A high gravity device and energy-optimized high gravity decarbonization system

By employing a trapezoidal packing clamp and annular protrusion design in a high-gravity rotating bed, combined with a spray pipe and dynamic-static disk structure, the gas-liquid distribution is optimized. Furthermore, by using a falling film reboiler and a molecular sieve catalyst, the problems of uneven gas-liquid distribution and high energy consumption are solved, achieving more efficient mass transfer and energy utilization.

CN117582802BActive Publication Date: 2026-02-06CHINA UNIV OF PETROLEUM (EAST CHINA)
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Patent Information

Application Number
CN202311613779.X
Authority / Receiving Office
CN · China
Patent Type
Patents(China)
Current Assignee / Owner
Filing Date
2023-11-29
Publication Date
2026-02-06
Estimated Expiration
2043-11-29

AI Technical Summary

Technical Problem

The uneven gas-liquid distribution in existing high-gravity rotating beds leads to reduced mass transfer efficiency, low liquid utilization, and high energy consumption.

Method used

The design employs a trapezoidal packing upper clamping plate and an annular raised packing lower clamping plate, combined with a spray pipe and dynamic and static disk structure, to optimize gas-liquid distribution; and uses a falling film reboiler and molecular sieve catalyst to improve mass transfer efficiency and energy utilization.

Benefits of technology

It improves the uniformity of gas-liquid distribution, reduces ineffective contact areas, enhances liquid utilization and mass transfer efficiency, and reduces energy consumption.

✦ Generated by Eureka AI based on patent content.

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Abstract

The application belongs to the field of gas-liquid mass transfer equipment, and provides an energy-optimized supergravity decarbonization system with a supergravity device. The supergravity device comprises a shell, a cavity in the shell, a rotating shaft, filler, an upper filler clamping plate and a lower filler clamping plate in the cavity, a liquid inlet, a liquid outlet, a gas inlet and a gas outlet on the shell, the filler being arranged between the upper filler clamping plate and the lower filler clamping plate, the upper filler clamping plate being trapezoidal, the lower filler clamping plate being provided with an annular protrusion, one end of the rotating shaft being arranged in the cavity and the other end of the rotating shaft extending out of the shell and being connected with a driving mechanism, the filler being symmetrically arranged on both sides of the rotating shaft, spray pipes being arranged on both sides of the rotating shaft and being connected with the liquid inlet. The supergravity device can improve the uniformity of gas-liquid distribution in the upper half of the filler, reduce the area of invalid gas-liquid contact, improve the utilization rate of liquid, and make the gas and liquid fully contact.
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Description

TECHNICAL FIELD

[0001] The present application belongs to the field of gas-liquid mass transfer equipment, and particularly relates to a supergravity device and an energy-optimized supergravity decarbonization system. BACKGROUND

[0002] The statements in this section merely provide background information related to the present application and do not necessarily constitute the prior art.

[0003] The supergravity reactor is a new type of industrial reactor, which utilizes the strong centrifugal force (or supergravity) generated by the high-speed rotating filler bed to continuously disperse and break the liquid to form a larger and continuously updated surface, so that the gas and liquid are fully contacted to obtain a better heat and mass transfer effect.

[0004] In the supergravity reactor, the liquid residence time in the rotating filler bed is generally short (<1s), but when a higher mass transfer effect is required, the filler thickness is generally increased to increase the residence time of the gas and liquid. Considering the mechanical stability of the rotation of the supergravity rotating bed, the rotating filler bed is generally placed in a vertical manner with the rotating shaft. Under the influence of the gravity of the earth, the liquid distribution is closer to the lower side of the filler as it is closer to the outer edge of the rotating shaft, which will cause most of the liquid to pass through the lower side of the filler and the gas to pass through the upper side of the filler with less liquid during the gas-liquid countercurrent mass transfer. The uneven distribution of gas and liquid reduces the mass transfer effect. SUMMARY

[0005] To solve the technical problems in the background art, the present application provides a supergravity device and an energy-optimized supergravity decarbonization system, wherein the supergravity device can improve the uniformity of the gas-liquid distribution in the upper half of the filler, reduce the area of invalid contact between the gas and liquid, and improve the utilization rate of the liquid to ensure sufficient contact between the gas and liquid.

[0006] To achieve the above-mentioned purposes, the present application adopts the following technical solutions:

[0007] The first aspect of the present application provides a supergravity device.

[0008] A supergravity device comprises:

[0009] A shell is provided with a cavity inside, and a rotating shaft, a filler, a lower filler clamp plate and an upper filler clamp plate are arranged in the cavity; the shell is further provided with a liquid inlet, a liquid outlet, a gas inlet and a gas outlet;

[0010] The filler is arranged between the upper filler clamp plate and the lower filler clamp plate, the upper filler clamp plate is trapezoidal, and the lower filler clamp plate is provided with an annular protrusion;

[0011] One end of the rotating shaft is arranged in the cavity, the other end extends out of the shell and is connected with a driving mechanism;

[0012] The fillers are symmetrically arranged on both sides of the rotating shaft, and the rotating shaft is provided with a spray pipe connected with the liquid inlet.

[0013] As an embodiment, the inner wall of the shell is further symmetrically provided with a static disc, and the rotating shaft is symmetrically provided with a dynamic disc, which is arranged opposite to the lower part of the static disc. The liquid on the inner wall of the shell flows into the inner circle of the dynamic disc through the upper surface of the static disc under the action of gravity, and is thrown out of the outer circle of the dynamic disc under the action of centrifugal force, and finally is led out by the liquid outlet.

[0014] As an embodiment, the vertical distance between the foot and the upper base of the trapezoidal upper clamping plate is obtained by calculating the average residence time of the liquid.

[0015] As an embodiment, the average residence time of the liquid and the liquid holdup rate are obtained by mutual derivation.

[0016] As an embodiment, the liquid inlet is used to introduce liquid and sprinkle it on the inner side of the filler through the spray pipe; and the liquid outlet is used to lead out the liquid thrown by the rotating shaft to the inner wall of the shell under the action of gravity.

[0017] As an embodiment, the gas inlet is used to introduce the gas to be purified, and the gas enters the filler from the outer edge of the rotating shaft under the action of gas pressure, and then contacts and mass transfer and heat transfer with the liquid in countercurrent, and the purified gas leaves the rotating shaft from the center of the rotating shaft, and finally is led out by the gas outlet.

[0018] As an embodiment, the rotating shaft extending out of the shell is connected with the shell through a bearing seal.

[0019] The second aspect of the present application provides an energy-optimized supergravity decarbonization system.

[0020] An energy-optimized supergravity decarbonization system comprises:

[0021] a first supergravity device, an amine-rich liquid tank, a lean-rich liquid heat exchanger, a steam-amine-rich liquid heat exchanger, a steam-cooling water heat exchanger, a lean amine liquid-cooling water heat exchanger, a tubular falling film reboiler, a gas-liquid separator, a second supergravity device, a lean amine liquid tank, and a CO2-water separator; wherein the first supergravity device and the second supergravity device are the same as the supergravity device described above;

[0022] The first supergravity device is connected with the uppermost end of the outer wall of the amine-rich liquid tank.

[0023] The amine-rich liquid output from the bottom of the amine-rich liquid tank is transported to the lean-rich liquid heat exchanger.

[0024] The rich liquid outlet of the lean-rich liquid heat exchanger is connected with the rich liquid inlet of the steam-amine-rich liquid heat exchanger, and the rich liquid outlet of the steam-amine-rich liquid heat exchanger is connected with the liquid inlet of the tubular falling film reboiler.

[0025] The molecular sieve regeneration solid catalyst is added to the path of the liquid flowing in the tube falling film reboiler; the material outlet of the tube falling film reboiler is connected with a gas-liquid separator, the liquid in the gas-liquid separator is sent to the liquid inlet of the second super gravity device, and the steam in the gas-liquid separator is introduced into the gas inlet of the second super gravity device;

[0026] The gas outlet of the second super gravity device sends the mixed gas of CO2 and steam to a steam-rich liquid heat exchanger, and the mixed gas after heat exchange is introduced into a steam-cooling water heat exchanger;

[0027] The condensed water output from the bottom of the CO2-water separator is sent to a lean amine liquid tank, the lean amine liquid tank is connected with the liquid outlet of the second super gravity device, the collected lean liquid is transported to a lean-rich liquid heat exchanger for heat exchange, and then is further cooled by a lean amine liquid-cooling water heat exchanger and then is sent to the first super gravity device as an absorption liquid.

[0028] As an embodiment, the lean-rich liquid heat exchanger, the steam-rich liquid heat exchanger, the steam-cooling water heat exchanger and the lean amine liquid-cooling water heat exchanger all adopt printed circuit heat exchangers (PCHE).

[0029] As an embodiment, the bottom of the rich amine liquid tank is connected with the inlet of a rich amine liquid pump, the outlet of the rich amine liquid pump is connected with a rich amine liquid regulating valve and the lean-rich liquid heat exchanger.

[0030] As an embodiment, the gas inlet of the first super gravity device is connected with a flue gas blower;

[0031] As an embodiment, the gas outlet of the second super gravity device is connected with a steam blower, for sending the mixed gas of CO2 and steam to the steam-rich liquid heat exchanger;

[0032] As an embodiment, the bottom of the CO2-water separator is connected with the inlet of a condensed water pump, for transporting the condensed water to the lean amine liquid tank;

[0033] As an embodiment, the lean liquid is transported to the lean-rich liquid heat exchanger for heat exchange by a lean liquid pump.

[0034] The beneficial effects of the present application are:

[0035] (1) The super gravity device of the present application considers the influence of the earth gravity on the liquid distribution in the packing, changes the clamping plate on the packing from a horizontal clamping plate to a trapezoidal clamping plate, improves the uniformity of the gas-liquid distribution in the upper half of the packing, and reduces the area of invalid gas-liquid contact; the present application increases annular protrusions on the lower clamping plate of the packing, promotes the liquid gathered at the bottom of the packing due to the influence of gravity to be lifted again, improves the liquid utilization rate, and makes the gas-liquid fully contact.

[0036] (2) The energy-optimized supergravity decarbonization system of the present application adopts a falling-film reboiler with higher heat exchange efficiency to replace the kettle-type reboiler, thereby reducing the heating power consumption and the equipment footprint; the present application further adds MCM-41 molecular sieve regenerated solid catalyst inside the falling-film reboiler to promote amine liquid stripping and further reduce the heating power consumption; the present application adds a second supergravity device as a stripping device, and the steam at the gas outlet of the device exchanges heat with the rich amine liquid heat exchanger, thereby recovering the heat released by steam condensation and further reducing the power consumption of the entire energy-optimized supergravity decarbonization system.

[0037] Advantages of the additional aspects of the present application will be given in part in the following description, will become apparent from the following description, or will be learned by practice of the present application. BRIEF DESCRIPTION OF DRAWINGS

[0038] The accompanying drawings, which form a part of the specification, are included to provide a further understanding of the application and are incorporated herein for explanation by illustrating a preferred embodiment of the present application.

[0039] Figure 1 is a supergravity device structure schematic diagram of the embodiment of the present application;

[0040] Figure 2 is a device packing lower clamp plan view of the embodiment of the present application;

[0041] Figure 3 is an energy-optimized supergravity decarbonization system schematic diagram of the embodiment of the present application.

[0042] wherein 1 is a spray pipe, 2 is packing, 3 is an external spray pipe, 4 is a static disc, 5 is a dynamic disc, 6 is a liquid outlet, 7 is a bearing seal, 8 is a shell, 9 is a gas inlet, 10 is packing lower clamp, 11 is packing upper clamp, 12 is a gas outlet, 13 is an annular protrusion, 14 is a flue gas blower, 15 is a first supergravity device, 16 is a rich amine liquid tank, 17 is a rich amine liquid regulating valve, 18 is a rich amine liquid pump, 19 is a lean-rich liquid heat exchanger, 20 is a steam-rich liquid heat exchanger, 21 is a steam-cooling water heat exchanger, 22 is a lean amine liquid-cooling water heat exchanger, 23 is a tubular falling-film reboiler, 24 is a gas-liquid separator, 25 is a hot liquid pump, 26 is a steam blower, 27 is a second supergravity device, 28 is a lean amine liquid tank, 29 is a CO2-water separator, 30 is a condensate pump, and 31 is a lean liquid pump. DETAILED DESCRIPTION

[0043] The present application will be further described below in conjunction with the drawings and embodiments.

[0044] It should be noted that the following detailed description is illustrative only, and is intended to provide further description in order to provide a thorough understanding of the present application. Unless otherwise defined, all technical and scientific terms used herein have the same meaning as commonly understood by one of ordinary skill in the art to which the application pertains.

[0045] It is also important to note that the use of the terms "example," "exemplary," "for instance," and "illustrative" herein does not denote a "preferred" embodiment, and that the singular forms "a," "an," and "the" include plural referents unless the context clearly dictates otherwise. It is to be understood that the terms "comprise," "comprising," "include," "including," and "contain," "containing," or variants thereof, do not preclude the presence of other elements or integers.

[0046] In the supergravity method gas purification absorption analysis process, the energy consumption mainly comes from the heating regeneration of rich amine solution. The regeneration process usually uses kettle type reboiler to further heat the rich liquid which is preliminarily heated by the lean-rich heat exchanger. The rich liquid is regenerated by the regeneration device and becomes hot lean liquid. The hot lean liquid exchanges heat with the cold rich liquid from the absorption device in the lean-rich heat exchanger. The lean liquid after heat exchange is further cooled and then transported to the absorption device as absorption liquid.

[0047] <supergravity device>

[0048] According to Figure 1 , the embodiment provides a supergravity device, which comprises a shell 8, a cavity in the shell 8, a rotating shaft, a filler 2, a filler lower clamping plate 10 and a filler upper clamping plate 11 in the cavity, a liquid inlet, a liquid outlet 6, a gas inlet 9 and a gas outlet 12 on the shell 8.

[0049] The filler 2 is arranged between the filler upper clamping plate 11 and the filler lower clamping plate 10, the filler upper clamping plate 11 is trapezoidal, and the filler lower clamping plate 10 is provided with an annular protrusion 13; one end of the rotating shaft is arranged in the cavity, the other end of the rotating shaft extends out of the shell 8 and is connected with a driving mechanism (such as a motor).

[0050] In the embodiment, the spray pipes 1 are symmetrically arranged, dynamic balance is maintained, the dynamic part has high stability when rotating at high speed, and the service life of the dynamic part is prolonged.

[0051] The inner wall of the shell 8 is also symmetrically provided with a static disc 4, the rotating shaft is symmetrically provided with a dynamic disc 5, and the dynamic disc 5 is arranged opposite to the lower side of the static disc 4. The liquid inlet is used to introduce liquid and spray the liquid on the inner side of the filler 2 through the spray pipe 1; the liquid on the inner wall of the shell 8 flows into the inner circle of the dynamic disc 5 through the upper surface of the static disc 4 under the action of gravity, is thrown out of the outer circle of the dynamic disc 5 under the action of centrifugal force, and is finally led out of the liquid outlet 6.

[0052] In one or more embodiments, the upper surface of the stationary disc 4 is inclined, funnel-shaped, which facilitates the flow of liquid under the action of gravity.

[0053] The gas inlet 9 is used to introduce the gas to be purified, which flows from the outer circle of the rotating disc 5 to the inner circle under the action of gas pressure, and then flows from the outer side of the packing 2 to the center of the packing. In the process of flowing, the gas contacts and mass transfers with the amine liquid countercurrently, and the purified flue gas leaves the rotor from the center of the rotor, and finally is led out by the gas outlet 12.

[0054] In this embodiment, the rotating shaft extending out of the shell 8 is connected to the shell 8 through a bearing seal 7.

[0055] The liquid enters through the liquid inlet, is sprinkled on the inner circumferential surface of the packing 2 through the spray pipe 1, and flows to the outer edge of the packing under the action of centrifugal force. In this process, the liquid is dispersed, cut, and broken by the large shear force of the packing to form a state that cannot be formed under normal working conditions, such as liquid filaments, liquid films, and liquid droplets. The surface area of the liquid is extremely large and constantly renewed. The tortuous flow channel in the packing further exacerbates the renewal of the liquid surface, thus forming excellent mass transfer and reaction conditions inside the rotating shaft.

[0056] This embodiment takes into account the effect of the earth's gravity on the distribution of liquid in the packing. The upper clamp plate 11 of the packing is a trapezoidal clamp plate, which improves the uniformity of the gas-liquid distribution in the upper half of the packing and reduces the area of ineffective gas-liquid contact. The annular protrusion 13 is added to the lower clamp plate 10 of the packing, as shown in Figure 2 which promotes the lifting of the liquid that converges at the bottom of the packing due to the effect of gravity, improves the utilization rate of the liquid, and enables the gas and liquid to fully contact. Then, the liquid is thrown by the rotor to the inner wall of the shell, and then flows into the inner circle of the rotating disc 5 through the upper surface of the stationary disc 4 under the action of gravity. The liquid is thrown out from the outer circle of the rotating disc 5 under the action of centrifugal force, and finally is led out by the liquid outlet 6. The gas is introduced into the cavity of the supergravity machine through the gas inlet 9, and flows from the outer circle of the rotating disc 5 to the inner circle under the action of gas pressure, and then flows from the outer side of the packing 2 to the center of the packing. In the process of flowing, the gas contacts and mass transfers with the liquid countercurrently, and the purified gas leaves the rotor from the center of the rotor, and finally is led out by the gas outlet 12.

[0057] In one or more embodiments, the vertical distance between the foot and the upper base of the trapezoidal clamp plate of the packing is obtained by calculating the average residence time of the liquid.

[0058] wherein the average residence time of the liquid and the liquid holdup rate are obtained from each other, as formula (2).

[0059] When foamed nickel is used as the packing, the correlation formula of the liquid holdup rate in the high-porosity packing is formula (1).

[0060] (1)

[0061] (2)

[0062] wherein take 100 m / s 2 , take 0.01 m / s, take 10 -6 m 2 / s, is the velocity of the liquid through the packing, is the kinematic viscosity of the liquid, is the volumetric flow of the liquid, is the average of the inner and outer radius of the packing, is the angular velocity of the rotor, r is the radius of the packing, and are the inner radius of the packing and the outer radius of the packing, respectively, is the axial height of the packing.

[0063] The following takes flue gas decarburization as an example:

[0064] The mixed solution of ethanolamine (MEA) and potassium carbonate (K2CO3) is used for flue gas decarburization. The lean amine solution enters the liquid inlet 1 and is sprayed on the inner circumferential surface of the packing 2 through the spray pipe. Under the action of centrifugal force, it flows to the outer edge of the packing. In this process, the liquid is dispersed, cut and broken by the huge shear force of the packing, forming a state that cannot be formed under normal working conditions such as liquid filament, liquid film and liquid droplet. The surface area of the liquid is very large and constantly updated. The tortuous flow channel in the packing further aggravates the update of the liquid surface, so that excellent mass transfer and reaction conditions are formed inside the rotor. Further, considering the influence of the earth's gravity on the liquid distribution in the packing, the clamping plate 11 on the packing is a trapezoidal clamping plate, which improves the uniformity of the gas-liquid distribution in the upper half of the packing and reduces the area of invalid gas-liquid contact. The annular protrusion 13 is added to the lower clamping plate 10 of the packing, which promotes the liquid gathered at the bottom of the packing due to gravity to be lifted again, improves the utilization rate of the liquid, and makes the gas and liquid fully contact. Then, the liquid is thrown to the inner wall of the shell by the rotor, and is led out by the liquid outlet 6 under the action of gravity. The flue gas is introduced into the cavity by the gas inlet 9, and enters the packing 2 from the outer edge of the rotor under the action of gas pressure. It is in countercurrent contact with the amine solution and mass transfer and heat transfer, and the purified flue gas leaves the rotor from the center of the rotor and is finally led out by the gas outlet 12.

[0065] The supergravity device of the embodiment considers the influence of the gravity of the earth on the liquid distribution in the filler, converts the clamping plate on the filler from a horizontal clamping plate into a trapezoidal clamping plate, improves the uniformity of the gas-liquid distribution in the upper half of the filler, and reduces the area of invalid gas-liquid contact; the application increases annular protrusions on the lower clamping plate of the filler, promotes the liquid gathered at the bottom of the filler due to the influence of gravity to be lifted again, improves the liquid utilization rate, and makes the gas and liquid fully contact.

[0066] <Energy-optimized supergravity decarbonization system>

[0067] According to Figure 3 , the embodiment provides an energy-optimized supergravity decarbonization system, which comprises a flue gas blower 14, a first supergravity device 15, a rich amine liquid tank 16, a rich amine liquid regulating valve 17, a rich amine liquid pump 18, a lean-rich liquid heat exchanger 19, a steam-rich liquid heat exchanger 20, a steam-cooling water heat exchanger 21, a lean amine liquid-cooling water heat exchanger 22, a tubular falling film reboiler 23, a gas-liquid separator 24, a hot liquid pump 25, a steam blower 26, a second supergravity device 27, a lean amine liquid tank 28, a CO2-water separator 29, a condensed water pump 30, and a lean liquid pump 31.

[0068] Among them, the first supergravity device 15 is used as a supergravity absorber, and the second supergravity device 27 is used as a supergravity desorber, and the first supergravity device and the second supergravity device are the same as the supergravity device described above.

[0069] Specifically, the flue gas blower 14 is connected with the gas inlet of the first supergravity device 15, the liquid outlet of the supergravity absorber is connected with the uppermost end of the outer wall of the rich amine liquid tank 16, the rich amine liquid flows along the tank wall, and the amine liquid foaming is reduced.

[0070] The bottom of the rich amine liquid tank 16 is connected with the inlet of the rich amine liquid pump 18, the outlet of the rich amine liquid pump 18 is connected with the rich amine liquid regulating valve 17 and the lean-rich liquid heat exchanger 19, and the rich amine liquid can be introduced into the liquid inlet of the absorption device to further absorb CO2 by opening the rich amine liquid regulating valve 17, so as to improve the actual CO2 load of the rich amine liquid. On the one hand, the liquid flow of the absorption device is increased, and the gas purification rate is improved; on the other hand, the rich amine liquid with high CO2 load can desorb more CO2 under unit energy consumption, improve the desorption efficiency of the desorption device, and reduce the system energy consumption.

[0071] The rich liquid outlet of the lean-rich liquid heat exchanger 19 is connected with the rich liquid inlet of the steam-rich liquid heat exchanger 20, and the rich liquid outlet of the steam-rich liquid heat exchanger 20 is connected with the liquid inlet of the tubular falling film reboiler 23.

[0072] The falling film reboiler has the following advantages: the solution flows in the reboiler in the form of a film, the heat transfer coefficient is high, the residence time is short, the material is not easy to deteriorate, the falling film reboiler is suitable for foaming materials, the liquid process does not form too much impact, the formation of foam is avoided, high-concentration and high-viscosity materials can be evaporated, low-temperature difference evaporation can be used, and the liquid holdup is small. The falling film reboiler can be operated quickly according to the changes in energy supply, feed quantity, concentration, etc.

[0073] The MCM-41 molecular sieve regeneration solid catalyst is added to the path through which the liquid in the tubular falling film reboiler 23 flows, so as to promote the amine liquid stripping.

[0074] The material outlet of the tubular falling film reboiler 23 is connected with the gas-liquid separator 24, the liquid in the gas-liquid separator 24 is sent to the liquid inlet of the second supergravity device 27 by the hot liquid pump 25, and the steam in the gas-liquid separator 24 is introduced into the gas inlet of the second supergravity device 27.

[0075] In the second supergravity device 27, the steam strips the hot amine liquid, the large concentration difference of the stripping product between the steam and the hot amine liquid makes CO2 quickly transfer from the liquid phase to the gas phase, meanwhile, part of the water vapor is liquefied to provide heat for the amine liquid stripping reaction, and the advantages of the supergravity machine in “three transfer and one reaction” accelerate the regeneration of the amine liquid. The steam blower 26 is connected with the gas outlet of the second supergravity device 27, the mixed gas of CO2 and water vapor is sent into the steam-rich liquid heat exchanger 20, the mixed gas after heat exchange is introduced into the steam-cooling water heat exchanger 21 for further cooling, the water vapor is condensed, and CO2 is purified.

[0076] The inlet of the condensate pump 30 is connected with the bottom of the CO2-water separator 29, the condensate is transported to the lean amine liquid tank 28, the lean amine liquid tank 28 is connected with the liquid outlet of the second supergravity device 27, the collected lean liquid is transported to the lean-rich liquid heat exchanger 19 by the lean liquid pump 31 for heat exchange, and then is further cooled by the lean amine liquid-cooling water heat exchanger 22 and then is sent into the first supergravity device 15 as the absorption liquid.

[0077] In one or more embodiments, the lean-rich liquid heat exchanger 19, the steam-rich liquid heat exchanger 20, the steam-cooling water heat exchanger 21 and the lean amine liquid-cooling water heat exchanger 22 all adopt printed circuit heat exchangers (PCHE). The PCHE is compact in design, and the volume of the PCHE is usually 4-6 times smaller than that of a traditional tube-shell heat exchanger and is lighter in weight under the same heat load and pressure drop.

[0078] It should be noted that in other embodiments, the specific models and structures of the lean-rich liquid heat exchanger, the steam-rich liquid heat exchanger, the steam-cooling water heat exchanger and the lean amine liquid-cooling water heat exchanger can be specifically selected by those skilled in the art according to actual needs, which will not be described in detail here.

[0079] The above merely provides the preferred embodiments of the present application, and is not used to limit the present application. For those skilled in the art, the present application can have various modifications and changes. Any modifications, equivalent replacements, improvements, etc. made within the principles and technical scope of the present application shall fall into the scope of the present application.

Claims

1. A high gravity device characterized in that, include: The housing has a cavity inside, and the cavity contains a rotating shaft, packing, a lower packing clamp plate, and an upper packing clamp plate; the housing is also provided with a liquid inlet, a liquid outlet, a gas inlet, and a gas outlet; The packing material is disposed between an upper packing clamp and a lower packing clamp. The upper packing clamp is trapezoidal, and the lower packing clamp has an annular protrusion. The vertical distance between the foot of the trapezoid and the top of the upper packing clamp is obtained by calculating the average liquid residence time. The average liquid residence time is derived from the liquid holdup. One end of the rotating shaft is located inside the cavity, and the other end extends out of the housing and is connected to the drive mechanism; The packing material is symmetrically arranged on both sides of the rotating shaft, and spray pipes are arranged on both sides of the rotating shaft. The spray pipes are connected to the liquid inlet.

2. The high gravity device as claimed in claim 1, wherein, The inner wall of the shell is also symmetrically provided with stationary disks, and the rotating shaft is symmetrically provided with moving disks. The moving disks are arranged directly below the stationary disks. Under the action of gravity, the liquid on the inner wall of the shell flows into the inner ring of the moving disk through the upper surface of the stationary disk, and is thrown out by the outer ring of the moving disk under the action of centrifugal force, and finally led out through the liquid outlet.

3. The high gravity device as claimed in claim 1, wherein, The gas inlet is used to introduce the gas to be purified, and under the action of gas pressure, it enters the packing from the outer edge of the rotating shaft. Then, it comes into countercurrent contact with the liquid and transfers mass and heat, so that the purified gas leaves the rotating shaft from the center and is finally led out from the gas outlet.

4. The high gravity device as claimed in claim 1, wherein, The shaft extending out of the housing is connected to the housing via a bearing seal.

5. An energy-optimized high-gravity decarburization system, characterized in that, include: The system comprises a first hypergravity device, a rich amine liquid tank, a lean-rich liquid heat exchanger, a steam-rich liquid heat exchanger, a steam-cooling water heat exchanger, a lean amine liquid-cooling water heat exchanger, a tubular falling film reboiler, a gas-liquid separator, a second hypergravity device, a lean amine liquid tank, and a CO2-water separator; wherein the first hypergravity device and the second hypergravity device are identical to the hypergravity device as described in any one of claims 1-4. The first hypergravity device is connected to the top of the outer wall of the amine liquid tank. The rich amine liquid output from the bottom of the rich amine liquid tank is transported to the lean-rich liquid heat exchanger; The rich liquid outlet of the lean-rich liquid heat exchanger is connected to the rich liquid inlet of the steam-rich liquid heat exchanger, and the rich liquid outlet of the steam-rich liquid heat exchanger is connected to the liquid inlet of the tubular falling film reboiler. A molecular sieve regenerated solid catalyst is added along the path through which the liquid flows inside the tubular falling film reboiler; the material outlet of the tubular falling film reboiler is connected to a gas-liquid separator, the liquid in the gas-liquid separator is sent to the liquid inlet of the second hypergravity device, and the steam in the gas-liquid separator is introduced into the gas inlet of the second hypergravity device. The gas outlet of the second hypergravity device sends a mixture of CO2 and water vapor into a steam-rich liquid heat exchanger, and the heat-exchanged mixture is then introduced into a steam-cooling water heat exchanger. The condensate output from the bottom of the CO2-water separator is sent to the lean amine liquid tank, which is connected to the liquid outlet of the second hypergravity device. The collected lean liquid is transported to the lean-rich liquid heat exchanger for heat exchange, and then further cooled by the lean amine liquid-cooling water heat exchanger before being sent to the first hypergravity device as the absorbent.

6. The energy-optimized supergravity decarbonization system of claim 5, wherein, The lean-rich liquid heat exchanger, the steam-rich liquid heat exchanger, the steam-cooling water heat exchanger, and the lean amine liquid-cooling water heat exchanger all use printed circuit heat exchangers (PCHEs).

7. The energy-optimized supergravity decarbonization system of claim 5, wherein, The bottom of the rich amine liquid tank is connected with the inlet of the rich amine liquid pump, the outlet of the rich amine liquid pump is connected with the rich-lean liquid heat exchanger and the rich amine liquid regulating valve.

8. The energy-optimized supergravity decarbonization system of claim 5, wherein, The gas inlet of the first supergravity device is connected with the flue gas blower; Or The gas outlet of the second supergravity device is connected with the steam blower, which is used for sending the mixed gas of CO2 and water vapor into the steam-rich liquid heat exchanger; Or The bottom of the CO2-water separator is connected with the inlet of the condensate pump, which is used for sending the condensate into the lean amine liquid tank; Or The lean liquid is sent to the rich-lean liquid heat exchanger by the lean liquid pump.

Citation Information

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