Process for the preparation of pirlindole enantiomers and its salts
A technology of enantiomers and pyrindole, applied in the field of preparing pyrindole enantiomers or their pharmaceutical salts, can solve the problem of low exothermic activity
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[0054] The present invention provides a method for the synthesis of the enantiomers of pyrindole which can be easily converted into the corresponding acid salts.
[0055] In one embodiment, the method of the present invention uses the intermediate compound of formula VI (S)-6-methyl-N-((S)-1-phenylethyl)-2,3,4,9-tetra Hydrogen-1H-carbazol-1-amine
[0056]
[0057] Compounds of formula VI can be prepared in two steps:
[0058] Compound 6-methyl-2,3,4,9-tetrahydro-1H-carbazol-1-ketone of formula IV and chiral auxiliary agent (S)-(-)-α-methylbenzylamine 1- condensation,
[0059]
[0060] Then: 2-stereoselective reduction with sodium borohydride.
[0061] Compounds of formula VI can be cyclized to produce compounds of formula VII (S)-8-methyl-3-((S)-1-phenylethyl)-2,3,3a,4,5,6-hexahydro- 1H-Pyrazino[3,2,1-jk]carbazole
[0062]
[0063] It can be subjected to catalytic hydrogenolysis to give compound (S)-pirindole of formula III.
[0064] In one embodiment, the prese...
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