Method for the dechlorination of polyvinyl chloride for the targeted production of high-value chlorine-containing chemicals and applications thereof

By reacting polyvinyl chloride (PVC) with aromatic alcohols under catalyst-free conditions, the problem of efficient conversion of chlorine in waste PVC has been solved, enabling the low-cost preparation of high-value chlorine-containing chemicals, which is suitable for the industrial production of various chlorine-containing aromatic compounds.

CN122301640BActive Publication Date: 2026-09-15ZHEJIANG UNIV
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Patent Information

Application Number
CN202610789124.5
Authority / Receiving Office
CN · China
Patent Type
Patents(China)
Current Assignee / Owner
Filing Date
2026-06-03
Publication Date
2026-09-15
Estimated Expiration
2046-06-03

AI Technical Summary

Technical Problem

Existing technologies are insufficient for efficiently and economically extracting and converting waste polyvinyl chloride into high-value chlorinated chemicals, especially aromatic chlorinated compounds. Furthermore, traditional methods require catalysts or electrocatalysis, resulting in high energy consumption and high costs.

Method used

Under catalyst-free conditions, the chlorine element in PVC is directionally converted into chlorinated aromatic compounds by reacting polyvinyl chloride with aromatic alcohols in a specific solvent, with controlled temperature and time. N-methylpyrrolidone and trace amounts of water are used as solvents, the reaction temperature is 100–300℃, and the time is more than 0.2 h.

Benefits of technology

It has achieved efficient and low-cost preparation of various chlorinated aromatic compounds from waste PVC, with a yield of up to 99%, simplified equipment requirements, reduced energy consumption, reduced side reactions, and has industrialization potential.

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Abstract

The application discloses a method for preparing high-value chlorine-containing chemicals from polyvinyl chloride (PVC) by dechlorination and orientation and application thereof, and belongs to the technical field of solid waste recycling. The method comprises the following steps: constructing a reaction system by using PVC, aromatic alcohol compounds and a solvent, and placing the reaction system in a temperature of 100-300 DEG C for reaction for greater than or equal to 0.2 h to obtain chlorine-containing aromatic compounds; the aromatic alcohol compounds include benzyl alcohol, 2-methylbenzyl alcohol, 3-methylbenzyl alcohol, 4-methylbenzyl alcohol, 4-tert-butylbenzyl alcohol, phenethyl alcohol, 4-bromobenzyl alcohol, p-chlorobenzyl alcohol, 4-hydroxymethyl benzonitrile or 4-hydroxymethyl diphenyl and the like. The method is economical and green, realizes the upgrading conversion of PVC to chlorine-containing aromatic compounds in a one-step method under the condition of no catalyst, is green and environment-friendly, and effectively and fully utilizes the chlorine resources.
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