Nano core-shell structure pore-forming agent and preparation method thereof

A technology of nano-core-shell and pore-forming agent is applied in the field of nano-core-shell structure pore-forming agent and its preparation, which can solve the problems of easy aggregation of pore structure, unstable structure of foam pore-forming agent, difficult control of pore size and the like.

Inactive Publication Date: 2021-08-10
WUHAN UNIV OF SCI & TECH
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

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Problems solved by technology

"A porous ceramic using straw as a pore-forming agent and its preparation method" (ZL201610118565.9) patent technology uses straw as a pore-forming agent to obtain porous ceramics. Easy to aggregate, and unable to achieve pore size regulation
"Porous corundum aggregate with core-shell structure and its preparation method" (ZL201410584015.7) patented technology, using foam method to prepare porous corundum balls with core-shell structure, but the structure of the foam pore former is unstable, and it is easy to form aggregates. hole, and the pore size is not easy to control

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0026] The preparation method of nano core-shell structure pore-forming agent, comprises the following steps:

[0027] (1) 0.5 gram average particle diameter is 100nm nano-carbon black is added 100 gram mass concentration and carry out ultrasonic dispersion in the ammonia solution of 15wt%, ultrasonic frequency is 20kHz, and dispersion time is 30 minutes, obtains nano-carbon black suspension;

[0028] (2) Under the condition of heating in a water bath at 70°C, add the obtained nano-carbon black suspension dropwise into an aqueous aluminum chloride solution with a concentration of 1.5 mol / L, and the mass ratio of the nano-carbon black suspension to the aqueous aluminum chloride solution is 20:100 , the dropping speed is 0.5 drop / s, and stirs evenly simultaneously, and the stirring speed is 100r / min, and the stirring time is 10 minutes to obtain the mixed solution;

[0029] (3) The obtained mixed solution was left to age for 6 hours, and then centrifuged at a speed of 3000r / min ...

Embodiment 2

[0032] The preparation method of nano core-shell structure pore-forming agent, comprises the following steps:

[0033] (1) 1 gram of average particle diameter is that the nano activated carbon of 400nm is added 100 grams of mass concentration in the aqueous ammonia solution of 20wt% to carry out ultrasonic dispersion, ultrasonic frequency is 30kHz, and dispersion speed is, and dispersion time is 30 minutes, obtains nano activated carbon suspension ;

[0034] (2) Under the condition of heating in a water bath at 90°C, add the obtained nano-activated carbon suspension dropwise into a 2mol / L aluminum nitrate aqueous solution, the mass ratio of the nano-activated carbon suspension to the aluminum nitrate aqueous solution is 30:100, and the dropping rate is 1 drop / s, while stirring evenly, the stirring speed is 200r / min, and the stirring time is 20 minutes to obtain a mixed solution;

[0035] (3) The resulting mixed solution was left to age for 8 hours, and then centrifuged at a ...

Embodiment 3

[0038] The preparation method of nano core-shell structure pore-forming agent, comprises the following steps:

[0039] (1) adding 1 gram of carbon nanospheres with an average particle diameter of 200nm into 100 grams of ammonia solution with a mass concentration of 25wt% for ultrasonic dispersion, the ultrasonic frequency is 40kHz, and the dispersion time is 30 minutes to obtain a suspension of carbon nanospheres;

[0040] (2) Under the condition of heating in a water bath at 80°C, the obtained nanocarbon sphere suspension was added dropwise to a 2.5mol / L aluminum chloride aqueous solution, and the mass ratio of the nanocarbon sphere suspension to the aluminum chloride aqueous solution was 30:100. The dropping rate is 2 drops / s, and the mixture is uniformly stirred at the same time, the stirring speed is 400r / min, and the stirring time is 30 minutes to obtain a mixed solution;

[0041] (3) The resulting mixed solution was left to age for 10 hours, and then centrifuged at a spe...

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Abstract

The invention discloses a preparation method of a nano core-shell structure pore-forming agent. The preparation method comprises the following steps: (1) adding nano carbon material particles into an ammonia water solution, and performing ultrasonic dispersion to obtain a nano carbon material suspension; (2) under a water bath heating condition, dropwise adding the obtained nanocarbon material suspension into a salt solution, and uniformly stirring to obtain a mixed solution; and (3) standing and aging the obtained mixed solution, then carrying out centrifugal separation, removing a supernatant to obtain a precipitate, drying the obtained precipitate, and then carrying out heat preservation to prepare the nano core-shell structure pore-forming agent. The nano core-shell structure pore-forming agent prepared by the invention has the characteristics of good high-temperature structural stability and adjustable pore diameter.

Description

technical field [0001] The invention belongs to the technical field of thermal insulation materials, and more specifically relates to a nano core-shell structure pore-forming agent and a preparation method thereof. Background technique [0002] In the context of industrial green transformation, modern high-temperature industries have put forward higher requirements for energy conservation and emission reduction. In this context, the development of high-efficiency thermal insulation materials has important practical significance for improving the quality and efficiency of high-temperature industries. Porogens are important materials for preparing high-efficiency thermal insulation materials, and their high-temperature structural stability directly determines the pore structure and performance of the prepared thermal insulation materials. With the development of high-temperature industry, it is required to develop porogens with good high-temperature structural stability and a...

Claims

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Application Information

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IPC IPC(8): C04B38/06C04B35/628
CPCC04B38/068C04B35/62813C04B35/62823
Inventor付绿平唐少鹏顾华志黄奥张美杰
OwnerWUHAN UNIV OF SCI & TECH