derivatization of another compound of formula (1) prepared according to the methods described herein. be able to. Compounds of formulas (1-a) through (1-h) are various subsets of formula (1).

[0170] Method I Compounds of formula (1-a) (i.e., R 7 and R 8 is as defined in Scheme 9) by a method comprising reacting a compound of Formula (10) with a reagent of Formula (4) in the presence of a base, as shown in Scheme 9. can be manufactured. [formation]

[0171] In scheme 9, R e is as disclosed herein, and R 7 , R 8 and R e can be substituted as disclosed herein.

[0172] Method I can be carried out in the presence of a suitable transition metal catalyst salt or complex and, if appropriate, in the presence of a ligand.

[0173] The resulting compound of formula (1-a) can then be converted to a compound of formula (1-b) in one or more steps.

[0174] Non-limiting examples of such transformations are described below.

[0175] U 1 is C 1 -C 6 Compounds of formula (1-a) that are alkoxy can be converted to U 2 is a hydroxyl group to compounds of formula (1-b).

[0176] U 2 A compound of formula (1-b) wherein is hydroxyl can be converted to U in the presence of a halogenating agent by known methods. 2 is halogen. Suitable halogenating reagents include, but are not limited to, phosphorus tribromide, phosphorus trichloride, phosphorus pentachloride, phosphorous trichloride, oxalyl chloride or thionyl chloride.

[0177] Compounds of formula (10) are commercially available or can be prepared by Method M described herein.

[0178] Compounds of formula (4) are commercially available or can be obtained by transforming or derivatizing another compound of formula (4) according to known methods.

[0179] Method J. Compounds of formula (1-c) (i.e., R 7 is defined in Scheme 10 for R 7a (1)) can be converted to the corresponding compound of formula (1-d) (i.e., R 7 is R defined in Scheme 10 7b A compound of formula (1) or (1-e) (i.e., R 7 is R defined in Scheme 10 7c can be converted into the following equation (1).

[0180] [formation]

[0181] In scheme 10, R e , R f , R g are as disclosed herein, and aliphatic and cyclic substituents R 7b , R 7c , R e , R f , R g can be substituted as disclosed herein.

[0182] Non-limiting examples of transformations can be performed according to the description provided in Method E.

[0183] U 1 is C 1 -C 6 Alkoxy compounds of formulas (1-c), (1-d) and (1-e) can be converted to U 1 is a hydroxyl group to compounds of formulas (1-c), (1-d) and (1-e). For example, by hydrolysis of the ester group with LiOH in THF / water.

[0184] U 1 Compounds of formulas (1-c), (1-d) and (1-e) where is hydroxyl can be converted to U in the presence of a halogenating agent using known methods. 1 can be further transformed into compounds of formulas (1-c), (1-d), (1-e) where is halogen. Suitable halogenating reagents include, but are not limited to, phosphorus tribromide, phosphorus trichloride, phosphorus pentachloride, phosphorous trichloride, oxalyl chloride or thionyl chloride.

[0185] Compounds of formula (1-c) can be prepared by one or more methods described herein.

[0186] Method K. Compounds of formula (1-f) (i.e., R 8 is H) can be converted to the corresponding compound of formula (1-g) (i.e., R 8 is R defined in Scheme 11 8a (i.e., R 8 is R defined in Scheme 11 8b can be converted into the following equation (1).

[0187] [formation]

[0188] In scheme 11, R h and R i are as disclosed herein, and aliphatic and cyclic substituents R 8a and R 8b can be substituted as disclosed herein.

[0189] Non-limiting examples of transformations can be performed according to the description provided in Method F.

[0190] U 1 is C 1 -C 6 Compounds of formulas (1-f), (1-g), (1-h) that are alkoxy can be converted to U 1 is a hydroxyl group to compounds of formulas (1-f), (1-g) and (1-h).

[0191] U 1 Compounds of formulas (1-f), (1-g), and (1-h), wherein is hydroxyl, can be converted to U in the presence of a halogenating agent using known methods. 1 can be further transformed to compounds of formulas (1-f), (1-g), (1-h) where is halogen. Suitable halogenating reagents include, but are not limited to, phosphorus tribromide, phosphorus trichloride, phosphorus pentachloride, phosphorous trichloride, oxalyl chloride or thionyl chloride.

[0192] Compound (1-f) can be prepared by one or more of the methods described herein.

[0193] Process for producing compounds of formula (3) Method L Compounds of formula (3) can be prepared by a process comprising reacting a compound of formula (10) with an amine of formula (2) or one of its salts, as shown in Scheme 12.

[0194] [formation]

[0195] Method L can be performed using the same conditions as Method A.

[0196] Compounds of formula (10) are commercially available or can be obtained by Method M.

[0197] Process for producing compounds of formula (10) Method M. Compounds of formula (10-a) (i.e., R 7 is a halogen) can be obtained by known methods (WO2000044755) of nucleophiles based on oxygen (ethanol), sulfur (thioethyl) or amino (methylamine) as shown in Scheme 13. In the presence of any, optionally in the presence of a base, compounds of formula (10-b) (i.e., R 7 can be converted to compounds of formula 10 as shown in scheme 13). [formation]

[0198] Compounds of formulas (10-a) and (10-b) can be prepared using conditions similar to those described in Method K. 1 (C 1 -C 6 alkoxy) can be converted to compounds of formula (10-a) and (10-b) substituted with hydroxyl or halogen.

[0199] Starting materials of formula (10-a) are commercially available.

[0200] The compounds of the invention can be prepared according to the methods described above. Nevertheless, the person skilled in the art understands that he can, based on his general knowledge and available publications, adapt these methods according to the specifics of each of the compounds of the invention that he wishes to synthesize. be done.

[0201] Compound (B) The active compound combinations according to the invention comprise, as compound (B), at least one further active compound selected from the group (1) inhibitors of ergosterol synthesis, (2) inhibitors of the respiratory chain at complex I or II, (3) inhibitors of the respiratory chain at complex III, (4) inhibitors of mitosis and cell division; (5) compounds with multisite action, (6) compounds capable of inducing host defenses; (7) inhibitors of amino acid and / or protein biosynthesis; (8) inhibitors of ATP production; (9) inhibitors of cell wall synthesis; (10) inhibitors of lipid and membrane synthesis, (11) inhibitors of melanin biosynthesis, (12) inhibitors of nucleic acid synthesis; (13) signaling inhibitors; (14) compounds capable of acting as uncouplers; (15) (15.001) abscisic acid, (15.002) benzazole, (15.003) betoxazine, (15.004) capcimycin, (15.005) carvone, (15.006) quinomethionate, (15.007) cufraneb, (15.008) cyflufenamide, (15.009) cymoxanil, (15.010) cyprosulfamide, (15.011) flutianil, (15.012) fosetyl-aluminum, (15.013) fosetyl-calcium, (15.014) fosetyl-sodium, (15.015) methyl isothiocyanate, (15.016) metrafenone, (15.017) milli Diomycin, (15.018) Natamycin, (15.019) Nickel Dimethyldithiocarbamate, (15.020) Nitrotar Isopropyl, (15.021) Oxamocarb, (15.022) Oxathiapiproline, (15.023) Oxyphenthine, (15.024) Pentachlorophenol and Its salts, (15.025) phosphorous acid and its salts, (15.026) propamocarb-fosetylate, (15.027) pyriophenone (clazaphenone), (15.028) tebufuroquine, (15.029) tecloftalam, (15.030) tolnifanide, (15.031) 1-(4) -{4-[(5R)-5-(2,6-difluorophenyl)-4,5-dihydro-1,2-oxazol-3-yl]-1,3-thiazol-2-yl}piperidine-1 -yl)-2-[5-methyl-3-(trifluoromethyl)-1H-pyrazol-1-yl]ethanone, (15.032)1-(4-{4-[(5S)-5-(2, 6-difluorophenyl)-4,5-dihydro-1,2-oxazol-3-yl]-1,3-thiazol-2-yl}piperidin-1-yl)-2-[5-methyl-3-( Trifluoromethyl)-1H-pyrazol-1-yl]ethanone, (15.033) 2-(6-benzylpyridin-2-yl)quinazoline, (15.034) dipimethitrone, (15.035) 2-[3,5-bis(difluoro Methyl)-1H-pyrazol-1-yl]-1-[4-(4-{5-[2-(prop-2-yn-1-yloxy)phenyl]-4,5-dihydro-1,2- Oxazol-3-yl}-1,3-thiazol-2-yl)piperidin-1-yl]ethanone, (15.036)2-[3,5-bis(difluoromethyl)-1H-pyrazol-1-yl]- 1-[4-(4-{5-[2-chloro-6-(prop-2-yn-1-yloxy)phenyl]-4,5-dihydro-1,2-oxazol-3-yl}-1 ,3-thiazol-2-yl)piperidin-1-yl]ethanone, (15.037)2-[3,5-bis(difluoromethyl)-1H-pyrazol-1-yl]-1-[4-(4- {5-[2-fluoro-6-(prop-2-yn-1-yloxy)phenyl]-4,5-dihydro-1,2-oxazol-3-yl}-1,3-thiazol-2-yl )piperidin-1-yl]ethanone, (15.038)2-[6-(3-fluoro-4-methoxyphenyl) -5-methylpyridin-2-yl]quinazoline, (15.039)2-{(5R)-3-[2-(1-{[3,5-bis(difluoromethyl)-1H-pyrazol-1-yl] Acetyl}piperidin-4-yl)-1,3-thiazol-4-yl]-4,5-dihydro-1,2-oxazol-5-yl}-3-chlorophenyl methanesulfonate, (15.040)2-{( 5S)-3-[2-(1-{[3,5-bis(difluoromethyl)-1H-pyrazol-1-yl]acetyl}piperidin-4-yl)-1,3-thiazol-4-yl] -4,5-dihydro-1,2-oxazol-5-yl}-3-chlorophenyl methanesulfonate, (15.041) ipflufenoquine, (15.042) 2-{2-fluoro-6-[(8-fluoro- 2-methylquinolin-3-yl)oxy]phenyl}propan-2-ol, (15.043) fluoxapiproline, (15.044) 2-{3-[2-(1-{[3,5-bis(difluoro Methyl)-1H-pyrazol-1-yl]acetyl}piperidin-4-yl)-1,3-thiazol-4-yl]-4,5-dihydro-1,2-oxazol-5-yl}phenyl methanesulfonate , (15.045) 2-phenylphenol and its salts, (15.046) 3-(4,4,5-trifluoro-3,3-dimethyl-3,4-dihydroisoquinolin-1-yl)quinoline, (15.047) quinofumeline , (15.048) 4-amino-5-fluoropyrimidin-2-ol (tautomer: 4-amino-5-fluoropyrimidin-2(1H)-one), (15.049) 4-oxo-4-[( 2-phenylethyl)amino]butanoic acid, (15.050) 5-amino-1,3,4-thiadiazol-2-thiol, (15.051) 5-chloro-N'-phenyl-N'-(prop-2-yne -1-yl)thiophene-2-sulfonohydrazide, (15.052)5-fluoro-2-[(4-fluorobenzyl)oxy]pyrimidin-4-amine, (15.053)5-fluoro-2-[(4- methylbenzyl)oxy]pyrimidin-4-amine, (15.054)9-fluoro-2,2-dimethyl-5-(quinolin-3-yl)-2,3-dihydro-1,4-benzoxazepine, ( 15.055) {6-[({[(Z)-(1-methyl-1H-tetrazol-5-yl)(phenyl)methylene]amino}oxy)methyl]pyridin-2-yl}carbamate but-3-yne -1-yl, (15.056) (2Z)-3-amino-2-cyano-3-phenylacrylate ethyl, (15.057) phenazine-1-carboxylic acid, (15.058) 3,4,5-trihydroxybenzoic acid propyl, (15.059) quinolin-8-ol, (15.060) quinolin-8-ol sulfate (2:1), (15.061) {6-[({[(1-methyl-1H-tetrazol-5-yl)( tert-butyl phenyl)methylene]amino}oxy)methyl]pyridin-2-yl}carbamate, (15.062)5-fluoro-4-imino-3-methyl-1-[(4-methylphenyl)sulfonyl]-3 ,4-dihydropyrimidin-2(1H)-one, (15.063) aminopyrifene, (15.064) (N'-[2-chloro-4-(2-fluorophenoxy)-5-methylphenyl]-N-ethyl -N-methylimidoformamide), (15.065)(N'-(2-chloro-5-methyl-4-phenoxyphenyl)-N-ethyl-N-methylimidoformamide), (15.066)(2-{2- [(7,8-difluoro-2-methylquinolin-3-yl)oxy]-6-fluorophenyl}propan-2-ol), (15.067)(5-bromo-1-(5,6-dimethylpyridine- 3-yl)-3,3-dimethyl-3,4-dihydroisoquinoline), (15.068)(3-(4, 4-difluoro-5,5-dimethyl-4,5-dihydrothieno[2,3-c]pyridin-7-yl)quinoline), (15.069)(1-(4,5-dimethyl-1H-benzimidazole-1 -yl)-4,4-difluoro-3,3-dimethyl-3,4-dihydroisoquinoline), (15.070)8-fluoro-3-(5-fluoro-3,3-dimethyl-3,4-dihydroisoquinoline) -1-yl)quinolone, (15.071)8-fluoro-3-(5-fluoro-3,3,4,4-tetramethyl-3,4-dihydroisoquinolin-1-yl)quinolone, (15.072)3- (4,4-difluoro-3,3-dimethyl-3,4-dihydroisoquinolin-1-yl)-8-fluoroquinoline, (15.073)(N-methyl-N-phenyl-4-[5-(trifluoro methyl)-1,2,4-oxadiazol-3-yl]benzamide), (15.074){4-[5-(trifluoromethyl)-1,2,4-oxadiazol-3-yl]phenyl}methyl carbamate, (15.075)(N-{4-[5-(trifluoromethyl)-1,2,4-oxadiazol-3-yl]benzyl}cyclopropanecarboxamide), (15.076)N-methyl -4-(5-(trifluoromethyl)-1,2,4-oxadiazol-3-yl]benzamide,(15.077)N-[(E)-methoxyiminomethyl]-4-[5-(trifluoromethyl) fluoromethyl)-1,2,4-oxadiazol-3-yl]benzamide, (15.078)N-[(Z)-methoxyiminomethyl]-4-[5-(trifluoromethyl)-1,2, 4-oxadiazol-3-yl]benzamide, (15.079)N-[4-[5-(trifluoromethyl)-1,2,4-oxadiazol-3-yl]phenyl]cyclopropanecarboxamide, ( 15.080) N-(2-fluorophenyl)-4-[5-(trifluoromethyl)-1,2,4-oxadiazol-3-yl]benzamide, (15.081) 2,2-difluoro-N-methyl -2-[4-[5-(trifluoromethyl)-1,2,4-oxadiazol-3-yl]phenyl]acetamide, (15.082)N-allyl-N-[[4-[5-( Trifluoromethyl)-1,2,4-oxadiazol-3-yl)phenyl]methyl]acetamide, (15.083)N-[(E)-N-methoxy-C-methyl-carbonimidoyl]-4- (5-(Trifluoromethyl)-1,2,4-oxadiazol-3-yl]benzamide, (15.084)N-[(Z)-N-methoxy-C-methyl-carbonimidoyl]-4- [5-(trifluoromethyl)-1,2,4-oxadiazol-3-yl]benzamide, (15.085)N-allyl-N-[[4-[5-(trifluoromethyl)-1,2 ,4-oxadiazol-3-yl]phenyl]methyl]propanamide, (15.086)4, 4-dimethyl-1-[[4-[5-(trifluoromethyl)-1,2,4-oxadiazol-3-yl]phenyl]methyl]pyrrolidin-2-one, (15.087)N-methyl- 4-[5-(trifluoromethyl)-1,2,4-oxadiazol-3-yl]benzenecarbothioamide, (15.088)5-methyl-1-[[4-[5-(trifluoromethyl) -1,2,4-oxadiazol-3-yl]phenyl]methyl]pyrrolidin-2-one, (15.089)N-((2,3-difluoro-4-[5-(trifluoromethyl)-1 ,2,4-oxadiazol-3-yl]phenyl]methyl]-3,3,3-trifluoro-propanamide, (15.090)1-methoxy-1-methyl-3-[[4-[5- (Trifluoromethyl)-1,2,4-oxadiazol-3-yl]phenyl]methyl]urea, (15.091)1,1-diethyl-3-[[4-[5-(trifluoromethyl)- 1,2,4-oxadiazol-3-yl]phenyl]methyl]urea, (15.092)N-[[4-[5-(trifluoromethyl)-1,2,4-oxadiazole-3- yl]phenyl]methyl]propanamide, (15.093)N-methoxy-N-[[4-[5-(trifluoromethyl)-1,2,4-oxadiazol-3-yl]phenyl]methyl]cyclo Propanecarboxamide, (15.094) 1-methoxy-3-methyl-1-[[4-[5-(trifluoromethyl)-1,2,4-oxadiazol-3-yl]phenyl]methyl]urea, ( 15.095) N-methoxy-N-[[4-[5-(trifluoromethyl)-1,2,4-oxadiazol-3-yl]phenyl]methyl)cyclopropanecarboxamide, (15.096)N,2- Dimethoxy-N-[[4-[5-(trifluoromethyl)-1,2,4-oxadiazol-3-yl]phenyl]methyl]propanamide, (15.097)N-ethyl-2-methyl-N -[[4-[5-(trifluoromethyl)-1,2,4-oxadiazol-3-yl)phenyl]methyl]propanamide, (15.098)1-methoxy-3-methyl-1-[[ 4-[5-(trifluoromethyl)-1,2,4-oxadiazol-3-yl]phenyl]methyl]urea, (15.099)1,3-dimethoxy-1-[[4-[5-( Trifluoromethyl)-1,2,4-oxadiazol-3-yl]phenyl]methyl]urea, (15.100)3-ethyl-1-methoxy-1-[[4-[5-(trifluoromethyl) -1,2,4-oxadiazol-3-yl]phenyl]methyl]urea, (15.101)1-[[4-[5-(trifluoromethyl)-1,2,4-oxadiazole-3 -yl]phenyl]methyl]piperidin-2-one, (15.102)4,4-dimethyl-2-[[4-[5-(trifluoromethyl)-1,2,4-oxadiazol-3-yl ]]phenyl]methyl]isoxazolidin-3-one, (15.103)5,5-dimethyl-2-[[4-[5-(trifluoromethyl)-1,2,4-oxadiazol-3-yl ]Phenyl]methyl]isoxazolidin-3-one, (15.104)3,3-dimethyl-1-[[4-[5-(trifluoromethyl)-1,2,4-oxadiazol-3-yl] Phenyl]methyl]piperidin-2-one, (15.105)1-[[3-fluoro-4-(5-(trifluoromethyl)-1,2,4-oxadiazol-3-yl]phenyl]methyl] Azepan-2-one, (15.106)4,4-dimethyl-2-[[4-(5-(trifluoromethyl)-1,2,4-oxadiazol-3-yl]phenyl]methyl]isoxazolidine -3-one, (15.107)5,5-dimethyl- 2-[[4-[5-(trifluoromethyl)-1,2,4-oxadiazol-3-yl]phenyl]methyl]isoxazolidin-3-one, (15.108)1-{4-[5 Ethyl -(trifluoromethyl)-1,2,4-oxadiazol-3-yl]benzyl}-1H-pyrazole-4-carboxylate, (15.109)N,N-dimethyl-1-{4-[5 -(trifluoromethyl)-1,2,4-oxadiazol-3-yl]benzyl}-1H-1,2,4-triazol-3-amine, (15.110)N-{2,3-difluoro- 4-[5-(trifluoromethyl)-1,2,4-oxadiazol-3-yl]benzyl}butanamide, (15.111)N-(1-methylcyclopropyl)-4-[5-(trifluoro Methyl)-1,2,4-oxadiazol-3-yl]benzamide, (15.112)N-(2,4-difluorophenyl)-4-[5-(trifluoromethyl)-1,2,4- Oxadiazol-3-yl]benzamide, (15.113) 1-(5,6-dimethylpyridin-3-yl)-4,4-difluoro-3,3-dimethyl-3,4-dihydroisoquinoline, (15.114) 1-(6-(difluoromethyl)-5-methyl-pyridin-3-yl)-4,4-difluoro-3,3-dimethyl-3,4-dihydroisoquinoline, (15.115)1-(5-(fluoro Methyl)-6-methyl-pyridin-3-yl)-4,4-difluoro-3,3-dimethyl-3,4-dihydroisoquinoline, (15.116)1-(6-(difluoromethyl)-5-methoxy- Pyridin-3-yl)-4,4-difluoro-3,3-dimethyl-3,4-dihydroisoquinoline, (15.117)4-[5-(trifluoromethyl)-1,2,4-oxadiazole- 3-yl]phenyldimethylcarbamate, (15.118)N-{4-[5-(trifluoromethyl)-1,2,4-oxadiazol-3-yl]phenyl}propanamide, (15.119)3 -[2-(1-{[5-methyl-3-(trifluoromethyl)-1H-pyrazol-1-yl]acetyl}piperidin-4-yl)-1,3-thiazol-4-yl]-1 ,5-dihydro-2,4-benzodioxepin-6-yl methanesulfonate, (15.120)9-fluoro-3-[2-(1-{[5-methyl-3-(trifluoromethyl) -1H-pyrazol-1-yl]acetyl}piperidin-4-yl)-1,3-thiazol-4-yl]-1,5-dihydro-2,4-benzodioxepin-6-yl methanesulfonic acid salt, (15.121)3-[2-(1-{[3,5-bis(difluoromethyl)-1H-pyrazol-1-yl]acetyl}piperidin-4-yl)-1,3-thiazol-4- yl]-1,5-dihydro-2,4-benzodioxepin-6-yl methanesulfonate, (15.122)3-[2-(1-{[3,5-bis(difluoromethyl)-1H -pyrazol-1-yl]acetyl}piperidin-4-yl)-1,3-thiazol-4-yl]-9-fluoro-1,5-dihydro-2,4-benzodioxepin-6-ylmethane sulfonate, (15.123) 1-(6,7-dimethylpyrazolo[1,5-a]pyridin-3-yl)-4,4-difluoro-3,3-dimethyl-3,4-dihydroisoquinoline, (15.124)8-fluoro-N-(4,4,4-trifluoro-2-methyl-1-phenylbutan-2-yl)quinoline-3-carboxamide, (15.125)8-fluoro-N-[(2S )-4,4,4-trifluoro-2-methyl-1-phenylbutan-2-yl]quinolin-3-carboxamide, (15.126)N-(2,4-dimethyl-1-phenylpentan-2-yl )-8-fluoroquinoline-3-carboxamide and (15.127)N-[(2S)-2,4-dimethyl-1-phenylpentan-2-yl]-8-fluoroquinoline-3-carboxamide other fungicides, (16) (16.001) Bacillus subtilis, particularly strain QST713 / AQ713 (having NRRL accession number B21661, described in US Pat. No. 7,094,592, SERENADE OPTI from Bayer CropScience LP, USA); (16.002) Bacillus amyloliquefaciens, particularly strain D747 (having accession number FERM BP-8234, described in U.S. Pat. No. 7,094,592; (16.003) Bacillus pumilus, especially strain BU F-33 (with NRRL accession number 50185); (16.004) Bacillus subtilis subspecies amylo Bacillus subtilis var. amyloliquefaciens strain FZB24 (available as Taegro® from Novozymes, USA); (16.005) having accession number NRRL B-50972 or accession number NRRL B-67129; Strains of Paenibacillus species as described in International Patent Publication No. WO2016 / 154297; and Fungi, such as (16.006) Aureobasidium pullulans, especially spores of strain DSM 14940; (16.007) spores of Aureobasidium pullulans, strain DSM 14941; (16.008) Aureobasidium pullulans, especially an antibacterial agent selected from the group of bacteria such as a mixture of spores of strains DSM14940 and DSM14941; (17) Bacteria such as (17.001) Bacillus subtilis, particularly strain QST713 / AQ713 (having accession number B21661 of NRRL, described in US Pat. No. 6,060,051, SERENADE OPTI from Bayer CropScience LP, USA) (17.002) Bacillus pumilus, particularly strain QST2808 (with accession number NRRL B-30087, described in US Pat. No. 6,245,551, SONATA from Bayer CropScience LP, USA); (17.003) Bacillus pumilus, especially strain GB34 (available as Yield Shield® from Bayer AG, Germany); (17.004) Bacillus pumilus, especially strain BU F-33 ( (17.005) Bacillus amyloliquefaciens, particularly strain D747 (having accession number FERM BP-8234, described in US Pat. No. 7,094,592, Certis, USA); (17.006) Bacillus subtilis Y1336 (registered as a biofungicide in Taiwan under registration numbers 4764, 5454, 5096 and 5277; BIOBAC® from Bion-Tech, Taiwan); (17.007) Bacillus amyloliquefaciens strain MBI 600 (available as SUBTILEX from BASF SE); (17.008) Bacillus subtilis strain GB03 (Kodiak® from Bayer AG, Germany); )); (17.009) Bacillus subtilis subsp. amyloliquefaciens strain FZB24 (as the fungicide TAEGRO® or TAEGRO® (EPA registration number 70127-5), Novozymes Biologicals, Salem, Virginia); Inc. or Syngenta Crop Protection, LLC, Greensboro, NC); (17.010) Bacillus mycoides isolate J (available as BmJ TGAI or WG from Certis, USA); (17.011) Bacillus licheniformis, particularly strain SB3086 (available from Novozymes as EcoGuard™ Biofungicide and Green Releaf); (17.012) having accession number NRRL B-50972 or accession number NRRL B-67129; A biological fungicide selected from the group of Paenibacillus sp. strains described in International Patent Publication No. WO2016 / 154297: (18) Fatty acids or derivatives such as (18.001) unsaturated and saturated C 12 -C 24 A composition comprising one or more fatty acids or derivatives thereof selected from fatty acids, salts thereof, esters thereof or mixtures of any of the foregoing, wherein at least 95% of said fatty acids or derivatives thereof is C 14 -C 20 (eg FLiPPER from AlphaBio Pesticides or Bayer AG).

[0202] Compound (B) is preferably (1.001) cyproconazole, (1.002) difenoconazole, (1.003) epoxiconazole, (1.004) fenhexamide, (1.005) fenpropidine, (1.006) fenpropimorph, (1.007) fenpyrazamine, (1.008) fluquinco Nazol, (1.009) flutriafol, (1.010) imazalil, (1.011) imazalil sulfate, (1.012) ipconazole, (1.013) metconazole, (1.014) microbutanil, (1.015) paclobutrazole, (1.016) prochloraz, (1.017) ) propiconazole, (1.018) prothioconazole, (1.019) pyrisoxazole, (1.020) spiroxamine, (1.021) tebuconazole, (1.022) tetraconazole, (1.023) triadimenol, (1.024) tridemorph, (1.025) tri Ticonazole, (1.026)(1R,2S,5S)-5-(4-chlorobenzyl)-2-(chloromethyl)-2-methyl-1-(1H-1,2,4-triazol-1-ylmethyl ) cyclopentanol, (1.027) (1S,2R,5R)-5-(4-chlorobenzyl)-2-(chloromethyl)-2-methyl-1-(1H-1,2,4-triazole-1 -ylmethyl)cyclopentanol, (1.028)(2R)-2-(1-chlorocyclopropyl)-4-[(1R)-2,2-dichlorocyclopropyl]-1-(1H-1,2,4 -triazol-1-yl)butan-2-ol, (1.029)(2R)-2-(1-chlorocyclopropyl)-4-[(1S)-2,2-dichlorocyclopropyl]-1-(1H -1,2,4-triazol-1-yl)butan-2-ol, (1.030)(2R)-2-[4-(4-chlorophenoxy)-2-(trifluoromethyl)phenyl]-1- (1H-1, 2,4-triazol-1-yl)propan-2-ol, (1.031)(2S)-2-(1-chlorocyclopropyl)-4-[(1R)-2,2-dichlorocyclopropyl]-1 -(1H-1,2,4-triazol-1-yl)butan-2-ol, (1.032)(2S)-2-(1-chlorocyclopropyl)-4-[(1S)-2,2- Dichlorocyclopropyl]-1-(1H-1,2,4-triazol-1-yl)butan-2-ol, (1.033)(2S)-2-[4-(4-chlorophenoxy)-2-( Trifluoromethyl)phenyl]-1-(1H-1,2,4-triazol-1-yl)propan-2-ol, (1.034)(R)-[3-(4-chloro-2-fluorophenyl) -5-(2,4-difluorophenyl)-1,2-oxazol-4-yl](pyridin-3-yl)methanol, (1.035)(S)-[3-(4-chloro-2-fluorophenyl )-5-(2,4-difluorophenyl)-1,2-oxazol-4-yl](pyridin-3-yl)methanol, (1.036)[3-(4-chloro-2-fluorophenyl)-5 -(2,4-difluorophenyl)-1,2-oxazol-4-yl](pyridin-3-yl)methanol, (1.037)1-({(2R,4S)-2-[2-chloro-4 -(4-chlorophenoxy)phenyl]-4-methyl-1,3-dioxolan-2-yl}methyl)-1H-1,2,4-triazole, (1.038)1-({(2S,4S)- 2-[2-chloro-4-(4-chlorophenoxy)phenyl]-4-methyl-1,3-dioxolan-2-yl}methyl)-1H-1,2,4-triazole, (1.039)1- {[3-(2-chlorophenyl)-2-(2,4-difluorophenyl)oxiran-2-yl]methyl}-1H-1,2,4-triazol-5-ylthiocyanate, (1.040)1-{[rel(2R,3R)-3-(2-chlorophenyl)-2-(2,4-difluorophenyl)oxiran-2-yl]methyl}-1H-1,2,4-triazol-5-ylthiocyanate, (1.041) 1-{[rel(2R,3S)-3-(2-chlorophenyl)-2-(2,4-difluorophenyl)oxiran-2-yl]methyl}-1H-1,2,4-triazole -5-ylthiocyanate, (1.042)2-[(2R,4R,5R)-1-(2,4-dichlorophenyl)-5-hydroxy-2,6,6-trimethylheptan-4-yl]-2, 4-dihydro-3H-1,2, 4-triazole-3-thione, (1.043)2-[(2R,4R,5S)-1-(2,4-dichlorophenyl)-5-hydroxy-2,6, 6-trimethylheptan-4-yl]-2,4-dihydro-3H-1,2,4-triazole-3-thione, (1.044)2-[(2R,4S,5R)-1-(2,4 -dichlorophenyl)-5-hydroxy-2,6,6-trimethylheptan-4-yl]-2,4-dihydro-3H-1,2,4-triazole-3-thione, (1.045)2-[(2R ,4S,5S)-1-(2, 4-dichlorophenyl)-5-hydroxy-2,6,6-trimethylheptan-4-yl]-2,4-dihydro-3H-1,2,4-triazole-3-thione, (1.046)2-[( 2S,4R,5R)-1-(2,4-dichlorophenyl)-5-hydroxy-2,6,6-trimethylheptan-4-yl]-2,4-dihydro-3H-1,2,4-triazole -3-thione, (1.047)2-[(2S,4R,5S)-1-(2,4-dichlorophenyl)-5-hydroxy-2,6,6-trimethylheptan-4-yl]-2,4 -dihydro-3H-1,2,4-triazole-3-thione, (1.048)2-[(2S,4S,5R)-1-(2,4-dichlorophenyl)-5-hydroxy-2,6,6 -trimethylheptan-4-yl]-2,4-dihydro-3H-1,2,4-triazole-3-thione, (1.049)2-[(2S,4S,5S)-1-(2,4- dichlorophenyl)-5-hydroxy-2,6,6-trimethylheptan-4-yl]-2,4-dihydro-3H-1,2,4-triazole-3-thione, (1.050)2-[1-( 2,4-dichlorophenyl)-5-hydroxy-2,6,6-trimethylheptan-4-yl]-2,4-dihydro-3H-1,2,4-triazole-3-thione, (1.051)2- [2-Chloro-4-(2,4-dichlorophenoxy)phenyl]-1-(1H-1,2,4-triazol-1-yl)propan-2-ol, (1.052)2-[2-chloro -4-(4-chlorophenoxy)phenyl]-1-(1H-1,2,4-triazol-1-yl)butan-2-ol, (1.053)2-[4-(4-chlorophenoxy)- 2-(trifluoromethyl)phenyl]-1-(1H-1,2,4-triazol-1-yl)butan-2-ol, (1.054)2-[4-(4-chlorophenoxy)-2- (trifluoromethyl)phenyl]-1-(1H-1,2,4-triazol-1-yl)pentan-2-ol, (1.055) mefentrifluconazole, (1.056) 2-{[3-(2 -chlorophenyl)-2-(2,4-difluorophenyl)oxiran-2-yl]methyl}-2,4-dihydro-3H-1,2,4-triazole-3-thione, (1.057)2-{[ rel(2R,3R)-3-(2-chlorophenyl)-2-(2,4-difluorophenyl)oxiran-2-yl]methyl}-2,4-dihydro-3H-1,2,4-triazole- 3-thione, (1.058)2-{[rel(2R,3S)-3-(2-chlorophenyl)-2-(2,4-difluorophenyl)oxiran-2-yl]methyl}-2,4-dihydro -3H-1,2,4-triazole-3-thione, (1.059)5-(4-chlorobenzyl)-2-(chloromethyl)-2-methyl-1-(1H-1,2,4-triazole -1-ylmethyl)cyclopentanol, (1.060)5-(allylsulfanyl)-1-{[3-(2-chlorophenyl)-2-(2,4-difluorophenyl)oxiran-2-yl]methyl}- 1H-1,2,4-triazole, (1.061)5-(allylsulfanyl)-1-{[rel(2R,3R)-3-(2-chlorophenyl)-2-(2,4-difluorophenyl)oxirane -2-yl]methyl}-1H-1,2,4-triazole, (1.062)5-(arylsulfanyl)-1-{[rel(2R,3S)-3-(2-chlorophenyl)-2-( 2,4-difluorophenyl)oxiran-2-yl]methyl}-1H-1,2, 4-triazole, (1.063)N'-(2,5-dimethyl-4-{[3-(1,1,2,2-tetrafluoroethoxy)phenyl]sulfanyl}phenyl)-N-ethyl-N-methyl imidoformamide, (1.064)N'-(2,5-dimethyl-4-{[3-(2,2,2-trifluoroethoxy)phenyl]sulfanyl}phenyl)N-ethyl-N-methylimidoformamide, ( 1.065) N'-(2,5-dimethyl-4-{[3-(2,2,3,3-tetrafluoropropoxy)phenyl]sulfanyl}phenyl)-N-ethyl-N-methyl-imidoformamide, ( 1.066) N'-(2,5-dimethyl-4-{[3-(pentafluoroethoxy)phenyl]sulfanyl}phenyl)-N-ethyl-N-methylimidoformamide, (1.067)N'-(2,5 -dimethyl-4-{3-[(1,1,2,2-tetrafluoroethyl)sulfanyl]phenoxy}phenyl)-N-ethyl-N-methylimidoformamide, (1.068)N'-(2,5- Dimethyl-4-{3-[(2,2,2-trifluoroethyl)sulfanyl]phenoxy}phenyl)-N-ethyl-N-methylimidoformamide, (1.069)N'-(2,5-dimethyl-4 -{3-[(2,2,3,3-tetrafluoropropyl)sulfanyl]phenoxy}phenyl)-N-ethyl-N-methylimidoformamide, (1.070)N'-(2,5-dimethyl-4- {3-[(pentafluoroethyl)sulfanyl]phenoxy}phenyl)-N-ethyl-N-methylimidoformamide, (1.071)N'-(2,5-dimethyl-4-phenoxyphenyl)-N-ethyl-N -methylimidoformamide, (1.072)N'-(4-{[3-(difluoromethoxy)phenyl]sulfanyl}-2,5-dimethylphenyl)-N-ethyl-N-methylimidoformamide, (1.073)N' -(4-{3-[(difluoromethyl)sulfanyl]phenoxy}-2,5-dimethylphenyl)-N-ethyl-N-methylimidoformamide, (1.074)N'-[5-bromo-6-(2 ,3-dihydro-1H-inden-2-yloxy)-2-methylpyridin-3-yl]-N-ethyl-N-methylimidoformamide, (1.075)N'-{4-[(4,5-dichloro -1,3-thiazol-2-yl)oxy]-2,5-dimethylphenyl}-N-ethyl-N-methylimidoformamide, (1.076)N'-{5-bromo-6-[(1R)- 1-(3,5-difluorophenyl)ethoxy]-2-methylpyridin-3-yl}-N-ethyl-N-methylimidoformamide, (1.077)N'-{5-bromo-6-[(1S) -1-(3, 5-difluorophenyl)ethoxy]-2-methylpyridin-3-yl}-N-ethyl-N-methylimidoformamide, (1.078)N'-{5-bromo-6-[(cis-4-isopropylcyclohexyl) oxy]-2-methylpyridin-3-yl}-N-ethyl-N-methylimidoformamide, (1.079)N'-{5-bromo-6-[(trans-4-isopropylcyclohexyl)oxy]-2- Methylpyridin-3-yl}-N-ethyl-N-methylimidoformamide, (1.080)N'-{5-bromo-6-[1-(3,5-difluorophenyl)ethoxy]-2-methylpyridine- 3-yl}-N-ethyl-N-methylimidoformamide, (1.081) ipfentifluconazole, (1.082) 2-[4-(4-chlorophenoxy)-2-(trifluoromethyl)phenyl] -1-(1H-1,2,4-triazol-1-yl)propan-2-ol, (1.083)2-[6-(4-bromophenoxy)-2-(trifluoromethyl)-3-pyridyl ]-1-(1,2,4-triazol-1-yl)propan-2-ol, (1.084)2-[6-(4-chlorophenoxy)-2-(trifluoromethyl)-3-pyridyl] -1-(1,2,4-triazol-1-yl)propan-2-ol, (1.085)3-[2-(1-chlorocyclopropyl)-3-(3-chloro-2-fluoro-phenyl )-2-hydroxy-propyl]imidazole-4-carbonitrile, (1.086)4-[[6-[rac-(2R)-2-(2,4-difluorophenyl)-1,1-difluoro-2- Hydroxy-3-(5-thioxo-4H-1,2,4-triazol-1-yl)propyl]-3-pyridyl]oxy]benzonitrile, (1.087)N-isopropyl-N'-[5-methoxy- 2-methyl-4-(2,2,2-trifluoro-1-hydroxy-1-phenylethyl)phenyl]-N-methylimidoformamide, (1.088)N'-{5-bromo-2-methyl-6 -[(1-propoxypropan-2-yl)oxy]pyridin-3-yl}-N-ethyl-N-methylimidoformamide, (1.089) hexaconazole, (1.090) penconazole, (1.091) fenbuconazole, (1.092) selected from the group consisting of methyl 2-[2-chloro-4-(4-chlorophenoxy)phenyl]-2-hydroxy-3-(1,2,4-triazol-1-yl)propanoate inhibitors of ergosterol synthesis, (2.001) benzovindiflupyr, (2.002) bixafen, (2.003) boscalid, (2.004) carboxin, (2.005) fluopyram, (2.006) flutolanil, (2.007) fluxapyroxad, (2.008) furametpyr, (2.009) isofetamide, (2.010) isopyrazam (anti-epimeric enantiomers 1R, 4S, 9S), (2.011) isopyrazam (anti-epimeric enantiomers 1S, 4R, 9R), (2.012) isopyrazam (anti-epimeric enantiomers 1RS, 4SR, 9SR) (2.013) isopyrazam (mixture of syn-epimeric racemate 1RS,4SR,9RS and anti-epimeric racemate !RS,4SR,9SR), (2.014) isopyrazam (syn-epimeric enantiomers 1R,4S,9R), (2.015) Isopyrazam (syn-epimeric enantiomer 1S,4R,9S), (2.016) Isopyrazam (syn-epimeric racemate 1RS, 4SR,9RS), (2.017) penflufen, (2.018) penthiopyrad, (2.019) pydiflumetofen, (2.020) pyraziflumide, (2.021) sedaxane, (2.022) 1,3-dimethyl-N-(1,1,3) -trimethyl-2,3-dihydro-1H-inden-4-yl)-1H-pyrazole-4-carboxamide, (2.023) 1,3-dimethyl-N-[(3R)-1,1,3-trimethyl- 2,3-dihydro-1H-inden-4-yl]-1H-pyrazole-4-carboxamide, (2.024)1,3-dimethyl-N-[(3S)-1,1,3-trimethyl-2,3 -dihydro-1H-inden-4-yl]-1H-pyrazole-4-carboxamide, (2.025) 1-methyl-3-(trifluoromethyl)-N-[2'-(trifluoromethyl)biphenyl-2- yl]-1H-pyrazole-4-carboxamide, (2.026) 2-fluoro-6-(trifluoromethyl)-N-(1,1,3-trimethyl-2,3-dihydro-1H-inden-4-yl ) benzamide, (2.027) 3-(difluoromethyl)-1-methyl-N-(1,1,3-trimethyl-2,3-dihydro-1H-inden-4-yl)-1H-pyrazole-4-carboxamide , (2.028) impylfluxam, (2.029) 3-(difluoromethyl)-1-methyl-N-[(3S)-1,1,3-trimethyl-2,3-dihydro-1H-indene-4- yl]-1H-pyrazole-4-carboxamide, (2.030) Fluindapyr, (2.031) 3-(difluoromethyl)-N-[(3R)-7-fluoro-1,1,3-trimethyl-2,3-dihydro -1H-inden-4-yl]-1-methyl-1H-pyrazole-4-carboxamide, (2.032)3-(difluoromethyl)-N-[(3S)-7-fluoro-1,1,3-trimethyl -2,3-dihydro-1H-inden-4-yl]-1-methyl-1H-pyrazole-4-carboxamide, (2.033)5,8-difluoro-N-[2-(2-fluoro-4-{[4-(Trifluoromethyl)pyridin-2-yl]oxy}phenyl)ethyl]quinazolin-4-amine, (2.034)N-(2-cyclopentyl-5-fluorobenzyl)-N-cyclopropyl-3-( Difluoromethyl)-5-fluoro-1-methyl-1H-pyrazole-4-carboxamide, (2.035)N-(2-tert-butyl-5-methylbenzyl)-N-cyclopropyl-3-(difluoromethyl)- 5-fluoro-1-methyl-1H-pyrazole-4-carboxamide, (2.036)N-(2-tert-butylbenzyl)-N-cyclopropyl-3-(difluoromethyl)-5-fluoro-1-methyl- 1H-pyrazole-4-carboxamide, (2.037)N-(5-chloro-2-ethylbenzyl)-N-cyclopropyl-3-(difluoromethyl)-5-fluoro-1-methyl-1H-pyrazole-4- Carboxamide, (2.038) Isoflurcipram, (2.039) N-[(1R,4S)-9-(dichloromethylene)-1,2,3,4-tetrahydro-1,4-methanonaphthalen-5-yl]- 3-(Difluoromethyl)-1-methyl-1H-pyrazole-4-carboxamide, (2.040)N- [(1S,4R)-9-(Dichloromethylene)-1,2,3,4-tetrahydro-1,4-methanonaphthalen-5-yl]-3-(difluoromethyl)-1-methyl-1H-pyrazole -4-carboxamide, (2.041) N-[1-(2,4-dichlorophenyl)-1-methoxypropan-2-yl]-3-(difluoromethyl)-1-methyl-1H-pyrazole-4-carboxamide, (2.042) N-[2-chloro-6-(trifluoromethyl)benzyl]-N-cyclopropyl-3-(difluoromethyl)-5-fluoro-1-methyl-1H-pyrazole-4-carboxamide, (2.043 ) N-[3-chloro-2-fluoro-6-(trifluoromethyl)benzyl]-N-cyclopropyl-3-(difluoromethyl)-5-fluoro-1-methyl-1H-pyrazole-4-carboxamide, (2.044) N-[5-chloro-2-(trifluoromethyl)benzyl]-N-cyclopropyl-3-(difluoromethyl)-5-fluoro-1-methyl-1H-pyrazole-4-carboxamide, (2.045) ) N-cyclopropyl-3-(difluoromethyl)-5-fluoro-1-methyl-N-[5-methyl-2-(trifluoromethyl)benzyl]-1H-pyrazole-4-carboxamide, (2.046)N -cyclopropyl-3-(difluoromethyl)-5-fluoro-N-(2-fluoro-6-isopropylbenzyl)-1-methyl-1H-pyrazole-4-carboxamide, (2.047)N-cyclopropyl-3- (Difluoromethyl)-5-fluoro-N-(2-isopropyl-5-methylbenzyl)-1-methyl-1H-pyrazole-4-carboxamide, (2.048) N-cyclopropyl-3-(difluoromethyl)-5 -fluoro-N-(2-isopropylbenzyl)-1-methyl-1H-pyrazole-4-carbothioamide, (2.049)N-cyclopropyl-3-(difluoromethyl)-5-fluoro-N-(2-isopropyl Benzyl)-1-methyl-1H-pyrazole-4-carboxamide, (2.050) N-cyclopropyl-3-(difluoromethyl)-5-fluoro-N-(5-fluoro-2-isopropylbenzyl)-1-methyl -1H-pyrazole-4-carboxamide, (2.051) N-cyclopropyl-3-(difluoromethyl)-N-(2-ethyl-4, 5-dimethylbenzyl)-5-fluoro-1-methyl-1H-pyrazole-4-carboxamide, (2.052) N-cyclopropyl-3-(difluoromethyl)-N-(2-ethyl-5-fluorobenzyl)- 5-fluoro-1-methyl-1H-pyrazole-4-carboxamide, (2.053) N-cyclopropyl-3-(difluoromethyl)-N-(2-ethyl-5-methylbenzyl)-5-fluoro-1- Methyl-1H-pyrazole-4-carboxamide, (2.054)N-Cyclopropyl-N-(2-cyclopropyl-5-fluorobenzyl)-3-(difluoromethyl)-5-fluoro-1-methyl-1H-pyrazole -4-carboxamide, (2.055) N-cyclopropyl-N-(2-cyclopropyl-5-methylbenzyl)-3-(difluoromethyl)-5-fluoro-1-methyl-1H-pyrazole-4-carboxamide, (2.056) N-cyclopropyl-N-(2-cyclopropylbenzyl)-3-(difluoromethyl)-5-fluoro-1-methyl-1H-pyrazole-4-carboxamide, (2.057) pyrapropoine, (2.058) N -[rac-(1S,2S)-2-(2,4-dichlorophenyl)cyclobutyl]-2-(trifluoromethyl)nicotinamide, (2.059)N-[(1S,2S)-2-(2,4 -dichlorophenyl)cyclobutyl]-2-(trifluoromethyl)nicotinamide, (2.060) an inhibitor of the respiratory chain at complex I or II selected from the group consisting of fulveneteram, (3.001) Amethoctrazine, (3.002) Amisulbrom, (3.003) Azoxystrobin, (3.004) Cumethoxystrobin, (3.005) Cumoxystrobin, (3.006) Cyazofamide, (3.007) Dimoxistrobin, (3.008) Enoxastrobin, (3.009) famoxadone, (3.010) phenamidone, (3.011) fluphenoxystrobin, (3.012) fluoxastrobin, (3.013) cresoxime-methyl, (3.014) metominostrobin, (3.015) orysastrobin, ( 3.016) picoxystrobin, (3.017) pyraclostrobin, (3.018) pyrametostrobin, (3.019) pyraoxystrobin, (3.020) trifloxystrobin, (3.021) (2E)-2-{2-[ ({[(1E)-1-(3-{[(E)-1-fluoro-2-phenylvinyl])oxy}phenyl)ethylidene]amino}oxy)methyl]phenyl}-2-(methoxyimino)- N-Methylacetamide, (3.022)(2E,3Z)-5-{[1-(4-chlorophenyl)-1H-pyrazol-3-yl]oxy}-2-(methoxyimino)-N,3-dimethylpenta -3-enamide, (3.023)(2R)-2-{2-[(2,5-dimethylphenoxy)methyl]phenyl}-2-methoxy-N-methylacetamide, (3.024)(2S)-2-{2-[(2,5-dimethylphenoxy)methyl]phenyl}-2-methoxy-N-methylacetamide, (3.025) fenpicoxamide, (3.026) mandestrobin, (3.027) N-(3-ethyl- 3,5,5-trimethylcyclohexyl)-3-formamide-2-hydroxybenzamide, (3.028)(2E,3Z)-5-{[1-(4-chloro-2-fluorophenyl)-1H-pyrazole-3 -yl]oxy}-2-(methoxyimino)-N,3-dimethylpent-3-enamide, (3.029){5-[3-(2,4-dimethylphenyl)-1H-pyrazol-1-yl] -2-methylbenzyl}methyl carbamate, (3.030) methyltetraprole, (3.031) florylpicoxamide, (3.032) (2S,3S)-3-(o-tolyl)butan-2-yl N-{an inhibitor of the respiratory chain at complex III selected from the group consisting of [4-methoxy-3-(propanoyloxy)-2-pyridyl]carbonyl}-L-alaninate; (4.001) carbendazim, (4.002) diethofencarb, (4.003) ethaboxam, (4.004) fluopicolide, (4.005) penciclon, (4.006) thiabendazole, (4.007) thiophanate-methyl, (4.008) zoxamide, (4.009) pyridaclomethyl, (4.010) 3-chloro-5-(4-chlorophenyl)-4-(2,6-difluorophenyl)-6-methylpyridazine, (4.011) 3-chloro-5-(6-chloropyridin-3-yl) -6-methyl-4-(2,4,6-trifluorophenyl)pyridazine, (4.012)4-(2-bromo-4-fluorophenyl)-N-(2,6-difluorophenyl)-1,3 -dimethyl-1H-pyrazol-5-amine, (4.013)4-(2-bromo-4-fluorophenyl)-N-(2-bromo-6-fluorophenyl)-1,3-dimethyl-1H-pyrazole- 5-amine, (4.014) 4-(2-bromo-4-fluorophenyl)-N-(2-bromophenyl)-1,3-dimethyl-1H-pyrazol-5-amine, (4.015) 4-(2 -bromo-4-fluorophenyl)-N-(2-chloro-6-fluorophenyl)-1,3-dimethyl-1H-pyrazol-5-amine, (4.016)4-(2-bromo-4-fluorophenyl )-N-(2-chlorophenyl)-1,3-dimethyl-1H-pyrazol-5-amine, (4.017)4-(2-bromo-4-fluorophenyl)-N-(2-fluorophenyl)-1 ,3-dimethyl-1H-pyrazol-5-amine, (4.018)4-(2-chloro-4-fluorophenyl)-N-(2,6-difluorophenyl)-1,3-dimethyl-1H-pyrazole- 5-amine, (4.019) 4-(2-chloro-4-fluorophenyl)-N-(2-chloro-6-fluorophenyl)-1,3-dimethyl-1H-pyrazol-5-amine, (4.020) 4-(2-chloro-4-fluorophenyl)-N-(2-chlorophenyl)-1,3-dimethyl-1H-pyrazol-5-amine, (4.021) 4-(2-chloro-4-fluorophenyl) -N-(2-fluorophenyl)-1,3-dimethyl-1H-pyrazol-5-amine, (4.022)4-(4-chlorophenyl)-5-(2,6-difluorophenyl)-3,6- Dimethylpyridazine, (4.023)N-(2-bromo-6-fluorophenyl)-4-(2-chloro-4-fluorophenyl)-1,3-dimethyl-1H-pyrazol-5-amine, (4.024)N -(2-bromophenyl)-4-(2-chloro-4-fluorophenyl)-1,3-dimethyl-1H-pyrazol-5-amine, (4.025)N-(4-chloro-2,6-difluoro An inhibitor of mitosis and cell division selected from the group consisting of phenyl)-4-(2-chloro-4-fluorophenyl)-1,3-dimethyl-1H-pyrazol-5-amine, (4.026) fluopimimide , (5.001) Bordeaux mixture, (5.002) captafol, (5.003) captan, (5.004) chlorothalonil, (5.005) copper hydroxide, (5.006) copper naphthenate, (5.007) copper oxide, (5.008) copper oxychloride, (5.009) ) copper (2+) sulfate, (5.010) dithianone, (5.011) dodine, (5.012) folpet, (5.013) mancozeb, (5.014) maneb, (5.015) metiram, (5.016) metiram zinc, (5.017) oxine copper (5.018) propineb, (5.019) sulfur preparations containing sulfur and calcium polysulfide, (5.020) thiram, (5.021) zineb, (5.022) ziram, (5.023) 6-ethyl-5,7-dioxo-6,7 -dihydro-5H-pyrrolo[3',4':5,6][1,4]dithiino[2,3-c][1,2]thiazole-3-carbonitrile, (6.001) acibenzolar-S-methyl A compound with multisite activity selected from the group consisting of (6.001) acibenzolar-S-methyl, (6.002) isotianil, (6.003) probenazole, (6.004) a compound capable of inducing host defenses selected from the group consisting of thiazinyl; (7.001) cyprodinil, (7.002) kasugamycin, (7.003) kasugamycin hydrochloride hydrate, (7.004) oxytetracycline, (7.005) pyrimethanil, (7.006) 3-(5-fluoro-3,3,4,4-tetramethyl) -3,4-dihydroisoquinolin-1-yl)quinolines, inhibitors of amino acid and / or protein biosynthesis, (8.001) an inhibitor of ATP production selected from the group consisting of silthiopham; (9.001) Bentiavalicarb, (9.002) Dimethomorph, (9.003) Flumorph, (9.004) Iprovalicarb, (9.005) Mandipropamide, (9.006) Pyrimorph, (9.007) Valifenalate, (9.008) (2E)-3-( 4-tert-butylphenyl)-3-(2-chloropyridin-4-yl)-1-(morpholin-4-yl)prop-2-en-1-one, (9.009)(2Z)-3-( Inhibition of cell wall synthesis selected from the group consisting of 4-tert-butylphenyl)-3-(2-chloropyridin-4-yl)-1-(morpholin-4-yl)prop-2-en-1-one agent, (10.001) propamocarb, (10.002) propamocarb hydrochloride, (10.003) an inhibitor of lipid and membrane synthesis selected from the group consisting of tolclofos-methyl; (11.001) tricyclazole, (11.002) an inhibitor of melanin biosynthesis selected from the group consisting of tolprocarb; an inhibitor of nucleic acid synthesis selected from the group consisting of (12.001) Benalaxyl, (12.002) Benalaxyl-M (Chiralaxyl), (12.003) Metalaxyl, (12.004) Metalaxyl-M (Mefenoxam); (13.001) fludioxonil, (13.002) iprodione, (13.003) procymidone, (13.004) proquinazide, (13.005) quinoxifene, (13.006) vinclozolin an inhibitor of signaling selected from the group; (14.001) fluazinam, (14.002) a compound capable of acting as an uncoupler selected from the group consisting of meptyldinocap, (15.001) Abscisic acid, (15.002) Benthazole, (15.003) Betoxazine, (15.004) Capcimycin, (15.005) Carvone, (15.006) Quinomethionato, (15.007) Cufraneb, (15.008) Cyflufenamide, (15.009) Cymoxanil, (15.0) 10) cyprosulfamide, (15.011) flutianil, (15.012) fosetyl-aluminum, (15.013) fosetyl-calcium, (15.014) fosetyl-sodium, (15.015) methyl isothiocyanate, (15.016) metrafenone, (15.017) millidiomycin, (15.018) Natamycin, (15.019) Nickel dimethyldithiocarbamate, (15.020) Nitrotal isopropyl, (15.021) Oxamocarb, (15.022) Oxathiapiproline, (15.023) Oxyphenthine, (15.024) Pentachlorophenol and its salts, (15.025) phosphorous acid and its salts, (15.026) propamocarb-fosetylate, (15.027) pyriophenone (clazaphenone), (15.028) tebufuroquine, (15.029) tecloftalam, (15.030) tolnifanide, (15.031) 1-(4-{4) -[(5R)-5-(2,6-difluorophenyl)-4,5-dihydro-1,2-oxazol-3-yl]-1,3-thiazol-2-yl}piperidin-1-yl) -2-[5-methyl-3-(trifluoromethyl)-1H-pyrazol-1-yl]ethanone, (15.032)1-(4-{4-[(5S)-5-(2,6-difluoro Phenyl)-4,5-dihydro-1,2-oxazol-3-yl]-1,3-thiazol-2-yl}piperidin-1-yl)-2-[5-methyl-3-(trifluoromethyl )-1H-pyrazol-1-yl]ethanone, (15.033) 2-(6-benzylpyridin-2-yl)quinazoline, (15.034) dipimethitrone, (15.035) 2-[3,5-bis(difluoromethyl)- 1H-pyrazol-1-yl]-1-[4-(4-{5-[2-(prop-2-yn-1-yloxy)phenyl]-4,5-dihydro-1,2-oxazole-3 -yl}-1,3-thiazol-2-yl)piperidin-1-yl]ethanone, (15.036)2-[3,5-bis(difluoromethyl)-1H-pyrazol-1-yl]-1-[ 4-(4-{5-[2-chloro-6-(prop-2-yn-1-yloxy)phenyl]-4,5-dihydro-1,2-oxazol-3-yl}-1,3- Thiazol-2-yl)piperidin-1-yl]ethanone, (15.037)2-[3,5-bis(difluoromethyl)-1H-pyrazol-1-yl]-1-[4-(4-{5- [2-fluoro-6-(prop-2-yn-1-yloxy)phenyl]-4,5-dihydro-1,2- Oxazol-3-yl}-1,3-thiazol-2-yl)piperidin-1-yl]ethanone, (15.038)2-[6-(3-fluoro-4-methoxyphenyl)-5-methylpyridine-2 -yl]quinazoline, (15.039)2-{(5R)-3-[2-(1-{[3,5-bis(difluoromethyl)-1H-pyrazol-1-yl]acetyl}piperidin-4-yl )-1,3-thiazol-4-yl]-4,5-dihydro-1,2-oxazol-5-yl}-3-chlorophenyl methanesulfonate, (15.040)2-{(5S)-3-[2 -(1-{[3,5-bis(difluoromethyl)-1H-pyrazol-1-yl]acetyl}piperidin-4-yl)-1,3-thiazol-4-yl]-4,5-dihydro- 1,2-oxazol-5-yl}-3-chlorophenyl methanesulfonate, (15.041) ipflufenoquine, (15.042) 2-{2-fluoro-6-[(8-fluoro-2-methylquinoline-3- yl)oxy]phenyl}propan-2-ol, (15.043)fluoxapiproline, (15.044)2-{3-[2-(1-{[3,5-bis(difluoromethyl)-1H-pyrazole- 1-yl]acetyl}piperidin-4-yl)-1,3-thiazol-4-yl]-4,5-dihydro-1,2-oxazol-5-yl}phenyl methanesulfonate, (15.045)2-phenyl Phenol and its salts, (15.046) 3-(4,4,5-trifluoro-3,3-dimethyl-3,4-dihydroisoquinolin-1-yl)quinoline, (15.047) quinofumeline, (15.048) 4-amino -5-fluoropyrimidin-2-ol (tautomer: 4-amino-5-fluoropyrimidin-2(1H)-one), (15.049) 4-oxo-4-[(2-phenylethyl)amino] Butanoic acid, (15.050) 5-amino-1,3,4-thiadiazol-2-thiol, (15.051) 5-chloro-N'-phenyl-N'-(prop-2-yn-1-yl)thiophene- 2-sulfonohydrazide, (15.052)5-fluoro-2-[(4-fluorobenzyl)oxy]pyrimidin-4-amine, (15.053)5-fluoro-2-[(4-methylbenzyl)oxy]pyrimidine- 4-amine, (15.054)9-fluoro-2,2-dimethyl-5-(quinolin-3-yl)-2,3-dihydro-1,4-benzoxazepine, (15.055) {6-[({[(Z)-(1-methyl-1H-tetrazol-5-yl)(phenyl)methylene]amino}oxy)methyl]pyridin-2-yl}carbamate but-3- In-1-yl, (15.056)(2Z)-3-amino-2-cyano-3-phenylacrylate ethyl, (15.057) phenazine-1-carboxylic acid, (15.058) 3,4,5-trihydroxybenzoin propyl acid, (15.059) quinolin-8-ol, (15.060) quinolin-8-ol sulfate (2:1), (15.061) {6-[({[(1-methyl-1H-tetrazol-5-yl) (Phenyl)methylene]amino}oxy)methyl]pyridin-2-yl}carbamate tert-butyl, (15.062)5-fluoro-4-imino-3-methyl-1-[(4-methylphenyl)sulfonyl]- 3,4-dihydropyrimidin-2(1H)-one, (15.063) aminopyrifene, (15.064) (N'-[2-chloro-4-(2-fluorophenoxy)-5-methylphenyl]-N- ethyl-N-methylimidoformamide), (15.065)(N'-(2-chloro-5-methyl-4-phenoxyphenyl)-N-ethyl-N-methylimidoformamide), (15.066)(2-{2 -[(7,8-difluoro-2-methylquinolin-3-yl)oxy]-6-fluorophenyl}propan-2-ol), (15.067)(5-bromo-1-(5,6-dimethylpyridine -3-yl)-3,3-dimethyl-3,4-dihydroisoquinoline), (15.068)(3-(4,4-difluoro-5,5-dimethyl-4,5-dihydrothieno[2,3-c ]pyridin-7-yl)quinoline), (15.069)(1-(4,5-dimethyl-1H-benzimidazol-1-yl)-4,4-difluoro-3,3-dimethyl-3,4-dihydro isoquinoline), (15.070)8-fluoro-3-(5-fluoro-3,3-dimethyl-3,4-dihydroisoquinolin-1-yl)quinolone, (15.071)8-fluoro-3-(5-fluoro- 3,3,4,4-tetramethyl-3,4-dihydroisoquinolin-1-yl)quinolone, (15.072)3-(4,4-difluoro-3,3-dimethyl-3,4-dihydroisoquinoline-1 -yl)-8-fluoroquinoline, (15.073)(N-methyl-N-phenyl-4-[5-(trifluoromethyl)-1,2,4-oxadiazol-3-yl]benzamide), ( 15.074) {4-[5-(trifluoromethyl)-1,2,4-oxadiazol-3-yl]phenyl}methyl carbamate, (15.075)(N-{4-[5-(trifluoromethyl )-1,2,4-oxadiazol-3-yl]benzyl}cyclopropanecarboxamide), (15.076)N-methyl-4-(5-(trifluoromethyl)-1,2,4-oxadiazole -3-yl]benzamide, (15.077)N-[(E)-methoxyiminomethyl]-4-[5-(trifluoromethyl)-1,2,4-oxadiazol-3-yl]benzamide, ( 15.078) N-[(Z)-methoxyiminomethyl]-4-[5-(trifluoromethyl)-1,2,4-oxadiazol-3-yl]benzamide, (15.079) N-[4-[ 5-(Trifluoromethyl)-1,2,4-oxadiazol-3-yl]phenyl]cyclopropanecarboxamide, (15.080)N-(2-fluorophenyl)-4-[5-(trifluoromethyl) -1,2,4-oxadiazol-3-yl]benzamide, (15.081)2,2-difluoro-N-methyl-2-[4-[5-(trifluoromethyl)-1,2,4- Oxadiazol-3-yl]phenyl]acetamide, (15.082)N-allyl-N-[[4-[5-(trifluoromethyl)-1,2,4-oxadiazol-3-yl)phenyl] methyl]acetamide, (15.083)N-[(E)-N-methoxy-C-methyl-carbonimidoyl]-4-(5-(trifluoromethyl)-1,2,4-oxadiazole-3- yl]benzamide, (15.084)N-[(Z)-N-methoxy-C-methyl-carbonimidoyl]-4-[5-(trifluoromethyl)-1,2,4-oxadiazole-3- yl]benzamide, (15.085) N-allyl-N-[[4-[5-(trifluoromethyl)-1,2,4-oxadiazol-3-yl]phenyl]methyl]propanamide, (15.086) 4,4-dimethyl-1-[[4-[5-(trifluoromethyl)-1,2,4-oxadiazol-3-yl]phenyl]methyl]pyrrolidin-2-one, (15.087)N- methyl-4- [5-(Trifluoromethyl)-1,2,4-oxadiazol-3-yl]benzenecarbothioamide, (15.088)5-methyl-1-[[4-[5-(trifluoromethyl)-1 ,2,4-oxadiazol-3-yl]phenyl]methyl]pyrrolidin-2-one, (15.089)N-((2,3-difluoro-4-[5-(trifluoromethyl)-1,2 ,4-oxadiazol-3-yl]phenyl]methyl]-3,3,3-trifluoro-propanamide, (15.090)1-methoxy-1-methyl-3-[[4-[5-(tri fluoromethyl)-1,2,4-oxadiazol-3-yl]phenyl]methyl]urea, (15.091)1,1-diethyl-3-[[4-[5-(trifluoromethyl)-1, 2,4-oxadiazol-3-yl]phenyl]methyl]urea, (15.092)N-[[4-[5-(trifluoromethyl)-1,2,4-oxadiazol-3-yl] Phenyl]methyl]propanamide, (15.093)N-Methoxy-N-[[4-[5-(trifluoromethyl)-1,2,4-oxadiazol-3-yl]phenyl]methyl]cyclopropanecarboxamide , (15.094) 1-Methoxy-3-methyl-1-[[4-[5-(trifluoromethyl)-1,2,4-oxadiazol-3-yl]phenyl]methyl]urea, (15.095) N-Methoxy-N-[[4-[5-(trifluoromethyl)-1,2,4-oxadiazol-3-yl]phenyl]methyl)cyclopropanecarboxamide, (15.096)N,2-dimethoxy- N-[[4-[5-(trifluoromethyl)-1,2,4-oxadiazol-3-yl]phenyl]methyl]propanamide, (15.097)N-ethyl-2-methyl-N-[ [4-[5-(trifluoromethyl)-1,2,4-oxadiazol-3-yl)phenyl]methyl]propanamide, (15.098)1-methoxy-3-methyl-1-[[4- [5-(Trifluoromethyl)-1,2,4-oxadiazol-3-yl]phenyl]methyl]urea, (15.099)1,3-dimethoxy-1-[[4-[5-(trifluoro) Methyl)-1,2,4-oxadiazol-3-yl]phenyl]methyl]urea, (15.100)3-ethyl-1-methoxy-1-[[4-[5-(trifluoromethyl)-1 ,2,4-oxadiazol-3-yl]phenyl]methyl]urea, (15.101)1- [[4-[5-(trifluoromethyl)-1,2,4-oxadiazol-3-yl]phenyl]methyl]piperidin-2-one, (15.102)4,4-dimethyl-2-[[ 4-[5-(trifluoromethyl)-1,2,4-oxadiazol-3-yl]]phenyl]methyl]isoxazolidin-3-one, (15.103)5,5-dimethyl-2-[[ 4-[5-(trifluoromethyl)-1,2,4-oxadiazol-3-yl]phenyl]methyl]isoxazolidin-3-one, (15.104)3,3-dimethyl-1-[[4 -[5-(trifluoromethyl)-1,2,4-oxadiazol-3-yl]phenyl]methyl]piperidin-2-one, (15.105)1-[[3-fluoro-4-(5- (Trifluoromethyl)-1,2,4-oxadiazol-3-yl]phenyl]methyl]azepan-2-one, (15.106)4,4-dimethyl-2-[[4-(5-(trifluoromethyl) fluoromethyl)-1,2,4-oxadiazol-3-yl]phenyl]methyl]isoxazolidin-3-one, (15.107)5,5-dimethyl-2-[[4-[5-(trifluoro Methyl)-1,2,4-oxadiazol-3-yl]phenyl]methyl]isoxazolidin-3-one, (15.108)1-{4-[5-(trifluoromethyl)-1,2,4 -oxadiazol-3-yl]benzyl}-1H-pyrazole-4-carboxylate, (15.109)N,N-dimethyl-1-{4-[5-(trifluoromethyl)-1,2,4 -oxadiazol-3-yl]benzyl}-1H-1,2,4-triazol-3-amine, (15.110)N-{2,3-difluoro-4-[5-(trifluoromethyl)-1 ,2,4-oxadiazol-3-yl]benzyl}butanamide, (15.111)N-(1-methylcyclopropyl)-4-[5-(trifluoromethyl)-1,2,4-oxadiazole -3-yl]benzamide, (15.112)N-(2,4-difluorophenyl)-4-[5-(trifluoromethyl)-1,2,4-oxadiazol-3-yl]benzamide, (15.113) ) 1-(5,6-dimethylpyridin-3-yl)-4,4-difluoro-3,3-dimethyl-3,4-dihydroisoquinoline, (15.114) 1-(6-(difluoromethyl)-5- Methyl-pyridin-3-yl)-4,4-difluoro-3,3-dimethyl-3,4-dihydroisoquinoline, (15.115)1-(5-(fluoromethyl)-6-methyl-pyridin-3-yl )-4,4-difluoro-3,3-dimethyl-3,4-dihydroisoquinoline, (15.116)1-(6-(difluoromethyl)-5-methoxy-pyridin-3-yl)-4,4-difluoro -3,3-dimethyl-3,4-dihydroisoquinoline, (15.117) 4-[5-(trifluoromethyl)-1,2,4-oxadiazol-3-yl]phenyldimethylcarbamate, (15.118) ) N-{4-[5-(trifluoromethyl)-1,2,4-oxadiazol-3-yl]phenyl}propanamide, (15.119) 3-[2-(1-{[5-methyl-3-(trifluoromethyl)-1H-pyrazol-1-yl]acetyl}piperidin-4-yl)-1,3-thiazol-4- yl]-1,5-dihydro-2,4-benzodioxepin-6-yl methanesulfonate, (15.120)9-fluoro-3-[2-(1-{[5-methyl-3-( Trifluoromethyl)-1H-pyrazol-1-yl]acetyl}piperidin-4-yl)-1,3-thiazol-4-yl]-1,5-dihydro-2,4-benzodioxepin-6- ylmethanesulfonate, (15.121)3-[2-(1-{[3,5-bis(difluoromethyl)-1H-pyrazol-1-yl]acetyl}piperidin-4-yl)-1,3- Thiazol-4-yl]-1,5-dihydro-2,4-benzodioxepin-6-yl methanesulfonate, (15.122)3-[2-(1-{[3,5-bis(difluoro Methyl)-1H-pyrazol-1-yl]acetyl}piperidin-4-yl)-1,3-thiazol-4-yl]-9-fluoro-1,5-dihydro-2,4-benzodioxepin- 6-ylmethanesulfonate, (15.123)1-(6,7-dimethylpyrazolo[1,5-a]pyridin-3-yl)-4,4-difluoro-3,3-dimethyl-3,4 -dihydroisoquinoline, (15.124)8-fluoro-N-(4,4,4-trifluoro-2-methyl-1-phenylbutan-2-yl)quinoline-3-carboxamide, (15.125)8-fluoro-N -[(2S)-4,4,4-trifluoro-2-methyl-1-phenylbutan-2-yl]quinoline-3-carboxamide, (15.126)N-(2,4-dimethyl-1-phenylpentane -2-yl)-8-fluoroquinoline-3-carboxamide and (15.127)N-[(2S)-2,4-dimethyl-1-phenylpentan-2-yl]-8-fluoroquinoline-3-carboxamide, (15.128) other fungicides selected from the group consisting of D-tagatose; (16.001) Bacillus subtilis, particularly strain QST713 / AQ713 (having NRRL accession number B21661, described in US Pat. No. 7,094,592, SERENADE OPTI or SERENADE ASO from Bayer CropScience LP, USA) (16.002) Bacillus amyloliquefaciens, particularly strain D747 (having accession number FERM BP-8234, described in US Pat. No. 7,094,592, from Certis, USA); (16.003) Bacillus pumilus, especially strain BU F-33 (with NRRL accession number 50185); (16.004) Bacillus subtilis subsp. amyloliquefaciens (Bacillus subtilis var. amyloliquefaciens) strain FZB24 (available as Taegro® from Novozymes, USA); Strains of Paenibacillus sp. as described in WO2016 / 154297; and fungi such as (16.006) spores of Aureobasidium pullulans, especially strain DSM 14940; (16.007) Aureobasidium. spores of pullulans strain DSM14941; (16.008) an antibacterial agent selected from the group consisting of a mixture of spores of Aureobasidium pullulans, in particular strains DSM14940 and DSM14941; (17.001) Bacillus subtilis, particularly strain QST713 / AQ713 (with NRRL accession number B21661 and described in US Pat. No. 6,060,051, available as SERENADE OPTI or SERENADE ASO from Bayer CropScience LP, USA) (17.002) Bacillus pumilus, particularly strain QST2808 (with accession number NRRL B-30087 and described in US Pat. No. 6,245,551, available as SONATA® from Bayer CropScience LP, USA); (17.003) Bacillus pumilus, especially strain GB34 (available as Yield Shield® from Bayer AG, Germany); (17.004) Bacillus pumilus, especially strain BU F-33 (NRRL accession number 50185; (17.005) Bacillus amyloliquefaciens, particularly strain D747 (having accession number FERM BP-8234, described in U.S. Pat. No. 7,094,592 as Double Nickel™ from Certis, USA); (17.006) Bacillus subtilis Y1336 (registered as a biofungicide in Taiwan under registration numbers 4764, 5454, 5096 and 5277, available as BIOBAC® WP from Bion-Tech, Taiwan); (17.007) Bacillus amyloliquefaciens strain MBI 600 (available as SUBTILEX from BASF SE); (17.008) Bacillus subtilis strain GB03 (available as Kodiak® from Bayer AG, Germany);( 17.009) Bacillus subtilis subsp. amyloliquefaciens strain FZB24 (as fungicide TAEGRO® or TAEGRO® (EPA registration number 70127-5) by Novozymes Biologicals Inc. Salem, Virginia or Greensboro, North Carolina). (17.010) Bacillus mycoides isolate J (available from Certis, USA as BmJ TGAI or WG); (17.011) Bacillus licheniformis , in particular strain SB3086 (available from Novozymes as EcoGuard™ Biofungicide and Green Releaf); (17.012) with accession number NRRL B-50972 or accession number NRRL B-67129, International Patent Publication No. WO2016 / 154297. a biological fungicide selected from the group consisting of strains of Paenibacillus sp. (18.001) unsaturated and saturated C 12 -C 24 A composition comprising one or more fatty acids or derivatives thereof selected from fatty acids, salts thereof, esters thereof or mixtures of any of the foregoing, wherein at least 95% of said fatty acids or derivatives thereof is C 14 -C 20(e.g. FLiPPER from AlphaBio Pesticides or Bayer AG) in the range of is selected from

[0203] Compound (B) is more preferably (1.001) cyproconazole, (1.002) difenoconazole, (1.003) epoxiconazole, (1.004) fenhexamide, (1.010) imazalil, (1.012) ipconazole, (1.013) metconazole, (1.017) propiconazole, (1.018) ) prothioconazole, (1.020) spiroxamine, (1.021) tebuconazole, (1.026) (1R,2S,5S)-5-(4-chlorobenzyl)-2-(chloromethyl)-2-methyl-1-(1H -1,2,4-triazol-1-ylmethyl)cyclopentanol, (1.027)(1S,2R,5R)-5-(4-chlorobenzyl)-2-(chloromethyl)-2-methyl-1- (1H-1,2,4-triazol-1-ylmethyl)cyclopentanol, (1.055) mefentrifluconazole, (1.059) 5-(4-chlorobenzyl)-2-(chloromethyl)-2-methyl- 1-(1H-1,2,4-triazol-1-ylmethyl)cyclopentanol, (1.081) ipfentifluconazole, (1.082) 2-[4-(4-chlorophenoxy)-2-( trifluoromethyl)phenyl]-1-(1H-1,2,4-triazol-1-yl)propan-2-ol and (1.092)2-[2-chloro-4-(4-chlorophenoxy)phenyl ]-methyl 2-hydroxy-3-(1,2,4-triazol-1-yl)propanoate, (2.001) benzovindiflupyr, (2.002) bixafen, (2.003) boscalid, (2.005) fluopyram, (2.007) fluxapyroxad, (2.009) isofetamide, (2.010) isopyrazam (anti-epimemeric enantiomers 1R, 4S, 9S) ), (2.011) isopyrazam (anti-epimeric enantiomers 1S, 4R, 9R), (2.012) isopyrazam (anti-epimeric racemates 1RS, 4SR, 9SR), (2.013) isopyrazam (syn-epimeric racemates 1RS, 4SR, (2.014) Isopyrazam (syn-epimeric enantiomers 1R,4S,9R), (2.015) Isopyrazam (syn-epimeric enantiomers 1S,4R,9S) (2.016) isopyrazam (syn-epimeric racemate 1RS,4SR,9RS), (2.017) penflufen, (2.018) penthiopyrad, (2.019) pydiflumetofen, (2.021) sedaxane, (2.028) impilfluxam, (2.030) Fluindapyr, (2.038) Isoflurcipram, (3.003) azoxystrobin, (3.007) dimoxystrobin, (3.012) fluoxastrobin, (3.013) cresoxime-methyl, (3.016) picoxystrobin, (3.017) pyraclostrobin, (3.020) trifle roxistrobin, (3.025) fenpicoxamide, (3.026) mandestrobin, (3.030) methyltetraprole, (3.031) florylpicoxamide, (4.005) pencychron, (4.007) thiophanate-methyl, (4.012) 4-(2-bromo-4-fluorophenyl)-N-(2,6-difluorophenyl)-1,3-dimethyl-1H-pyrazole-5 -amine, (4.015) 4-(2-bromo-4-fluorophenyl)-N-(2-chloro-6-fluorophenyl)-1,3-dimethyl-1H-pyrazol-5-amine, (4.025)N -(4-chloro-2,6-difluorophenyl)-4-(2-chloro-4-fluorophenyl)-1,3-dimethyl-1H-pyrazol-5-amine, (5.003) captan, (5.004) chlorothalonil, (5.010) dithianone, (5.011) dodine, (5.012) folpet, (5.013) mancozeb, (5.015) methiram, (5.018) propineb, (6.002) isotianil, (7.001) cyprodinil, (7.005) pyrimethanil, (12.003) metalaxyl, (12.004) metalaxyl-M (mefenoxam), (13.001) fludioxonil, (13.002) iprodione, (13.004) proquinazide, (13.005) quinoxifene, (14.001) Fluazinam, (14.002) Meptyldinocap, (15.008) cyflufenamide, (15.010) cyprosulfamide, (15.011) flutianil, (15.012) fosetyl-aluminium, (15.016) metrafenone, (15.027) pyriophenone (clazafenone), (15.047) quinofumeline, (15.048) 4-amino- 5-fluoropyrimidin-2-ol (tautomer: 4-amino-5-fluoropyrimidin-2(1H)-one), (15.052) 5-fluoro-2-[(4-fluorobenzyl)oxy]pyrimidine -4-amine, (15.053) 5-fluoro-2-[(4-methylbenzyl)oxy]pyrimidin-4-amine, (15.062) 5-fluoro-4-imino-3-methyl-1-[(4- methylphenyl)sulfonyl]-3,4-dihydropyrimidin-2(1H)-one, (15.063) aminopyrifene, (15.064)(N'-[2-chloro-4-(2-fluorophenoxy)-5- methylphenyl]-N-ethyl-N-methylimidoformamide), (16.001) Bacillus subtilis, particularly strain QST713 / AQ713 (having NRRL accession number B21661, described in US Pat. No. 7,094,592, SERENADE OPTI or SERENADE ASO from Bayer CropScience LP, USA) available as (17.001) Bacillus subtilis, particularly strain QST713 / AQ713 (with NRRL accession number B21661, described in US Pat. No. 6,060,051, available as SERENADE OPTI or SERENADE ASO from Bayer CropScience LP, USA) (17.002) Bacillus pumilus, particularly strain QST2808 (with accession number NRRL B-30087 and described in US Pat. No. 6,245,551, available as SONATA® from Bayer CropScience LP, USA); (17.003) Bacillus pumilus, in particular strain GB34 (available as Yield Shield® from Bayer AG, Germany); (17.008) Bacillus subtilis strain GB03 (as Kodiak® from Bayer AG, Germany); (17.009) Bacillus subtilis subsp. amyloliquefaciens strain FZB24 (as fungicide TAEGRO® or TAEGRO® (EPA registration number 70127-5), Novozymes Biologicals Inc., Salem, Virginia); (17.011) Bacillus licheniformis, particularly strain SB3086 (available from Novozymes as EcoGuard™ Biofungicide and Green Releaf); (17.012) a biological fungicide selected from the group consisting of strains of Paenibacillus sp. having accession number NRRL B-50972 or accession number NRRL B-67129 and described in International Patent Publication No. WO2016 / 154297; (18.001) unsaturated and saturated C 12 -C 24 A composition comprising one or more fatty acids or derivatives thereof selected from fatty acids, salts thereof, esters thereof or mixtures of any of the foregoing, wherein at least 95% of said fatty acids or derivatives thereof is C 14 -C 20 (e.g. FLiPPER from AlphaBio Pesticides or Bayer AG) in the range of is selected from

[0204] Compound (B) is even more preferably (1.002) Difenoconazole, (1.004) Fenhexamide, (1.010) Imazalil, (1.012) Ipconazole, (1.018) Prothioconazole, (1.020) Spiroxamine, (1.021) Tebuconazole, (1.026) (1R,2S,5S)- 5-(4-chlorobenzyl)-2-(chloromethyl)-2-methyl-1-(1H-1,2,4-triazol-1-ylmethyl)cyclopentanol, (1.027)(1S,2R,5R )-5-(4-chlorobenzyl)-2-(chloromethyl)-2-methyl-1-(1H-1,2,4-triazol-1-ylmethyl)cyclopentanol, (1.055) mefentrifluconazole , (1.059) 5-(4-chlorobenzyl)-2-(chloromethyl)-2-methyl-1-(1H-1,2,4-triazol-1-ylmethyl)cyclopentanol, (1.081) ipfen Trifluconazole (ipfentifluconazole), (1.082)2-[4-(4-chlorophenoxy)-2-(trifluoromethyl)phenyl]-1-(1H-1,2,4-triazol-1-yl)propane- 2-ol and (1.092) methyl 2-[2-chloro-4-(4-chlorophenoxy)phenyl]-2-hydroxy-3-(1,2,4-triazol-1-yl)propanoate, (2.001) benzovindiflupyr, (2.002) bixafen, (2.003) boscalid, (2.005) fluopyram, (2.007) fluxapyroxad, (2.017) penflufen, (2.018) penthiopyrad, (2.019) pydiflumetofen, ( 2.021) sedaxane, (2.028) impilfluxam, (2.030) fluindapyr, (2.038) isoflurcipram, (3.003) azoxystrobin, (3.012) fluoxastrobin, (3.016) picoxystrobin, (3.017) pyraclostrobin, (3.020) trifloxystrobin, (3.025) fenpicoxamide, (3.026) mandestrobin, (3.030) methyltetraprole, (3.031) florylpicoxamide, (4.005) pencychron, (4.007) thiophanate-methyl, (4.012) 4-(2-bromo-4-fluorophenyl)-N-(2,6-difluorophenyl)-1,3-dimethyl-1H-pyrazole-5 -amine, (4.015) 4-(2-bromo-4-fluorophenyl)-N-(2-chloro-6-fluorophenyl)-1,3-dimethyl-1H-pyrazol-5-amine, (4.025)N -(4-chloro-2,6-difluorophenyl)-4-(2-chloro-4-fluorophenyl)-1,3-dimethyl-1H-pyrazol-5-amine, (5.003) captan, (5.004) chlorothalonil, (5.010) dithianone, (5.012) folpet, (5.013) mancozeb, (5.015) metiram, (5.018) propineb, (6.002) isotianil, (7.005) pyrimethanil, (12.003) metalaxyl, (12.004) metalaxyl-M (mefenoxam), (13.001) fludioxonil, (13.004) proquinazide, (13.005) quinoxifene, (14.001) Fluazinam, (14.002) Meptyldinocap, (15.008) cyflufenamide, (15.012) fosetyl-aluminium, (15.016) metrafenone, (15.027) pyriophenone (clazafenone), (15.047) quinofumeline, (15.048) 4-amino-5-fluoropyrimidin-2-ol (tautomers) : 4-amino-5-fluoropyrimidin-2(1H)-one), (15.052)5-fluoro-2-[(4-fluorobenzyl)oxy]pyrimidin-4-amine, (15.062)5-fluoro-4 -imino-3-methyl-1-[(4-methylphenyl)sulfonyl]-3,4-dihydropyrimidin-2(1H)-one, (15.064)(N'-[2-chloro-4-(2- fluorophenoxy)-5-methylphenyl]-N-ethyl-N-methylimidoformamide), (16.001) Bacillus subtilis, particularly strain QST713 / AQ713 (having NRRL accession number B21661, described in US Pat. No. 7,094,592, SERENADE OPTI or SERENADE ASO from Bayer CropScience LP, USA) available as (17.001) Bacillus subtilis, particularly strain QST713 / AQ713 (with NRRL accession number B21661, described in US Pat. No. 6,060,051, available as SERENADE OPTI or SERENADE ASO from Bayer CropScience LP, USA) (17.012) a biological organism selected from the group consisting of strains of Paenibacillus sp. having accession number NRRL B-50972 or accession number NRRL B-67129 and described in International Patent Publication No. WO2016 / 154297; Fungicide, (18.001) unsaturated and saturated C 12 -C 24 A composition comprising one or more fatty acids or derivatives thereof selected from fatty acids, salts thereof, esters thereof or mixtures of any of the foregoing, wherein at least 95% of said fatty acids or derivatives thereof is C 14 -C 20 (e.g. FLiPPER from AlphaBio Pesticides or Bayer AG) in the range of is selected from

[0205] Compound (B) is most preferably (1.002) difenoconazole, (1.018) prothioconazole, (1.020) spiroxamine, (1.021) tebuconazole, (1.055) mefentrifluconazole, (2.002) Bixafen, (2.005) Fluopyram, (2.028) Impylfluxam, (2.038) Isoflurcipram, (3.020) trifloxystrobin, (3.025) fenpicoxamide, (5.003) captan, (5.010) dithianone, (5.012) folpet, (5.013) mancozeb, (5.018) propineb, (6.002) isotianil, (7.005) pyrimethanil, (13.001) fludioxonil, (13.004) proquinazide, (13.005) quinoxifene, (15.012) Fosetyl-aluminum, (15.016) Metraphenone, (15.064) (N'-[2-chloro-4-(2-fluorophenoxy)-5-methylphenyl]-N-ethyl-N-methylimidoformamide), (18.001) unsaturated and saturated C 12 -C 24 A composition comprising one or more fatty acids or derivatives thereof selected from fatty acids, salts thereof, esters thereof or mixtures of any of the foregoing, wherein at least 95% of said fatty acids or derivatives thereof is C 14 -C 20 (e.g. FLiPPER from AlphaBio Pesticides or Bayer AG) in the range of is selected from

[0206] The combination of compounds of the invention may contain one, two or more compounds (B). Preferably, the combination of compounds of the invention comprises one or two compounds (B).

[0207] When two or more compounds (B) are present, those compounds may be selected from different groups (1)-(18). For example, when one compound (B) is selected from group (1), additional compounds (B) may be selected from groups (2) to (18).

[0208] Preferred compound combinations are selected from the group (G1) consisting of the following mixtures: (I-655)+(1.001), (I-655)+(1.002), (I-655)+(1.003), (I-655)+(1.004), (I-655)+(1.005), (I-655)+(1.006), (I-655)+(1.007), (I-655)+(1.008), (I-655)+(1.009), (I-655)+(1.010), (I-655)+(1.011), (I-655)+(1.012), (I-655)+(1.013), (I-655)+(1.014), (I-655)+(1.015), (I-655)+(1.016), (I-655)+(1.017), (I-655)+(1.018), (I-655)+(1.019), (I-655)+(1.020), (I-655)+(1.021), (I-655)+(1.022), (I-655)+(1.023), (I-655)+(1.024), (I-655)+(1.025), (I-655)+(1.026), (I-655)+(1.027), (I-655)+(1.028), (I-655)+(1.029), (I-655)+(1.030), (I-655)+(1.031), (I-655)+(1.032), (I-655)+(1.033), (I-655)+(1.034), (I-655)+(1.035), (I-655)+(1.036), (I-655)+(1.037), (I-655)+(1.038), (I-655)+(1.039), (I-655)+(1.040), (I-655)+(1.041), (I-655)+(1.042), (I-655)+(1.043), (I-655)+(1.044), (I-655)+(1.045), (I-655)+(1.046), (I-655)+(1.047), (I-655)+(1.048), (I-655)+(1.049), (I-655)+(1.050), (I-655)+(1.051), (I-655)+(1.052), (I-655)+(1.053), (I-655)+(1.054), (I-655)+(1.055), (I-655)+(1.056), (I-655)+(1.057), (I-655)+(1.058), (I-655)+(1.059), (I-655)+(1.060), (I-655)+(1.061), (I-655)+(1.062), (I-655)+(1.063), (I-655)+(1.064), (I-655)+(1.065), (I-655)+(1.066), (I-655)+(1.067), (I-655)+(1.068), (I-655)+(1.069), (I-655)+(1.070), (I-655)+(1.071), (I-655)+(1.072), (I-655)+(1.073), (I-655)+(1.074), (I-655)+(1.075), (I-655)+(1.076), (I-655)+(1.077), (I-655)+(1.078), (I-655)+(1.079), (I-655)+(1.080), (I-655)+(1.081), (I-655)+(1.082), (I-655)+(1.083), (I-655)+(1.084), (I-655)+(1.085), (I-655)+(1.086), (I-655)+(1.087), (I-655)+(1.088), (I-655)+(1.089), (I-655)+(1.090), (I-655)+(1.091), (I-655)+(1.092), (I-655)+(2.001), (I-655)+(2.002), (I-655)+(2.003), (I-655)+(2.004), (I-655)+(2.005), (I-655)+(2.006), (I-655)+(2.007), (I-655)+(2.008), (I-655)+(2.009), (I-655)+(2.010), (I-655)+(2.011), (I-655)+(2.012), (I-655)+(2.013), (I-655)+(2.014), (I-655)+(2.015), (I-655)+(2.016), (I-655)+(2.017), (I-655)+(2.018), (I-655)+(2.019), (I-655)+(2.020), (I-655)+(2.021), (I-655)+(2.022), (I-655)+(2.023), (I-655)+(2.024), (I-655)+(2.025), (I-655)+(2.026), (I-655)+(2.027), (I-655)+(2.028), (I-655)+(2.029), (I-655)+(2.030), (I-655)+(2.031), (I-655)+(2.032), (I-655)+(2.033), (I-655)+(2.034), (I-655)+(2.035), (I-655)+(2.036), (I-655)+(2.037), (I-655)+(2.038), (I-655)+(2.039), (I-655)+(2.040), (I-655)+(2.041), (I-655)+(2.042), (I-655)+(2.043), (I-655)+(2.044), (I-655)+(2.045), (I-655)+(2.046), (I-655)+(2.047), (I-655)+(2.048), (I-655)+(2.049), (I-655)+(2.050), (I-655)+(2.051), (I-655)+(2.052), (I-655)+(2.053), (I-655)+(2.054), (I-655)+(2.055), (I-655)+(2.056), (I-655)+(2.057), (I-655)+(2.058), (I-655)+(2.059), (I-655)+(2.060), (I-655)+(3.001), (I-655)+(3.002), (I-655)+(3.003), (I-655)+(3.004), (I-655)+(3.005), (I-655)+(3.006), (I-655)+(3.007), (I-655)+(3.008), (I-655)+(3.009), (I-655)+(3.010), (I-655)+(3.011), (I-655)+(3.012), (I-655)+(3.013), (I-655)+(3.014), (I-655)+(3.015), (I-655)+(3.016), (I-655)+(3.017), (I-655)+(3.018), (I-655)+(3.019), (I-655)+(3.020), (I-655)+(3.021), (I-655)+(3.022), (I-655)+(3.023), (I-655)+(3.024), (I-655)+(3.025), (I-655)+(3.026), (I-655)+(3.027), (I-655)+(3.028), (I-655)+(3.029), (I-655)+(3.030), (I-655)+(3.031), (I-655)+(3.032), (I-655)+(4.001), (I-655)+(4.002), (I-655)+(4.003), (I-655)+(4.004), (I-655)+(4.005), (I-655)+(4.006), (I-655)+(4.007), (I-655)+(4.008), (I-655)+(4.009), (I-655)+(4.010), (I-655)+(4.011), (I-655)+(4.012), (I-655)+(4.013), (I-655)+(4.014), (I-655)+(4.015), (I-655)+(4.016), (I-655)+(4.017), (I-655)+(4.018), (I-655)+(4.019), (I-655)+(4.020), (I-655)+(4.021), (I-655)+(4.022), (I-655)+(4.023), (I-655)+(4.024), (I-655)+(4.025), (I-655)+(4.026), (I-655)+(5.001), (I-655)+(5.002), (I-655)+(5.003), (I-655)+(5.004), (I-655)+(5.005), (I-655)+(5.006), (I-655)+(5.007), (I-655)+(5.008), (I-655)+(5.009), (I-655)+(5.010), (I-655)+(5.011), (I-655)+(5.012), (I-655)+(5.013), (I-655)+(5.014), (I-655)+(5.015), (I-655)+(5.016), (I-655)+(5.017), (I-655)+(5.018), (I-655)+(5.019), (I-655)+(5.020), (I-655)+(5.021), (I-655)+(5.022), (I-655)+(5.023), (I-655)+(6.001), (I-655)+(6.002), (I-655)+(6.003), (I-655)+(6.004), (I-655)+(7.001), (I-655)+(7.002), (I-655)+(7.003), (I-655)+(7.004), (I-655)+(7.005), (I-655)+(7.006), (I-655)+(8.001), (I-655)+(9.001), (I-655)+(9.002), (I-655)+(9.003), (I-655)+(9.004), (I-655)+(9.005), (I-655)+(9.006), (I-655)+(9.007), (I-655)+(9.008), (I-655)+(9.009), (I-655)+(10.001), (I-655)+(10.002), (I-655)+(10.003), (I-655)+(11.001), (I-655)+(11.002), (I-655)+(12.001), (I-655)+(12.002), (I-655)+(12.003), (I-655)+(12.004), (I-655)+(13.001), (I-655)+(13.002), (I-655)+(13.003), (I-655)+(13.004), (I-655)+(13.005), (I-655)+(13.006), (I-655)+(14.001), (I-655)+(14.002), (I-655)+(15.001), (I-655)+(15.002), (I-655)+(15.003), (I-655)+(15.004), (I-655)+(15.005), (I-655)+(15.006), (I-655)+(15.007), (I-655)+(15.008), (I-655)+(15.009), (I-655)+(15.010), (I-655)+(15.011), (I-655)+(15.012), (I-655)+(15.013), (I-655)+(15.014), (I-655)+(15.015), (I-655)+(15.016), (I-655)+(15.017), (I-655)+(15.018), (I-655)+(15.019), (I-655)+(15.020), (I-655)+(15.021), (I-655)+(15.022), (I-655)+(15.023), (I-655)+(15.024), (I-655)+(15.025), (I-655)+(15.026), (I-655)+(15.027), (I-655)+(15.028), (I-655)+(15.029), (I-655)+(15.030), (I-655)+(15.031), (I-655)+(15.032), (I-655)+(15.033), (I-655)+(15.034), (I-655)+(15.035), (I-655)+(15.036), (I-655)+(15.037), (I-655)+(15.038), (I-655)+(15.039), (I-655)+(15.040), (I-655)+(15.041), (I-655)+(15.042), (I-655)+(15.043), (I-655)+(15.044), (I-655)+(15.045), (I-655)+(15.046), (I-655)+(15.047), (I-655)+(15.048), (I-655)+(15.049), (I-655)+(15.050), (I-655)+(15.051), (I-655)+(15.052), (I-655)+(15.053), (I-655)+(15.054), (I-655)+(15.055), (I-655)+(15.056), (I-655)+(15.057), (I-655)+(15.058), (I-655)+(15.059), (I-655)+(15.060), (I-655)+(15.061), (I-655)+(15.062), (I-655)+(15.063), (I-655)+(15.064), (I-655)+(15.065), (I-655)+(15.066), (I-655)+(15.067), (I-655)+(15.068), (I-655)+(15.069), (I-655)+(15.070), (I-655)+(15.071), (I-655)+(15.072), (I-655)+(15.073), (I-655)+(15.074), (I-655)+(15.075), (I-655)+(15.076), (I-655)+(15.077), (I-655)+(15.078), (I-655)+(15.079), (I-655)+(15.080), (I-655)+(15.081), (I-655)+(15.082), (I-655)+(15.083), (I-655)+(15.084), (I-655) + (15.085), (I-655) + (15.086), (I-655)+(15.087), (I-655)+(15.088), (I-655)+(15.089), (I-655)+(15.090), (I-655)+(15.091), (I-655)+(15.092), (I-655)+(15.093), (I-655)+(15.094), (I-655)+(15.095), (I-655)+(15.096), (I-655)+(15.097), (I-655)+(15.098), (I-655)+(15.099), (I-655)+(15.100), (I-655)+(15.101), (I-655)+(15.102), (I-655)+(15.103), (I-655)+(15.104), (I-655)+(15.105), (I-655)+(15.106), (I-655)+(15.107), (I-655)+(15.108), (I-655)+(15.109), (I-655)+(15.110), (I-655)+(15.111), (I-655)+(15.112), (I-655)+(15.113), (I-655)+(15.114), (I-655)+(15.115), (I-655)+(15.116), (I-655)+(15.117), (I-655)+(15.118), (I-655)+(15.119), (I-655)+(15.120), (I-655)+(15.121), (I-655)+(15.122), (I-655)+(15.123), (I-655)+(15.124), (I-655)+(15.125), (I-655)+(15.126), (I-655)+(15.127), (I-655)+(15.128), (I-655)+(16.001), (I-655)+(16.002), (I-655)+(16.003), (I-655)+(16.004), (I-655)+(16.005), (I-655)+(16.006), (I-655)+(16.007), (I-655)+(16.008), (I-655)+(17.001), (I-655)+(17.002), (I-655)+(17.003), (I-655)+(17.004), (I-655)+(17.005), (I-655)+(17.006), (I-655)+(17.007), (I-655)+(17.008), (I-655)+(17.009), (I-655)+(17.010), (I-655)+(17.011), (I-655)+(17.012) and (I-655)+(18.001).

[0209] Preferred compound combinations are also selected from the group (G2) consisting of the following mixtures: (I-667)+(1.001), (I-667)+(1.002), (I-667)+(1.003), (I-667)+(1.004), (I-667)+(1.005), (I-667)+(1.006), (I-667)+(1.007), (I-667)+(1.008), (I-667)+(1.009), (I-667)+(1.010), (I-667)+(1.011), (I-667)+(1.012), (I-667)+(1.013), (I-667)+(1.014), (I-667)+(1.015), (I-667)+(1.016), (I-667)+(1.017), (I-667)+(1.018), (I-667)+(1.019), (I-667)+(1.020), (I-667)+(1.021), (I-667)+(1.022), (I-667)+(1.023), (I-667)+(1.024), (I-667)+(1.025), (I-667)+(1.026), (I-667)+(1.027), (I-667)+(1.028), (I-667)+(1.029), (I-667)+(1.030), (I-667)+(1.031), (I-667)+(1.032), (I-667)+(1.033), (I-667)+(1.034), (I-667)+(1.035), (I-667)+(1.036), (I-667)+(1.037), (I-667)+(1.038), (I-667)+(1.039), (I-667)+(1.040), (I-667)+(1.041), (I-667)+(1.042), (I-667)+(1.043), (I-667)+(1.044), (I-667)+(1.045), (I-667)+(1.046), (I-667)+(1.047), (I-667)+(1.048), (I-667)+(1.049), (I-667)+(1.050), (I-667)+(1.051), (I-667)+(1.052), (I-667)+(1.053), (I-667)+(1.054), (I-667)+(1.055), (I-667)+(1.056), (I-667)+(1.057), (I-667)+(1.058), (I-667)+(1.059), (I-667)+(1.060), (I-667)+(1.061), (I-667)+(1.062), (I-667)+(1.063), (I-667)+(1.064), (I-667)+(1.065), (I-667)+(1.066), (I-667)+(1.067), (I-667)+(1.068), (I-667)+(1.069), (I-667)+(1.070), (I-667)+(1.071), (I-667)+(1.072), (I-667)+(1.073), (I-667)+(1.074), (I-667)+(1.075), (I-667)+(1.076), (I-667)+(1.077), (I-667)+(1.078), (I-667)+(1.079), (I-667)+(1.080), (I-667)+(1.081), (I-667)+(1.082), (I-667)+(1.083), (I-667)+(1.084), (I-667)+(1.085), (I-667)+(1.086), (I-667)+(1.087), (I-667)+(1.088), (I-667)+(1.089), (I-667)+(1.090), (I-667)+(1.091), (I-667)+(1.092), (I-667)+(2.001), (I-667)+(2.002), (I-667)+(2.003), (I-667)+(2.004), (I-667)+(2.005), (I-667)+(2.006), (I-667)+(2.007), (I-667)+(2.008), (I-667)+(2.009), (I-667)+(2.010), (I-667)+(2.011), (I-667)+(2.012), (I-667)+(2.013), (I-667)+(2.014), (I-667)+(2.015), (I-667)+(2.016), (I-667)+(2.017), (I-667)+(2.018), (I-667)+(2.019), (I-667)+(2.020), (I-667)+(2.021), (I-667)+(2.022), (I-667)+(2.023), (I-667)+(2.024), (I-667)+(2.025), (I-667)+(2.026), (I-667)+(2.027), (I-667)+(2.028), (I-667)+(2.029), (I-667)+(2.030), (I-667)+(2.031), (I-667)+(2.032), (I-667)+(2.033), (I-667)+(2.034), (I-667)+(2.035), (I-667)+(2.036), (I-667)+(2.037), (I-667)+(2.038), (I-667)+(2.039), (I-667)+(2.040), (I-667)+(2.041), (I-667)+(2.042), (I-667)+(2.043), (I-667)+(2.044), (I-667)+(2.045), (I-667)+(2.046), (I-667)+(2.047), (I-667)+(2.048), (I-667)+(2.049), (I-667)+(2.050), (I-667)+(2.051), (I-667)+(2.052), (I-667)+(2.053), (I-667)+(2.054), (I-667)+(2.055), (I-667)+(2.056), (I-667)+(2.057), (I-667)+(2.058), (I-667)+(2.059), (I-667)+(2.060), (I-667)+(3.001), (I-667)+(3.002), (I-667)+(3.003), (I-667)+(3.004), (I-667)+(3.005), (I-667)+(3.006), (I-667)+(3.007), (I-667)+(3.008), (I-667)+(3.009), (I-667)+(3.010), (I-667)+(3.011), (I-667)+(3.012), (I-667)+(3.013), (I-667)+(3.014), (I-667)+(3.015), (I-667)+(3.016), (I-667)+(3.017), (I-667)+(3.018), (I-667)+(3.019), (I-667)+(3.020), (I-667)+(3.021), (I-667)+(3.022), (I-667)+(3.023), (I-667)+(3.024), (I-667)+(3.025), (I-667)+(3.026), (I-667)+(3.027), (I-667)+(3.028), (I-667)+(3.029), (I-667)+(3.030), (I-667)+(3.031), (I-667)+(3.032), (I-667)+(4.001), (I-667)+(4.002), (I-667)+(4.003), (I-667)+(4.004), (I-667)+(4.005), (I-667)+(4.006), (I-667)+(4.007), (I-667)+(4.008), (I-667)+(4.009), (I-667)+(4.010), (I-667)+(4.011), (I-667)+(4.012), (I-667)+(4.013), (I-667)+(4.014), (I-667)+(4.015), (I-667)+(4.016), (I-667)+(4.017), (I-667)+(4.018), (I-667)+(4.019), (I-667)+(4.020), (I-667)+(4.021), (I-667)+(4.022), (I-667)+(4.023), (I-667)+(4.024), (I-667)+(4.025), (I-667)+(4.026), (I-667)+(5.001), (I-667)+(5.002), (I-667)+(5.003), (I-667)+(5.004), (I-667)+(5.005), (I-667)+(5.006), (I-667)+(5.007), (I-667)+(5.008), (I-667)+(5.009), (I-667)+(5.010), (I-667)+(5.011), (I-667)+(5.012), (I-667)+(5.013), (I-667)+(5.014), (I-667)+(5.015), (I-667)+(5.016), (I-667)+(5.017), (I-667)+(5.018), (I-667)+(5.019), (I-667)+(5.020), (I-667)+(5.021), (I-667)+(5.022), (I-667)+(5.023), (I-667)+(6.001), (I-667)+(6.002), (I-667)+(6.003), (I-667)+(6.004), (I-667)+(7.001), (I-667)+(7.002), (I-667)+(7.003), (I-667)+(7.004), (I-667)+(7.005), (I-667)+(7.006), (I-667)+(8.001), (I-667)+(9.001), (I-667)+(9.002), (I-667)+(9.003), (I-667)+(9.004), (I-667)+(9.005), (I-667)+(9.006), (I-667)+(9.007), (I-667)+(9.008), (I-667)+(9.009), (I-667)+(10.001), (I-667)+(10.002), (I-667)+(10.003), (I-667)+(11.001), (I-667)+(11.002), (I-667)+(12.001), (I-667)+(12.002), (I-667)+(12.003), (I-667)+(12.004), (I-667)+(13.001), (I-667)+(13.002), (I-667)+(13.003), (I-667)+(13.004), (I-667)+(13.005), (I-667)+(13.006), (I-667)+(14.001), (I-667)+(14.002), (I-667)+(15.001), (I-667)+(15.002), (I-667)+(15.003), (I-667)+(15.004), (I-667)+(15.005), (I-667)+(15.006), (I-667)+(15.007), (I-667)+(15.008), (I-667)+(15.009), (I-667)+(15.010), (I-667)+(15.011), (I-667)+(15.012), (I-667)+(15.013), (I-667)+(15.014), (I-667)+(15.015), (I-667)+(15.016), (I-667)+(15.017), (I-667)+(15.018), (I-667)+(15.019), (I-667)+(15.020), (I-667)+(15.021), (I-667)+(15.022), (I-667)+(15.023), (I-667)+(15.024), (I-667)+(15.025), (I-667)+(15.026), (I-667)+(15.027), (I-667)+(15.028), (I-667)+(15.029), (I-667)+(15.030), (I-667)+(15.031), (I-667)+(15.032), (I-667)+(15.033), (I-667)+(15.034), (I-667)+(15.035), (I-667)+(15.036), (I-667)+(15.037), (I-667)+(15.038), (I-667)+(15.039), (I-667)+(15.040), (I-667)+(15.041), (I-667)+(15.042), (I-667)+(15.043), (I-667)+(15.044), (I-667)+(15.045), (I-667)+(15.046), (I-667)+(15.047), (I-667)+(15.048), (I-667)+(15.049), (I-667)+(15.050), (I-667)+(15.051), (I-667)+(15.052), (I-667)+(15.053), (I-667)+(15.054), (I-667)+(15.055), (I-667)+(15.056), (I-667)+(15.057), (I-667)+(15.058), (I-667)+(15.059), (I-667)+(15.060), (I-667)+(15.061), (I-667)+(15.062), (I-667)+(15.063), (I-667)+(15.064), (I-667)+(15.065), (I-667)+(15.066), (I-667)+(15.067), (I-667)+(15.068), (I-667)+(15.069), (I-667)+(15.070), (I-667)+(15.071), (I-667)+(15.072), (I-667)+(15.073), (I-667)+(15.074), (I-667)+(15.075), (I-667)+(15.076), (I-667)+(15.077), (I-667)+(15.078), (I-667)+(15.079), (I-667)+(15.080), (I-667)+(15.081), (I-667)+(15.082), (I-667)+(15.083), (I-667)+(15.084), (I-667)+(15.085), (I-667)+(15.086), (I-667)+(15.087), (I-667)+(15.088), (I-667)+(15.089), (I-667)+(15.090), (I-667)+(15.091), (I-667)+(15.092), (I-667)+(15.093), (I-667)+(15.094), (I-667)+(15.095), (I-667)+(15.096), (I-667)+(15.097), (I-667)+(15.098), (I-667)+(15.099), (I-667)+(15.100), (I-667)+(15.101), (I-667)+(15.102), (I-667)+(15.103), (I-667)+(15.104), (I-667)+(15.105), (I-667)+(15.106), (I-667)+(15.107), (I-667)+(15.108), (I-667)+(15.109), (I-667)+(15.110), (I-667)+(15.111), (I-667)+(15.112), (I-667)+(15.113), (I-667)+(15.114), (I-667)+(15.115), (I-667)+(15.116), (I-667)+(15.117), (I-667)+(15.118), (I-667)+(15.119), (I-667)+(15.120), (I-667)+(15.121), (I-667)+(15.122), (I-667)+(15.123), (I-667)+(15.124), (I-667)+(15.125), (I-667)+(15.126), (I-667)+(15.127), (I-667)+(15.128), (I-667)+(16.001), (I-667)+(16.002), (I-667)+(16.003), (I-667)+(16.004), (I-667)+(16.005), (I-667)+(16.006), (I-667)+(16.007), (I-667)+(16.008), (I-667)+(17.001), (I-667)+(17.002), (I-667)+(17.003), (I-667)+(17.004), (I-667)+(17.005), (I-667)+(17.006), (I-667)+(17.007), (I-667)+(17.008), (I-667)+(17.009), (I-667)+(17.010), (I-667)+(17.011), (I-667)+(17.012) and (I-667)+(18.001).

[0210] Preferred compound combinations are also selected from the group (G3) consisting of the following mixtures: (I-746)+(1.001), (I-746)+(1.002), (I-746)+(1.003), (I-746)+(1.004), (I-746)+(1.005), (I-746)+(1.006), (I-746)+(1.007), (I-746)+(1.008), (I-746)+(1.009), (I-746)+(1.010), (I-746)+(1.011), (I-746)+(1.012), (I-746)+(1.013), (I-746)+(1.014), (I-746)+(1.015), (I-746)+(1.016), (I-746)+(1.017), (I-746)+(1.018), (I-746)+(1.019), (I-746)+(1.020), (I-746)+(1.021), (I-746)+(1.022), (I-746)+(1.023), (I-746)+(1.024), (I-746)+(1.025), (I-746)+(1.026), (I-746)+(1.027), (I-746)+(1.028), (I-746)+(1.029), (I-746)+(1.030), (I-746)+(1.031), (I-746)+(1.032), (I-746)+(1.033), (I-746)+(1.034), (I-746)+(1.035), (I-746)+(1.036), (I-746)+(1.037), (I-746)+(1.038), (I-746)+(1.039), (I-746)+(1.040), (I-746)+(1.041), (I-746)+(1.042), (I-746)+(1.043), (I-746)+(1.044), (I-746)+(1.045), (I-746)+(1.046), (I-746)+(1.047), (I-746)+(1.048), (I-746)+(1.049), (I-746)+(1.050), (I-746)+(1.051), (I-746)+(1.052), (I-746)+(1.053), (I-746)+(1.054), (I-746)+(1.055), (I-746)+(1.056), (I-746)+(1.057), (I-746)+(1.058), (I-746)+(1.059), (I-746)+(1.060), (I-746)+(1.061), (I-746)+(1.062), (I-746)+(1.063), (I-746)+(1.064), (I-746)+(1.065), (I-746)+(1.066), (I-746)+(1.067), (I-746)+(1.068), (I-746)+(1.069), (I-746)+(1.070), (I-746)+(1.071), (I-746)+(1.072), (I-746)+(1.073), (I-746)+(1.074), (I-746)+(1.075), (I-746)+(1.076), (I-746)+(1.077), (I-746)+(1.078), (I-746)+(1.079), (I-746)+(1.080), (I-746)+(1.081), (I-746)+(1.082), (I-746)+(1.083), (I-746)+(1.084), (I-746)+(1.085), (I-746)+(1.086), (I-746)+(1.087), (I-746)+(1.088), (I-746)+(1.089), (I-746)+(1.090), (I-746)+(1.091), (I-746)+(1.092), (I-746)+(2.001), (I-746)+(2.002), (I-746)+(2.003), (I-746)+(2.004), (I-746)+(2.005), (I-746)+(2.006), (I-746)+(2.007), (I-746)+(2.008), (I-746)+(2.009), (I-746)+(2.010), (I-746)+(2.011), (I-746)+(2.012), (I-746)+(2.013), (I-746)+(2.014), (I-746)+(2.015), (I-746)+(2.016), (I-746)+(2.017), (I-746)+(2.018), (I-746)+(2.019), (I-746)+(2.020), (I-746)+(2.021), (I-746)+(2.022), (I-746)+(2.023), (I-746)+(2.024), (I-746)+(2.025), (I-746)+(2.026), (I-746)+(2.027), (I-746)+(2.028), (I-746)+(2.029), (I-746)+(2.030), (I-746)+(2.031), (I-746)+(2.032), (I-746)+(2.033), (I-746)+(2.034), (I-746)+(2.035), (I-746)+(2.036), (I-746)+(2.037), (I-746)+(2.038), (I-746)+(2.039), (I-746)+(2.040), (I-746)+(2.041), (I-746)+(2.042), (I-746)+(2.043), (I-746)+(2.044), (I-746)+(2.045), (I-746)+(2.046), (I-746)+(2.047), (I-746)+(2.048), (I-746)+(2.049), (I-746)+(2.050), (I-746)+(2.051), (I-746)+(2.052), (I-746)+(2.053), (I-746)+(2.054), (I-746)+(2.055), (I-746)+(2.056), (I-746)+(2.057), (I-746)+(2.058), (I-746)+(2.059), (I-746)+(2.060), (I-746)+(3.001), (I-746)+(3.002), (I-746)+(3.003), (I-746)+(3.004), (I-746)+(3.005), (I-746)+(3.006), (I-746)+(3.007), (I-746)+(3.008), (I-746)+(3.009), (I-746)+(3.010), (I-746)+(3.011), (I-746)+(3.012), (I-746)+(3.013), (I-746)+(3.014), (I-746)+(3.015), (I-746)+(3.016), (I-746)+(3.017), (I-746)+(3.018), (I-746)+(3.019), (I-746)+(3.020), (I-746)+(3.021), (I-746)+(3.022), (I-746)+(3.023), (I-746)+(3.024), (I-746)+(3.025), (I-746)+(3.026), (I-746)+(3.027), (I-746)+(3.028), (I-746)+(3.029), (I-746)+(3.030), (I-746)+(3.031), (I-746)+(3.032), (I-746)+(4.001), (I-746)+(4.002), (I-746)+(4.003), (I-746)+(4.004), (I-746)+(4.005), (I-746)+(4.006), (I-746)+(4.007), (I-746)+(4.008), (I-746)+(4.009), (I-746)+(4.010), (I-746)+(4.011), (I-746)+(4.012), (I-746)+(4.013), (I-746)+(4.014), (I-746)+(4.015), (I-746)+(4.016), (I-746)+(4.017), (I-746)+(4.018), (I-746)+(4.019), (I-746)+(4.020), (I-746)+(4.021), (I-746)+(4.022), (I-746)+(4.023), (I-746)+(4.024), (I-746)+(4.025), (I-746)+(4.026), (I-746)+(5.001), (I-746)+(5.002), (I-746)+(5.003), (I-746)+(5.004), (I-746)+(5.005), (I-746)+(5.006), (I-746)+(5.007), (I-746)+(5.008), (I-746)+(5.009), (I-746)+(5.010), (I-746)+(5.011), (I-746)+(5.012), (I-746)+(5.013), (I-746)+(5.014), (I-746)+(5.015), (I-746)+(5.016), (I-746)+(5.017), (I-746)+(5.018), (I-746)+(5.019), (I-746)+(5.020), (I-746)+(5.021), (I-746)+(5.022), (I-746)+(5.023), (I-746)+(6.001), (I-746)+(6.002), (I-746)+(6.003), (I-746)+(6.004), (I-746)+(7.001), (I-746)+(7.002), (I-746)+(7.003), (I-746)+(7.004), (I-746)+(7.005), (I-746)+(7.006), (I-746)+(8.001), (I-746)+(9.001), (I-746)+(9.002), (I-746)+(9.003), (I-746)+(9.004), (I-746)+(9.005), (I-746)+(9.006), (I-746)+(9.007), (I-746)+(9.008), (I-746)+(9.009), (I-746)+(10.001), (I-746)+(10.002), (I-746)+(10.003), (I-746)+(11.001), (I-746)+(11.002), (I-746)+(12.001), (I-746)+(12.002), (I-746)+(12.003), (I-746)+(12.004), (I-746)+(13.001), (I-746)+(13.002), (I-746)+(13.003), (I-746)+(13.004), (I-746)+(13.005), (I-746)+(13.006), (I-746)+(14.001), (I-746)+(14.002), (I-746)+(15.001), (I-746)+(15.002), (I-746)+(15.003), (I-746)+(15.004), (I-746)+(15.005), (I-746)+(15.006), (I-746)+(15.007), (I-746)+(15.008), (I-746)+(15.009), (I-746)+(15.010), (I-746)+(15.011), (I-746)+(15.012), (I-746)+(15.013), (I-746)+(15.014), (I-746)+(15.015), (I-746)+(15.016), (I-746)+(15.017), (I-746)+(15.018), (I-746)+(15.019), (I-746)+(15.020), (I-746)+(15.021), (I-746)+(15.022), (I-746)+(15.023), (I-746)+(15.024), (I-746)+(15.025), (I-746)+(15.026), (I-746)+(15.027), (I-746)+(15.028), (I-746)+(15.029), (I-746)+(15.030), (I-746)+(15.031), (I-746)+(15.032), (I-746)+(15.033), (I-746)+(15.034), (I-746)+(15.035), (I-746)+(15.036), (I-746)+(15.037), (I-746)+(15.038), (I-746)+(15.039), (I-746)+(15.040), (I-746)+(15.041), (I-746)+(15.042), (I-746)+(15.043), (I-746)+(15.044), (I-746)+(15.045), (I-746)+(15.046), (I-746)+(15.047), (I-746)+(15.048), (I-746)+(15.049), (I-746)+(15.050), (I-746)+(15.051), (I-746)+(15.052), (I-746)+(15.053), (I-746)+(15.054), (I-746)+(15.055), (I-746)+(15.056), (I-746)+(15.057), (I-746)+(15.058), (I-746)+(15.059), (I-746)+(15.060), (I-746)+(15.061), (I-746)+(15.062), (I-746)+(15.063), (I-746)+(15.064), (I-746)+(15.065), (I-746)+(15.066), (I-746)+(15.067), (I-746)+(15.068), (I-746)+(15.069), (I-746)+(15.070), (I-746)+(15.071), (I-746)+(15.072), (I-746)+(15.073), (I-746)+(15.074), (I-746)+(15.075), (I-746)+(15.076), (I-746)+(15.077), (I-746)+(15.078), (I-746)+(15.079), (I-746)+(15.080), (I-746)+(15.081), (I-746)+(15.082), (I-746)+(15.083), (I-746)+(15.084), (I-746)+(15.085), (I-746)+(15.086), (I-746)+(15.087), (I-746)+(15.088), (I-746)+(15.089), (I-746)+(15.090), (I-746)+(15.091), (I-746)+(15.092), (I-746)+(15.093), (I-746)+(15.094), (I-746)+(15.095), (I-746)+(15.096), (I-746)+(15.097), (I-746)+(15.098), (I-746)+(15.099), (I-746)+(15.100), (I-746)+(15.101), (I-746)+(15.102), (I-746)+(15.103), (I-746)+(15.104), (I-746)+(15.105), (I-746)+(15.106), (I-746)+(15.107), (I-746)+(15.108), (I-746)+(15.109), (I-746)+(15.110), (I-746)+(15.111), (I-746)+(15.112), (I-746)+(15.113), (I-746)+(15.114), (I-746)+(15.115), (I-746)+(15.116), (I-746)+(15.117), (I-746)+(15.118), (I-746)+(15.119), (I-746)+(15.120), (I-746)+(15.121), (I-746)+(15.122), (I-746)+(15.123), (I-746)+(15.124), (I-746)+(15.125), (I-746)+(15.126), (I-746)+(15.127), (I-746)+(15.128), (I-746)+(16.001), (I-746)+(16.002), (I-746)+(16.003), (I-746)+(16.004), (I-746)+(16.005), (I-746)+(16.006), (I-746)+(16.007), (I-746)+(16.008), (I-746)+(17.001), (I-746)+(17.002), (I-746)+(17.003), (I-746)+(17.004), (I-746)+(17.005), (I-746)+(17.006), (I-746)+(17.007), (I-746)+(17.008), (I-746)+(17.009), (I-746)+(17.010), (I-746)+(17.011), (I-746)+(17.012) and (I-746)+(18.001).

[0211] Preferred compound combinations are also selected from the group (G4) consisting of the following mixtures: (I-749)+(1.001), (I-749)+(1.002), (I-749)+(1.003), (I-749)+(1.004), (I-749)+(1.005), (I-749)+(1.006), (I-749)+(1.007), (I-749)+(1.008), (I-749)+(1.009), (I-749)+(1.010), (I-749)+(1.011), (I-749)+(1.012), (I-749)+(1.013), (I-749)+(1.014), (I-749)+(1.015), (I-749)+(1.016), (I-749)+(1.017), (I-749)+(1.018), (I-749)+(1.019), (I-749)+(1.020), (I-749)+(1.021), (I-749)+(1.022), (I-749)+(1.023), (I-749)+(1.024), (I-749)+(1.025), (I-749)+(1.026), (I-749)+(1.027), (I-749)+(1.028), (I-749)+(1.029), (I-749)+(1.030), (I-749)+(1.031), (I-749)+(1.032), (I-749)+(1.033), (I-749)+(1.034), (I-749)+(1.035), (I-749)+(1.036), (I-749)+(1.037), (I-749)+(1.038), (I-749)+(1.039), (I-749)+(1.040), (I-749)+(1.041), (I-749)+(1.042), (I-749)+(1.043), (I-749)+(1.044), (I-749)+(1.045), (I-749)+(1.046), (I-749)+(1.047), (I-749)+(1.048), (I-749)+(1.049), (I-749)+(1.050), (I-749)+(1.051), (I-749)+(1.052), (I-749)+(1.053), (I-749)+(1.054), (I-749)+(1.055), (I-749)+(1.056), (I-749)+(1.057), (I-749)+(1.058), (I-749)+(1.059), (I-749)+(1.060), (I-749)+(1.061), (I-749)+(1.062), (I-749)+(1.063), (I-749)+(1.064), (I-749)+(1.065), (I-749)+(1.066), (I-749)+(1.067), (I-749)+(1.068), (I-749)+(1.069), (I-749)+(1.070), (I-749)+(1.071), (I-749)+(1.072), (I-749)+(1.073), (I-749)+(1.074), (I-749)+(1.075), (I-749)+(1.076), (I-749)+(1.077), (I-749)+(1.078), (I-749)+(1.079), (I-749)+(1.080), (I-749)+(1.081), (I-749)+(1.082), (I-749)+(1.083), (I-749)+(1.084), (I-749)+(1.085), (I-749)+(1.086), (I-749)+(1.087), (I-749)+(1.088), (I-749)+(1.089), (I-749)+(1.090), (I-749)+(1.091), (I-749)+(1.092), (I-749)+(2.001), (I-749)+(2.002), (I-749)+(2.003), (I-749)+(2.004), (I-749)+(2.005), (I-749)+(2.006), (I-749)+(2.007), (I-749)+(2.008), (I-749)+(2.009), (I-749)+(2.010), (I-749)+(2.011), (I-749)+(2.012), (I-749)+(2.013), (I-749)+(2.014), (I-749)+(2.015), (I-749)+(2.016), (I-749)+(2.017), (I-749)+(2.018), (I-749)+(2.019), (I-749)+(2.020), (I-749)+(2.021), (I-749)+(2.022), (I-749)+(2.023), (I-749)+(2.024), (I-749)+(2.025), (I-749)+(2.026), (I-749)+(2.027), (I-749)+(2.028), (I-749)+(2.029), (I-749)+(2.030), (I-749)+(2.031), (I-749)+(2.032), (I-749)+(2.033), (I-749)+(2.034), (I-749)+(2.035), (I-749)+(2.036), (I-749)+(2.037), (I-749)+(2.038), (I-749)+(2.039), (I-749)+(2.040), (I-749)+(2.041), (I-749)+(2.042), (I-749)+(2.043), (I-749)+(2.044), (I-749)+(2.045), (I-749)+(2.046), (I-749)+(2.047), (I-749)+(2.048), (I-749)+(2.049), (I-749)+(2.050), (I-749)+(2.051), (I-749)+(2.052), (I-749)+(2.053), (I-749)+(2.054), (I-749)+(2.055), (I-749)+(2.056), (I-749)+(2.057), (I-749)+(2.058), (I-749)+(2.059), (I-749)+(2.060), (I-749)+(3.001), (I-749)+(3.002), (I-749)+(3.003), (I-749)+(3.004), (I-749)+(3.005), (I-749)+(3.006), (I-749)+(3.007), (I-749)+(3.008), (I-749)+(3.009), (I-749)+(3.010), (I-749)+(3.011), (I-749)+(3.012), (I-749)+(3.013), (I-749)+(3.014), (I-749)+(3.015), (I-749)+(3.016), (I-749)+(3.017), (I-749)+(3.018), (I-749)+(3.019), (I-749)+(3.020), (I-749)+(3.021), (I-749)+(3.022), (I-749)+(3.023), (I-749)+(3.024), (I-749)+(3.025), (I-749)+(3.026), (I-749)+(3.027), (I-749)+(3.028), (I-749)+(3.029), (I-749)+(3.030), (I-749)+(3.030), (I-749)+(3.031), (I-749)+(4.001), (I-749)+(4.002), (I-749)+(4.003), (I-749)+(4.004), (I-749)+(4.005), (I-749)+(4.006), (I-749)+(4.007), (I-749)+(4.008), (I-749)+(4.009), (I-749)+(4.010), (I-749)+(4.011), (I-749)+(4.012), (I-749)+(4.013), (I-749)+(4.014), (I-749)+(4.015), (I-749)+(4.016), (I-749)+(4.017), (I-749)+(4.018), (I-749)+(4.019), (I-749)+(4.020), (I-749)+(4.021), (I-749)+(4.022), (I-749)+(4.023), (I-749)+(4.024), (I-749)+(4.025), (I-749)+(4.026), (I-749)+(5.001), (I-749)+(5.002), (I-749)+(5.003), (I-749)+(5.004), (I-749)+(5.005), (I-749)+(5.006), (I-749)+(5.007), (I-749)+(5.008), (I-749)+(5.009), (I-749)+(5.010), (I-749)+(5.011), (I-749)+(5.012), (I-749)+(5.013), (I-749)+(5.014), (I-749)+(5.015), (I-749)+(5.016), (I-749)+(5.017), (I-749)+(5.018), (I-749)+(5.019), (I-749)+(5.020), (I-749)+(5.021), (I-749)+(5.022), (I-749)+(5.023), (I-749)+(6.001), (I-749)+(6.002), (I-749)+(6.003), (I-749)+(6.004), (I-749)+(7.001), (I-749)+(7.002), (I-749)+(7.003), (I-749)+(7.004), (I-749)+(7.005), (I-749)+(7.006), (I-749)+(8.001), (I-749)+(9.001), (I-749)+(9.002), (I-749)+(9.003), (I-749)+(9.004), (I-749)+(9.005), (I-749)+(9.006), (I-749)+(9.007), (I-749)+(9.008), (I-749)+(9.009), (I-749)+(10.001), (I-749)+(10.002), (I-749)+(10.003), (I-749)+(11.001), (I-749)+(11.002), (I-749)+(12.001), (I-749)+(12.002), (I-749)+(12.003), (I-749)+(12.004), (I-749)+(13.001), (I-749)+(13.002), (I-749)+(13.003), (I-749)+(13.004), (I-749)+(13.005), (I-749)+(13.006), (I-749)+(14.001), (I-749)+(14.002), (I-749)+(15.001), (I-749)+(15.002), (I-749)+(15.003), (I-749)+(15.004), (I-749)+(15.005), (I-749)+(15.006), (I-749)+(15.007), (I-749)+(15.008), (I-749)+(15.009), (I-749)+(15.010), (I-749)+(15.011), (I-749)+(15.012), (I-749)+(15.013), (I-749)+(15.014), (I-749)+(15.015), (I-749)+(15.016), (I-749)+(15.017), (I-749)+(15.018), (I-749)+(15.019), (I-749)+(15.020), (I-749)+(15.021), (I-749)+(15.022), (I-749)+(15.023), (I-749)+(15.024), (I-749)+(15.025), (I-749)+(15.026), (I-749)+(15.027), (I-749)+(15.028), (I-749)+(15.029), (I-749)+(15.030), (I-749)+(15.031), (I-749)+(15.032), (I-749)+(15.033), (I-749)+(15.034), (I-749)+(15.035), (I-749)+(15.036), (I-749)+(15.037), (I-749)+(15.038), (I-749)+(15.039), (I-749)+(15.040), (I-749)+(15.041), (I-749)+(15.042), (I-749)+(15.043), (I-749)+(15.044), (I-749)+(15.045), (I-749)+(15.046), (I-749)+(15.047), (I-749)+(15.048), (I-749)+(15.049), (I-749)+(15.050), (I-749)+(15.051), (I-749)+(15.052), (I-749)+(15.053), (I-749)+(15.054), (I-749)+(15.055), (I-749)+(15.056), (I-749)+(15.057), (I-749)+(15.058), (I-749)+(15.059), (I-749)+(15.060), (I-749)+(15.061), (I-749)+(15.062), (I-749)+(15.063), (I-749)+(15.064), (I-749)+(15.065), (I-749)+(15.066), (I-749)+(15.067), (I-749)+(15.068), (I-749)+(15.069), (I-749)+(15.070), (I-749)+(15.071), (I-749)+(15.072), (I-749)+(15.073), (I-749)+(15.074), (I-749)+(15.075), (I-749)+(15.076), (I-749)+(15.077), (I-749)+(15.078), (I-749)+(15.079), (I-749)+(15.080), (I-749)+(15.081), (I-749)+(15.082), (I-749)+(15.083), (I-749)+(15.084), (I-749)+(15.085), (I-749)+(15.086), (I-749)+(15.087), (I-749)+(15.088), (I-749)+(15.089), (I-749)+(15.090), (I-749)+(15.091), (I-749)+(15.092), (I-749)+(15.093), (I-749)+(15.094), (I-749)+(15.095), (I-749)+(15.096), (I-749)+(15.097), (I-749)+(15.098), (I-749)+(15.099), (I-749)+(15.100), (I-749)+(15.101), (I-749)+(15.102), (I-749)+(15.103), (I-749)+(15.104), (I-749)+(15.105), (I-749)+(15.106), (I-749)+(15.107), (I-749)+(15.108), (I-749)+(15.109), (I-749)+(15.110), (I-749)+(15.111), (I-749)+(15.112), (I-749)+(15.113), (I-749)+(15.114), (I-749)+(15.115), (I-749)+(15.116), (I-749)+(15.117), (I-749)+(15.118), (I-749)+(15.119), (I-749)+(15.120), (I-749)+(15.121), (I-749)+(15.122), (I-749)+(15.123), (I-749)+(15.124), (I-749)+(15.125), (I-749)+(15.126), (I-749)+(15.127), (I-749)+(15.128), (I-749)+(16.1001), (I-749)+(16.1002), (I-749)+(16.1003), (I-749)+(16.1004), (I-749)+(16.1005), (I-749)+(16.2001), (I-749)+(16.2002), (I-749)+(16.2003), (I-749)+(17.001), (I-749)+(17.002), (I-749)+(17.003), (I-749)+(17.004), (I-749)+(17.005), (I-749)+(17.006), (I-749)+(17.007), (I-749)+(17.008), (I-749)+(17.009), (I-749)+(17.010), (I-749)+(17.011), (I-749)+(17.012) and (I-749)+(18.001).

[0212] Preferred compound combinations are also selected from the group (G5) consisting of the following mixtures: (I-784)+(1.001), (I-784)+(1.002), (I-784)+(1.003), (I-784)+(1.004), (I-784)+(1.005), (I-784)+(1.006), (I-784)+(1.007), (I-784)+(1.008), (I-784)+(1.009), (I-784)+(1.010), (I-784)+(1.011), (I-784)+(1.012), (I-784)+(1.013), (I-784)+(1.014), (I-784)+(1.015), (I-784)+(1.016), (I-784)+(1.017), (I-784)+(1.018), (I-784)+(1.019), (I-784)+(1.020), (I-784)+(1.021), (I-784)+(1.022), (I-784)+(1.023), (I-784)+(1.024), (I-784)+(1.025), (I-784)+(1.026), (I-784)+(1.027), (I-784)+(1.028), (I-784)+(1.029), (I-784)+(1.030), (I-784)+(1.031), (I-784)+(1.032), (I-784)+(1.033), (I-784)+(1.034), (I-784)+(1.035), (I-784)+(1.036), (I-784)+(1.037), (I-784)+(1.038), (I-784)+(1.039), (I-784)+(1.040), (I-784)+(1.041), (I-784)+(1.042), (I-784)+(1.043), (I-784)+(1.044), (I-784)+(1.045), (I-784)+(1.046), (I-784)+(1.047), (I-784)+(1.048), (I-784)+(1.049), (I-784)+(1.050), (I-784)+(1.051), (I-784)+(1.052), (I-784)+(1.053), (I-784)+(1.054), (I-784)+(1.055), (I-784)+(1.056), (I-784)+(1.057), (I-784)+(1.058), (I-784)+(1.059), (I-784)+(1.060), (I-784)+(1.061), (I-784)+(1.062), (I-784)+(1.063), (I-784)+(1.064), (I-784)+(1.065), (I-784)+(1.066), (I-784)+(1.067), (I-784)+(1.068), (I-784)+(1.069), (I-784)+(1.070), (I-784)+(1.071), (I-784)+(1.072), (I-784)+(1.073), (I-784)+(1.074), (I-784)+(1.075), (I-784)+(1.076), (I-784)+(1.077), (I-784)+(1.078), (I-784)+(1.079), (I-784)+(1.080), (I-784)+(1.081), (I-784)+(1.082), (I-784)+(1.083), (I-784)+(1.084), (I-784)+(1.085), (I-784)+(1.086), (I-784)+(1.087), (I-784)+(1.088), (I-784)+(1.089), (I-784)+(1.090), (I-784)+(1.091), (I-784)+(1.092), (I-784)+(2.001), (I-784)+(2.002), (I-784)+(2.003), (I-784)+(2.004), (I-784)+(2.005), (I-784)+(2.006), (I-784)+(2.007), (I-784)+(2.008), (I-784)+(2.009), (I-784)+(2.010), (I-784)+(2.011), (I-784)+(2.012), (I-784)+(2.013), (I-784)+(2.014), (I-784)+(2.015), (I-784)+(2.016), (I-784)+(2.017), (I-784)+(2.018), (I-784)+(2.019), (I-784)+(2.020), (I-784)+(2.021), (I-784)+(2.022), (I-784)+(2.023), (I-784)+(2.024), (I-784)+(2.025), (I-784)+(2.026), (I-784)+(2.027), (I-784)+(2.028), (I-784)+(2.029), (I-784)+(2.030), (I-784)+(2.031), (I-784)+(2.032), (I-784)+(2.033), (I-784)+(2.034), (I-784)+(2.035), (I-784)+(2.036), (I-784)+(2.037), (I-784)+(2.038), (I-784)+(2.039), (I-784)+(2.040), (I-784)+(2.041), (I-784)+(2.042), (I-784)+(2.043), (I-784)+(2.044), (I-784)+(2.045), (I-784)+(2.046), (I-784)+(2.047), (I-784)+(2.048), (I-784)+(2.049), (I-784)+(2.050), (I-784)+(2.051), (I-784)+(2.052), (I-784)+(2.053), (I-784)+(2.054), (I-784)+(2.055), (I-784)+(2.056), (I-784)+(2.057), (I-784)+(2.058), (I-784)+(2.059), (I-784)+(2.060), (I-784)+(3.001), (I-784)+(3.002), (I-784)+(3.003), (I-784)+(3.004), (I-784)+(3.005), (I-784)+(3.006), (I-784)+(3.007), (I-784)+(3.008), (I-784)+(3.009), (I-784)+(3.010), (I-784)+(3.011), (I-784)+(3.012), (I-784)+(3.013), (I-784)+(3.014), (I-784)+(3.015), (I-784)+(3.016), (I-784)+(3.017), (I-784)+(3.018), (I-784)+(3.019), (I-784)+(3.020), (I-784)+(3.021), (I-784)+(3.022), (I-784)+(3.023), (I-784)+(3.024), (I-784)+(3.025), (I-784)+(3.026), (I-784)+(3.027), (I-784)+(3.028), (I-784)+(3.029), (I-784)+(3.030), (I-784)+(3.031), (I-784)+(3.032), (I-784)+(4.001), (I-784)+(4.002), (I-784)+(4.003), (I-784)+(4.004), (I-784)+(4.005), (I-784)+(4.006), (I-784)+(4.007), (I-784)+(4.008), (I-784)+(4.009), (I-784)+(4.010), (I-784)+(4.011), (I-784)+(4.012), (I-784)+(4.013), (I-784)+(4.014), (I-784)+(4.015), (I-784)+(4.016), (I-784)+(4.017), (I-784)+(4.018), (I-784)+(4.019), (I-784)+(4.020), (I-784)+(4.021), (I-784)+(4.022), (I-784)+(4.023), (I-784)+(4.024), (I-784)+(4.025), (I-784)+(4.026), (I-784)+(5.001), (I-784)+(5.002), (I-784)+(5.003), (I-784)+(5.004), (I-784)+(5.005), (I-784)+(5.006), (I-784)+(5.007), (I-784)+(5.008), (I-784)+(5.009), (I-784)+(5.010), (I-784)+(5.011), (I-784)+(5.012), (I-784)+(5.013), (I-784)+(5.014), (I-784)+(5.015), (I-784)+(5.016), (I-784)+(5.017), (I-784)+(5.018), (I-784)+(5.019), (I-784)+(5.020), (I-784)+(5.021), (I-784)+(5.022), (I-784)+(5.023), (I-784)+(6.001), (I-784)+(6.002), (I-784)+(6.003), (I-784)+(6.004), (I-784)+(7.001), (I-784)+(7.002), (I-784)+(7.003), (I-784)+(7.004), (I-784)+(7.005), (I-784)+(7.006), (I-784)+(8.001), (I-784)+(9.001), (I-784)+(9.002), (I-784)+(9.003), (I-784)+(9.004), (I-784)+(9.005), (I-784)+(9.006), (I-784)+(9.007), (I-784)+(9.008), (I-784)+(9.009), (I-784)+(10.001), (I-784)+(10.002), (I-784)+(10.003), (I-784)+(11.001), (I-784)+(11.002), (I-784)+(12.001), (I-784)+(12.002), (I-784)+(12.003), (I-784)+(12.004), (I-784)+(13.001), (I-784)+(13.002), (I-784)+(13.003), (I-784)+(13.004), (I-784)+(13.005), (I-784)+(13.006), (I-784)+(14.001), (I-784)+(14.002), (I-784)+(15.001), (I-784)+(15.002), (I-784)+(15.003), (I-784)+(15.004), (I-784)+(15.005), (I-784)+(15.006), (I-784)+(15.007), (I-784)+(15.008), (I-784)+(15.009), (I-784)+(15.010), (I-784)+(15.011), (I-784)+(15.012), (I-784)+(15.013), (I-784)+(15.014), (I-784)+(15.015), (I-784)+(15.016), (I-784)+(15.017), (I-784)+(15.018), (I-784)+(15.019), (I-784)+(15.020), (I-784)+(15.021), (I-784)+(15.022), (I-784)+(15.023), (I-784)+(15.024), (I-784)+(15.025), (I-784)+(15.026), (I-784)+(15.027), (I-784)+(15.028), (I-784)+(15.029), (I-784)+(15.030), (I-784)+(15.031), (I-784)+(15.032), (I-784)+(15.033), (I-784)+(15.034), (I-784)+(15.035), (I-784)+(15.036), (I-784)+(15.037), (I-784)+(15.038), (I-784)+(15.039), (I-784)+(15.040), (I-784)+(15.041), (I-784)+(15.042), (I-784)+(15.043), (I-784)+(15.044), (I-784)+(15.045), (I-784)+(15.046), (I-784)+(15.047), (I-784)+(15.048), (I-784)+(15.049), (I-784)+(15.050), (I-784)+(15.051), (I-784)+(15.052), (I-784)+(15.053), (I-784)+(15.054), (I-784)+(15.055), (I-784)+(15.056), (I-784)+(15.057), (I-784)+(15.058), (I-784)+(15.059), (I-784)+(15.060), (I-784)+(15.061), (I-784)+(15.062), (I-784)+(15.063), (I-784)+(15.064), (I-784)+(15.065), (I-784)+(15.066), (I-784)+(15.067), (I-784)+(15.068), (I-784)+(15.069), (I-784)+(15.070), (I-784)+(15.071), (I-784)+(15.072), (I-784)+(15.073), (I-784)+(15.074), (I-784)+(15.075), (I-784)+(15.076), (I-784)+(15.077), (I-784)+(15.078), (I-784)+(15.079), (I-784)+(15.080), (I-784)+(15.081), (I-784)+(15.082), (I-784)+(15.083), (I-784)+(15.084), (I-784)+(15.085), (I-784)+(15.086), (I-784)+(15.087), (I-784)+(15.088), (I-784)+(15.089), (I-784)+(15.090), (I-784)+(15.091), (I-784)+(15.092), (I-784)+(15.093), (I-784)+(15.094), (I-784)+(15.095), (I-784)+(15.096), (I-784)+(15.097), (I-784)+(15.098), (I-784)+(15.099), (I-784)+(15.100), (I-784)+(15.101), (I-784)+(15.102), (I-784)+(15.103), (I-784)+(15.104), (I-784)+(15.105), (I-784)+(15.106), (I-784)+(15.107), (I-784)+(15.108), (I-784)+(15.109), (I-784)+(15.110), (I-784)+(15.111), (I-784)+(15.112), (I-784)+(15.113), (I-784)+(15.114), (I-784)+(15.115), (I-784)+(15.116), (I-784)+(15.117), (I-784)+(15.118), (I-784)+(15.119), (I-784)+(15.120), (I-784)+(15.121), (I-784)+(15.122), (I-784)+(15.123), (I-784)+(15.124), (I-784)+(15.125), (I-784)+(15.126), (I-784)+(15.127), (I-784)+(15.128), (I-784)+(16.001), (I-784)+(16.002), (I-784)+(16.003), (I-784)+(16.004), (I-784)+(16.005), (I-784)+(16.006), (I-784)+(16.007), (I-784)+(16.008), (I-784)+(17.001), (I-784)+(17.002), (I-784)+(17.003), (I-784)+(17.004), (I-784)+(17.005), (I-784)+(17.006), (I-784)+(17.007), (I-784)+(17.008), (I-784)+(17.009), (I-784)+(17.010), (I-784)+(17.011), (I-784)+(17.012) and (I-784)+(18.001).

[0213] Preferred compound combinations are also selected from the group (G6) consisting of the following mixtures: (I-840)+(1.001), (I-840)+(1.002), (I-840)+(1.003), (I-840)+(1.004), (I-840)+(1.005), (I-840)+(1.006), (I-840)+(1.007), (I-840)+(1.008), (I-840)+(1.009), (I-840)+(1.010), (I-840)+(1.011), (I-840)+(1.012), (I-840)+(1.013), (I-840)+(1.014), (I-840)+(1.015), (I-840)+(1.016), (I-840)+(1.017), (I-840)+(1.018), (I-840)+(1.019), (I-840)+(1.020), (I-840)+(1.021), (I-840)+(1.022), (I-840)+(1.023), (I-840)+(1.024), (I-840)+(1.025), (I-840)+(1.026), (I-840)+(1.027), (I-840)+(1.028), (I-840)+(1.029), (I-840)+(1.030), (I-840)+(1.031), (I-840)+(1.032), (I-840)+(1.033), (I-840)+(1.034), (I-840)+(1.035), (I-840)+(1.036), (I-840)+(1.037), (I-840)+(1.038), (I-840)+(1.039), (I-840)+(1.040), (I-840)+(1.041), (I-840)+(1.042), (I-840)+(1.043), (I-840)+(1.044), (I-840)+(1.045), (I-840)+(1.046), (I-840)+(1.047), (I-840)+(1.048), (I-840)+(1.049), (I-840)+(1.050), (I-840)+(1.051), (I-840)+(1.052), (I-840)+(1.053), (I-840)+(1.054), (I-840)+(1.055), (I-840)+(1.056), (I-840)+(1.057), (I-840)+(1.058), (I-840)+(1.059), (I-840)+(1.060), (I-840)+(1.061), (I-840)+(1.062), (I-840)+(1.063), (I-840)+(1.064), (I-840)+(1.065), (I-840)+(1.066), (I-840)+(1.067), (I-840)+(1.068), (I-840)+(1.069), (I-840)+(1.070), (I-840)+(1.071), (I-840)+(1.072), (I-840)+(1.073), (I-840)+(1.074), (I-840)+(1.075), (I-840)+(1.076), (I-840)+(1.077), (I-840)+(1.078), (I-840)+(1.079), (I-840)+(1.080), (I-840)+(1.081), (I-840)+(1.082), (I-840)+(1.083), (I-840)+(1.084), (I-840)+(1.085), (I-840)+(1.086), (I-840)+(1.087), (I-840)+(1.088), (I-840)+(1.089), (I-840)+(1.090), (I-840)+(1.091), (I-840)+(1.092), (I-840)+(2.001), (I-840)+(2.002), (I-840)+(2.003), (I-840)+(2.004), (I-840)+(2.005), (I-840)+(2.006), (I-840)+(2.007), (I-840)+(2.008), (I-840)+(2.009), (I-840)+(2.010), (I-840)+(2.011), (I-840)+(2.012), (I-840)+(2.013), (I-840)+(2.014), (I-840)+(2.015), (I-840)+(2.016), (I-840)+(2.017), (I-840)+(2.018), (I-840)+(2.019), (I-840)+(2.020), (I-840)+(2.021), (I-840)+(2.022), (I-840)+(2.023), (I-840)+(2.024), (I-840)+(2.025), (I-840)+(2.026), (I-840)+(2.027), (I-840)+(2.028), (I-840)+(2.029), (I-840)+(2.030), (I-840)+(2.031), (I-840)+(2.032), (I-840)+(2.033), (I-840)+(2.034), (I-840)+(2.035), (I-840)+(2.036), (I-840)+(2.037), (I-840)+(2.038), (I-840)+(2.039), (I-840)+(2.040), (I-840)+(2.041), (I-840)+(2.042), (I-840)+(2.043), (I-840)+(2.044), (I-840)+(2.045), (I-840)+(2.046), (I-840)+(2.047), (I-840)+(2.048), (I-840)+(2.049), (I-840)+(2.050), (I-840)+(2.051), (I-840)+(2.052), (I-840)+(2.053), (I-840)+(2.054), (I-840)+(2.055), (I-840)+(2.056), (I-840)+(2.057), (I-840)+(2.058), (I-840)+(2.059), (I-840)+(2.060), (I-840)+(3.001), (I-840)+(3.002), (I-840)+(3.003), (I-840)+(3.004), (I-840)+(3.005), (I-840)+(3.006), (I-840)+(3.007), (I-840)+(3.008), (I-840)+(3.009), (I-840)+(3.010), (I-840)+(3.011), (I-840)+(3.012), (I-840)+(3.013), (I-840)+(3.014), (I-840)+(3.015), (I-840)+(3.016), (I-840)+(3.017), (I-840)+(3.018), (I-840)+(3.019), (I-840)+(3.020), (I-840)+(3.021), (I-840)+(3.022), (I-840)+(3.023), (I-840)+(3.024), (I-840)+(3.025), (I-840)+(3.026), (I-840)+(3.027), (I-840)+(3.028), (I-840)+(3.029), (I-840)+(3.030), (I-840)+(3.031), (I-840)+(3.032), (I-840)+(4.001), (I-840)+(4.002), (I-840)+(4.003), (I-840)+(4.004), (I-840)+(4.005), (I-840)+(4.006), (I-840)+(4.007), (I-840)+(4.008), (I-840)+(4.009), (I-840)+(4.010), (I-840)+(4.011), (I-840)+(4.012), (I-840)+(4.013), (I-840)+(4.014), (I-840)+(4.015), (I-840)+(4.016), (I-840)+(4.017), (I-840)+(4.018), (I-840)+(4.019), (I-840)+(4.020), (I-840)+(4.021), (I-840)+(4.022), (I-840)+(4.023), (I-840)+(4.024), (I-840)+(4.025), (I-840)+(4.026), (I-840)+(5.001), (I-840)+(5.002), (I-840)+(5.003), (I-840)+(5.004), (I-840)+(5.005), (I-840)+(5.006), (I-840)+(5.007), (I-840)+(5.008), (I-840)+(5.009), (I-840)+(5.010), (I-840)+(5.011), (I-840)+(5.012), (I-840)+(5.013), (I-840)+(5.014), (I-840)+(5.015), (I-840)+(5.016), (I-840)+(5.017), (I-840)+(5.018), (I-840)+(5.019), (I-840)+(5.020), (I-840)+(5.021), (I-840)+(5.022), (I-840)+(5.023), (I-840)+(6.001), (I-840)+(6.002), (I-840)+(6.003), (I-840)+(6.004), (I-840)+(7.001), (I-840)+(7.002), (I-840)+(7.003), (I-840)+(7.004), (I-840)+(7.005), (I-840)+(7.006), (I-840)+(8.001), (I-840)+(9.001), (I-840)+(9.002), (I-840)+(9.003), (I-840)+(9.004), (I-840)+(9.005), (I-840)+(9.006), (I-840)+(9.007), (I-840)+(9.008), (I-840)+(9.009), (I-840)+(10.001), (I-840)+(10.002), (I-840)+(10.003), (I-840)+(11.001), (I-840)+(11.002), (I-840)+(12.001), (I-840)+(12.002), (I-840)+(12.003), (I-840)+(12.004), (I-840)+(13.001), (I-840)+(13.002), (I-840)+(13.003), (I-840)+(13.004), (I-840)+(13.005), (I-840)+(13.006), (I-840)+(14.001), (I-840)+(14.002), (I-840)+(15.001), (I-840)+(15.002), (I-840)+(15.003), (I-840)+(15.004), (I-840)+(15.005), (I-840)+(15.006), (I-840)+(15.007), (I-840)+(15.008), (I-840)+(15.009), (I-840)+(15.010), (I-840)+(15.011), (I-840)+(15.012), (I-840)+(15.013), (I-840)+(15.014), (I-840)+(15.015), (I-840)+(15.016), (I-840)+(15.017), (I-840)+(15.018), (I-840)+(15.019), (I-840)+(15.020), (I-840)+(15.021), (I-840)+(15.022), (I-840)+(15.023), (I-840)+(15.024), (I-840)+(15.025), (I-840)+(15.026), (I-840)+(15.027), (I-840)+(15.028), (I-840)+(15.029), (I-840)+(15.030), (I-840)+(15.031), (I-840)+(15.032), (I-840)+(15.033), (I-840)+(15.034), (I-840)+(15.035), (I-840)+(15.036), (I-840)+(15.037), (I-840)+(15.038), (I-840)+(15.039), (I-840)+(15.040), (I-840)+(15.041), (I-840)+(15.042), (I-840)+(15.043), (I-840)+(15.044), (I-840)+(15.045), (I-840)+(15.046), (I-840)+(15.047), (I-840)+(15.048), (I-840)+(15.049), (I-840)+(15.050), (I-840)+(15.051), (I-840)+(15.052), (I-840)+(15.053), (I-840)+(15.054), (I-840)+(15.055), (I-840)+(15.056), (I-840)+(15.057), (I-840)+(15.058), (I-840)+(15.059), (I-840)+(15.060), (I-840)+(15.061), (I-840)+(15.062), (I-840)+(15.063), (I-840)+(15.064), (I-840)+(15.065), (I-840)+(15.066), (I-840)+(15.067), (I-840)+(15.068), (I-840)+(15.069), (I-840)+(15.070), (I-840)+(15.071), (I-840)+(15.072), (I-840)+(15.073), (I-840)+(15.074), (I-840)+(15.075), (I-840)+(15.076), (I-840)+(15.077), (I-840)+(15.078), (I-840)+(15.079), (I-840)+(15.080), (I-840)+(15.081), (I-840)+(15.082), (I-840)+(15.083), (I-840)+(15.084), (I-840)+(15.085), (I-840)+(15.086), (I-840)+(15.087), (I-840)+(15.088), (I-840)+(15.089), (I-840)+(15.090), (I-840)+(15.091), (I-840)+(15.092), (I-840)+(15.093), (I-840)+(15.094), (I-840)+(15.095), (I-840)+(15.096), (I-840)+(15.097), (I-840)+(15.098), (I-840)+(15.099), (I-840)+(15.100), (I-840)+(15.101), (I-840)+(15.102), (I-840)+(15.103), (I-840)+(15.104), (I-840)+(15.105), (I-840)+(15.106), (I-840)+(15.107), (I-840)+(15.108), (I-840)+(15.109), (I-840)+(15.110), (I-840)+(15.111), (I-840)+(15.112), (I-840)+(15.113), (I-840)+(15.114), (I-840)+(15.115), (I-840)+(15.116), (I-840)+(15.117), (I-840)+(15.118), (I-840)+(15.119), (I-840)+(15.120), (I-840)+(15.121), (I-840)+(15.122), (I-840)+(15.123), (I-840)+(15.124), (I-840)+(15.125), (I-840)+(15.126), (I-840)+(15.127), (I-840)+(15.128), (I-840)+(16.001), (I-840)+(16.002), (I-840)+(16.003), (I-840)+(16.004), (I-840)+(16.005), (I-840)+(16.006), (I-840)+(16.007), (I-840)+(16.008), (I-840)+(17.001), (I-840)+(17.002), (I-840)+(17.003), (I-840)+(17.004), (I-840)+(17.005), (I-840)+(17.006), (I-840)+(17.007), (I-840)+(17.008), (I-840)+(17.009), (I-840)+(17.010), (I-840)+(17.011), (I-840)+(17.012) and (I-840)+(18.001).

[0214] More preferably, the combination of compounds is selected from mixtures belonging to groups (G1), (G3) and (G4).

[0215] An even more preferred combination of compounds is selected from the group (G1-A) consisting of the following mixtures: (I-655)+(1.002), (I-655)+(1.004), (I-655)+(1.010), (I-655)+(1.012), (I-655)+(1.018), (I-655)+(1.020), (I-655)+(1.021), (I-655)+(1.026), (I-655)+(1.027), (I-655)+(1.055), (I-655)+(1.059), (I-655)+(1.081), (I-655)+(1.082), (I-655)+(1.092), (I-655)+(2.001), (I-655)+(2.002), (I-655)+(2.003), (I-655)+(2.005), (I-655)+(2.007), (I-655)+(2.017), (I-655)+(2.018), (I-655)+(2.019), (I-655)+(2.021), (I-655)+(2.028), (I-655)+(2.030), (I-655)+(2.038), (I-655)+(3.003), (I-655)+(3.012), (I-655)+(3.016), (I-655)+(3.017), (I-655)+(3.020), (I-655)+(3.025), (I-655)+(3.026), (I-655)+(3.030), (I-655)+(3.031), (I-655)+(4.005), (I-655)+(4.007), (I-655)+(4.012), (I-655)+(4.015), (I-655)+(4.025), (I-655)+(5.003), (I-655)+(5.004), (I-655)+(5.010), (I-655)+(5.012), (I-655)+(5.013), (I-655)+(5.015), (I-655)+(5.018), (I-655)+(6.002), (I-655)+(7.005), (I-655)+(9.004), (I-655)+(12.003), (I-655)+(12.004), (I-655)+(13.001), (I-655)+(13.004), (I-655)+(13.005), (I-655)+(14.001), (I-655)+(14.002), (I-655)+(15.008), (I-655)+(15.012), (I-655)+(15.016), (I-655)+(15.027), (I-655)+(15.047), (I-655)+(15.048), (I-655)+(15.052), (I-655)+(15.062), (I-655)+(15.064), (I-655)+(16.001), (I-655)+(17.001), (I-655)+(17.012) and (I-655)+(18.001).

[0216] Even more preferred combinations of compounds are also selected from the group (G3-A) consisting of the following mixtures: (I-746)+(1.002), (I-746)+(1.004), (I-746)+(1.010), (I-746)+(1.012), (I-746)+(1.018), (I-746)+(1.020), (I-746)+(1.021), (I-746)+(1.026), (I-746)+(1.027), (I-746)+(1.055), (I-746)+(1.059), (I-746)+(1.081), (I-746)+(1.082), (I-746)+(1.092), (I-746)+(2.001), (I-746)+(2.002), (I-746)+(2.003), (I-746)+(2.005), (I-746)+(2.007), (I-746)+(2.017), (I-746)+(2.018), (I-746)+(2.019), (I-746)+(2.021), (I-746)+(2.028), (I-746)+(2.030), (I-746)+(2.038), (I-746)+(3.003), (I-746)+(3.012), (I-746)+(3.016), (I-746)+(3.017), (I-746)+(3.020), (I-746)+(3.025), (I-746)+(3.026), (I-746)+(3.030), (I-746)+(3.031), (I-746)+(4.005), (I-746)+(4.007), (I-746)+(4.012), (I-746)+(4.015), (I-746)+(4.025), (I-746)+(5.003), (I-746)+(5.004), (I-746)+(5.010), (I-746)+(5.012), (I-746)+(5.013), (I-746)+(5.015), (I-746)+(5.018), (I-746)+(6.002), (I-746)+(7.005), (I-746)+(9.004), (I-746)+(12.003), (I-746)+(12.004), (I-746)+(13.001), (I-746)+(13.004), (I-746)+(13.005), (I-746)+(14.001), (I-746)+(14.002), (I-746)+(15.008), (I-746)+(15.012), (I-746)+(15.016), (I-746)+(15.027), (I-746)+(15.047), (I-746)+(15.048), (I-746)+(15.052), (I-746)+(15.062), (I-746)+(15.064), (I-746)+(16.001), (I-746)+(17.001), (I-746)+(17.012) and (I-746)+(18.001).

[0217] An even more preferred combination of compounds is also selected from the group (G4-A) consisting of the following mixtures: (I-749)+(1.002), (I-749)+(1.004), (I-749)+(1.010), (I-749)+(1.012), (I-749)+(1.018), (I-749)+(1.020), (I-749)+(1.021), (I-749)+(1.026), (I-749)+(1.027), (I-749)+(1.055), (I-749)+(1.059), (I-749)+(1.081), (I-749)+(1.082), (I-749)+(1.092), (I-749)+(2.001), (I-749)+(2.002), (I-749)+(2.003), (I-749)+(2.005), (I-749)+(2.007), (I-749)+(2.017), (I-749)+(2.018), (I-749)+(2.019), (I-749)+(2.021), (I-749)+(2.028), (I-749)+(2.030), (I-749)+(2.038), (I-749)+(3.003), (I-749)+(3.012), (I-749)+(3.016), (I-749)+(3.017), (I-749)+(3.020), (I-749)+(3.025), (I-749)+(3.026), (I-749)+(3.030), (I-749)+(3.031), (I-749)+(4.005), (I-749)+(4.007), (I-749)+(4.012), (I-749)+(4.015), (I-749)+(4.025), (I-749)+(5.003), (I-749)+(5.004), (I-749)+(5.010), (I-749)+(5.012), (I-749)+(5.013), (I-749)+(5.015), (I-749)+(5.018), (I-749)+(6.002), (I-749)+(7.005), (I-749)+(9.004), (I-749)+(12.003), (I-749)+(12.004), (I-749)+(13.001), (I-749)+(13.004), (I-749)+(13.005), (I-749)+(14.001), (I-749)+(14.002), (I-749)+(15.008), (I-749)+(15.012), (I-749)+(15.016), (I-749)+(15.027), (I-749)+(15.047), (I-749)+(15.048), (I-749)+(15.052), (I-749)+(15.062), (I-749)+(15.064), (I-749)+(16.001), (I-749)+(17.001), (I-749)+(17.012) and (I-749)+(18.001).

[0218] An even more preferred combination of compounds is selected from the group (G1-A) consisting of the following mixtures: (I-655)+(1.002), (I-655)+(1.018), (I-655)+(1.020), (I-655)+(1.021), (I-655)+(1.055), (I-655)+(2.002), (I-655)+(2.005), (I-655)+(2.028), (I-655)+(2.038), (I-655)+(3.020), (I-655)+(3.025), (I-655)+(5.003), (I-655)+(5.010), (I-655)+(5.012), (I-655)+(5.013), (I-655)+(5.018), (I-655)+(6.002), (I-655)+(7.005), (I-655)+(13.001), (I-655)+(13.004), (I-655)+(13.005), (I-655)+(15.012), (I-655)+(15.016), (I-655)+(15.064) and (I-655)+(18.001).

[0219] An even more preferred combination of compounds is also selected from the group (G3-A) consisting of the following mixtures: (I-746)+(1.002), (I-746)+(1.018), (I-746)+(1.020), (I-746)+(1.021), (I-746)+(1.055), (I-746)+(2.002), (I-746)+(2.005), (I-746)+(2.028), (I-746)+(2.038), (I-746)+(3.020), (I-746)+(3.025), (I-746)+(5.003), (I-746)+(5.010), (I-746)+(5.012), (I-746)+(5.013), (I-746)+(5.018), (I-746)+(6.002), (I-746)+(7.005), (I-746)+(13.001), (I-746)+(13.004), (I-746)+(13.005), (I-746)+(15.012), (I-746)+(15.016), (I-746)+(15.064) and (I-746)+(18.001).

[0220] An even more preferred combination of compounds is also selected from the group (G4-A) consisting of the following mixtures: (I-749)+(1.002), (I-749)+(1.018), (I-749)+(1.020), (I-749)+(1.021), (I-749)+(1.055), (I-749)+(2.002), (I-749)+(2.005), (I-749)+(2.028), (I-749)+(2.038), (I-749)+(3.020), (I-749)+(3.025), (I-749)+(5.003), (I-749)+(5.010), (I-749)+(5.012), (I-749)+(5.013), (I-749)+(5.018), (I-749)+(6.002), (I-749)+(7.005), (I-749)+(13.001), (I-749)+(13.004), (I-749)+(13.005), (I-749)+(15.012), (I-749)+(15.016), (I-749)+(15.064) and (I-749)+(18.001).

[0221] When two compounds (B) are present in the combination of the invention, preferred compound combinations are selected from the group (G1-C) consisting of the following mixtures: (I-655)+(1.001)+(1.002), (I-655)+(1.001)+(1.003), (I-655)+(1.001)+(1.004), (I-655)+(1.001) )+(1.005), (I-655)+(1.001)+(1.006), (I-655)+(1.001)+(1.007), (I-655)+(1.001)+(1.008), (I -655)+(1.001)+(1.009), (I-655)+(1.001)+(1.010), (I-655)+(1.001)+(1.011), (I-655)+(1.001)+ (1.012), (I-655)+(1.001)+(1.013), (I-655)+(1.001)+(1.014), (I-655)+(1.001)+(1.015), (I-655 )+(1.001)+(1.016), (I-655)+(1.001)+(1.017), (I-655)+(1.001)+(1.018), (I-655)+(1.001)+(1.019) ), (I-655)+(1.001)+(1.020), (I-655)+(1.001)+(1.021), (I-655)+(1.001)+(1.022), (I-655)+ (1.001)+(1.023), (I-655)+(1.001)+(1.024), (I-655)+(1.001)+(1.025), (I-655)+(1.001)+(1.026), (I-655)+(1.001)+(1.027), (I-655)+(1.001)+(1.028), (I-655)+(1.001)+(1.029), (I-655)+(1.001) )+(1.030), (I-655)+(1.001)+(1.031), (I-655)+(1.001)+(1.032), (I-655)+(1.001)+(1.033), (I -655)+(1.001)+(1.034), (I-655)+(1.001)+(1.035), (I-655)+(1.001)+(1.036), (I-655)+(1.001)+ (1.037), (I-655)+(1.001)+(1.038), (I-655)+(1.001)+(1.039), (I-655)+(1.001)+(1.040), (I-655 )+(1.001)+(1.041), (I-655)+(1.001)+(1.042), (I-655)+(1.001)+(1.043), (I-655)+(1.001)+(1.044 ), (I-655)+(1.001)+(1.045), (I-655)+(1.001)+(1.046), (I-655)+(1.001)+(1.047), (I-655)+ (1.001)+(1.048), (I-655)+(1.001)+(1.049), (I-655)+(1.001)+(1.050), (I-655)+(1.001)+(1.051), (I-655)+(1.001)+(1.052), (I-655)+(1.001)+(1.053), (I-655)+(1.001)+(1.054), (I-655)+(1.001) )+(1.055), (I-655)+(1.001)+(1.056), (I-655)+(1.001)+(1.057), (I-655)+(1.001)+(1.058), (I -655)+(1.001)+(1.059), (I-655)+(1.001)+(1.060), (I-655)+(1.001)+(1.061), (I-655)+(1.001)+(1.062), (I-655)+(1.001)+(1.063), (I-655)+(1.001)+(1.064), (I-655)+(1.001) )+(1.065), (I-655)+(1.001)+(1.066), (I-655)+(1.001)+(1.067), (I-655)+(1.001)+(1.068), (I -655)+(1.001)+(1.069), (I-655)+(1.001)+(1.070), (I-655)+(1.001)+(1.071), (I-655)+(1.001)+ (1.072), (I-655)+(1.001)+(1.073), (I-655)+(1.001)+(1.074), (I-655)+(1.001)+(1.075), (I-655 )+(1.001)+(1.076), (I-655)+(1.001)+(1.077), (I-655)+(1.001)+(1.078), (I-655)+(1.001)+(1.079) ), (I-655)+(1.001)+(1.080), (I-655)+(1.001)+(1.081), (I-655)+(1.001)+(1.082), (I-655)+ (1.001)+(1.083), (I-655)+(1.001)+(1.084), (I-655)+(1.001)+(1.085), (I-655)+(1.001)+(1.086), (I-655)+(1.001)+(1.087), (I-655)+(1.001)+(1.088), (I-655)+(1.001)+(1.089), (I-655)+(1.001) )+(1.090), (I-655)+(1.001)+(1.091), (I-655)+(1.001)+(1.092), (I-655)+(1.001)+(2.001), (I -655)+(1.001)+(2.002), (I-655)+(1.001)+(2.003), (I-655)+(1.001)+(2.004), (I-655)+(1.001)+ (2.005), (I-655)+(1.001)+(2.006), (I-655)+(1.001)+(2.007), (I-655)+(1.001)+(2.008), (I-655 )+(1.001)+(2.009), (I-655)+(1.001)+(2.010), (I-655)+(1.001)+(2.011), (I-655)+(1.001)+(2.012) ), (I-655)+(1.001)+(2.013), (I-655)+(1.001)+(2.014), (I-655)+(1.001)+(2.015), (I-655)+ (1.001)+(2.016), (I-655)+(1.001)+(2.017), (I-655)+(1.001)+(2.018), (I-655)+(1.001)+(2.019), (I-655)+(1.001)+(2.020), (I-655)+(1.001)+(2.021), (I-655)+(1.001)+(2.022), (I-655)+(1.001) )+(2.023), (I-655)+(1.001)+(2.024), (I-655)+(1.001)+(2.025), (I-655)+(1.001)+(2.026), (I -655)+(1.001)+(2.027), (I-655)+(1.001)+(2.028), (I-655)+(1.001)+(2.029), (I-655)+(1.001)+ (2.030), (I-655)+(1.001)+(2.031), (I-655)+(1.001)+(2.032), (I-655)+(1.001)+(2.033), (I-655 ) + (1.001) + (2.034), (I-655)+(1.001)+(2.035), (I-655)+(1.001)+(2.036), (I-655)+(1.001)+(2.037), (I-655)+(1.001) )+(2.038), (I-655)+(1.001)+(2.039), (I-655)+(1.001)+(2.040), (I-655)+(1.001)+(2.041), (I -655)+(1.001)+(2.042), (I-655)+(1.001)+(2.043), (I-655)+(1.001)+(2.044), (I-655)+(1.001)+ (2.045), (I-655)+(1.001)+(2.046), (I-655)+(1.001)+(2.047), (I-655)+(1.001)+(2.048), (I-655 )+(1.001)+(2.049), (I-655)+(1.001)+(2.050), (I-655)+(1.001)+(2.051), (I-655)+(1.001)+(2.052) ), (I-655)+(1.001)+(2.053), (I-655)+(1.001)+(2.054), (I-655)+(1.001)+(2.055), (I-655)+(1.001)+(2.056), (I-655)+(1.001)+(2.057), (I-655)+(1.001) )+(2.058), (I-655)+(1.001)+(2.059), (I-655)+(1.001)+(3.001), (I-655)+(1.001)+(3.002), (I -655)+(1.001)+(3.003), (I-655)+(1.001)+(3.004), (I-655)+(1.001)+(3.005), (I-655)+(1.001)+ (3.006), (I-655)+(1.001)+(3.007), (I-655)+(1.001)+(3.008), (I-655)+(1.001)+(3.009), (I-655 )+(1.001)+(3.010), (I-655)+(1.001)+(3.011), (I-655)+(1.001)+(3.012), (I-655)+(1.001)+(3.013) ), (I-655)+(1.001)+(3.014), (I-655)+(1.001)+(3.015), (I-655)+(1.001)+(3.016), (I-655)+ (1.001)+(3.017), (I-655)+(1.001)+(3.018), (I-655)+(1.001)+(3.019), (I-655)+(1.001)+(3.020), (I-655)+(1.001)+(3.021), (I-655)+(1.001)+(3.022), (I-655)+(1.001)+(3.023), (I-655)+(1.001) )+(3.024), (I-655)+(1.001)+(3.025), (I-655)+(1.001)+(3.026), (I-655)+(1.001)+(3.027), (I -655)+(1.001)+(3.028), (I-655)+(1.001)+(3.029), (I-655)+(1.001)+(3.030), (I-655)+(1.001)+(3.031), (I-655)+(1.001)+(5.001), (I-655)+(1.001)+(5.002), (I-655)+(1.001) )+(5.003), (I-655)+(1.001)+(5.004), (I-655)+(1.001)+(5.005), (I-655)+(1.001)+(5.006), (I -655)+(1.001)+(5.007), (I-655)+(1.001)+(5.008), (I-655)+(1.001)+(5.009), (I-655)+(1.001)+ (5.010), (I-655)+(1.001)+(5.011), (I-655)+(1.001)+(5.012), (I-655)+(1.001)+(5.013), (I-655 )+(1.001)+(5.014), (I-655)+(1.001)+(5.015), (I-655)+(1.001)+(5.016), (I-655)+(1.001)+(5.017) ), (I-655)+(1.001)+(5.018), (I-655)+(1.001)+(5.019), (I-655)+(1.001)+(5.020), (I-655)+ (1.001)+(5.021), (I-655)+(1.001)+(5.022), (I-655)+(1.001)+(5.023), (I-655)+(1.001)+(6.001), (I-655)+(1.001)+(6.002), (I-655)+(1.001)+(6.003), (I-655)+(1.001)+(6.004), (I-655)+(1.001) )+(7.001), (I-655)+(1.001)+(7.002), (I-655)+(1.001)+(7.003), (I-655)+(1.001)+(7.004), (I -655)+(1.001)+(7.005), (I-655)+(1.001)+(7.006), (I-655)+(1.001)+(9.001), (I-655)+(1.001)+ (9.002), (I-655)+(1.001)+(9.003), (I-655)+(1.001)+(9.004), (I-655)+(1.001)+(9.005), (I-655) ) + (1.001) + (9.006), (I-655)+(1.001)+(9.007), (I-655)+(1.001)+(9.008), (I-655)+(1.001)+(9.009), (I-655)+(1.001) )+(14.001), (I-655)+(1.001)+(14.002), (I-655)+(1.001)+(15.008), (I-655)+(1.001)+(15.011), (I -655)+(1.001)+(15.012), (I-655)+(1.001)+(15.016), (I-655)+(1.001)+(15.025), (I-655)+(1.001)+ (15.027), (I-655)+(1.001)+(15.047), (I-655)+(1.001)+(15.063), (I-655)+(1.001)+(15.064), (I-655 )+(1.001)+(16.001), (I-655)+(1.001)+(16.002), (I-655)+(1.001)+(16.003), (I-655)+(1.001)+(16.004) ), (I-655)+(1.001)+(16.005), (I-655)+(1.001)+(16.006), (I-655)+(1.001)+(16.007), (I-655)+ (1.001)+(16.008), (I-655)+(1.001)+(17.001), (I-655)+(1.001)+(17.002), (I-655)+(1.001)+(17.003), (I-655)+(1.001)+(17.004), (I-655)+(1.001)+(17.005), (I-655)+(1.001)+(17.006), (I-655)+(1.001) )+(17.007), (I-655)+(1.001)+(17.008), (I-655)+(1.001)+(17.009), (I-655)+(1.001)+(17.010), (I -655)+(1.001)+(17.011), (I-655)+(1.001)+(17.012), (I-655)+(1.001)+(18.001), (I-655)+(1.002)+(1.003), (I-655)+(1.002)+(1.004), (I-655)+(1.002)+(1.005), (I-655)+(1.002) )+(1.006), (I-655)+(1.002)+(1.007), (I-655)+(1.002)+(1.008), (I-655)+(1.002)+(1.009), (I -655)+(1.002)+(1.010), (I-655)+(1.002)+(1.011), (I-655)+(1.002)+(1.012), (I-655)+(1.002)+ (1.013), (I-655)+(1.002)+(1.014), (I-655)+(1.002)+(1.015), (I-655)+(1.002)+(1.016), (I-655 )+(1.002)+(1.017), (I-655)+(1.002)+(1.018), (I-655)+(1.002)+(1.019), (I-655)+(1.002)+(1.020) ), (I-655)+(1.002)+(1.021), (I-655)+(1.002)+(1.022), (I-655)+(1.002)+(1.023), (I-655)+ (1.002)+(1.024), (I-655)+(1.002)+(1.025), (I-655)+(1.002)+(1.026), (I-655)+(1.002)+(1.027), (I-655)+(1.002)+(1.028), (I-655)+(1.002)+(1.029), (I-655)+(1.002)+(1.030), (I-655)+(1.002) )+(1.031), (I-655)+(1.002)+(1.032), (I-655)+(1.002)+(1.033), (I-655)+(1.002)+(1.034), (I -655)+(1.002)+(1.035), (I-655)+(1.002)+(1.036), (I-655)+(1.002)+(1.037), (I-655)+(1.002)+ (1.038), (I-655)+(1.002)+(1.039), (I-655)+(1.002)+(1.040), (I-655)+(1.002)+(1.041), (I-655 )+(1.002)+(1.042), (I-655)+(1.002)+(1.043), (I-655)+(1.002)+(1.044), (I-655)+(1.002)+(1.045) ), (I-655)+(1.002)+(1.046), (I-655)+(1.002)+(1.047), (I-655)+(1.002)+(1.048), (I-655)+(1.002)+(1.049), (I-655)+(1.002)+(1.050), (I-655)+(1.002) )+(1.051), (I-655)+(1.002)+(1.052), (I-655)+(1.002)+(1.053), (I-655)+(1.002)+(1.054), (I -655)+(1.002)+(1.055), (I-655)+(1.002)+(1.056), (I-655)+(1.002)+(1.057), (I-655)+(1.002)+ (1.058), (I-655)+(1.002)+(1.059), (I-655)+(1.002)+(1.060), (I-655)+(1.002)+(1.061), (I-655 )+(1.002)+(1.062), (I-655)+(1.002)+(1.063), (I-655)+(1.002)+(1.064), (I-655)+(1.002)+(1.065) ), (I-655)+(1.002)+(1.066), (I-655)+(1.002)+(1.067), (I-655)+(1.002)+(1.068), (I-655)+ (1.002)+(1.069), (I-655)+(1.002)+(1.070), (I-655)+(1.002)+(1.071), (I-655)+(1.002)+(1.072), (I-655)+(1.002)+(1.073), (I-655)+(1.002)+(1.074), (I-655)+(1.002)+(1.075), (I-655)+(1.002) )+(1.076), (I-655)+(1.002)+(1.077), (I-655)+(1.002)+(1.078), (I-655)+(1.002)+(1.079), (I -655)+(1.002)+(1.080), (I-655)+(1.002)+(1.081), (I-655)+(1.002)+(1.082), (I-655)+(1.002)+ (1.083), (I-655)+(1.002)+(1.084), (I-655)+(1.002)+(1.085), (I-655)+(1.002)+(1.086), (I-655 )+(1.002)+(1.087), (I-655)+(1.002)+(1.088), (I-655)+(1.002)+(1.089), (I-655)+(1.002)+(1.090) ), 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(I-655)+(1.014)+(2.059), (I-655)+(1.014)+(3.001 ), (I-655)+(1.014)+(3.002), (I-655)+(1.014)+(3.003), (I-655)+(1.014)+(3.004), (I-655)+ (1.014)+(3.005), (I-655)+(1.014)+(3.006), (I-655)+(1.014)+(3.007), (I-655)+(1.014)+(3.008), (I-655)+(1.014)+(3.009), (I-655)+(1.014)+(3.010), (I-655)+(1.014)+(3.011), (I-655)+(1.014) )+(3.012), (I-655)+(1.014)+(3.013), (I-655)+(1.014)+(3.014), (I-655)+(1.014)+(3.015), (I -655)+(1.014)+(3.016), (I-655)+(1.014)+(3.017), (I-655)+(1.014)+(3.018), (I-655)+(1.014)+ (3.019), (I-655)+(1.014)+(3.020), (I-655)+(1.014)+(3.021), (I-655)+(1.014)+(3.022), (I-655 )+(1.014)+(3.023), (I-655)+(1.014)+(3.024), (I-655)+(1.014)+(3.025), (I-655)+(1.014)+(3.026) ), (I-655)+(1.014)+(3.027), (I-655)+(1.014)+(3.028), (I-655)+(1.014)+(3.029), (I-655)+(1.014)+(3.030), (I-655)+(1.014)+(3.031), (I-655)+(1.014) )+(5.001), (I-655)+(1.014)+(5.002), (I-655)+(1.014)+(5.003), (I-655)+(1.014)+(5.004), (I -655)+(1.014)+(5.005), (I-655)+(1.014)+(5.006), (I-655)+(1.014)+(5.007), (I-655)+(1.014)+ (5.008), (I-655)+(1.014)+(5.009), (I-655)+(1.014)+(5.010), (I-655)+(1.014)+(5.011), (I-655 )+(1.014)+(5.012), (I-655)+(1.014)+(5.013), (I-655)+(1.014)+(5.014), (I-655)+(1.014)+(5.015) ), (I-655)+(1.014)+(5.016), (I-655)+(1.014)+(5.017), (I-655)+(1.014)+(5.018), (I-655)+ (1.014)+(5.019), (I-655)+(1.014)+(5.020), (I-655)+(1.014)+(5.021), (I-655)+(1.014)+(5.022), (I-655)+(1.014)+(5.023), (I-655)+(1.014)+(6.001), (I-655)+(1.014)+(6.002), (I-655)+(1.014) )+(6.003), (I-655)+(1.014)+(6.004), (I-655)+(1.014)+(7.001), (I-655)+(1.014)+(7.002), (I -655)+(1.014)+(7.003), (I-655)+(1.014)+(7.004), (I-655)+(1.014)+(7.005), (I-655)+(1.014)+ (7.006), (I-655)+(1.014)+(9.001), (I-655)+(1.014)+(9.002), (I-655)+(1.014)+(9.003), (I-655 )+(1.014)+(9.004), (I-655)+(1.014)+(9.005), (I-655)+(1.014)+(9.006), (I-655)+(1.014)+(9.007 ), (I-655)+(1.014)+(9.008), (I-655)+(1.014)+(9.009), (I-655)+(1.014)+(14.001), (I-655)+(1.014)+(14.002), (I-655)+(1.014)+(15.008), (I-655)+(1.014) )+(15.011), (I-655)+(1.014)+(15.012), (I-655)+(1.014)+(15.016), (I-655)+(1.014)+(15.025), (I -655)+(1.014)+(15.027), (I-655)+(1.014)+(15.047), (I-655)+(1.014)+(15.063), (I-655)+(1.014)+ (15.064), (I-655)+(1.014)+(16.001), (I-655)+(1.014)+(16.002), (I-655)+(1.014)+(16.003), (I-655 )+(1.014)+(16.004), (I-655)+(1.014)+(16.005), (I-655)+(1.014)+(16.006), (I-655)+(1.014)+(16.007 ), (I-655)+(1.014)+(16.008), (I-655)+(1.014)+(17.001), (I-655)+(1.014)+(17.002), (I-655)+ (1.014)+(17.003), (I-655)+(1.014)+(17.004), (I-655)+(1.014)+(17.005), (I-655)+(1.014)+(17.006), (I-655)+(1.014)+(17.007), (I-655)+(1.014)+(17.008), (I-655)+(1.014)+(17.009), (I-655)+(1.014) )+(17.010), (I-655)+(1.014)+(17.011), (I-655)+(1.014)+(17.012), (I-655)+(1.014)+(18.001), (I-655)+(1.015)+(1.016), (I-655)+(1.015)+(1.017), (I-655)+(1.015)+(1.018), (I-655)+(1.015) )+(1.019), (I-655)+(1.015)+(1.020), (I-655)+(1.015)+(1.021), (I-655)+(1.015)+(1.022), (I -655)+(1.015)+(1.023), (I-655)+(1.015)+(1.024), (I-655)+(1.015)+(1.025), (I-655)+(1.015)+ (1.026), (I-655)+(1.015)+(1.027), (I-655)+(1.015)+(1.028), (I-655)+(1.015)+(1.029), (I-655 )+(1.015)+(1.030), (I-655)+(1.015)+(1.031), (I-655)+(1.015)+(1.032), (I-655)+(1.015)+(1.033 ), (I-655)+(1.015)+(1.034), (I-655)+(1.015)+(1.035), (I-655)+(1.015)+(1.036), (I-655)+ (1.015)+(1.037), (I-655)+(1.015)+(1.038), (I-655)+(1.015)+(1.039), (I-655)+(1.015)+(1.040), (I-655)+(1.015)+(1.041), (I-655)+(1.015)+(1.042), (I-655)+(1.015)+(1.043), (I-655)+(1.015) )+(1.044), (I-655)+(1.015)+(1.045), (I-655)+(1.015)+(1.046), (I-655)+(1.015)+(1.047), (I -655)+(1.015)+(1.048), (I-655)+(1.015)+(1.049), (I-655)+(1.015)+(1.050), (I-655)+(1.015)+ (1.051), (I-655)+(1.015)+(1.052), (I-655)+(1.015)+(1.053), (I-655)+(1.015)+(1.054), (I-655 )+(1.015)+(1.055), (I-655)+(1.015)+(1.056), (I-655)+(1.015)+(1.057), (I-655)+(1.015)+(1.058) ), (I-655)+(1.015)+(1.059), (I-655)+(1.015)+(1.060), (I-655)+(1.015)+(1.061), (I-655)+ (1.015)+(1.062), (I-655)+(1.015)+(1.063), (I-655)+(1.015)+(1.064), (I-655)+(1.015)+(1.065), (I-655)+(1.015)+(1.066), (I-655)+(1.015)+(1.067), (I-655)+(1.015)+(1.068), (I-655)+(1.015) )+(1.069), (I-655)+(1.015)+(1.070), (I-655)+(1.015)+(1.071), (I-655)+(1.015)+(1.072), (I -655)+(1.015)+(1.073), (I-655)+(1.015)+(1.074), (I-655)+(1.015)+(1.075), (I-655)+(1.015)+ (1.076), (I-655)+(1.015)+(1.077), (I-655)+(1.015)+(1.078), (I-655)+(1.015)+(1.079), (I-655 )+(1.015)+(1.080), (I-655)+(1.015)+(1.081), (I-655)+(1.015)+(1.082), (I-655)+(1.015)+(1.083) ), (I-655)+(1.015)+(1.084), (I-655)+(1.015)+(1.085), (I-655)+(1.015)+(1.086), (I-655)+ (1.015)+(1.087), (I-655)+(1.015)+(1.088), (I-655)+(1.015)+(1.089), (I-655)+(1.015)+(1.090), (I-655)+(1.015)+(1.091), (I-655)+(1.015)+(1.092), (I-655)+(1.015)+(2.001), (I-655)+(1.015) )+(2.002), (I-655)+(1.015)+(2.003), (I-655)+(1.015)+(2.004), (I-655)+(1.015)+(2.005), (I -655)+(1.015)+(2.006), (I-655)+(1.015)+(2.007), (I-655)+(1.015)+(2.008), (I-655)+(1.015)+ (2.009), (I-655)+(1.015)+(2.010), (I-655)+(1.015)+(2.011), (I-655)+(1.015)+(2.012), (I-655 )+(1.015)+(2.013), (I-655)+(1.015)+(2.014), (I-655)+(1.015)+(2.015), (I-655)+(1.015)+(2.016) ), (I-655)+(1.015)+(2.017), (I-655)+(1.015)+(2.018), (I-655)+(1.015)+(2.019), (I-655)+ (1.015)+(2.020), (I-655)+(1.015)+(2.021), (I-655)+(1.015)+(2.022), (I-655)+(1.015)+(2.023), (I-655)+(1.015)+(2.024), (I-655)+(1.015)+(2.025), (I-655)+(1.015)+(2.026), (I-655)+(1.015) )+(2.027), (I-655)+(1.015)+(2.028), (I-655)+(1.015)+(2.029), (I-655)+(1.015)+(2.030), (I -655)+(1.015)+(2.031), (I-655)+(1.015)+(2.032), (I-655)+(1.015)+(2.033), (I-655)+(1.015)+ (2.034), (I-655)+(1.015)+(2.035), (I-655)+(1.015)+(2.036), (I-655)+(1.015)+(2.037), (I-655 )+(1.015)+(2.038), (I-655)+(1.015)+(2.039), (I-655)+(1.015)+(2.040), (I-655)+(1.015)+(2.041) ), (I-655)+(1.015)+(2.042), (I-655)+(1.015)+(2.043), (I-655)+(1.015)+(2.044), (I-655)+ (1.015)+(2.045), (I-655)+(1.015)+(2.046), (I-655)+(1.015)+(2.047), (I-655)+(1.015)+(2.048), (I-655)+(1.015)+(2.049), (I-655)+(1.015)+(2.050), (I-655)+(1.015)+(2.051), (I-655)+(1.015) )+(2.052), (I-655)+(1.015)+(2.053), (I-655)+(1.015)+(2.054), (I-655)+(1.015)+(2.055), (I -655)+(1.015)+(2.056), (I-655)+(1.015)+(2.057), (I-655)+(1.015)+(2.058), (I-655)+(1.015)+(2.059), (I-655)+(1.015)+(3.001), (I-655)+(1.015)+(3.002), (I-655)+(1.015) )+(3.003), (I-655)+(1.015)+(3.004), (I-655)+(1.015)+(3.005), (I-655)+(1.015)+(3.006), (I -655)+(1.015)+(3.007), (I-655)+(1.015)+(3.008), (I-655)+(1.015)+(3.009), (I-655)+(1.015)+ (3.010), (I-655)+(1.015)+(3.011), (I-655)+(1.015)+(3.012), (I-655)+(1.015)+(3.013), (I-655 )+(1.015)+(3.014), (I-655)+(1.015)+(3.015), (I-655)+(1.015)+(3.016), (I-655)+(1.015)+(3.017 ), (I-655)+(1.015)+(3.018), (I-655)+(1.015)+(3.019), (I-655)+(1.015)+(3.020), (I-655)+ (1.015)+(3.021), (I-655)+(1.015)+(3.022), (I-655)+(1.015)+(3.023), (I-655)+(1.015)+(3.024), (I-655)+(1.015)+(3.025), (I-655)+(1.015)+(3.026), (I-655)+(1.015)+(3.027), (I-655)+(1.015) )+(3.028), (I-655)+(1.015)+(3.029), (I-655)+(1.015)+(3.030), (I-655)+(1.015)+(3.031), (I -655)+(1.015)+(5.001), (I-655)+(1.015)+(5.002), (I-655)+(1.015)+(5.003), (I-655)+(1.015)+(5.004), (I-655)+(1.015)+(5.005), (I-655)+(1.015)+(5.006), (I-655)+(1.015) )+(5.007), (I-655)+(1.015)+(5.008), (I-655)+(1.015)+(5.009), (I-655)+(1.015)+(5.010), (I -655)+(1.015)+(5.011), (I-655)+(1.015)+(5.012), (I-655)+(1.015)+(5.013), (I-655)+(1.015)+ (5.014), (I-655)+(1.015)+(5.015), (I-655)+(1.015)+(5.016), (I-655)+(1.015)+(5.017...

Claims

1. (A) (I-655) 6-chloro-3-(3-cyclopropyl-2-fluorophenoxy)-N-[2-(2,4-dimethylphenyl)-2,2-difluoroethyl]-5-methylpyridazine-4-carboxamide, (I-746) 6-chloro-N-[2-(2-chloro-4-methylphenyl)-2,2-difluoroethyl]-3-(3-cyclopropyl-2-fluorophenoxy)-5-methylpyridazine-4-carboxamide and (I-749) 6-chloro-3-(3-cyclopropyl-2-fluorophenoxy)-N-[2-(3,4-dimethylphenyl)-2,2-difluoroethyl]-5-methylpyridazine-4-carboxamide At least one compound of formula (I) selected from the group consisting of 【Chemistry 1】 and (B) (1.002) difenoconazole, (1.018) prothioconazole, (1.020) spiroxamine, (1.021) tebuconazole, (1.055) mefentrifluconazole, (2.002) bixafen, (2.005) fluopyram, (2.028) impirfluxam, (2.038) isoflucipram, (3.020) trifloxystrobin, (3.025) fenpicoxamide, (5.003) captan, (5.010) dithianon, (5.012) folpet, ( 5.013) mancozeb, (5.018) propineb, (6.002) isotianil, (7.005) pyrimethanil, (13.001) fludioxonil, (13.004) proquinazid, (13.005) quinoxyfen, (15.012) fosetyl-aluminum, (15.016) metrafenone, (15.064) (N'-[2-chloro-4-(2-fluorophenoxy)-5-methylphenyl]-N-ethyl-N-methylimidoformamide) and (18.001) unsaturated and saturated C at least one further active compound selected from the group consisting of a composition comprising one or more fatty acids selected from C 12 -C 24 fatty acids, salts thereof or derivatives thereof, or a mixture of any of the above, wherein at least 95% of the fatty acids are in the C 14 -C 20 range (e.g. FLiPPER® from AlphaBio Pesticides or Bayer AG); A combination of active compounds comprising:

2. The combination of active compounds according to claim 1, wherein (A) is (I-655) 6-chloro-3-(3-cyclopropyl-2-fluorophenoxy)-N-[2-(2,4-dimethylphenyl)-2,2-difluoroethyl]-5-methylpyridazine-4-carboxamide.

3. The combination of active compounds according to claim 1, wherein (A) is (I-746) 6-chloro-N-[2-(2-chloro-4-methylphenyl)-2,2-difluoroethyl]-3-(3-cyclopropyl-2-fluorophenoxy)-5-methylpyridazine-4-carboxamide.

4. The combination of active compounds according to claim 1, wherein (A) is (I-749) 6-chloro-3-(3-cyclopropyl-2-fluorophenoxy)-N-[2-(3,4-dimethylphenyl)-2,2-difluoroethyl]-5-methylpyridazine-4-carboxamide.

5. The compound (B) is selected from the group consisting of: (1.002) difenoconazole, (1.018) prothioconazole, (1.020) spiroxamine, (1.021) tebuconazole, (1.055) mefentrifluconazole, (2.002) bixafen, (2.005) fluopyram, (2.028) impirfluxam, (2.038) isoflucipram, (3.020) trifloxystrobin, (3.025) fenpicoxamide, (5.003) captan, (5.010) dithianon, (5.012) folpet, (5.013) manco 5. A combination of active compounds according to any one of claims 1 to 4 selected from the group consisting of zeb, (5.018) propineb, (6.002) isotianil, (7.005) pyrimethanil, (13.001) fludioxonil, (13.004) proquinazid, (13.005) quinoxyfen, (15.012) fosetyl-aluminium, (15.016) metrafenone and (15.064) (N'-[2-chloro-4-(2-fluorophenoxy)-5-methylphenyl]-N-ethyl-N-methylimidoformamide).

6. 10. A composition for controlling phytopathogenic harmful fungi in crop protection and material protection, characterized in addition to at least one extender and / or surfactant by a quantity of a combination of active compounds according to at least one of claims 1 to 5.

7. Method for controlling phytopathogenic harmful fungi in crop protection and material protection, characterized in that a combination of active compounds according to at least one of claims 1 to 5 or a composition according to claim 6 is applied to the phytopathogenic harmful fungi and / or their habitat.

8. Use of a combination of active compounds according to at least one of claims 1 to 5 or a composition according to claim 6 for controlling phytopathogenic harmful fungi in crop protection and material protection.

9. Use of a combination of active compounds according to at least one of claims 1 to 5 or a composition according to claim 6 for the treatment of transgenic plants.

10. Use of a combination of active compounds according to at least one of claims 1 to 5 or of a composition according to claim 6 for the treatment of seeds.

11. The use according to claim 10, wherein the seed is a seed of a transgenic plant.

12. Seeds coated with a combination of active compounds according to at least one of claims 1 to 5 or with a composition according to claim 6.

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