Photoresist compositions and methods of forming photolithographic patterns
A technology of photoresist and photolithography pattern, which is applied in the field of electronic device manufacturing, and can solve problems such as differential photospeed and CD uniformity
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[0066] Preparation of photoresist composition
[0067] Photoresists used in accordance with the present invention are generally prepared according to known procedures. For example, the photoresist composition of the present invention can be prepared by dissolving photoresist components in a solvent component. The ideal total solids content of a photoresist will depend on various factors such as the specific polymers in the composition, final layer thickness and exposure wavelength. Typically the solids content of the photoresist varies from 1 to 10 wt%, more typically from 2 to 5 wt%, based on the total weight of the photoresist composition.
[0068] The photoresist compositions of the present invention find particular utility in negative tone development processes as described below.
[0069] negative tone developing method
[0070] The present invention further provides methods of forming a photoresist relief image and producing electronic devices using the photoresist of...
Embodiment
[0088] Matrix Polymer Synthesis
[0089] The following monomers were employed in the synthesis of the copolymers used in the examples:
[0090] A. Leaving group monomer
[0091]
[0092] B. Lactone group monomer
[0093]
[0094] C. Polar group monomer
[0095]
[0096] A representative example of the polymerization process is given below and all other copolymers were prepared using a similar process with different initiator loading conditions to control molecular weight.
[0097] Synthesis of Poly(MCPMA / NLM)(P-17)
[0098] MCPMA (17.234 g) and NLM (22.766 g) monomers were dissolved in 60 g propylene glycol methyl ether acetate (PGMEA). The monomer solution was degassed by bubbling nitrogen for 20 minutes. PGMEA (31.938 g) was added to a 500 mL three-necked flask equipped with a condenser and mechanical stirrer and degassed by bubbling nitrogen for 20 minutes. The solvent in the reaction flask was then warmed to 80°C. V601 (dimethyl-2,2-azobisisobutyrate) (2.83...
Embodiment 39
[0141] 2.526 g polymer P-17 was dissolved in 29.070 g PGMEA, 19.380 g cyclohexanone and 48.450 g methyl-2-hydroxyisobutyrate. To this mixture was added 0.484 g of "PAGA" described below, 0.029 g of 1-(tert-butoxycarbonyl)-4-hydroxypiperidine quencher, and 0.062 g of PnBMA. The resulting mixture was rolled on a roller for 6 hours and then filtered through a Teflon filter with a 0.2 micron pore size.
[0142]
PUM
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