A current supply system and control method for a large-scale alkaline water electrolyzer

Abstract

This invention relates to a current supply system and control method for a large-scale alkaline water electrolyzer. The system includes a host computer, a rectifier circuit module, a terminal block module, a monitoring module, and an electrolyzer. The rectifier circuit module includes a rectifier circuit and a rectifier circuit control unit. The terminal block module includes multiple terminals and multiple terminal block control units. The rectifier circuit is used to input current to each terminal block, and the rectifier circuit control unit is used to control the output current of the rectifier circuit. The terminals are used to input current values ​​to the electrolyzer, and the terminal block control unit is used to control the output current of the terminals. The monitoring module is used to monitor the operating parameters of the electrolyzer. Compared with the prior art, this invention provides a rectifier circuit control unit to control the output current of the rectifier circuit, and a terminal block control unit to control the output current of the terminals, thereby controlling the total current input to the electrolyzer and the current input to the electrolyzer from each terminal block.

Description

Technical Field

[0001] This invention relates to the field of water electrolysis for hydrogen production, and in particular to a current supply system and control method for a large-scale alkaline water electrolyzer. Background Technology

[0002] Electrolysis of water is one of the most important methods for producing high-purity hydrogen, and alkaline electrolysis of water is the oldest and most widely used technology in this field. With increasing demand for renewable energy, the need for large-scale high-purity hydrogen production is also growing stronger. To address this issue, large-scale alkaline water electrolyzers are needed. Generally, hydrogen is produced by electrolyzing the power supply and the positive and negative terminals of the electrolyzer through a rectifier circuit. However, when large-scale alkaline water electrolyzers use traditional wiring power supply methods, they are not stable enough under high-power and variable-power conditions, and the accuracy of current control cannot be guaranteed. Therefore, research on the control of high-power alkaline water electrolyzers is crucial.

[0003] A literature search of existing technologies revealed that current industrial research largely focuses on controlling the current in electrolyzers solely by controlling the magnitude of the rectifier circuit current. For example, Chinese patent CN202110089016.4 discloses "A Current Source Type PWM Rectifier Electrolysis Water Hydrogen Production System and Control Method," which proposes a method using a three-phase current source type PWM rectifier and a control unit to achieve current sharing control. Its advantages include the large capacity and high reliability of the current source type rectifier, making it suitable for large-scale production. However, for large-scale alkaline water electrolyzers, current research has not yet addressed the issue of uneven electrode reaction intensity across different regions within the electrolyzer under high-power conditions. Summary of the Invention

[0004] The purpose of this invention is to overcome the defects of the prior art by providing a current supply system and control method for a large alkaline water electrolyzer.

[0005] The objective of this invention can be achieved through the following technical solutions:

[0006] A current supply system for a large alkaline water electrolyzer includes a host computer, a rectifier circuit module, a terminal block module, a monitoring module, and an electrolyzer. The rectifier circuit module includes a rectifier circuit and a rectifier circuit control unit, and the terminal block module includes multiple terminals and multiple terminal block control units.

[0007] The host computer is connected to the rectifier circuit control unit, the terminal control unit, and the monitoring module;

[0008] The rectifier circuit is connected to the terminals and is used to input current to each terminal. The rectifier circuit control unit is connected to the rectifier circuit and is used to control the output current of the rectifier circuit.

[0009] The terminals are installed on the electrolytic cell and are used to input current to the electrolytic cell. The number of terminal control units corresponds to the number of terminals and is connected to the terminals to control the output current of the terminals.

[0010] The monitoring module is installed on the electrolytic cell and is used to monitor the operating parameters of the electrolytic cell.

[0011] Preferably, it also includes a trigger circuit, which is connected to the host computer and the rectifier circuit and is used to trigger the rectifier circuit.

[0012] Preferably, the monitoring module includes multiple temperature sensors and multiple pressure sensors, which are installed inside the electrolytic cell to acquire temperature, hydrogen pressure, and oxygen pressure values ​​within the electrolytic cell.

[0013] Preferably, the monitoring module includes a current sensor and a power acquisition unit. The current sensor is installed inside the electrolytic cell and is used to acquire the output current values ​​of the rectifier circuit and each terminal. The power acquisition unit is used to acquire the input power of the electrolytic cell.

[0014] Preferably, it also includes a fault protection module, which is connected to the rectifier circuit and is used to cut off the output current of the rectifier circuit.

[0015] Preferably, the fault protection module is connected to the host computer, and the fault protection module receives control signals from the host computer and operates accordingly.

[0016] Preferably, the fault protection module is connected to the monitoring module, and the fault protection module has a built-in processor chip. The processor chip receives the electrolytic cell operating parameters given by the monitoring module and operates accordingly.

[0017] Preferably, it also includes an alarm module, which is connected to the fault protection module and is used to output an alarm signal.

[0018] A method for controlling the current of a large-scale alkaline water electrolyzer includes the following steps:

[0019] S1. Obtain the operating parameters of the electrolyzer, including the input power, temperature inside the electrolyzer, current inside the electrolyzer, hydrogen pressure and oxygen pressure, and then proceed to step S2.

[0020] S2. Determine the current state of the electrolytic cell based on the operating parameters. If it is under stable operating conditions, proceed to step S3. If it is under variable operating conditions, proceed to step S4.

[0021] S3. If the electrolytic cell operates in the low - power range, determine the set value of the current in the electrolytic cell according to the input power, adjust the output current of the rectifier circuit to the set value, and return to step S1. If the electrolytic cell operates in the high - power range, determine the set value of the current in the electrolytic cell according to the input power, adjust the output current of the rectifier circuit to the set value, and then adjust the output current of each terminal post until each area in the electrolytic cell operates stably, and return to step S1;

[0022] S4. If the input power needs to increase, calculate the current change amount according to the power change, determine the set value of the current in the electrolytic cell, adjust the output current of the rectifier circuit to be lower than the set value, and then increase the output current of each terminal post until the current in the electrolytic cell increases to the set value, and return to step S1. If the input power needs to decrease, calculate the current change amount according to the power change, determine the set value of the current in the electrolytic cell, adjust the output current of the rectifier circuit to be higher than the set value, and then decrease the output current of each terminal post until the current in the electrolytic cell decreases to the set value, and return to step S1.

[0023] Preferably, in step S2, if the electrolytic cell is in a fault state condition, then execute step S5, as follows:

[0024] Step S5. The electrolytic cell stops operating, adjust the output current of the rectifier circuit to zero, restart after the fault is cleared, and return to step S1.

[0025] Preferably, in step S3, the rated input power of the electrolytic cell is X0, and the working range is 0.3X0 - 1.2X0. Obtain the input power X1. If 0.3X0 ≤ X1 ≤ 0.8X0, then the electrolytic cell operates in the low - power range. If 0.8X0 < X1 ≤ 1.2X0, then the electrolytic cell operates in the high - power range.

[0026] Preferably, in step S4, calculate the current change amount according to the power change, determine the set value I of the current in the electrolytic cell. When the input power needs to increase, adjust the output current of the rectifier circuit to 0.9I, and then increase the output current of each terminal post to I. When the input power needs to decrease, adjust the output current of the rectifier circuit to 1.1I, and then decrease the output current of each terminal post to I.

[0027] Compared with the prior art, the present invention has the following beneficial effects:

[0028] (1) On the one hand, a rectifier - circuit control unit is provided to control the output current of the rectifier circuit, so that the total current input to the electrolytic cell can be controlled. On the other hand, a terminal - post control unit is provided to control the output current of the terminal posts, so that the current input to the electrolytic cell by each terminal post can be controlled. Therefore, the present application can accurately control the current in the electrolytic cell, and the control is more flexible and the controllable range is wider.

[0029] (2) Under stable operating conditions, depending on the input power, if the electrolyzer operates in the low power range, only the rectifier circuit control unit needs to control the total current, and the terminal control unit does not need to be turned on. This can improve the system operating efficiency, reduce module operation, and reduce costs. If the electrolyzer operates in the high power range, the rectifier circuit control unit controls the total current to stabilize, ensuring the overall power and hydrogen production efficiency, while the terminal control unit performs auxiliary control to improve the current distribution in the electrolyzer, avoid excessively violent reactions in some areas, increase the stability of the electrolyzer operation, and improve the service life of the electrolyzer, thus greatly improving economic benefits.

[0030] (3) Considering that the current will fluctuate when the input power changes, the output current of the rectifier circuit is adjusted to be slightly greater than or less than the set value, and then slowly adjusted through the terminal control unit to ensure stable current control, thereby avoiding the problem of current instability caused by current fluctuation when the power changes. Attached Figure Description

[0031] Figure 1 A schematic diagram of the current supply system for a large-scale alkaline water electrolysis cell;

[0032] Figure 2 A flowchart of the current control method for a large-scale alkaline water electrolysis cell;

[0033] Attached reference numerals: 1. Host computer, 2. Trigger circuit, 3. Rectifier circuit, 4. Rectifier circuit control unit, 5. Terminal block, 6. Terminal block control unit, 7. Electrolytic cell, 8. Monitoring module. Detailed Implementation

[0034] The present invention will now be described in detail with reference to the accompanying drawings and specific embodiments. These embodiments are based on the technical solution of the present invention and provide detailed implementation methods and specific operating procedures. However, the scope of protection of the present invention is not limited to the following embodiments.

[0035] In the accompanying drawings, components with the same structure are indicated by the same numerical designation, and components with similar structures or functions are indicated by similar numerical designations. The dimensions and thicknesses of each component shown in the drawings are arbitrary, and the present invention does not limit the dimensions and thicknesses of each component. To make the illustrations clearer, some components are appropriately exaggerated in the drawings.

[0036] Example 1:

[0037] Through the inventors' research, it has been found that for large electrolytic cells, under high power and variable power conditions, the electrode reactions in different regions are not uniformly intense. Existing power supply systems can generally only adjust the total input current of the electrolytic cell, thus failing to guarantee the current stability of the electrolytic cell under high power and variable power conditions. Therefore, this application provides a current supply system for large-scale alkaline water electrolytic cells.

[0038] A current supply system for a large alkaline water electrolyzer, such as Figure 1 As shown, it includes: host computer 1, trigger circuit 2, rectifier circuit module, terminal module, monitoring module 8 and electrolytic cell 7. The rectifier circuit module includes rectifier circuit 3 and rectifier circuit control unit 4. The terminal module includes multiple terminals 5 and multiple terminal control units 6.

[0039] The host computer 1 is connected to the trigger circuit 2, the rectifier circuit control unit 4, the terminal control unit 6, and the monitoring module 8. The host computer 1 can be a computer, microprocessor, control cabinet, etc., or it can be understood as a control unit, main control unit, etc. The trigger circuit 2 is used to trigger the rectifier circuit 3. The rectifier circuit 3 is connected to the terminal 5 and is used to input current to each terminal 5. The rectifier circuit control unit 4 is connected to the rectifier circuit 3 and is used to control the output current of the rectifier circuit 3. The terminal 5 is installed on the electrolytic cell 7 and is used to input current to the electrolytic cell 7. The number of terminal control units 6 corresponds to the number of terminal 5 and is connected to the terminal 5 to control the output current of the terminal 5. The monitoring module 8 is installed on the electrolytic cell 7 and is used to monitor the operating parameters of the electrolytic cell 7.

[0040] The monitoring module 8 includes multiple temperature sensors installed inside the electrolytic cell 7 to acquire the temperature value within the cell. It also includes multiple pressure sensors installed inside the cell to acquire the hydrogen and oxygen pressure values. Furthermore, the monitoring module 8 includes a current sensor installed inside the cell to acquire the output current values ​​of the rectifier circuit 3 and each terminal 5. Finally, the monitoring module 8 includes a power acquisition unit to acquire the input power of the electrolytic cell 7. The monitoring module 8 can acquire real-time operating parameters of the electrolytic cell 7, such as the cell temperature, the current flowing through the cell, the hydrogen pressure, the oxygen pressure, the input power, and the pressure difference between hydrogen and oxygen.

[0041] In addition, the current supply system also includes a fault protection module. Fault states include input overvoltage, input undervoltage, input overcurrent, output overcurrent, overtemperature of electrolytic cell 7, and excessive hydrogen-oxygen pressure difference, etc. The fault protection module is connected to the rectifier circuit 3 and is used to cut off the output current of the rectifier circuit 3. The fault protection module can be manually switched on or off, allowing the operator to determine whether the electrolytic cell 7 is in a fault state and thus achieve fault protection; alternatively, the fault protection module can be connected to the host computer 1, receiving control signals from the host computer 1 and operating accordingly. The fault protection module can also be connected to the monitoring module 8, with a built-in processor chip or judgment circuit, etc. The processor chip receives the operating parameters of the electrolytic cell 7 from the monitoring module 8 and determines the fault state and operation. Furthermore, an alarm module can be included, connected to the fault protection module, for outputting alarm signals, such as using a buzzer and LED lights to achieve audible and visual alarms. It should be understood that the above-mentioned fault states and their judgment conditions are common knowledge in the field and will not be elaborated further here.

[0042] In the technical solution of this invention, on the one hand, a rectifier circuit control unit 4 is provided to control the output current of the rectifier circuit 3, thereby allowing the operator to conveniently control the total current input to the electrolytic cell 7. On the other hand, a terminal control unit 6 is provided to control the output current of the terminals 5, thereby allowing the operator to control the current input to the electrolytic cell 7 at each terminal 5, i.e., to control the current at various points within the electrolytic cell 7. In summary, existing technical solutions can basically only control the total current input to the electrolytic cell 7. For electrolytic cells 7 with multiple terminals 5, it is not possible to provide current control at each point. The structural design of this application enables current control of the electrolytic cell 7 from both global and local perspectives. It can control the overall current input to the electrolytic cell 7 as well as the input current at different terminals 5, significantly improving the current control accuracy of the electrolytic cell 7. This ensures stable reactions at various points within the electrolytic cell 7, thereby extending the lifespan of the electrolytic cell 7 and improving its operational stability.

[0043] It should be understood that the present invention does not limit the trigger circuit 2, rectifier control circuit, terminal 5 control circuit, fault protection module, alarm module, etc. Those skilled in the art can implement them according to conventional understanding, such as using a pulse circuit as the trigger circuit 2, adjusting the output current through resistor adjustment, judging the fault through a judgment circuit, cutting off the current through an on / off switch, triggering the alarm circuit through a switching switch, etc., which will not be elaborated here.

[0044] A current control method for a large-scale alkaline water electrolyzer, applicable to alkaline water electrolyzers with multiple current input terminals, includes the following steps:

[0045] S1. Obtain the operating parameters of the electrolyzer, including the input power, temperature inside the electrolyzer, current inside the electrolyzer, hydrogen pressure and oxygen pressure, and then proceed to step S2.

[0046] S2. Determine the current state of the electrolytic cell based on the working parameters. If it is under stable operating conditions, proceed to step S3. If it is under variable operating conditions, proceed to step S4. If the electrolytic cell is under fault conditions, proceed to step S5.

[0047] S3. If the electrolytic cell is operating in the low power range, determine the set value of the current in the electrolytic cell according to the input power, adjust the output current of the rectifier circuit to the set value, and return to step S1. If the electrolytic cell is operating in the high power range, determine the set value of the current in the electrolytic cell according to the input power, adjust the output current of the rectifier circuit to the set value, and then adjust the output current of each terminal until each area in the electrolytic cell is operating stably, and return to step S1.

[0048] S4. If the input power needs to be increased, calculate the change in current based on the power change, determine the set value of the current in the electrolytic cell, adjust the output current of the rectifier circuit to be lower than the set value, and then increase the output current of each terminal until the current in the electrolytic cell slowly increases to the set value, and return to step S1. If the input power needs to be decreased, calculate the change in current based on the power change, determine the set value of the current in the electrolytic cell, adjust the output current of the rectifier circuit to be higher than the set value, and then decrease the output current of each terminal until the current in the electrolytic cell slowly decreases to the set value, and return to step S1.

[0049] Step S5: In the fault state, execute the fault protection shutdown, shut down the electrolytic cell, adjust the output current of the rectifier circuit to zero, and restart after the fault is cleared, then return to step S1.

[0050] like Figure 2 As shown, Figure 2 A flowchart of the current control method described above is provided in this embodiment. First, it is determined whether a fault has occurred. Then, control is performed by distinguishing between stable operating conditions and variable operating conditions. Under stable operating conditions, control is performed based on low power range and high power range. Under variable operating conditions, control is performed based on the increase and decrease of input power.

[0051] For an electrolytic cell with a multi-terminal design, the output current of the terminal is the current inside the electrolytic cell in the area corresponding to the terminal. To avoid overly intense reactions in some areas, two-level regulation of the current in the rectifier circuit and the terminal is performed under high-power intervals and variable-power conditions. The terminal control unit assists in controlling the current inside the electrolytic cell, which can fully improve the current distribution inside the electrolytic cell. This application enables the electrolytic cell to operate stably under different working conditions. While the current of the electrolytic cell is stable, the control accuracy of the current is improved, ensuring that the reactions in all areas of the electrolytic cell tend to be stable, thereby enhancing the safety and efficiency of hydrogen production.

[0052] Specifically, in step S2, according to the input power magnitude required by the host computer, the set value of the current inside the electrolytic cell can be determined. Then, the rectifier circuit is triggered through the trigger circuit, and the input current is sent into the electrolytic cell for electrolysis. The electrolytic cell then feeds back data such as temperature, pressure difference, and current magnitude to the host computer through the monitoring module. Whether the electrolytic cell fails is judged based on multiple data such as temperature, pressure difference, and current. The stability of the current is judged through the current data. Then, the input power is obtained in real time, and different current control methods are selected in combination with the change of the input power.

[0053] Specifically, in step S3, the rated input power of the electrolytic cell is X0, and the working range is 0.3X0 to 1.2X0. The input power X1 is obtained. If 0.3X0 ≤ X1 ≤ 0.8X0, the electrolytic cell operates in the low-power interval and requires a relatively small current inside the electrolytic cell. At this time, the current is low and the overall operation is relatively stable. Therefore, the host computer gives an input signal, and the output current of the rectifier circuit is adjusted to the set value according to the input power. The current inside the electrolytic cell is stabilized near the set value through the rectifier circuit control unit. If 0.8X0 < X1 ≤ 1.2X0, the electrolytic cell operates in the high-power interval and requires a relatively large current inside the electrolytic cell. At this time, the current is large and the electrolytic cell may operate unstably. Therefore, after the output current of the rectifier circuit is adjusted to the set value, the terminal current control unit is used to control the magnitude of the current inside the electrolytic cell to ensure stable operation in all areas. It should be understood that for those skilled in the art, they can set the power ranges of the low-power interval and the high-power interval by themselves according to their actual working conditions, the working parameters of the electrolytic cell, and working experience. This embodiment only gives a better suggestion and is not limited here.

[0054] Specifically, in step S4, the change in current is calculated based on the power change to determine the set value I of the current in the electrolytic cell. When the input power needs to be increased, the output current of the rectifier circuit is adjusted to 0.9I, and then the output current of each terminal is increased to I. Of course, if the current density already exceeds 0.9I, the rectifier circuit control unit does not need to be adjusted further; the current is directly increased slowly to I through the terminal current control unit. When the input power needs to be decreased, the output current of the rectifier circuit is adjusted to 1.1I, and then the output current of each terminal is decreased to I. Of course, if the current density is already below 1.1I, the rectifier circuit control unit does not need to be adjusted further; the current is directly decreased slowly to I through the terminal current control unit. It should be understood that those skilled in the art can set the difference between the output current of the rectifier circuit and the set value I themselves. For example, when the input power increases, the output current of the rectifier circuit can be adjusted to 0.95I, 0.89I, etc., and when the input power decreases, the output current of the rectifier circuit can be adjusted to 1.08I, 1.12I, etc. This embodiment only provides a preferred suggestion and does not impose any limitations.

[0055] Specifically, in step S5, the fault states include input overvoltage, input undervoltage, input overcurrent, output overcurrent, electrolytic cell overtemperature, and excessive hydrogen-oxygen pressure difference. The trigger circuit can be cut off to make the output current of the rectifier circuit zero, and the process can return to step S1 after the fault is cleared.

[0056] The preferred embodiments of the present invention have been described in detail above. It should be understood that those skilled in the art can make numerous modifications and variations based on the concept of the present invention without creative effort. Therefore, all technical solutions that can be obtained by those skilled in the art based on the concept of the present invention through logical analysis, reasoning, or limited experimentation on the basis of existing technology should be within the scope of protection defined by the claims.

Claims

1. A current supply system for a large-scale alkaline water electrolysis cell, characterized in that, It includes a host computer, a rectifier circuit module, a terminal block module, a monitoring module, and an electrolytic cell. The rectifier circuit module includes a rectifier circuit and a rectifier circuit control unit. The terminal block module includes multiple terminals and multiple terminal block control units. The host computer is connected to the rectifier circuit control unit, the terminal control unit, and the monitoring module; The rectifier circuit is connected to the terminals and is used to input current to each terminal. The rectifier circuit control unit is connected to the rectifier circuit and is used to control the output current of the rectifier circuit. The terminals are installed on the electrolytic cell and are used to input current to the electrolytic cell. The number of terminal control units corresponds to the number of terminals and is connected to the terminals to control the output current of the terminals. The monitoring module is installed on the electrolytic cell and is used to monitor the operating parameters of the electrolytic cell; The monitoring module includes multiple temperature sensors and multiple pressure sensors, which are installed inside the electrolytic cell to acquire the temperature, hydrogen pressure, and oxygen pressure values ​​inside the electrolytic cell. The monitoring module includes a current sensor and a power acquisition unit. The current sensor is installed inside the electrolytic cell and is used to acquire the output current values ​​of the rectifier circuit and each terminal. The power acquisition unit is used to acquire the input power of the electrolytic cell.

2. The current supply system for a large-scale alkaline water electrolysis cell according to claim 1, characterized in that, It also includes a trigger circuit, which is connected to the host computer and the rectifier circuit and is used to trigger the rectifier circuit.

3. The current supply system for a large-scale alkaline water electrolysis cell according to claim 1, characterized in that, It also includes a fault protection module, which is connected to the rectifier circuit and is used to cut off the output current of the rectifier circuit.

4. The current supply system for a large-scale alkaline water electrolysis cell according to claim 3, characterized in that, It also includes an alarm module, which is connected to the fault protection module and is used to output alarm signals.

5. A method for controlling the current of a large-scale alkaline water electrolysis cell, characterized in that, Based on the large-scale alkaline water electrolysis cell current supply system as described in any one of claims 1-4, the system includes the following steps: S1. Obtain the operating parameters of the electrolyzer, including the input power, temperature inside the electrolyzer, current inside the electrolyzer, hydrogen pressure and oxygen pressure, and then proceed to step S2. S2. Determine the current state of the electrolytic cell based on the operating parameters. If it is under stable operating conditions, proceed to step S3. If it is under variable operating conditions, proceed to step S4. S3. If the electrolytic cell is operating in the low power range, determine the set value of the current in the electrolytic cell according to the input power, adjust the output current of the rectifier circuit to the set value, and return to step S1. If the electrolytic cell is operating in the high power range, determine the set value of the current in the electrolytic cell according to the input power, adjust the output current of the rectifier circuit to the set value, and then adjust the output current of each terminal until each area in the electrolytic cell is operating stably, and return to step S1. S4. If the input power needs to be increased, calculate the current change amount according to the power change, determine the set value of the current in the electrolytic cell, adjust the output current of the rectifier circuit to be lower than the set value, and then increase the output current of each terminal until the current in the electrolytic cell increases to the set value, and return to step S1. If the input power needs to be decreased, calculate the current change amount according to the power change, determine the set value of the current in the electrolytic cell, adjust the output current of the rectifier circuit to be higher than the set value, and then decrease the output current of each terminal until the current in the electrolytic cell decreases to the set value, and return to step S1.

6. The current control method for a large-scale alkaline water electrolysis cell according to claim 5, characterized in that, In step S2, if the electrolytic cell is in a fault state condition, then execute step S5 as follows: Step S5. Stop the electrolytic cell, adjust the output current of the rectifier circuit to zero, restart after the fault is cleared, and return to step S1.

7. The current control method for a large-scale alkaline water electrolysis cell according to claim 5, characterized in that, In step S3, the rated input power of the electrolytic cell is X0, and the working range is 0.3X0~1.2X0. Obtain the input power X1. If 0.3X0≤X1≤0.8X0, the electrolytic cell operates in the low power range. If 0.8X0<X1≤1.2X0, the electrolytic cell operates in the high power range.

8. The current control method for a large-scale alkaline water electrolysis cell according to claim 5, characterized in that, In step S4, calculate the current change amount according to the power change, determine the set value I of the current in the electrolytic cell. When the input power needs to be increased, adjust the output current of the rectifier circuit to 0.9I, and then increase the output current of each terminal to I. When the input power needs to be decreased, adjust the output current of the rectifier circuit to 1.1I, and then decrease the output current of each terminal to I.

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