Polymer additives for powder coatings
a technology of polymer additives and powder coatings, which is applied in the direction of powdery paints, synthetic resin layered products, coatings, etc., can solve the problems of brittleness of durable powder compositions, non-durable films, and inability to give the desired durability, etc., to achieve improved flow and leveling characteristics, increased flexibility, and increased toughness
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example 1
[0033] An acrylic polymer grafted with caprolactone-based chains modified with anhydride was prepared as follows:
[0034] To 325 parts by weight of a commercially available hydroxyl functional acrylic polymer (JONCRYL 587, from S.C. Johnson & Son) was added 3.25 parts by weight of stannous octoate and 1235 parts by weight of ε-caprolactone. The resultant mixture was heated to react in a nitrogen atmosphere at a temperature of 180° C. The reaction was allowed to progress for 4 hours at that temperature. The reaction was then cooled to 120° C. and 62.6 parts by weight of hexahydrophthalic anhydride were added. The reaction was allowed to progress until no anhydride groups were detected by infrared spectroscopy analysis of the material.
[0035] The reaction product was then cooled, discharged and analyzed. The determined acid value was 17.9 mg KOH / gram, and hydroxy value was 4.9 mg KOH / gram. Analysis of the polymer by GPC (using linear polystyrene standards) showed the polymer to have an...
example 2
[0036] An acrylic polymer grafted with caprolactone-based chains modified with anhydride was prepared as follows:
[0037] To 160 parts by weight of JONCRYL 587 was added 3.42 parts by weight of stannous octoate and 1520 parts by weight of ε-caprolactone. The resultant mixture was heated to react in a nitrogen atmosphere at a temperature of 170° C. The reaction was allowed to progress for 4 hours at that temperature. The reaction was then cooled to 120° C. and 30.8 parts by weight of hexahydrophthalic anhydride were added. The reaction was allowed to progress until no anhydride groups were detected by infrared spectroscopy analysis of the material.
[0038] The reaction product was then cooled, discharged and analyzed. The determined acid value was 9.7 mg KOH / gram, and hydroxy value was 3.2 mg KOH / gram. Analysis of the polymer by GPC (using linear polystyrene standards) showed the polymer to have an Mw value of 215,933, and an Mn value of 9293. The melting temperature was determined to ...
example 3
[0039] An acrylic polymer grafted with caprolactone-based chains was prepared as follows:
[0040] To 355 parts by weight of JONCRYL 587 was added 3.41 parts by weight of stannous octoate and 1349 parts by weight of ε-caprolactone. The resultant mixture was heated to react in a nitrogen atmosphere at a temperature of 180° C. The reaction was allowed to progress for 4 hours at that temperature.
[0041] The reaction product was then cooled, discharged and analyzed. The determined acid value was 2.7 mg KOH / gram, and hydroxy value was 20.7 mg KOH / gram. Analysis of the polymer by GPC (using linear polystyrene standards) showed the polymer to have an Mw value of 66,489, and an Mn value of 4,877. The melting temperature was determined to be 56.3° C. by differential scanning calorimetry, and no glass transition temperature was observed.
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