Method for preparing chromium formate by reducing chromic anhydride with formic acid

A technology of chromium formate and chromic anhydride, which is applied in carboxylate preparation, organic chemistry, etc., can solve problems such as environmental pollution, high energy consumption, and long process, and achieve good economic and social benefits, low energy consumption, and a good reaction process short effect

Inactive Publication Date: 2011-02-23
SHAANXI UNIV OF SCI & TECH
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

The preparation method is divided into two stages. The first stage needs to add sulfuric acid and other reducing agents, mainly to reduce Cr(VI) to Cr(III), and then add alkali to generate Cr(OH) 3 Precipitation, after filtration to give Cr(OH) 3 , after filtration, waste liquid containing sulfate will be produced, which will pollute the environment; the second stage is to use formic acid to dissolve Cr(OH) 3 Chromium formate is generated, and after cooling down, chromium formate crystallizes, and crude chromium formate is obtained by filtration. The whole preparation process is very long and consumes a lot of energy, and waste liquid containing Cr(Ⅲ) will be generated, which will pollute the environment

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0011] 1) At first, get 100 parts of industrial chromic anhydride by mass parts and dissolve with 100 parts of water, join in the reactor that reflux condenser is housed;

[0012] 2) Next, slowly add 200 parts of industrial formic acid to the above reaction kettle. During the addition process, the reaction solution is kept at a slight boiling reflux. After adding the industrial formic acid, heat to keep the reaction solution at a slight boiling reflux for 30 minutes;

[0013] 3) Finally, the reaction solution was cooled to 10° C., crystallized for 3 hours, filtered through a filter cloth, and the solid obtained by the filtration was crude chromium formate.

Embodiment 2

[0015] 1) First, get 100 parts of industrial chromic anhydride by mass parts and dissolve with 130 parts of water, join in the reactor that reflux condenser is housed;

[0016] 2) Next, slowly add 240 parts of industrial formic acid to the above reaction kettle. During the addition process, the reaction solution is kept at a slight boiling backflow. After adding the industrial formic acid, heat to keep the reaction solution at a slight boiling backflow for 30 minutes;

[0017] 3) Finally, the reaction solution was cooled to 20° C., crystallized for 4 hours, filtered through a filter cloth, and the solid obtained by filtering was crude chromium formate.

Embodiment 3

[0019] 1) First, get 100 parts of industrial chromic anhydride by mass parts and dissolve with 200 parts of water, join in the reactor that reflux condenser is housed;

[0020] 2) Next, slowly add 280 parts of industrial formic acid to the above reaction kettle. During the addition process, the reaction solution is kept at a slight boiling reflux. After adding the industrial formic acid, heat to keep the reaction solution at a slight boiling reflux for 30 minutes;

[0021] 3) Finally, the reaction solution was cooled to 13° C., crystallized for 3.5 hours, and filtered through a filter cloth, and the solid obtained by filtering was crude chromium formate.

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Abstract

The invention discloses a method for preparing chromium formate by reducing chromic anhydride with formic acid, which comprises the following steps of: firstly, dissolving industrial chromic anhydride by using water, and adding the solution into a reaction kettle provided with a reflux condenser; secondly, adding industrial formic acid into the reaction kettle, keeping the reaction solution slightly boiled with heating after the industrial formic acid is added, and refluxing the reaction solution for 30 minutes; and finally, cooling the reaction solution to between 10 and 20 DEG C, crystallizing the solution for 3 to 4 hours, and filtering the solution through filter cloth, wherein the filtered solid is rough chromium formate. The formic acid in the reaction plays a role of a reducing agent, and also plays a role of a coordination agent; sulfuric acid and other reducing agents are not needed in the preparation process, so waste liquid containing sulfate is not produced, and environmental pollution is not caused; the formic acid can directly reduce Cr(VI) in the chromic anhydride into Cr(III) and is coordinated with the Cr(III) to directly generate the chromium formate, the temperature is reduced after the reaction is finished, the chromium formate is directly crystallized, and the rough chromium formate is obtained after filtration, so the whole reaction has short flow and low energy consumption, and the residual solution can be recycled so as not to cause environmental pollution.

Description

technical field [0001] The invention relates to the preparation technology of fine chemical products, in particular to a method for preparing chromium formate by reducing chromic anhydride with formic acid. Background technique [0002] Chromium formate is a fine chemical product with a wide range of uses. It can be used as a flower penetration agent for ceramics, a printing and dyeing auxiliary agent, a leather tanning agent, an electroplating material, a raw material for the synthesis of metal complex dyes, and a catalyst for the synthesis of polymer materials. [0003] At present, the main preparation of chromium formate is to use reducing agents, such as glucose, sulfur dioxide, sodium thiosulfate and other reducing agents, to reduce sodium dichromate, potassium dichromate or chromic anhydride under acidic conditions, and to make sodium dichromate, dichromate Cr(Ⅵ) in potassium chromate or chromic anhydride is reduced to Cr(Ⅲ), and then Cr(Ⅲ) is changed to Cr(OH) under a...

Claims

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Application Information

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IPC IPC(8): C07C53/06C07C51/41
Inventor马兴元马小鹏马君
OwnerSHAANXI UNIV OF SCI & TECH