Solid composition containing dimethyl sulfide and dextrin

Abstract

The purpose of the present invention is to provide a solid composition having an excellent ability to retain dimethyl sulfide.　A solid composition containing dimethyl sulfide to which a dextrin having a molecular weight of 50,000 or greater is added.

Description

[Technical field]

[0001] The present invention relates to a solid composition containing dimethyl sulfide and dextrin. [Background technology]

[0002] A common powdering method for obtaining instant tea is the spray drying method, which is suitable for continuous mass production. Spray drying is a method in which fine droplets are sprayed into hot air to instantly evaporate water. The residence time exposed to high temperatures is short, and the amount of heat given is consumed as latent heat of evaporation, so the heat load on the liquid contents is suppressed, and powder with little deterioration in quality can be obtained. The higher the concentration of the liquid contents to be spray-dried, the higher the retention rate of the aromatic components contained in the liquid after spray drying. This can be explained by the selective diffusion theory, and when the solute concentration is low in the droplets during drying, the diffusion coefficient of the aromatic components is low, and the aromatic components volatilize at the same time as the water evaporates. However, the higher the solute concentration, the higher the diffusion coefficient of the aromatic components, and the water evaporates faster than the migration of the aromatic components, leaving the aroma. Therefore, in order to obtain high-quality instant tea, it is important to produce a tea concentrate containing a high concentration of aromatic components.

[0003] The methods of concentrating tea extract can be classified into three types based on the principle of whether water is separated into a solid, liquid, or gas phase: freeze concentration (aqueous phase-solid), membrane concentration (aqueous phase-liquid), and evaporation concentration (aqueous phase-gas). Of these, evaporation concentration places a large thermal load on the contents, making it difficult to obtain a concentrated liquid that retains the aroma components of tea, which are susceptible to thermal deterioration. In addition, freeze concentration has high hurdles to practical use, such as the long concentration time and cost, and it is difficult to achieve a high concentration in the first place. For this reason, concentration by these two methods has not been widely adopted. On the other hand, membrane concentration is a method of increasing the solute concentration by applying pressure to water through a membrane with fine holes, so evaporation and freezing are not necessary, making it possible to concentrate at low cost without causing any change in quality.

[0004] Furthermore, as a method for producing a tea concentrate, it is known to add dextrin, which is a type of excipient and has a molecular structure in which sugars are linked in a chain, to a tea extract. For example, it has been reported that the extract can be concentrated without decreasing the concentration efficiency by adding acyclic dextrin or cyclic dextrin with an average degree of polymerization of 4 to 10 to an extract of tea leaves, roasted grains, or roasted beans before concentrating the extract, and then performing membrane concentration at 40°C (Patent Document 1).

[0005] It is also known that certain dextrins improve the solubility of instant tea after spray drying. For example, it has been reported that instant tea with excellent flavor and immediate solubility can be produced by spray drying tea containing dextrin with an average degree of polymerization of 4 to 10 or a combination of this with cyclic dextrin in a state in which carbon dioxide is dissolved (Patent Document 2). It has also been reported that instant tea with excellent flavor and immediate solubility can be provided by adding resistant dextrin to tea extract and spray drying the mixture (Patent Document 3). [Prior art documents] [Patent documents]

[0006] [Patent Document 1] Japanese Patent Application Publication No. 3-36491 [Patent Document 2] Japanese Patent Application Publication No. 3-35898 [Patent Document 3] JP 2009-17867 A Summary of the Invention [Problem to be solved by the invention]

[0007] Among tea beverages, the so-called high-grade green tea has a characteristic aroma called "green laver aroma," and it is known that dimethyl sulfide and the like have the aroma of green laver. However, since dimethyl sulfide is easily volatilized, it has not always been possible to sufficiently retain dimethyl sulfide at a high concentration in a solid composition in the production of a solid composition containing dimethyl sulfide. Therefore, the present invention aims to provide a solid composition that has excellent dimethyl sulfide retention and gives a strong green laver aroma when made into a beverage using water, hot water, or the like. [Means for solving the problem]

[0008] As a result of intensive research to solve the above problems, the present inventors have focused on dextrin in the production of a solid composition containing dimethyl sulfide, and have found that by preparing a solid composition containing polymeric dextrin, dimethyl sulfide can be maintained at a high concentration in the solid composition. Based on this finding, the present inventors have completed the present invention.

[0009] The present invention relates to, but is not limited to, the following: (1) A solid composition containing dimethyl sulfide and dextrin, The content of dimethyl sulfide in the composition is 2.1 μg per 1 g of the composition (2.1 μg / g) or more; The composition comprises dextrin having a molecular weight of 50,000 or more. (2) The composition according to (1), wherein the proportion of dextrin having a molecular weight of 50,000 or more in the molecular weight distribution of the composition is 5 to 35%. (3) The composition according to (1) or (2), wherein the proportion of dextrin having a molecular weight of 50,000 to 200,000 in the molecular weight distribution of the composition is 2 to 30%. (4) The composition according to any one of (1) to (3), wherein the proportion of dextrin having a molecular weight of 200,000 to 350,000 in the molecular weight distribution of the composition is 0.3 to 6%. (5) The composition according to any one of (1) to (4), wherein the proportion of dextrin having a molecular weight of 250,000 or more in the molecular weight distribution of the composition is 0.9 to 10%. (6) The composition according to any one of (1) to (5), wherein the proportion of dextrin having a molecular weight of 350,000 or more in the molecular weight distribution of the composition is 0.2 to 4%. (7) The composition according to any one of (1) to (6), which contains two or more types of dextrin. (8) The composition according to any one of (1) to (7), comprising a linear dextrin and a cyclic dextrin. (9) The composition according to any one of (1) to (8), further comprising one or more fragrance components selected from the group consisting of β-ionone, α-ionone, β-cyclocitral, (z)-3-hexenol, 1-penten-3-ol, hexanal, and nerolidol. (10) The composition according to any one of (1) to (9), which is a powder composition. (11) The composition according to any one of (1) to (10), which contains a tea leaf extract. (12) The composition according to (11), wherein the tea leaf extract is an extract of sencha tea leaves. (13) A food or drink comprising the composition according to any one of (1) to (12). (14) The food or beverage according to (13), which is a beverage. (15) The food or beverage according to (14), which is a tea beverage. (16) A food or beverage containing dimethyl sulfide and dextrin, The dimethyl sulfide content in the food or beverage is 20.3 ppb (w / w) or more per 1.0% solids concentration (Brix), The food or drink described above, which contains dextrin having a molecular weight of 50,000 or more. Effect of the Invention

[0010] According to the present invention, a solid composition capable of retaining dimethyl sulfide at a high concentration can be provided. In the present invention, dimethyl sulfide contained in a solution before drying in a production process can be retained at a high concentration in a solid composition after drying. Therefore, by utilizing the present invention, it is possible to provide a solid composition rich in dimethyl sulfide.

[0011] The solid composition of the present invention can be used to prepare a tea beverage by adding water or hot water, and can provide a strong aroma of green laver when consumed. In addition, the solid composition of the present invention is very light compared to beverages, and therefore is convenient to transport.

[0012] Furthermore, the solid composition of the present invention can be used as a food ingredient. The number and variety of foods having a tea flavor have been increasing in recent years. The solid composition of the present invention can be used to impart a green laver aroma to confectioneries such as cakes, castella cakes, candies, cookies, jellies, puddings, and chocolates. DETAILED DESCRIPTION OF THE PREFERRED EMBODIMENTS

[0013] 1. Solid composition One aspect of the present invention is a solid composition containing dimethyl sulfide and dextrin, the composition having a dimethyl sulfide content of 2.1 μg or more per 1 g of the composition (2.1 μg / g) and containing dextrin having a molecular weight of 50,000 or more. By adopting such a constitution, it is possible to maintain a high dimethyl sulfide content in the solid composition, and to provide a solid composition that has a strong green laver aroma when made into a beverage using water, hot water, or the like. Here, the "green laver aroma" in this specification means an aroma that is a mixture of a faint roasted aroma, a sweet aroma, and a smell like the seashore.

[0014] 1-1.Dimethyl sulfide The solid composition of the present invention contains dimethyl sulfide, which is an organic sulfur compound represented by the formula (CH3)2S and is known as an aromatic component that exhibits the aroma of green laver.

[0015] The content of dimethyl sulfide in the solid composition of the present invention is not particularly limited, but is, for example, 2.1 μg (2.1 μg / g) or more per 1 g of solid composition, preferably 2.2 μg / g or more, more preferably 2.3 μg / g or more, even more preferably 2.4 μg / g or more, and particularly preferably 2.5 μg / g or more. The content of dimethyl sulfide in the above range allows the green laver aroma to be exhibited. The upper limit of the content of dimethyl sulfide in the solid composition of the present invention is not particularly limited, but is, for example, 50,000 μg (50,000 μg / g) or less per 1 g of solid composition, preferably 40,000 μg / g or less, more preferably 25,000 μg / g or less, even more preferably 5,000 μg / g or less, and particularly preferably 2,500 μg / g or less. The content of dimethyl sulfide in the solid composition of the present invention is typically 2.1 to 50,000 μg per 1 g of solid composition (2.1 to 50,000 μg / g), preferably 2.2 to 40,000 μg / g, more preferably 2.3 to 25,000 μg / g, even more preferably 2.4 to 5,000 μg / g, and particularly preferably 2.5 to 2,500 μg / g.

[0016] In the present invention, the content of dimethyl sulfide in the solid composition can be measured using gas chromatography (GC). In addition, an example of an analytical device is a flash GC nose HERACLES II (Alpha Moss Japan). Specifically, the solid composition of the present invention is dissolved in water to prepare a solution, and the content of dimethyl sulfide can be measured using the solution under the following conditions. Gas Chromatography Equipment: Flash GC Nose HERACLES II Column 1: MXT-5 (low polarity 10m, 180μm ID, 0.4μm) Column 2: MXT-WAX (high polarity 10m, 180μm ID, 0.4μm) Carrier gas flow rate: Hydrogen 1.6mL / min Flame ionization detector (FID) temperature: 260℃ Injector temperature: 200℃ Oven temperature: 40℃(5 seconds)~1.5℃ / sec~250℃(90 seconds) Injection time: 125 seconds Trapping temperature: Adsorption 50℃, Desorption 240℃ Trapping time: Adsorption 130 seconds, pre-heating 35 seconds The conditions for the measurement sample can be set as shown in the Examples described later. After measuring the content of dimethyl sulfide in the dissolution liquid, the content of dimethyl sulfide in the solid composition can be calculated backward from the amount of the solid composition dissolved in water.

[0017] In the solid composition of the present invention, dimethyl sulfide may be used in the form of a purified or crude product, or an extract containing dimethyl sulfide may be used. As the extract containing dimethyl sulfide, a naturally derived extract may be used, and both a plant extract and an animal extract may be used. In the present invention, it is preferable to use a plant extract, and it is more preferable to use a tea leaf extract among plants. Here, although not particularly limited, it is preferable that the tea leaf extract containing dimethyl sulfide is a different type of tea leaf extract from the tea leaf extract described below. That is, when the tea leaf extract described in the section "1-4. Tea leaf extract" described below is used as the first tea leaf extract, the tea leaf extract containing dimethyl sulfide can be used as the second tea leaf extract different from it.

[0018] As the raw material tea leaves for the tea leaf extract containing dimethyl sulfide, preferably non-fermented tea is used, and specifically, green tea such as crude tea, sencha, gyokuro, kabusecha, tencha, bancha, and roasted tea are exemplified. The tea leaf extract containing dimethyl sulfide may be extracted from only one type of tea leaves, or may be extracted by blending multiple types of tea leaves. In the present invention, the tea leaf extract containing dimethyl sulfide is preferably a green tea leaf extract, and more preferably an extract of tea leaves such as kabusecha, gyokuro, and tencha that have been shaded from the sun and grown under cover before picking. By using an extract of tea leaves such as kabusecha, gyokuro, and tencha that have been shaded from the sun and grown under cover before picking, aromatic components other than dimethyl sulfide derived from the tea leaves can be contained, and a more excellent flavor that is characteristic of high-quality tea can be imparted to the solid composition.

[0019] When a tea leaf extract containing dimethyl sulfide is used, its content is not particularly limited, and the content of dimethyl sulfide in the solid composition of the present invention can be adjusted so that it is within the range described above.

[0020] 1-2.Dextrin The solid composition of the present invention contains dextrin. Dextrin is a general term for carbohydrates obtained by hydrolysis of starch or glycogen. In the present invention, dextrin can be used as an excipient for forming a solid composition, and the molecular weight distribution in the solid composition of the present invention can be adjusted depending on the weight average molecular weight of the dextrin used and its content in the composition.

[0021] The content of dextrin in the solid composition of the present invention is not particularly limited, but is, for example, 10 to 70% by weight, preferably 20 to 65% by weight, more preferably 30 to 60% by weight. In the present invention, a commercially available product can be used as the dextrin. The content of dextrin in the solid composition can be measured by sugar analysis using a method known to those skilled in the art.

[0022] In this specification, high molecular weight dextrin means dextrin having a molecular weight of 10,000 or more, and low molecular weight dextrin means dextrin having a molecular weight of less than 10,000.

[0023] The solid composition of the present invention contains a dextrin having a molecular weight of at least 50,000. The presence of such a dextrin having a large molecular weight makes it possible to maintain a high concentration of dimethyl sulfide in the solid composition.

[0024] On the other hand, when there is too much dextrin with a large molecular weight, for example, when the proportion of dextrin with a molecular weight of 50,000 or more exceeds 45%, the viscosity of the composition before solidification becomes too high, making it difficult to perform a drying treatment, and tends to make it difficult to obtain a solid composition. In the molecular weight distribution of the solid composition of the present invention, the proportion of dextrin with a molecular weight of 50,000 or more is preferably 5 to 35%, more preferably 5.5 to 30%, even more preferably 6.0 to 25%, and particularly preferably 6.5 to 23%.

[0025] In the present invention, the molecular weight distribution in the solid composition can be examined by gel permeation chromatography (GPC) analysis. Specifically, the molecular weight distribution in the solid composition can be examined under the following conditions. Equipment: Sampling injector: 231 XL (GILSON) Pump: 305 (GILSON) Column oven: CTO-10AS VP (Shimadzu Corporation) Detector: RID-10A (Shimadzu Corporation) Columns: connected in series in the following order [Pump] → TSKgel Guard Column PWxl (6.0mm ID×4cm) (Tosoh) → TSKgel G4000PWxl (particle size 10 μm, 7.8 mm ID x 30 cm) (Tosoh) → TSKgel G3000PWxl (particle size 7 μm, 7.8 mm ID x 30 cm) (Tosoh) → [Detector] Analysis data system: LabSolutions (Shimadzu Corporation) Flow rate: 1mL / min Injection volume: 50μL Mobile phase: 0.1 mol / L sodium nitrate solution Column temperature: 50℃ The preparation of the analysis sample can be carried out as shown in the Examples below. The ratio of components of various molecular weights in the molecular weight distribution can also be determined as shown in the Examples below, specifically, by calculating the ratio of the target peak area to the sum of the obtained peak areas (total peak area).

[0026] In the molecular weight distribution of the solid composition of the present invention, the proportion of dextrin having a molecular weight of 100,000 or more is not particularly limited, but is, for example, 2.0 to 25%, preferably 3.0 to 20%, more preferably 4.0 to 15%. In the molecular weight distribution of the solid composition of the present invention, the proportion of dextrin having a molecular weight of 150,000 or more is not particularly limited, but is, for example, 1.0 to 20%, preferably 2.0 to 15%, more preferably 2.5 to 9.0%. In the molecular weight distribution of the solid composition of the present invention, the proportion of dextrin having a molecular weight of 200,000 or more is not particularly limited, but is, for example, 0.5 to 12%, preferably 1.0 to 9.0%, more preferably 1.5 to 6.0%. In the molecular weight distribution of the solid composition of the present invention, the proportion of dextrin having a molecular weight of 250,000 or more is not particularly limited, but is, for example, 0.9 to 10%, preferably 1.00 to 5.0%, more preferably 1.10 to 3.5%. In addition, in the molecular weight distribution of the solid composition of the present invention, the proportion of dextrin having a molecular weight of 300,000 or more is not particularly limited, but is, for example, 0.40 to 8.0%, preferably 0.50 to 5.0%, more preferably 0.60 to 2.0%. In addition, in the molecular weight distribution of the solid composition of the present invention, the proportion of dextrin having a molecular weight of 350,000 or more is not particularly limited, but is, for example, 0.2 to 4%, preferably 0.30 to 2.5%, more preferably 0.40 to 1.5%. In addition, in the molecular weight distribution of the solid composition of the present invention, the proportion of dextrin having a molecular weight of 400,000 or more is not particularly limited, but is, for example, 0.10 to 3.0%, preferably 0.20 to 2.0%, more preferably 0.30 to 1.0%. In the molecular weight distribution of the solid composition of the present invention, the proportion of dextrin having a molecular weight of 450,000 or more is not particularly limited, but is, for example, 0.05 to 1.5%, preferably 0.10 to 1.0%, and more preferably 0.20 to 0.6%. In the molecular weight distribution of the solid composition of the present invention, the proportion of dextrin having a molecular weight of 500,000 or more is not particularly limited, but is, for example, 0.05 to 1.2%, preferably 0.08 to 0.8%, and more preferably 0.10 to 0.5%.

[0027] In the molecular weight distribution of the solid composition of the present invention, the proportion of dextrin having a molecular weight of 50,000 or more and less than 200,000 is not particularly limited, but is, for example, 2 to 30%, preferably 3.5 to 25%, and more preferably 4.5 to 18%. In the molecular weight distribution of the solid composition of the present invention, the proportion of dextrin having a molecular weight of 200,000 or more and less than 350,000 is not particularly limited, but is, for example, 0.3 to 6.0%, preferably 0.50 to 5.0%, and more preferably 0.60 to 4.0%.

[0028] In the molecular weight distribution of the solid composition of the present invention, the proportion of components having a molecular weight of less than 50,000 is not particularly limited. In the molecular weight distribution of the solid composition of the present invention, the proportion of components having a molecular weight of less than 3,000 is, for example, 35% or more, preferably 40% or more, more preferably 45% or more. In addition, in the molecular weight distribution of the solid composition of the present invention, the proportion of components having a molecular weight of 3,000 or more and less than 10,000 is, for example, 5.0% or more, preferably 8.0% or more, more preferably 10% or more. In the molecular weight distribution of the solid composition of the present invention, the proportion of components having a molecular weight of 10,000 or more and less than 50,000 is, for example, 2.0 to 30%, preferably 4.0 to 25%, more preferably 6.0 to 20%.

[0029] The proportion of dextrin having a molecular weight of 50,000 or more in the solid composition of the present invention is not particularly limited, but within the range of a molecular weight of 50,000 or more and less than 500,000, it is preferable that the proportion decreases as the molecular weight increases. That is, the proportion of dextrin with a molecular weight of 100,000 or more and less than 150,000 is smaller than the proportion of dextrin with a molecular weight of 50,000 or more and less than 100,000, the proportion of dextrin with a molecular weight of 150,000 or more and less than 200,000 is smaller than the proportion of dextrin with a molecular weight of 100,000 or more and less than 150,000, the proportion of dextrin with a molecular weight of 200,000 or more and less than 250,000 is smaller than the proportion of dextrin with a molecular weight of 150,000 or more and less than 200,000, the proportion of dextrin with a molecular weight of 250,000 or more and less than 300,000 is smaller than the proportion of dextrin with a molecular weight of 200,000 or more and less than 250,000, It is preferable that the proportion of dextrin having a molecular weight of 300,000 or more and less than 350,000 is smaller than the proportion of dextrin having a molecular weight of 250,000 or more and less than 300,000; the proportion of dextrin having a molecular weight of 350,000 or more and less than 400,000 is smaller than the proportion of dextrin having a molecular weight of 300,000 or more and less than 350,000; the proportion of dextrin having a molecular weight of 400,000 or more and less than 450,000 is smaller than the proportion of dextrin having a molecular weight of 350,000 or more and less than 400,000; and the proportion of dextrin having a molecular weight of 450,000 or more and less than 500,000 is smaller than the proportion of dextrin having a molecular weight of 400,000 or more and less than 450,000.

[0030] As described above, in the present invention, the molecular weight distribution in the solid composition can be adjusted by the type of dextrin used. The dextrin used in the present invention is not particularly limited, and for example, linear dextrin or cyclic dextrin can be used. Here, in this specification, "linear dextrin" means dextrin in which glucose is bonded in a linear or branched chain and does not form a ring structure or a spiral structure. In addition, in this specification, "cyclic dextrin" means dextrin in which glucose is bonded to form a ring structure and does not form a spiral structure.

[0031] The linear dextrin is not particularly limited, and for example, linear dextrin having a DE (dextrose equivalent) of 1 to 25 or linear dextrin having a weight average molecular weight of 500 to 160,000 can be used. In the present invention, not only one type of linear dextrin but also two or more types can be used in combination. A preferred embodiment of the present invention is the use of two types of linear dextrin. When two types of linear dextrin are used, for example, a combination of a linear dextrin having a DE of 2 to 5 and a linear dextrin having a DE of 16 to 20, or a combination of a linear dextrin having a weight average molecular weight of 90,000 to 140,000 and a linear dextrin having a weight average molecular weight of 600 to 1,200 can be used.

[0032] When a linear dextrin is used, the content of the linear dextrin in the solid composition of the present invention is, for example, 0 to 65% by weight, preferably 10 to 60% by weight, and more preferably 15 to 55% by weight. When a linear dextrin with DE2 to 5 and a linear dextrin with DE16 to 20 are used as two types of linear dextrin, the content of the linear dextrin with DE2 to 5 in the solid composition of the present invention is, for example, 0 to 60% by weight, preferably 5 to 50% by weight, and more preferably 10 to 45% by weight, and the content of the linear dextrin with DE16 to 20 is, for example, 0 to 60% by weight, preferably 5 to 50% by weight, and more preferably 10 to 45% by weight. The content ratio (weight ratio) of linear dextrins having DE2 to 5 to linear dextrins having DE16 to 20 is, for example, 4:0.5 to 0.5:5, preferably 3:1 to 1:5, and more preferably 2:1 to 1:4.

[0033] Furthermore, when a linear dextrin having a weight-average molecular weight of 90,000 to 140,000 and a linear dextrin having a weight-average molecular weight of 600 to 1,200 are used as two types of linear dextrins, the content of the linear dextrin having a weight-average molecular weight of 90,000 to 140,000 in the solid composition of the present invention is, for example, 0 to 65% by weight, preferably 10 to 60% by weight, and more preferably 15 to 55% by weight, and the content of the linear dextrin having a weight-average molecular weight of 600 to 1,200 is, for example, 5 to 60% by weight, preferably 5 to 50% by weight, and more preferably 10 to 45% by weight. The content ratio (weight ratio) of the linear dextrin having a weight average molecular weight of 90,000 to 140,000 to the linear dextrin having a weight average molecular weight of 600 to 1,200 is, for example, 5:1 to 1:3, preferably 3:1 to 1:2, and more preferably 2:1 to 1:1.

[0034] As the cyclic dextrin, for example, cyclodextrin can be used. In the present invention, any of α-cyclodextrin, β-cyclodextrin, and γ-cyclodextrin can be used, but α-cyclodextrin is preferably used. The weight-average molecular weight of the cyclic dextrin used in the present invention is not particularly limited, but is, for example, 700 to 1,300, preferably 800 to 1,200, and more preferably 900 to 1,100. When a cyclic dextrin is used, the content of the cyclic dextrin in the solid composition of the present invention is, for example, 0.5 to 15% by weight, preferably 1 to 12% by weight, and more preferably 3 to 10% by weight.

[0035] When linear dextrin and cyclic dextrin are used, the content ratio (weight ratio) of the linear dextrin to the cyclic dextrin is, for example, 20:1 to 2:1, preferably 15:1 to 3:1, and more preferably 12:1 to 5:1.

[0036] 1-3. Other aromatic ingredients The solid composition of the present invention may further contain, in addition to the above-mentioned dimethyl sulfide, one or more aroma components selected from the group consisting of β-ionone, α-ionone, β-cyclocitral, (z)-3-hexenol, 1-penten-3-ol, hexanal and nerolidol. By including these aroma components in the solid composition of the present invention, a more well-balanced green laver aroma can be presented.

[0037] The content of β-ionone in the solid composition of the present invention is not particularly limited, but is, for example, 0.31 to 5,000 μg per 1 g of solid composition (0.31 to 5,000 μg / g), preferably 0.5 to 3,500 μg / g, more preferably 0.65 to 2,000 μg / g, even more preferably 0.8 to 1,500 μg / g, and particularly preferably 1 to 1,000 μg / g.

[0038] The content of α-ionone in the solid composition of the present invention is not particularly limited, but is, for example, 0.01 to 200 μg per 1 g of solid composition (0.1 to 200 μg / g), preferably 0.025 to 150 μg / g, more preferably 0.05 to 100 μg / g, even more preferably 0.075 to 75 μg / g, and particularly preferably 0.1 to 50 μg / g.

[0039] The content of β-cyclocitral in the solid composition of the present invention is not particularly limited, but is, for example, 0.01 to 200 μg per 1 g of solid composition (0.1 to 200 μg / g), preferably 0.025 to 150 μg / g, more preferably 0.1 to 100 μg / g, even more preferably 0.5 to 75 μg / g, and particularly preferably 1 to 50 μg / g.

[0040] The content of (z)-3-hexenol in the solid composition of the present invention is not particularly limited, but is, for example, 0.1 to 1,000 μg per 1 g of solid composition (0.1 to 1,000 μg / g), preferably 0.5 to 750 μg / g, more preferably 1 to 500 μg / g, even more preferably 5 to 350 μg / g, and particularly preferably 10 to 200 μg / g.

[0041] The content of 1-penten-3-ol in the solid composition of the present invention is not particularly limited, but is, for example, 0.1 to 1,000 μg per 1 g of solid composition (0.1 to 1,000 μg / g), preferably 0.5 to 750 μg / g, more preferably 1 to 500 μg / g, even more preferably 5 to 350 μg / g, and particularly preferably 10 to 200 μg / g.

[0042] The content of hexanal in the solid composition of the present invention is not particularly limited, but is, for example, 0.01 to 200 μg per 1 g of solid composition (0.01 to 200 μg / g), preferably 0.05 to 100 μg / g, more preferably 0.1 to 50 μg / g, even more preferably 0.5 to 25 μg / g, and particularly preferably 1 to 10 μg / g.

[0043] The content of nerolidol in the solid composition of the present invention is not particularly limited, but is, for example, 0.01 to 200 μg per 1 g of solid composition (0.1 to 200 μg / g), preferably 0.025 to 150 μg / g, more preferably 0.1 to 100 μg / g, even more preferably 0.5 to 75 μg / g, and particularly preferably 1 to 50 μg / g.

[0044] In the present invention, the content of β-ionone in the solid composition can be measured by gas chromatography (GC) in the same manner as the content of dimethyl sulfide described above. Specifically, the solid composition of the present invention is dissolved in water to prepare a solution, and the content of β-ionone can be measured by using the solution under the same conditions as the measurement of the content of dimethyl sulfide described above.

[0045] In the present invention, the contents of α-ionone, β-cyclocitral, (z)-3-hexenol, 1-penten-3-ol, hexanal and nerolidol in the solid composition can be measured by gas chromatography mass spectrometry (GC / MS). Specifically, the contents of the aromatic components can be measured under the following conditions. Equipment: GC: Agilent Technologies GC7890B MS: Agilent Technologies 5977A HS: Gestel MPS Tube: Tenax TA, Carbon bx1000 Column: HP-INNOWAX 60m x 0.25mmi.d. df=0.25μm Temperature conditions: 40℃ (4 minutes) ~ 5℃ / min ~ 260℃ Carrier gas flow rate: He 1.5 ml / min Injection method: splitless Ion source temperature: 260℃ The conditions for the measurement sample can be set as shown in the examples described later.

[0046] Since the solid composition of the present invention contains tea leaf extract, the solid composition of the present invention may contain aroma components derived from tea leaves. Examples of such aroma components include, but are not limited to, pentanal (valeraldehyde), 2-methylpropanal (isobutyraldehyde), nonanal, trimethylpyrazine, 1-octen-3-ol, 2-ethyl-3,5-dimethylpyrazine, 2-ethyl-3,6-dimethylpyrazine, 2,4-heptadiene-6-one, 2,3-diethyl-5-methylpyrazine, 2-methyl-3-n-propylpyrazine, benzaldehyde, ethyl decanoate, acetyl thiazoline, ethyl acetophenone, and p-cresol.

[0047] 1-4.Tea leaf extract The solid composition of the present invention contains tea leaf extract. Here, in the present specification, "tea leaf extract" means a component extracted from tea leaves. In the present invention, tea leaves obtained from plants of the genus Camellia and the family Theaceae (such as Camellia sinensis (L) O. Kuntze) can be used. The tea leaves used in the present invention can be classified into non-fermented tea, semi-fermented tea, and fermented tea according to the processing method. Examples of non-fermented tea include green tea such as crude tea, sencha, gyokuro, kabusecha, tencha, bancha, hojicha, kettle tea, kikucha, bocha, and budcha. Examples of semi-fermented tea include oolong tea such as iron guanyin, colored tea, golden gui, and Wuyi rock tea. Examples of fermented tea include black tea such as Darjeeling, Assam, and Sri Lanka. In the present invention, only one type of tea leaf may be used alone, or multiple types of tea leaves may be blended and used. The tea leaves are not particularly limited as long as they are parts from which aromatic components can be extracted, and leaves, stems, etc. can be used as appropriate, and the form is also not limited to large leaves, powder, etc. In the present invention, although there is no particular limitation, an extract of green tea leaves is preferably used, and an extract of sencha tea leaves is more preferably used.

[0048] The content of tea leaf extract in the powder composition of the present invention is not particularly limited, but is, for example, 30 to 90% by weight, preferably 35 to 80% by weight, and more preferably 40 to 70% by weight. When the content of tea leaf extract is within the above range, the aroma and flavor derived from tea leaves can be fully felt.

[0049] 1-5.Other additives In addition to the various components listed above, the solid composition of the present invention may contain additives commonly used in foods and beverages, such as antioxidants, preservatives, pH adjusters, sweeteners, nutritional fortifiers, thickening stabilizers, emulsifiers, dietary fiber, and quality stabilizers, within the range that does not impair the effects of the present invention.

[0050] 1-6. Uses of solid compositions The solid composition of the present invention can be contained in food and drink (beverages and foods). That is, in the present invention, food and drink containing the above-mentioned solid composition can be provided. The solid composition of the present invention is preferably contained in a liquid to make a beverage, and most preferably dissolved in water or hot water and consumed as a tea beverage. From this point of view, the solid composition of the present invention can be provided as instant tea. Here, in this specification, "instant tea" means a solution using tea leaf extract as a raw material, which is dried and processed into a solid form. Tea beverages include non-fermented teas (green tea, etc.), semi-fermented teas (oolong tea, etc.), and fermented teas (black tea, etc.), and specifically, there can be mentioned steamed non-fermented teas (green teas) such as Sencha, Bancha, Houjicha, Gyokuro, Kabusecha, and Tencha; non-fermented teas such as Ureshino tea, Aoyagi tea, and various Chinese teas; semi-fermented teas such as Baozhong tea, Tieguanyin tea, and Oolong tea; fermented teas such as black tea, Awa Bancha, and Pu-erh tea. The tea beverage in which the solid composition of the present invention is used is preferably green tea. That is, the solid composition of the present invention can be provided as instant green tea.

[0051] When the solid composition of the present invention is added to a liquid such as water or hot water, the content of the solid composition in the solution is not particularly limited, but is, for example, 0.01 to 20% by weight, preferably 0.05 to 10% by weight, and more preferably 0.1 to 5.0% by weight. The content of the solid composition in the solution may be adjusted so that the content of dimethyl sulfide in the solution is, for example, 1 to 2,500 ppb (w / w), preferably 5 to 2,000 ppb (w / w), more preferably 10 to 1,000 ppb (w / w), and even more preferably 100 to 500 ppb (w / w), or the content of β-ionone in the solution is, for example, 0.05 to 100 ppb, preferably 0.2 to 80 ppb, more preferably 0.4 to 60 ppb, and even more preferably 4 to 40 ppb.

[0052] The solid composition of the present invention can also be added to food. Examples of such foods include Japanese and Western confectionery, such as cakes, castella, candies, cookies, jellies, puddings, and chocolates, and frozen desserts such as ice cream, popsicles, and sherbets, as well as snacks, and can also be used in bread and dairy products. When the solid composition of the present invention is added to food, the amount of the composition added can be appropriately determined depending on the type of food, etc.

[0053] When the solid composition of the present invention is added to a food, the amount of the solid composition added can be appropriately set according to the type of food, etc. The solid composition of the present invention can be added to a food so that the content of the solid composition in the food is, for example, 0.01 to 20% by weight, preferably 0.05 to 10.0% by weight, more preferably 0.1 to 5.0% by weight, and even more preferably 0.5 to 5.0% by weight. For example, the solid composition of the present invention can be added to a food so that the content of β-ionone in the food is 0.05 to 100 ppb, preferably 0.2 to 80 ppb, more preferably 0.4 to 60 ppb, and even more preferably 4 to 40 ppb.

[0054] The amount of the solid composition of the present invention to be added to a food can also be determined based on the content of dimethyl sulfide as an index. For example, the solid composition of the present invention can be added to a food so that the content of dimethyl sulfide in the food is 1 to 2,500 ppb (w / w), preferably 5 to 2,000 ppb (w / w), more preferably 10 to 1,000 ppb (w / w), and even more preferably 100 to 500 ppb (w / w).

[0055] In one embodiment, the present invention relates to a food or drink (beverage and food) containing dimethyl sulfide and dextrin, the food or drink containing dextrin having a molecular weight of not less than 50,000. The content of dimethyl sulfide in the food or drink is preferably not less than 20.3 ppb (w / w) per 1.0% solids concentration (Brix), more preferably 20.8 to 485,000 ppb (w / w), 21.3 to 380,000 ppb (w / w), 22.3 to 242,100 ppb (w / w), or 23.1 to 48,400 ppb (w / w) per 1.0% Brix, and even more preferably 24.1 to 24,200 ppb (w / w) per 1.0% Brix. The solid content concentration (Brix) value is a value obtained by converting the refractive index measured at 20°C using a saccharometer or refractometer into the mass / mass percent of a sucrose solution based on the conversion table of ICUMSA (International Commission on Uniform Methods of Sugar Analysis), and represents the soluble solid content in the composition. The type of food and drink (beverages and foods) is not particularly limited, but examples of beverages include steamed unfermented teas (green teas) such as Sencha, Bancha, Houjicha, Gyokuro, Kabusecha, and Tencha; unfermented teas such as Ureshinocha, Aoyagicha, and various Chinese teas; semi-fermented teas such as Baozhongcha, Tieguanyincha, and Oolong tea; and fermented teas such as black tea, Awabancha, and Pu-erh tea. Examples of foods include cakes, castella, candies, cookies, jellies, puddings, and chocolates, ice cream, popsicles, sherbets, and other cold desserts, snacks, bread, and dairy products.

[0056] 2. Manufacturing method The solid composition of the present invention can be produced through a process of preparing a solution containing dimethyl sulfide and dextrin as described above, and a process of drying the obtained solution. The solution may contain the above-mentioned tea leaf extract and various components in addition to dimethyl sulfide and dextrin. The blending amount of each component can be appropriately set as long as it does not impair the effects of the present invention, and the order in which the various components are blended is not particularly limited. In addition, water may be used as the solvent for the solution, or the tea leaf extract may be used as it is. The blending amount of dextrin in the solution before solidification can be adjusted so that the content of dextrin in the soluble solid content of the solution is the content in the above-mentioned solid composition.

[0057] The solution can be dried using a method conventionally known to those skilled in the art. For example, spray drying, freeze drying, hot air drying, vacuum drying, and other methods can be used. In the present invention, spray drying is preferably used. The conditions for spray drying, such as temperature and time, are not particularly limited, and can be appropriately adjusted to solidify the solution.

[0058] In addition to the above steps, the production of the solid composition of the present invention may include a step of concentrating a solution containing dimethyl sulfide and dextrin, a step of sterilizing the solution, etc. All steps can be carried out using methods conventionally known to those skilled in the art.

[0059] As for dimethyl sulfide, a tea leaf extract containing dimethyl sulfide (second tea leaf extract) may be used as described above. A solution containing dimethyl sulfide and dextrin can be prepared by mixing the first tea leaf extract (tea leaf extract described in the above section "1-4. Tea Leaf Extract") with the second tea leaf extract. Although not particularly limited, the tea leaf extract containing dimethyl sulfide (second tea leaf extract) can be produced through a process of distilling tea leaves. The tea leaves used as the raw material for the second tea leaf extract are as described above, and in the present invention, tea leaves such as kabusecha, gyokuro, and tencha that have been shaded from sunlight and grown under cover before picking can be used as the raw material.

[0060] As a method for distilling tea leaves to obtain a tea leaf extract (second tea leaf extract) containing dimethyl sulfide, a steam distillation method is typically used. The steam distillation method is a method in which steam is passed through the raw material (tea leaves) and the aromatic components distilled along with the steam are cooled and condensed. For the steam distillation method, methods such as atmospheric pressure steam distillation, reduced pressure steam distillation, and gas-liquid multistage countercurrent contact distillation (spinning cone column) can be adopted, and in the present invention, it is preferable to use the atmospheric pressure steam distillation method. In addition, in the steam distillation of tea leaves, a blowing type steam distillation is typically performed. The blowing type steam distillation is a method in which steam is directly brought into contact with the raw material (tea leaves) placed in a container such as a basket, and the steam obtained through the raw material is collected and cooled to obtain a distillate.

[0061] As for the tea leaf extract (second tea leaf extract) containing dimethyl sulfide, various aromatic components can be concentrated through a process of further concentrating the extract obtained by steam distillation. As such a concentration method, distillation concentration is typically performed. In distillation concentration, for example, a method can be adopted in which the tea leaf extract is put into a distillation pot, heated from the bottom to boil, and the aromatic components are recovered together with the steam. In the distillation concentration method, either atmospheric distillation concentration or reduced pressure distillation concentration can be used, and in the present invention, reduced pressure distillation concentration is preferably used. In addition, when performing distillation concentration, an operation called salting out may be performed. By performing the salting out process, the polarity of the salt attracts water molecules in the distillate put into the distillation pot, and the volatilization of organic compounds can be promoted. The salting out process can be performed by adding a salt such as sodium chloride to the distillate to be concentrated.

[0062] Furthermore, the tea leaf extract containing dimethyl sulfide (second tea leaf extract) may be produced through a step of activated carbon treatment. By carrying out the activated carbon treatment, the amount of unnecessary aroma components can be reduced. Here, in this specification, "activated carbon" means a porous material mainly composed of carbon, which is produced from a carbon material such as wood through an activation reaction at high temperature.

[0063] 3. Methods for enhancing the aroma of green laver in food and beverages The solid composition of the present invention obtained as described above can be added to food and drink, and can enhance the aroma of green laver in the food and drink. Therefore, in another aspect, the present invention also provides a method for enhancing the aroma of green laver in a food and drink, comprising the step of adding the solid composition obtained through the above steps to the food and drink. EXAMPLES

[0064] The present invention will be described below based on examples, but the present invention is not limited to these examples.

[0065] 1. Preparation of Solid Composition (i) Preparation of solid composition stock solution A solid composition stock solution was prepared using tea leaf extract solid raw material (tea solid raw material; product name GT204S, raw material: green tea (produced in China)), linear dextrin A (Matsutani Chemical, TK-16, weight average molecular weight: 910, DE: 18), linear dextrin B (Sanwa Starch Industry, Sandec #30, weight average molecular weight: 120,000, DE: 2-5), and cyclic dextrin (Cyclochem, α-cyclodextrin, weight average molecular weight: 973). Specifically, each raw material was mixed in the ratio shown in Table 1 below to prepare a total of 6,000 g of a powder mixture, to which 14,000 g of water was added to prepare a total of 20,000 g (Brix 30%) of a solid composition stock solution. The above tea leaf extract solid raw material (tea solid raw material) was obtained by drying and solidifying the extract of tea leaves, and does not contain dextrin.

[0066] [Table 1]

[0067] (ii) Preparation of a Dimethyl Sulfide-Rich Distillate Apart from the above (i), a tea leaf extract containing a high concentration of dimethyl sulfide was prepared. Specifically, 12 kg of commercially available Kabuse tea leaves were mixed with 12 kg of water, and the tea leaves were wetted by stirring by hand so as not to cause a bias in the moisture content of the tea leaves. Next, the tea leaves were placed in a basket installed in a steam distillation pot, and steam distillation was performed by blowing in steam under the conditions of a steam pressure of 0.25 MPa, a steam flow rate of 16 kg / hr, and a steam temperature of 100°C (normal pressure). The cooling refrigerant temperature was set to 4°C for the outward flow and 6°C for the return flow, and condensation was performed at a refrigerant flow rate of 30 L / min to collect the distillate. The distillate was collected for 30 minutes after the start of distillation. This operation was performed four times to obtain a total of 28 kg of distillate.

[0068] 1.52g of powdered activated carbon derived from wood (Shirasagi WP-Z, Osaka Gas Chemicals) with an average pore size of 3nm was added to 22.4kg of the obtained distillate, and the mixture was stirred with a stirrer for 10 minutes to perform activated carbon treatment. The activated carbon in the distillate was removed using filter paper (ADVANTEC, No.2). The treatment temperature for the activated carbon treatment was 5.7℃. The liquid not treated with activated carbon and the treated liquid were mixed in a 1:4 ratio to obtain 28kg of distillate.

[0069] (iii) Preparation of solid compositions 6L of the distillate obtained in (ii) above was added to 14L of the solid composition stock solution obtained in (i) above and mixed. A part of the pre-drying stock solution for preparing the solid composition prepared as described above was taken out as a sample for measuring the concentration of aroma components, and then the pre-drying stock solution was spray-dried using a spray dryer to prepare a solid composition. The drying conditions were an inlet hot air temperature of 160°C and an outlet hot air temperature of 110°C.

[0070] 2. Molecular weight distribution in solid composition The molecular weight distribution of the soluble molecules contained in the above-mentioned various solid compositions was measured. Each solid composition was diluted with 0.1 mol / L sodium nitrate solution to a concentration of 1% (w / v) to prepare an analytical sample, and the molecular weight distribution was measured using gel permeation chromatography (GPC) analysis. The gel permeation chromatography analysis conditions were as follows. Equipment: Sampling injector: 231 XL (GILSON) Pump: 305 (GILSON) Column oven: CTO-10AS VP (Shimadzu Corporation) Detector: RID-10A (Shimadzu Corporation) Columns: connected in series in the following order [Pump] → TSKgel Guard Column PWxl (6.0mm ID×4cm) (Tosoh) → TSKgel G4000PWxl (particle size 10 μm, 7.8 mm ID x 30 cm) (Tosoh) → TSKgel G3000PWxl (particle size 7 μm, 7.8 mm ID x 30 cm) (Tosoh) → [Detector] Analysis data system: LabSolutions (Shimadzu Corporation) Flow rate: 1mL / min Injection volume: 50μL Mobile phase: 0.1 mol / L sodium nitrate solution Column temperature: 50℃

[0071] Using STANDARD P-82 (Shodex, Showa Denko) as a standard solution, the retention times of eight types of molecular weight were first detected, and a calibration curve was created based on the detection results. Then, the peak area ratio (ratio to the total peak area) for each molecular size contained in the sample was calculated from the total peak area detected at each retention time in the analytical sample. The results of the molecular weight distribution in various samples are shown in Table 2.

[0072] [Table 2]

[0073] In addition, in the molecular weight distribution of Table 2, the percentage of dextrin having a molecular weight of 50,000 or more, the percentage of dextrin having a molecular weight of 100,000 or more, the percentage of dextrin having a molecular weight of 150,000 or more, the percentage of dextrin having a molecular weight of 200,000 or more, the percentage of dextrin having a molecular weight of 250,000 or more, the percentage of dextrin having a molecular weight of 300,000 or more, the percentage of dextrin having a molecular weight of 350,000 or more, the percentage of dextrin having a molecular weight of 400,000 or more, the percentage of dextrin having a molecular weight of 450,000 or more, and the percentage of dextrin having a molecular weight of 500,000 or more are calculated and the results are shown in Table 3. In addition, in the molecular weight distribution of Table 2, the percentage of dextrin having a molecular weight of 50,000 or more and less than 200,000, and the percentage of dextrin having a molecular weight of 200,000 or more and less than 350,000 are calculated and the results are shown in Table 3.

[0074] [Table 3]

[0075] As shown in Tables 2 and 3 above, peaks of dextrins with molecular weights of 50,000 or more were confirmed in Samples 2 to 4, which contain the high molecular weight dextrin linear dextrin B. Note that, since no peaks were observed in the molecular weight region of 50,000 or more in Sample 1, which does not contain the high molecular weight dextrin linear dextrin B (see Tables 2 and 3), the peaks detected in the molecular weight region of 50,000 or more in this test are believed to be due to high molecular weight dextrins.

[0076] 3. Evaluation of aroma component retention The undried stock solution and solid composition obtained as described above were diluted or dissolved in water so that the solid content concentration (Brix) value was 4%. The solid content concentration (Brix) value is a value obtained by converting the refractive index measured at 20°C using a saccharometer or refractometer, etc., into the mass / mass percentage of the sucrose solution based on the conversion table of ICUMSA (International Commission on Uniform Methods of Sugar Analysis), and represents the soluble solid content in the composition. 10 mL of the obtained solution was placed in a vial containing 3 g of sodium chloride, and the vial was sealed and introduced into a gas chromatography analyzer (Alpha Moss Japan, Flash GC Nose HERACLES II). Analysis of dimethyl sulfide in various solutions was performed under the conditions shown below. Incubation: 60℃, 15 min. Syringe: Temperature: 70℃, Post-injection cleaning: 90 seconds Headspace injection: 5000 μl at 250 μl / sec Column 1: MXT-5 (low polarity 10m, 180μm ID, 0.4μm) Column 2: MXT-WAX (high polarity 10m, 180μm ID, 0.4μm) Carrier gas flow rate: Hydrogen 1.6mL / min Flame ionization detector (FID) temperature: 260℃ Injector temperature: 200℃ Oven temperature: 40℃(5 seconds)~1.5℃ / sec~250℃(90 seconds) Injection time: 125 seconds Trapping temperature: Adsorption 50℃, Desorption 240℃ Trapping time: Adsorption 130 seconds, pre-heating 35 seconds

[0077] The retention rate of dimethyl sulfide before and after spray drying was calculated from the integrated value of the total peak area from the data obtained by the analysis. The content of dimethyl sulfide in the solid composition after drying was also determined.

[0078] [Table 4]

[0079] As shown by the above results, Samples 2 to 4 (see Table 3), which contain high molecular weight dextrins of 50,000 or more, showed higher dimethyl sulfide retention rates than Sample 1, which does not contain high molecular weight dextrins of 50,000 or more (see Table 4). This result shows that when a solid composition contains dextrins of 50,000 or more in molecular weight, the retention rate of dimethyl sulfide is improved.

[0080] 4. Sensory evaluation 0.58 g of the solid composition of samples 1 to 4 obtained as described above was dissolved in water to adjust to 100 g, and a sample for sensory evaluation was obtained. The Brix value of the sample for sensory evaluation was about 0.6%. The converted value of the dimethyl sulfide content in the sample for sensory evaluation prepared as described above is shown in Table 5.

[0081] [Table 5]

[0082] A sensory evaluation was carried out for each of the prepared samples by five panelists who were well trained in flavor evaluation. The sensory evaluation involved rating the degree of green laver aroma felt in the samples on the following five-point scale, scoring in 0.1-point increments, and finally calculating the average score. In the sensory evaluation, the above base sample (sample 1) was given a score of 3 points, and the various samples were evaluated. 1: Almost no green seaweed aroma 2: I don't really notice the green seaweed scent. 3: Feel the aroma of green laver 4: The green laver aroma lasts (the green laver aroma is excellent) 5: The green laver scent lasts longer (the green laver scent is excellent)

[0083] [Table 6]

[0084] As described above, samples 2 to 4, which contain high molecular weight dextrin with a molecular weight of 50,000 or more and have a high dimethyl sulfide retention rate, were shown to have a longer-lasting green laver aroma compared to sample 1, which does not contain high molecular weight dextrin with a molecular weight of 50,000 or more. The above results also showed that in beverage form, the green laver aroma is longer-lasting when the beverage contains 12.2 ppb or more of dimethyl sulfide per 0.6% solids concentration (Brix) or 20.3 ppb or more of dimethyl sulfide converted to a 1.0% solids concentration (Brix).

Claims

1. A solid composition containing dimethyl sulfide and dextrin, The content of dimethyl sulfide in the composition is 2.1 μg per 1 gram of the composition (2.1 μg / g) or more; Contains dextrin with a molecular weight of 50,000 or more, The composition, wherein the dextrin comprises linear dextrin and cyclic dextrin.

2. 2. The composition according to claim 1, wherein the proportion of dextrin having a molecular weight of 50,000 or more in the molecular weight distribution of the composition is 5 to 35%.

3. 3. The composition according to claim 1, wherein the proportion of dextrin having a molecular weight of 50,000 to 200,000 in the molecular weight distribution of the composition is 2 to 30%.

4. 4. The composition according to claim 1, wherein the proportion of dextrin having a molecular weight of 200,000 to 350,000 in the molecular weight distribution of the composition is 0.3 to 6%.

5. 5. The composition according to claim 1, wherein the proportion of dextrin having a molecular weight of 250,000 or more in the molecular weight distribution of the composition is 0.9 to 10%.

6. 6. The composition according to claim 1, wherein the proportion of dextrin having a molecular weight of 350,000 or more in the molecular weight distribution of the composition is 0.2 to 4%.

7. The composition according to any one of claims 1 to 6, which contains two or more types of dextrin.

8. The composition according to any one of claims 1 to 7, further comprising one or more fragrance components selected from the group consisting of β-ionone, α-ionone, β-cyclocitral, (z)-3-hexenol, 1-penten-3-ol, hexanal and nerolidol.

9. The composition according to any one of claims 1 to 8, wherein the composition is a powder composition.

10. The composition according to any one of claims 1 to 9, which contains a tea leaf extract.

11. The composition according to claim 10, wherein the tea leaf extract is a Sencha tea leaf extract.

12. A food or drink comprising the composition according to any one of claims 1 to 11.

13. The food or drink according to claim 12, which is a beverage.

14. The food or beverage according to claim 13, which is a tea beverage.

15. A food or drink containing dimethyl sulfide and dextrin, The content of dimethyl sulfide in the food or beverage is 20.3 ppb (w / w) or more per 1.0% solids concentration (Brix), Contains dextrin with a molecular weight of 50,000 or more, The food or beverage, wherein the dextrin comprises linear dextrin and cyclic dextrin.

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