The invention provides a compound chocolate Chinese herbal composition for treating and improving menstrual syndrome of females. The composition comprises cocoa powder, sugar, skim milk, plant oil, salt, carrageenan, natural flavor, Chinese angelica, folium artemisiae argyi, Ligusticum wallichii, achyranthes root, cinnamon, peach seed, corydalis tuber, tree peony bark, Chinese herbaceous peony, flying squirrel feces, safflower, betel nut, balloonflower root, fennel, Poria cocos, wrinkled giant hyssop, magnolia cortex, atractylodes rhizome, perilla, dried orange peel, dahurian angelica root, yeast, ginger, cape jasmine, nutgrass galingale rhizome, licorice, ginseng, combined spicebush, divaricate saposhnikovia root, bitter organe, astragalus, etc. After scientific concentration, the above-mentioned components are combined according to demands of the pathological degree of menorrhalgia syndrome of females and pharmacological characteristics to form a compound Chinese herbal composition for treating menstrual menorrhalgia syndrome and a compound Chinese herbal composition for treating myoma of uterus; and the two compound Chinese herbal compositions have different efficacy and are then mixed with a cocoa chocolate powder composition so as to compose the special compound chocolate Chinese herbal composition or health care food composition capable of treating and improving a variety of uncomfortable symptoms caused by the menstrual syndrome.