Preparation method of Co@NC-CNT / DME catalyst and matching used recyclable stirring device

By preparing PDA-modified Co@CN-CNTs/DME immobilized catalysts and a matching recyclable stirring device, the problems of low catalyst activity and inability to be reused were solved, achieving catalyst stability and efficient utilization, and improving the efficiency of catalytic reactions.

CN118162184BActive Publication Date: 2026-05-29ZHENGZHOU UNIV

Patent Information

Authority / Receiving Office
CN · China
Patent Type
Patents(China)
Current Assignee / Owner
ZHENGZHOU UNIV
Filing Date
2024-03-11
Publication Date
2026-05-29

AI Technical Summary

Technical Problem

Existing catalysts suffer from low catalytic activity and cannot be reused. In particular, immobilized catalysts are prone to deformation and breakage during stirring, and uneven contact with the solution leads to reduced catalytic efficiency.

Method used

The Co@NC-CNT/DME catalyst preparation method involves preparing CNTs/DME precursors, ZIF-67-CNTs/DME, Co@CN-CNTs/DME, and PDA modification to form a PDA-modified Co@CN-CNTs/DME immobilized catalyst. A recyclable stirring device, including a mounting plate, a central shaft, and a water flow dispersion plate, is used to prevent the catalyst from deforming and breaking during the stirring process.

Benefits of technology

This approach enables the reuse of catalysts, reduces the amount of Co ion leaching, improves the dispersion and catalytic activity of catalytic active sites, enhances the stability and durability of catalysts, and improves the efficiency of catalytic reactions.

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Abstract

The present application relates to a kind of Co@NC-CNT / DME catalyst preparation method and matching use recyclable stirring device.Preparation method includes:1) preparation CNTs / DME precursor;2) preparation ZIF-67-CNTs / DME;3) preparation Co@CN-CNTs / DME;4) PDA modification immobilized Co@CN-CNTs / DME.Can obtain immobilized Co@CN-CNTs / DME catalyst.The above-mentioned catalyst can be fitted on the mounting column on the mounting plate of recyclable stirring device when using, the immobilized catalyst of the present application cooperates with the recyclable stirring device of the present application, so that the immobilized catalyst of the present application not only can be reused, but also has lower Co ion leaching amount, has good catalytic activity.
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