Layered oxide positive electrode material and preparation method thereof, and application to sodium battery

By performing three-point doping and shuttle ion doping on layered oxide cathode materials, the problems of structural instability and slow sodium ion diffusion during charge and discharge processes were solved, thereby improving the cycle stability and diffusion rate of the material.

CN121687944BActive Publication Date: 2026-05-19SHENZHEN INST OF ADVANCED TECH CHINESE ACAD OF SCI
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Patent Information

Application Number
CN202610197021.X
Authority / Receiving Office
CN · China
Patent Type
Patents(China)
Current Assignee / Owner
Filing Date
2026-02-11
Publication Date
2026-05-19
Estimated Expiration
2046-02-11

AI Technical Summary

Technical Problem

Layered oxide cathode materials are prone to harmful phase transitions and structural degradation during charge-discharge cycles, leading to blockage of ion channels and hindered sodium ion diffusion, which affects long-term cycle stability and coulombic efficiency.

Method used

A three-point doping strategy is adopted, which involves doping the sodium storage layer, the cation sites of the transition metal layer, and the anion sites of the transition metal layer, and introducing shuttle ion doping, which shuttles between the transition metal layer and the sodium storage layer to dynamically fill vacancies, thereby stabilizing the material structure and improving the sodium ion diffusion rate.

Benefits of technology

It improves the structural stability and sodium ion diffusion rate of the material, enhances the material's flexibility, solves the problems of cycling instability and slow diffusion, and achieves better cycling performance and electrochemical performance.

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Abstract

The application relates to the technical field of battery materials, in particular to a layered oxide positive electrode material, a preparation method thereof and application to a sodium battery. The expression of the layered oxide positive electrode material is: AB2Y2X2O12, wherein, A is a sodium storage layer site doping element, B is a transition metal layer cation site doping element, C is a transition metal layer anion site doping element, and Y is a shuttle ion doping element. In the charging and discharging process of the layered oxide positive electrode material, the shuttle ion shuttles between the transition metal layer and the sodium storage layer, which can improve the stability and sodium ion diffusion rate of the material, and effectively solve the problems of unstable iron-manganese-based layer oxygen circulation, low coulomb efficiency and slow sodium ion diffusion rate.
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