Seawater electrolysis method, medium and equipment

Abstract

According to the seawater electrolysis method, the medium and the equipment, reaction conditions of a catalyst and component contents and distribution states of different surfaces of an electrode are analyzed by introducing a neural network model, the relationship among morphology, a structure and catalytic activity and the influence of electro-catalytic selectivity of the relationship are further investigated, and by summarizing synthesis conditions, the seawater electrolysis efficiency is improved. And the relevance between the catalyst and the electrocatalytic activity is established. By means of the scheme, the influence rule of the electrode component content and the distribution state on the catalyst performance can be summarized, then targeted synthesis of catalysts with different components is studied, and the optimal catalytic composition and structure are determined. And adding the optimal catalyst into an electrolysis device, and electrolyzing seawater to prepare the hypochlorous acid solution. Compared with the prior art, the seawater electrolysis efficiency can be improved, and power consumption is effectively saved.

Description

Technical Field

[0001] The invention relates to the technical field of water source desalination, and in particular to a seawater electrolysis method, medium and equipment. Background Art

[0002] At present, the industrial electrolysis of seawater to produce hypochlorous acid generally only uses titanium plates as cathode materials, which has the problem of low activity, and the electrolysis efficiency is affected by the relevant parameters of the electrode surface and the pH gradient of the electrolyte. Different pH gradients have different effects on the hydrogen production efficiency and hypochlorous acid production efficiency, as well as the reaction voltage and energy consumption. How to achieve low-energy electrolysis of seawater to produce high-value-added chemical products such as hydrogen and hypochlorous acid has always been a research topic in this field. Summary of the invention

[0003] Therefore, it is necessary to provide a technical solution for seawater electrolysis to solve the problems of high energy consumption and low seawater electrolysis efficiency in the prior art seawater electrolysis methods.

[0004] To solve the above problems, in a first aspect, the present application provides a seawater electrolysis method, the method comprising the following steps:

[0005] constructing a transition metal electrode, and modifying the surface of the transition metal electrode to obtain a modified transition metal electrode;

[0006] Inputting the initial catalyst reaction conditions and the initial experimental result data into the first neural network model for iterative updating to obtain improved catalyst reaction conditions, and preparing catalysts on different surfaces of the transition metal electrode under the improved catalyst reaction conditions;

[0007] Inputting the component contents and distribution states of different surfaces of the sample electrode into the trained second neural network model, analyzing the influence of the component contents and distribution states of different surfaces of the sample electrode on the correlation of the catalyst activity, and obtaining a mapping relationship between the component contents and distribution states and catalyst-related parameters, wherein the catalyst-related parameters include catalyst components and structures;

[0008] Obtaining the component content and distribution state of different surfaces of the transition metal electrode, obtaining the optimal relevant parameters of catalysts on different surfaces according to the mapping relationship, and obtaining the optimal catalyst according to the optimal relevant parameters;

[0009] The optimal catalyst is added to an electrolysis device to electrolyze seawater to prepare a hypochlorous acid solution.

[0010] Furthermore, constructing a transition metal electrode and modifying the surface of the transition metal electrode comprises:

[0011] A multi-component high entropy alloy transition metal electrode is constructed by electrolysis and electrodeposition combined with a high-temperature atmosphere calcination method, and the surface of the transition metal electrode is modified by phosphating and sulfiding methods.

[0012] Furthermore, the method further comprises:

[0013] By utilizing the cocktail effect of high entropy alloys, multiple non-precious metals are alloyed, and the specific surface area of ​​transition metal electrodes is increased through local low-dimensional nano-scaling.

[0014] Furthermore, the initial catalyst reaction conditions include reaction solvent, reaction ligand and basic reaction parameters, and the basic reaction parameters include reaction time, temperature and concentration.

[0015] Furthermore, the analysis of the influence of the component content and distribution state of different surfaces of the sample electrode on the correlation of the catalyst activity includes:

[0016] The characterization technology is used to focus on the surface structure and element valence state differences of the transition metal electrode, and correlated with the improved catalyst reaction conditions to obtain the influence of the component content and distribution state of different surfaces on the correlation of catalyst activity.

[0017] Furthermore, the method comprises:

[0018] When electrolyzing seawater, a pH gradient acid-base asymmetric electrolytic cell is constructed, specifically including:

[0019] Acidic seawater is used as the cathode and alkaline seawater as the anode, and a corresponding pH gradient is provided for the cathode and anode reactions.

[0020] Furthermore, the electrolysis device comprises a reaction barrel (1), a fourth connecting pipe (48) is fixedly connected to the right side of the top of the reaction barrel (1), a dustproof pipe is fixedly connected to the front end of the fourth connecting pipe (48), a compensation component is arranged at the top of the left side of the dustproof pipe, a third connecting pipe (46) is fixedly connected to the bottom of the left side of the dustproof pipe, a first control valve is fixedly connected to the bottom of the third connecting pipe (46), an ejector (44) is fixedly connected to the bottom of the first control valve, a delivery pump (43) is fixedly connected to the right side of the ejector (44), a second connecting pipe (42) is fixedly connected to the top of the delivery pump (43), a three-way valve (41) is fixedly connected to the rear side of the top of the second connecting pipe (42), a connecting pipe (5) is fixedly connected to the right side of the three-way valve (41), a first connecting pipe (4) is fixedly connected to the left side of the three-way valve (41), the first connecting pipe (4) is fixedly connected to the reaction barrel (1), and a refinement component is arranged on the inner side of the bottom of the reaction barrel (1).

[0021] Furthermore, the refinement component comprises a second connecting rod, a support ring is fixedly connected to the inner side of the bottom end of the reaction barrel (1), a first air inlet pipe is fixedly connected to the middle end of the inner side of the support ring, and a spiral tube is fixedly connected to the right side of the first air inlet pipe.

[0022] In a second aspect, the present application provides a computer-readable storage medium having a computer program stored thereon, which, when executed by a processor, implements the seawater electrolysis method as described in the first aspect of the present application.

[0023] In a third aspect, the present application provides an electronic device having a computer program stored thereon, comprising a processor and a storage medium, wherein the storage medium stores a computer program, and when the computer program is executed by the processor, the seawater electrolysis method as described in the first aspect of the present application is implemented.

[0024] Different from the prior art, the seawater electrolysis method, medium and equipment of the present application analyze the reaction conditions of the catalyst, the component content and distribution state of different electrode surfaces by introducing a neural network model, further investigate the relationship between morphology, structure and catalytic activity and the influence of its electrocatalytic selectivity, and establish its correlation with electrocatalytic activity by summarizing the synthesis conditions. Through the scheme of the present application, it is possible to summarize the influence of the electrode component content and distribution state on the performance of the catalyst, and then study the targeted synthesis of catalysts of different components to establish the optimal catalytic composition and structure. Then, the optimal catalyst is added to the electrolysis device, and seawater is electrolyzed to prepare a hypochlorous acid solution. Compared with the prior art, it can improve the efficiency of seawater electrolysis and effectively save power consumption. BRIEF DESCRIPTION OF THE DRAWINGS

[0025] In order to more clearly illustrate the technical solutions in the embodiments of the present invention, the drawings required for use in the description of the embodiments will be briefly introduced below. Obviously, the drawings described below are only some embodiments of the present invention. For ordinary technicians in this field, other drawings can be obtained based on these drawings without paying creative work.

[0026] Figure 1 This is a flow chart of a seawater electrolysis method according to an exemplary embodiment of the present application;

[0027] Figure 2 This is a schematic diagram of the electrolysis of seawater according to an exemplary embodiment of the present application;

[0028] Figure 3 A schematic diagram of a technical route for reducing energy consumption for electrolyzing seawater according to an exemplary embodiment of the present application;

[0029] Figure 4 This is a schematic structural diagram of an electrolysis device according to an exemplary embodiment of the present application;

[0030] Figure 5 A schematic diagram of a module of an electronic device according to an exemplary embodiment of the present application;

[0031] Description of reference numerals:

[0032] 1. Reaction barrel;

[0033] 11. Support leg;

[0034] 2. Motor;

[0035] 4. First connecting pipe;

[0036] 41. Three-way valve;

[0037] 42. Second connecting pipe;

[0038] 43. Delivery pump;

[0039] 44. Ejector;

[0040] 46. ​​third connecting pipe;

[0041] 48. Fourth connecting pipe;

[0042] 5. Connecting pipe;

[0043] 51. Compensation bottle;

[0044] 10. Electronic equipment;

[0045] 101. Processor;

[0046] 102. Storage medium. DETAILED DESCRIPTION

[0047] In order to explain the technical content, structural features, achieved objectives and effects of the technical solution in detail, the following is a detailed description in conjunction with specific embodiments and accompanying drawings.

[0048] The following embodiments of the technical solution of the present application are described in detail in conjunction with the accompanying drawings. The following embodiments are only used to more clearly illustrate the technical solution of the present application, and are therefore only used as examples, and cannot be used to limit the scope of protection of the present application.

[0049] Unless otherwise defined, all technical and scientific terms used herein have the same meaning as commonly understood by technicians in the technical field to which this application belongs; the terms used herein are only for the purpose of describing specific embodiments and are not intended to limit this application; the terms "including" and "having" in the specification and claims of this application and the above-mentioned figure descriptions and any variations thereof are intended to cover non-exclusive inclusions.

[0050] In the description of the embodiments of the present application, the technical terms "first", "second", etc. are only used to distinguish different objects, and cannot be understood as indicating or implying relative importance or implicitly indicating the number, specific order or primary and secondary relationship of the indicated technical features. In the description of the embodiments of the present application, the meaning of "multiple" is more than two, unless otherwise clearly and specifically defined.

[0051] Reference to "embodiments" herein means that a particular feature, structure, or characteristic described in conjunction with the embodiments may be included in at least one embodiment of the present application. The appearance of the phrase in various locations in the specification does not necessarily refer to the same embodiment, nor is it an independent or alternative embodiment that is mutually exclusive with other embodiments. It is explicitly and implicitly understood by those skilled in the art that the embodiments described herein may be combined with other embodiments.

[0052] In the description of the embodiments of the present application, the term "and / or" is only a description of the association relationship of the associated objects, indicating that there may be three relationships. For example, A and / or B can represent: A exists alone, A and B exist at the same time, and B exists alone. In addition, the character " / " in this article generally indicates that the associated objects before and after are in an "or" relationship.

[0053] In the description of the embodiments of the present application, the term "multiple" refers to more than two (including two). Similarly, "multiple groups" refers to more than two groups (including two groups), and "multiple pieces" refers to more than two pieces (including two pieces).

[0054] In the description of the embodiments of the present application, the technical terms "center", "longitudinal", "lateral", "length", "width", "thickness", "up", "down", "front", "back", "left", "right", "vertical", "horizontal", "top", "bottom", "inside", "outside", "clockwise", "counterclockwise", "axial", "radial", "circumferential", etc. indicate orientations or positional relationships based on the orientations or positional relationships shown in the accompanying drawings, which are only for the convenience of describing the embodiments of the present application and simplifying the description, and do not indicate or imply that the referred device or element must have a specific orientation, be constructed and operated in a specific orientation, and therefore should not be understood as a limitation on the embodiments of the present application.

[0055] In the description of the embodiments of the present application, unless otherwise clearly specified and limited, technical terms such as "installed", "connected", "connected", "fixed" and the like should be understood in a broad sense. For example, it can be a fixed connection, a detachable connection, or an integrated connection; it can be a mechanical connection or an electrical connection; it can be a direct connection or an indirect connection through an intermediate medium, and it can be the internal connection of two elements or the interaction relationship between two elements. For ordinary technicians in this field, the specific meanings of the above terms in the embodiments of the present application can be understood according to the specific circumstances.

[0056] In the first aspect, Figure 1 As shown, the present application provides a method for electrolyzing seawater, the method comprising the following steps:

[0057] First, enter step S101 to construct a transition metal electrode, and modify the surface of the transition metal electrode to obtain a modified transition metal electrode;

[0058] Then, step S102 is entered to input the initial catalyst reaction conditions and the initial experimental result data into the first neural network model for iterative update to obtain improved catalyst reaction conditions, and under the improved catalyst reaction conditions, catalysts on different surfaces of the transition metal electrode are obtained;

[0059] Then, step S103 is entered to input the component content and distribution state of different surfaces of the sample electrode into the trained second neural network model, and the influence of the component content and distribution state of different surfaces of the sample electrode on the correlation of catalyst activity is analyzed to obtain a mapping relationship between the component content and distribution state and catalyst-related parameters, wherein the catalyst-related parameters include catalyst components and structures;

[0060] Then, step S104 is entered to obtain the component content and distribution state of different surfaces of the transition metal electrode, obtain the optimal relevant parameters of catalysts on different surfaces according to the mapping relationship, and obtain the optimal catalyst according to the optimal relevant parameters;

[0061] Then, the process proceeds to step S105 to add the optimal catalyst into the electrolysis device to electrolyze seawater to prepare a hypochlorous acid solution.

[0062] In step S101, the transition metal electrode refers to an electrode using transition metals (such as titanium, tungsten, molybdenum, chromium, etc.) as electrode materials. These metals are characterized by having multiple oxidation states and good electrical conductivity, making them very useful in electrochemical reactions. They are widely used in various electrochemical devices and catalysts, such as fuel cells, electrolyzers, and batteries.

[0063] In step S102, the initial catalyst reaction conditions include the reaction solvent, the reaction ligand and the reaction base parameters, which include the reaction time, temperature and concentration. Iterative updates through the first neural network model can enable the catalyst to achieve the purpose of controllable morphology. Among them, the regulation of different atmosphere pyrolysis for the adjustment of catalyst different elements can be achieved by regulating the catalyst with uniform structure and uniform particle size.

[0064] In step S103, the analysis of the influence of the component content and distribution state of different surfaces of the sample electrode on the correlation of the catalyst activity includes: using characterization technology to focus on the surface structure and element valence state differences of the transition metal electrode, and correlating them with the improved catalyst reaction conditions to obtain the influence of the component content and distribution state of different surfaces on the correlation of the catalyst activity.

[0065] Among them, characterization techniques include the use of X-ray diffractometer (XRD), scanning electron microscope, transmission electron microscope, X-ray photoelectron spectroscopy (XPS), etc., focusing on the surface structure of the electrode, the difference in element valence states, and correlating them with the synthetic preparation conditions to derive the differences in reaction conditions and material structure.

[0066] The first neural network model and the second neural network model can be a convolutional neural network (CNN) or a recurrent neural network (RNN) and their variants (such as LSTM, GRU).

[0067] In steps S104 and S105, by studying the control methods of catalyst morphology such as electrochemical control conditions and temperature control, the relationship between morphology, structure and catalytic activity and the influence of electrocatalytic selectivity are further investigated. By summarizing the synthesis conditions, the correlation with electrocatalytic activity is established. After conducting a systematic study, the influence of the electrode component content and distribution state on the catalyst performance (i.e., the mapping relationship) is summarized, so as to carry out targeted synthesis of catalysts of different components and establish the optimal catalytic composition and structure. Then, the optimal catalyst is added to the electrolysis device, and seawater is electrolyzed to prepare a hypochlorous acid solution. Compared with the prior art, it can improve the efficiency of seawater electrolysis and effectively save power consumption.

[0068] In some embodiments, the construction of a transition metal electrode and modification of the surface of the transition metal electrode include: constructing a multinary high entropy alloy transition metal electrode by electrolysis and electrodeposition combined with a high-temperature atmosphere calcination method, and modifying the surface of the transition metal electrode by phosphating and sulfiding methods.

[0069] In some embodiments, the method further includes: utilizing the cocktail effect of high entropy alloys to alloy multiple non-precious metals, which can improve the intrinsic activity and stability of the catalytic material. And increasing the specific surface area of ​​the transition metal electrode through local low-dimensional nano-crystallization. Through local low-dimensional nano-crystallization, the specific surface area of ​​the seawater electrolysis electrode can be increased, more active sites are exposed, the current required by the electrode is achieved, and the voltage is reduced at the same time.

[0070] In some embodiments, the method includes: constructing a pH gradient acid-base asymmetric electrolysis cell when electrolyzing seawater, specifically including: using acidic seawater as the cathode, using alkaline seawater as the anode, and providing corresponding pH gradients for cathode and anode reactions.

[0071] like Figure 2 Shown is a schematic diagram of the electrolysis of seawater according to an exemplary embodiment of the present application. Figure 2 It is an acid-base pH gradient mixed chemical coupling system based on hydrogen production by electrolysis of seawater and electrosynthesis of sodium hypochlorite. Acidic seawater is used as the cathode and alkaline seawater is used as the anode, and a suitable pH gradient is provided for the cathode and anode reactions. Since the hydrogen evolution reaction is kinetically fast in acidic media, while oxygen or chlorine evolution reactions are more easily carried out in alkaline media, acid / base mixed electrolysis can provide a more suitable pH environment for the cathode and anode. In addition, the acidic cathode avoids metal precipitation, improves electrode stability, and regulates the pH gradient effect. While effectively reducing energy consumption, a multifunctional energy-saving acid-base mixed electrolysis new device for seawater hydrogen chloride production and sodium hypochlorite co-production is realized, achieving the effect of reducing costs and increasing efficiency.

[0072] like Figure 3 As shown in FIG. 1 , it is a schematic diagram of a technical route for reducing energy consumption in electrolyzing seawater according to an exemplary embodiment of the present application. In view of the technical problems that enterprises need to solve urgently, such as high energy consumption, low yield and concentration in the electrolysis process of seawater, this project constructs an acid-base pH gradient mixed chemical coupling electrolysis system for seawater. First, a laboratory simulation module study is conducted to select electrode materials and optimize operating parameters, and then intelligent integration and amplification application tests are carried out. The technical route adopted is as follows: Figure 3 As shown, it mainly includes:

[0073] (1) Square meter level electrode preparation: Multi-component high entropy alloy transition metal electrodes are constructed by electrolysis and electrodeposition combined with high temperature atmosphere calcination. The electrode surface is modified by phosphating and sulfiding. Catalysts with different surfaces are prepared by regulating and optimizing the reaction solvent, ligand, and reaction conditions (time, temperature, concentration, etc.) to achieve the purpose of controllable morphology.

[0074] (2) Characterization of electrode physicochemical properties: Using advanced characterization techniques such as X-ray diffractometer (XRD), scanning electron microscopy, transmission electron microscopy, and X-ray photoelectron spectroscopy (XPS), we focus on the surface structure and element valence state differences of the electrodes, and correlate them with the synthesis and preparation conditions to obtain the differences between reaction conditions and material structures; at the same time, we analyze the control methods of catalyst morphology such as electrochemical control conditions and temperature control, and further investigate the relationship between morphology, structure and catalytic activity and its influence on electrocatalytic selectivity. By summarizing the synthesis conditions and establishing their correlation with electrocatalytic activity, we finally determine the optimal catalytic composition and structure.

[0075] (3) Construction and performance optimization of a 500W pH gradient seawater electrolyzer

[0076] Based on the optimization of electrodes, a new electrolytic cell was designed, focusing on the effects of different acid-base gradients on reaction voltage and reaction current, as well as the effect of pH changes on energy saving. The stability of the electrolytic cell was tested at different pH values, and the best pH gradient was obtained through system optimization to achieve the lowest working energy consumption and the highest reaction current and stability.

[0077] like Figure 4 As shown, the electrolysis device comprises a reaction barrel (1), a fourth connecting pipe (48) is fixedly connected to the right side of the top of the reaction barrel (1), a dustproof pipe is fixedly connected to the front end of the fourth connecting pipe (48), a compensation component is arranged at the top of the left side of the dustproof pipe, a third connecting pipe (46) is fixedly connected to the bottom of the left side of the dustproof pipe, a first control valve is fixedly connected to the bottom of the third connecting pipe (46), an ejector (44) is fixedly connected to the bottom of the first control valve, a delivery pump (43) is fixedly connected to the right side of the ejector (44), a second connecting pipe (42) is fixedly connected to the top of the delivery pump (43), a three-way valve (41) is fixedly connected to the rear side of the top of the second connecting pipe (42), a connecting pipe (5) is fixedly connected to the right side of the three-way valve (41), a first connecting pipe (4) is fixedly connected to the left side of the three-way valve (41), the first connecting pipe (4) is fixedly connected to the reaction barrel (1), and a refinement component is arranged on the inner side of the bottom of the reaction barrel (1).

[0078] Furthermore, the refinement component comprises a second connecting rod, a support ring is fixedly connected to the inner side of the bottom end of the reaction barrel (1), a first air inlet pipe is fixedly connected to the middle end of the inner side of the support ring, and a spiral tube is fixedly connected to the right side of the first air inlet pipe.

[0079] In some embodiments, a motor (2) is fixedly connected to the top of the reaction barrel (1), the compensation component includes a compensation bottle (51), and evenly distributed support legs (11) are fixedly connected to the outer side of the bottom end of the reaction barrel (1).

[0080] In some embodiments, the electrolysis device can also prepare hypochlorous acid solution by respectively introducing chlorine gas and sodium hydroxide solution into the anode and cathode. The working principle is as follows: when the electrolysis device is running, the sodium hydroxide solution is first transported into the reaction barrel through the second control valve, and the mixing blade is driven to rotate by the motor using the transmission rod, and the top solution is transported downward while stirring the solution, and then chlorine gas is transported into the spiral tube through the first air inlet pipe, and the chlorine gas is refined into bubbles with smaller diameters through the spiral tube, and the refined chlorine gas bubbles are transported to the sodium hydroxide solution for reaction, and then the second connecting pipe, the three-way valve and the delivery pump are used to transport the chlorine gas into the reaction barrel. The first connecting tube extracts the top solution and transports it back to the reaction through the ejector. During the process, the third connecting tube and the fourth connecting tube are used to extract the gas at the top of the reaction barrel through the ejector, and are remixed inside the right side of the ejector and then ejected at high speed, so that the reaction continues in the reaction barrel. At the same time, a vortex is formed in the reaction barrel by the high-speed ejected gas-liquid mixed fluid, thereby increasing the lateral stress of the bubbles, so that the bubbles can stay in the same water layer for a longer time and react for a long time. After the mixing is completed, the first connecting tube and the connecting tube are connected by rotating the three-way valve, so that cleaning water can be transported to the reaction barrel to facilitate subsequent cleaning.

[0081] In a second aspect, the present invention further provides a computer-readable storage medium having a computer program stored thereon, which, when executed by a processor, implements the text content intelligent segmentation method based on variable vector length as described in the first aspect of the present invention.

[0082] The computer-readable storage medium may be a volatile memory or a non-volatile memory, or may include both volatile and non-volatile memories.

[0083] The non-volatile memory can be a read-only memory (ROM), a programmable read-only memory (PROM), an erasable programmable read-only memory (EPROM), an electrically erasable programmable read-only memory (EEPROM), a ferromagnetic random access memory (FRAM), a flash memory, a magnetic surface memory, an optical disc, or a compact disc read-only memory (CD ROM); the magnetic surface memory can be a disk memory or a tape memory.

[0084] The volatile memory may be a random access memory (RAM), which is used as an external cache. By way of example but not limitation, many forms of RAM are available, such as static random access memory (SRAM), synchronous static random access memory (SSRAM), dynamic random access memory (DRAM), synchronous dynamic random access memory (SDRAM), double data rate synchronous dynamic random access memory (DDRSDRAM), enhanced synchronous dynamic random access memory (ESDRAM), synchronous link dynamic random access memory (SLDRAM), direct memory bus random access memory (DRRAM). The computer-readable storage medium described in the embodiments of the present invention is intended to include these and any other suitable types of memory.

[0085] like Figure 5 As shown, in a third aspect, the present invention provides an electronic device 10, comprising a processor 101 and a storage medium 102, wherein a computer program is stored on the storage medium, and when the computer program is executed by the processor, the text content intelligent segmentation method based on variable vector length as described in the first aspect of the present invention is implemented.

[0086] In some embodiments, the processor can be implemented by software, hardware, firmware or a combination thereof, and can use a circuit, a single or multiple application-specific integrated circuits (Application Specific Integrated Circuit, ASIC), a digital signal processor (Digital Signal Processor, DSP), a digital signal processing device (Digital Signal Processing Device, DSPD), a programmable logic device (Programmable Logic Device, PLD), a field programmable gate array (Field Programmable Gate Array, FPGA), a central processing unit (Central Processing Unit, CPU), a controller, a microcontroller, at least one of a microprocessor, so that the processor can execute part of the steps or all of the steps or any combination of the steps in the method for intelligent segmentation of text content based on variable vector length described in the various embodiments of the present application.

[0087] It should be noted that, although the above embodiments have been described in this article, this does not limit the scope of patent protection of this application. Therefore, based on the innovative concept of this application, changes and modifications made to the embodiments of this article, or equivalent structures or equivalent process changes made using the contents of the specification and drawings of this application, directly or indirectly applying the above technical solutions to other related technical fields are all included in the scope of patent protection of this application.

Claims

1. A method for electrolyzing seawater, characterized in that: The method comprises the following steps: constructing a transition metal electrode, and modifying the surface of the transition metal electrode to obtain a modified transition metal electrode; Inputting the initial catalyst reaction conditions and the initial experimental result data into the first neural network model for iterative updating to obtain improved catalyst reaction conditions, and preparing catalysts on different surfaces of the transition metal electrode under the improved catalyst reaction conditions; Inputting the component contents and distribution states of different surfaces of the sample electrode into the trained second neural network model, analyzing the influence of the component contents and distribution states of different surfaces of the sample electrode on the correlation of the catalyst activity, and obtaining a mapping relationship between the component contents and distribution states and catalyst-related parameters, wherein the catalyst-related parameters include catalyst components and structures; Obtaining the component content and distribution state of different surfaces of the transition metal electrode, obtaining the optimal relevant parameters of catalysts on different surfaces according to the mapping relationship, and obtaining the optimal catalyst according to the optimal relevant parameters; The optimal catalyst is added to an electrolysis device to electrolyze seawater to prepare a hypochlorous acid solution.

2. The seawater electrolysis method according to claim 1, characterized in that: The step of constructing a transition metal electrode and modifying the surface of the transition metal electrode comprises: A multi-component high entropy alloy transition metal electrode is constructed by electrolysis and electrodeposition combined with a high-temperature atmosphere calcination method, and the surface of the transition metal electrode is modified by phosphating and sulfiding methods.

3. The seawater electrolysis method according to claim 1, characterized in that: The method further comprises: By utilizing the cocktail effect of high entropy alloys, multiple non-precious metals are alloyed, and the specific surface area of ​​transition metal electrodes is increased through local low-dimensional nano-scaling.

4. The seawater electrolysis method according to claim 1, characterized in that: The initial catalyst reaction conditions include reaction solvent, reaction ligand and reaction basic parameters, and the reaction basic parameters include reaction time, temperature and concentration.

5. The seawater electrolysis method according to claim 1, characterized in that: The influence of the component content and distribution state of different surfaces of the analyzed sample electrode on the correlation of the catalyst activity includes: The characterization technology is used to focus on the surface structure and element valence state differences of the transition metal electrode, and correlated with the improved catalyst reaction conditions to obtain the influence of the component content and distribution state of different surfaces on the correlation of catalyst activity.

6. The seawater electrolysis method according to claim 1, characterized in that: The method comprises: When electrolyzing seawater, a pH gradient acid-base asymmetric electrolytic cell is constructed, specifically including: Acidic seawater is used as the cathode and alkaline seawater as the anode, and a corresponding pH gradient is provided for the cathode and anode reactions.

7. The seawater electrolysis method according to claim 1, characterized in that: The electrolysis device comprises a reaction barrel (1), a fourth connecting pipe (48) is fixedly connected to the right side of the top of the reaction barrel (1), a dustproof pipe is fixedly connected to the front end of the fourth connecting pipe (48), a compensation component is arranged at the top of the left side of the dustproof pipe, a third connecting pipe (46) is fixedly connected to the bottom of the left side of the dustproof pipe, a first control valve is fixedly connected to the bottom of the third connecting pipe (46), an ejector (44) is fixedly connected to the bottom of the first control valve, a delivery pump (43) is fixedly connected to the right side of the ejector (44), a second connecting pipe (42) is fixedly connected to the top of the delivery pump (43), a three-way valve (41) is fixedly connected to the rear side of the top of the second connecting pipe (42), a connecting pipe (5) is fixedly connected to the right side of the three-way valve (41), a first connecting pipe (4) is fixedly connected to the left side of the three-way valve (41), the first connecting pipe (4) is fixedly connected to the reaction barrel (1), and a refinement component is arranged on the inner side of the bottom of the reaction barrel (1).

8. The seawater electrolysis method according to claim 7, characterized in that: The refinement assembly comprises a second connecting rod, a support ring is fixedly connected to the inner side of the bottom end of the reaction barrel (1), a first air inlet pipe is fixedly connected to the middle end of the inner side of the support ring, and a spiral pipe is fixedly connected to the right side of the first air inlet pipe.

9. A computer-readable storage medium having a computer program stored thereon, characterized in that: When the program is executed by a processor, the seawater electrolysis method according to any one of claims 1 to 8 is implemented.

10. An electronic device having a computer program stored thereon, characterized in that: It comprises a processor and a storage medium, wherein the storage medium stores a computer program, and when the computer program is executed by the processor, the seawater electrolysis method according to any one of claims 1 to 8 is implemented.

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