Parallel calculation method
A technology of parallel computing and computing methods, applied in computing, organic chemistry methods, computational theoretical chemistry, etc., can solve problems such as shortening the integration calculation time
Patent Information
- Authority / Receiving Office
- CN · China
- Patent Type
- Applications(China)
- Current Assignee / Owner
- Publication Date
- 2005-12-28
- Estimated Expiration
- Not applicable · inactive patent
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Abstract
Description
technical field
[0001] The present invention relates to a kind of comprehensive self-consistent field theory (Multi configuration Self-Consistent Field: MSCF) method and configuration interaction (Configuration Interaction: CI) method in the molecular orbital method that has no experience. Parallel Computational Methods for Energy and Energy Gradients. Background technique
[0002] Among non-empirical molecular orbital calculation methods, the above-mentioned MCSCF method and CI method are known as representative calculation methods that can use electron correlation. In the MSCCF method, the differential of the total energy E and the coordinates of the nucleus, that is, the energy gradient (force acting on the nucleus) is obtained as in Equations (1) and (2).
[0003] E = Σ ab MO γ ab h ab + 1 2 ...
Examples
Embodiment Construction
[0056] Embodiments of the present invention will be described below.
[0057] The inventor of the present application believes that: because the two-electron integral of the atomic orbital base layer and the differential of the atomic nucleus coordinates are independent of each other, in the transformation from the atomic orbital base layer to the molecular orbital base layer, the labels r and s of the atomic orbital are parallelized, that is , for the above-mentioned plurality of processors, designate the labels r and s of the atomic orbitals to be calculated, and process the data separately to make the granularity uniform by processing all combinations of t and u by each processor. Although the marks r and s are parallelized, since all combinations of t and u are calculated by each processor, an average of 10,000 floating decimal point operations are required for each two-electron integral, so each processor needs to perform 10000N 2 Times of operations can ensure a suffici...