Multi-layer coating film forming method
A multi-layer coating and coating technology, applied in chemical instruments and methods, coatings, layered products, etc., can solve the problems of coating uniformity and water resistance deterioration, and achieve excellent water resistance and clear images. The effect of excellent degree and high reversibility
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preparation example Construction
[0037] The preparation method of the hydroxyl-containing polyester resin (A1) is not particularly limited, and conventional methods can be used, for example, by heating the acid component (a1-1) and the alcohol component in a gaseous nitrogen stream at about 150 to about 250°C (a1-2) is carried out for about 5-10 hours to realize the esterification reaction or transesterification reaction of the acid component (a1-1) and the alcohol component (a1-2).
[0038] In the case of such an esterification or transesterification reaction of the acid component (a1-1) and the alcohol component (a1-2), the reactants may be added all at once or in portions. It is also possible to first synthesize a hydroxyl group-containing polyester resin and then react it with an acid anhydride to initiate half-esterification; or to first synthesize a carboxyl group-containing polyester resin and then add the alcohol component (a1-2) thereto.
[0039] In the case of the above esterification or transesteri...
Embodiment
[0164] Hereinafter, the present invention will be explained more specifically with reference to examples, but it should be understood that the present invention is not limited thereto. Hereinafter, "parts" and "%" mean "parts by mass" and "% by mass".
[0165] Preparation of hydroxyl-containing polyester resin solution (A1)
preparation Embodiment 1
[0167] Add 89 parts of neopentyl glycol, 20 parts of trimethylolpropane, 83 parts of isophthalic acid, 44 parts of adipic di acid and 23 parts of 1,2-cyclohexanedicarboxylic anhydride. After raising the temperature from 160°C to 230°C in the reactor over 3 hours, the water of condensation thus formed was distilled off with a water separator while maintaining 230°C. Continue the reaction until the acid value of the product reaches 3 mg KOH / g. With a 50 / 50 (mass) xylene / SWAZOL 1000 (trade name, COSMO Oil Co., Ltd., aromatic hydrocarbon solvent derived from petroleum) mixed solvent, the product was diluted to a solid content of 60% to obtain a hydroxyl-containing poly Ester resin solution (A1-1). The content of the alicyclic polybasic acid (a1-1-2) in the acid component (a1-1) of the obtained hydroxyl group-containing polyester resin was 16 mol% based on the total amount of the acid component (a1-1). The polyester resin had an acid value of 3 mgKOH / g, a hydroxyl value of 67 mg...
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