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A kind of c/sic composite material and preparation method

A composite material and material density technology, which is applied in the field of C/SiC composite materials and preparation, can solve the problems of reducing the porosity of C/SiC composite materials, the effect is not obvious, and the porosity is reduced, so as to improve the ablation resistance and improve the Mechanical properties, the effect of small molecular weight

Active Publication Date: 2021-11-30
AEROSPACE INST OF ADVANCED MATERIALS & PROCESSING TECH
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

In order to further reduce the porosity of C / SiC composites, low-molecular-weight polycarbosilane was used for PIP process at the end of the composite process, and the porosity was reduced to a certain extent, but the effect was not obvious

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0028] 1. The carbon fiber prefabricated body with carbon cloth laminated stitching structure is used, and the low-density C / C composite material is prepared by chemical vapor deposition (CVI) to a density of 0.95g / cm 3 .

[0029] 2. Using the polycarbosilane precursor solution as the impregnation solution, the SiC matrix is ​​densified by the PIP process to a density of 1.4g / cm 3 .

[0030] 3. Using the zirconium precursor solution as the impregnating solution, the PIP process is used for densification, and the number of cycles is 2;

[0031] 4. Using the polycarbosilane precursor solution as the impregnation solution, the SiC matrix is ​​densified by the PIP process until the material density increases by ≤1%.

[0032] The C / SiC composite material prepared in this example is used for testing, the density is GJB / T8133.14 "Test Method for Physical and Chemical Properties of Electric Carbon Products Part 14: Bulk Density", and the open porosity is HB5367.3-86 "Carbon Graphit...

Embodiment 2

[0034] 1. The carbon fiber prefabricated body with carbon cloth laminated stitching structure is used, and the low-density C / C composite material is prepared by chemical vapor deposition (CVI) to a density of 0.95g / cm 3 .

[0035] 2. Using the polycarbosilane precursor solution as the impregnation solution, the SiC matrix is ​​densified by the PIP process to a density of 1.6g / cm 3 .

[0036] 3. Using the zirconium precursor solution as the impregnation solution, the PIP process is used for densification, and the number of cycles is 3 times.

[0037] 4. Using the polycarbosilane precursor solution as the impregnation solution, the SiC matrix is ​​densified by the PIP process until the material density increases by ≤1%.

[0038] The C / SiC composite material prepared by this example is used for testing (the test method is the same as in Example 1), and the porosity of this example is 4.0%. Compared with the C / SiC composite material (the same total number of PIP times) prepared ...

Embodiment 3、4

[0040] Examples 3 and 4 adopt the zirconium precursor PIP process for densification, the number of cycles is 1 and 6 respectively, and the rest are the same as the process of Example 1.

[0041] The C / SiC composite material prepared by this example 3 is used for testing (the test method is the same as in Example 1), and the porosity of this embodiment is 4.7%, which is compared with the C / SiC composite material prepared by conventional processes (the same total number of PIPs) , the open porosity is reduced by 20%, and the tensile strength is increased by 9%.

[0042] The C / SiC composite material prepared by this example 4 is used for testing (the test method is the same as in Example 1), and the porosity of this embodiment is 4.6%, which is compared with the C / SiC composite material prepared by conventional processes (the same total number of PIPs) , the open porosity was reduced by 28%, and the tensile strength was increased by 11%.

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Abstract

The invention provides a C / SiC composite material and a preparation method, which are prepared by a CVI process and a PIP process. During the PIP process, a zirconium precursor is used for several times of PIP process densification. In the present invention, the zirconium precursor solution is used for densification by the PIP process. Because the zirconium precursor has a small molecular weight, a low viscosity, and a large immersion depth, and the zirconium precursor cracking product is a dense powder, it will not cause volume expansion and generate holes inside the material. .

Description

technical field [0001] The invention relates to a C / SiC composite material and a preparation method, belonging to the technical field of SiC composite materials. Background technique [0002] C / SiC composite materials have a series of excellent properties such as low density, high temperature resistance, high specific modulus, high specific strength and thermal shock resistance, and are widely used in the aerospace field. The PIP process is one of the main preparation processes for preparing C / SiC composites. The PIP silicon carbide process technology is to impregnate the polycarbosilane solution into the porous carbon fiber prefabricated body under a certain degree of vacuum, then undergo pressure impregnation and pressure curing, and finally crack the polycarbosilane at a certain temperature to obtain a SiC matrix, thereby obtaining C. / SiC composites. Due to the overflow of a large number of small molecules during the cracking process of polycarbosilane, the cracked pro...

Claims

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Application Information

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Patent Type & Authority Patents(China)
IPC IPC(8): C04B35/80C04B35/83C04B35/52C04B35/622
CPCC04B35/83C04B35/52C04B35/622C04B2235/3826C04B2235/77
Inventor 李晓东刘俊鹏霍鹏飞孙同臣王涛裴雨辰
Owner AEROSPACE INST OF ADVANCED MATERIALS & PROCESSING TECH