Production method of liquid carbamate prepolymer and resin composition
A technology of urethane and production method, which is applied in the field of isocyanate group-terminated urethane prepolymer, and can solve the problems of poor performance such as heat resistance and light resistance resistance
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[0035] The present invention is explained in more detail with reference to the following examples, but the present invention should not be limited by these examples. All "parts" and "%" are by weight unless otherwise specified. In addition, "molecular weight" means the molecular weight calculated from the hydroxyl value.
[0036] Reference example 1
[0037] will be equipped with stirrer, thermometer, N 2 The inlet tube and the four-necked flask of the air-cooled condenser were installed in a jacketed resistance heater, and 1500 parts of polytetramethylene ether glycol (PTGM, molecular weight: 1300) and 1000 parts of ε-hexane were charged into the flask. Lactone monomer (hereinafter referred to as ε-CL) (PTMG / ε-CL=60 / 40). By blowing in N 2 After uniform mixing with stirring, 0.075 parts of tetraisopropyl titanate (30 ppm to the total amount added) was added, and heating was started to increase the temperature to 180°C. Thereafter, the whole was maintained at 180° C. for 5...
example 2
[0039] Synthesize product in the mode of reference example 1, just replace 1500 parts of molecular weight with the PTMG of 1000 molecular weight as 1300 with 1500 parts of molecular weight. The OH value of the product was 64.6 (molecular weight: 1737).
[0040] Reference example 3
[0041] Synthesize product in the mode of reference example 1, just replace 1500 parts of molecular weight with the copolymer of 1250 parts of THF and methyl-THF (PTGL produced by Hodogaya Chemical Co., Ltd., the PTGL) (molecular weight is 1000) that molecular weight is 1300 PTMG, and Change 1000 parts of ε-caprolactone into 1250 parts. The OH value of the product was 55.1 (molecular weight: 2036).
example 4
[0043] Synthesize product in the mode of reference example 1, just replace 1500 parts of PTMG with molecular weight of 1300 with 1250 parts of PTMG of molecular weight of 650, replace 1250 parts of epsilon-caprolactone with 1250 parts of valerolactone monomers. The OH value of the product was 85.0 (molecular weight: 1320).
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