Branched waterborne polyurethane leather edge oil and preparation method thereof
A water-based polyurethane and leather edge technology, applied in the field of polymer material production, can solve the problems of poor water resistance, solvent resistance and heat resistance, and achieve the effects of easy solubility, simple operation process and excellent fluidity
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Embodiment 1
[0034] Step (1): Preparation of hydroxyl-terminated branched monomer (HPAE)
[0035] Add 10.5g of diethanolamine (DEA) and 10mL of methanol into a three-necked flask, and stir at room temperature until the DEA is completely dissolved, then measure 17mL of methyl acrylate (MA) and slowly add it dropwise to the flask. After the dropwise addition, the temperature is raised to 40 ℃, reacted for 3h, and finally obtained AB by vacuum filtration 2 monomer.
[0036] Using the nucleated "one-step method", trimethylolpropane (TMP) is the central core, according to TMP and AB 2 Molar ratio is 1:3 and takes by weighing TMP, and catalyst p-toluenesulfonic acid is 2% (AB 2 Monomer and TMP mass and percentage), and AB 2 The monomer was slowly added dropwise to the three-neck flask. Raise the temperature to 110°C and start stirring, and react for 2.5 hours. After the reaction is stopped, the crude product is evaporated in vacuo, dissolved in acetone, reprecipitated with dichloromethane, a...
Embodiment 2
[0044] Step (1): Preparation of hydroxyl-terminated branched monomer (HPAE)
[0045] Add 10.5g of diethanolamine (DEA) and 10mL of methanol into a three-necked flask, and stir at room temperature until DEA is completely dissolved, then measure 17mL of methyl acrylate (MA) and slowly drop it into the flask. After the dropwise addition, the temperature is raised to 35 ℃, reacted for 3.5h, and finally obtained AB by vacuum filtration 2 monomer.
[0046] Using the nucleated "one-step method", trimethylolpropane (TMP) is the central core, according to TMP and AB 2 Molar ratio is 1:3 and takes by weighing TMP, and catalyst p-toluenesulfonic acid is 2% (AB 2 Monomer and TMP mass and percentage), and AB 2 The monomer was slowly added dropwise to the three-neck flask. Raise the temperature to 120°C and start stirring, and react for 2 hours. After the reaction stops, the crude product is evaporated in vacuo, dissolved in acetone, reprecipitated with dichloromethane, and extracted wi...
Embodiment 3
[0050] Step (1): Preparation of hydroxyl-terminated branched monomer (HPAE)
[0051] Take 10.5g of diethanolamine (DEA) and 10mL of methanol into a three-necked flask, and stir at room temperature until the DEA is completely dissolved, then measure 17mL of methyl acrylate (MA) and slowly add it dropwise to the flask, and after the dropwise addition, the temperature is raised to 30 ℃, reacted for 4h, and finally obtained AB by vacuum filtration 2 monomer.
[0052] Using the nucleated "one-step method", trimethylolpropane (TMP) is the central core, according to TMP and AB 2 Molar ratio is 1:3 and takes by weighing TMP, and catalyst p-toluenesulfonic acid is 2% (AB 2 Monomer and TMP mass and percentage), and AB 2 The monomer was slowly added dropwise to the three-neck flask. Raise the temperature to 100°C and start stirring, and react for 3 hours. After the reaction stops, the crude product is evaporated in vacuo, dissolved in acetone, reprecipitated with dichloromethane, and...
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