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Preparation method of hydrogenation catalyst

A technology for hydrogenation catalysts and catalyst carriers, which is applied in the direction of catalyst carriers, molecular sieve catalysts, chemical instruments and methods, etc. It can solve the problems of amorphous silicon-aluminum agglomeration, blockage of molecular sieves, reduction of catalyst specific surface area and pore volume, etc. Uniform distribution, the effect of improving performance

Active Publication Date: 2013-05-15
CHINA PETROLEUM & CHEM CORP +1
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

In this method, amorphous silicon-alumina is prone to agglomeration, and it is also easy to enter the pores of the other party or block the orifice of the molecular sieve, which affects the distribution of amorphous silicon-alumina on the molecular sieve, and the connectivity between molecular sieve and amorphous silicon-alumina channels is poor. The specific surface area and pore volume of the catalyst are reduced, and the distribution of the active metal of the catalyst is uneven, which affects the performance of the catalyst

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0030] Add 365g of solid aluminum chloride into 3.5 liters of distilled water while heating and stirring until dissolved to obtain aluminum chloride solution (a). Add an appropriate amount of distilled water to the concentrated ammonia water and dilute it into about 10wt% dilute ammonia water (b), and dissolve 14 g of octadecylamine in 350 ml of absolute ethanol to form a solution (c). In the stirring state, add 35g modified Y-type molecular sieve Y-1 (SiO 2 / Al 2 o 3 The molar ratio is 11.0, the unit cell constant is 24.42?, and the relative crystallinity is 95%), stirred for 1 hour, filtered, and dried at 100°C for 4 hours to obtain (d). Take a stainless steel reaction tank, add (a) into the tank, stir and heat to 60°C, open the valve of the container containing (b), and control the system in the tank to drop to pH=4.0 within 10 minutes, at this time, add Add (d) into the tank, continue to add (b) dropwise, and control the dropwise addition of the tank system to pH=8.0 wi...

Embodiment 2

[0033] 465g of solid aluminum sulfate was added to 3.5 liters of distilled water while heating and stirring until dissolved to obtain aluminum sulfate solution (a). Add an appropriate amount of distilled water to the concentrated ammonia water and dilute it into about 10wt% dilute ammonia water (b), and dissolve 28g of hexadecylamine in 1L of ethanol to form a solution (c). In the stirring state, add 139g modified Y-type molecular sieve Y-1 (SiO 2 / Al 2 o 3 The molar ratio is 11.0, the unit cell constant is 24.42?, and the relative crystallinity is 95%), stirred for 1 h, filtered to obtain a filter cake, and dried at 110°C for 12 h to obtain (d). Take a stainless steel reaction tank, add (a) into the tank, stir and heat to 60°C, open the valve of the container containing (b), and control the system in the tank to drop to pH=4.0 within 10 minutes, at this time, add Add (d) into the tank, continue to add (b) dropwise, and control the dropwise addition of the tank system to pH...

Embodiment 3

[0037] 230g of solid aluminum sulfate was added to 1.5 liters of distilled water while heating and stirring until dissolved to obtain aluminum sulfate solution (a). Prepare the solid sodium metaaluminate to a concentration of 20g Al 2 o 3 / l sodium aluminate solution (b), 55g decylamine is dissolved in 2.5L ethanol, forms solution (c). In the stirring state, add 548g modified Y-type molecular sieve Y-1 (SiO 2 / Al 2 o 3 The molar ratio is 11.0, the unit cell constant is 24.42 ?, and the relative crystallinity is 95%), and stirred for 1 h to obtain (d). Take a stainless steel reaction tank, put 1L of deionized water into it, stir and heat it to 60°C, open the valves of the containers containing (a), (b) and (d) at the same time, control the pH of the system to 8.0, and control it within 45 minutes Drip (a) and (d) off. Keep the temperature at 60°C, pH=8.0, age for 1 hour, filter the material in the tank, wash until there is no sulfate ion, wash twice with absolute ethanol,...

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Abstract

The invention discloses a preparation method of a hydrogenation catalyst. The preparation method comprises the following steps of preparing a catalyst carrier material and introducing a hydrogenation active component by a dipping method or a coprecipitation method to obtain the hydrogenation catalyst. The preparation process of the catalyst carrier material comprises the following steps of adding a mixture of a molecular sieve and an organic amine into amorphous alumina in gelling, after amorphous alumina gelling, carrying out aging, and then carrying out filtration, washing and drying to obtain the catalyst carrier material. The preparation method realizes ordered arrangement and uniform deposition of the alumina on the surface of the molecular sieve, improves the binding strength of the molecular sieve and the alumina, avoids agglomeration of the amorphous alumina and the molecular sieve and channel blocking caused by the agglomeration, realizes mutual communication of channels of the alumina and the molecular sieve, fully develops synergism of the alumina and the molecular sieve, and improves catalyst use performances. The hydrogenation catalyst obtained by the preparation method can be used for various hydrogenation processes.

Description

technical field [0001] The invention relates to a method for preparing a hydrogenation catalyst, in particular to a method for preparing a hydrogenation catalyst containing molecular sieves. Background technique [0002] The rapid development of the world economy and the gradual heavy and inferior quality of crude oil have made the market more interested in light oil products (sea, land and air transportation oil, agricultural oil and heating oil, etc.) and chemical raw materials (light aromatics, olefins and ethylene) The demand for cracking raw materials, etc.) is increasing year by year; in order to protect the living environment of human beings, various environmental protection laws and regulations are gradually promulgated, and increasingly stringent requirements are put forward for the cleanliness of various oil products. Hydrocracking technology is one of the important means for the secondary processing of crude oil and the lightening of heavy oil. Because of its str...

Claims

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Application Information

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Patent Type & Authority Applications(China)
IPC IPC(8): B01J29/16B01J29/78B01J32/00C10G47/20
Inventor 蒋广安张晔方向晨王继锋
Owner CHINA PETROLEUM & CHEM CORP