Heat-sensitive recording material
A heat-sensitive recording material and heat-sensitive technology, applied in the field of color developers, can solve the problems of medium durability of text and images, expensive formula, complex recording layer, etc.
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[0114] Preparation of compounds of formula (I) according to the invention.
[0115] Compounds I-XXXII (Table 2) were prepared as follows:
[0116] Step A - Preparation of Nitroaryl Sulfonanilides
[0117] To a mixture of 55 mmol aromatic amine and 50 mmol pyridine was added portionwise 50 mmol nitroarylsulfonyl chloride with stirring. The mixture was briefly (5-10 min) warmed to 95-100° C., cooled and triturated with 100-150 ml hydrochloric acid (2 mol / l). After suction filtration, it is washed neutral with water and dried. The nitroarylsulfonanilide was used in step B without prior purification.
[0118] Step B - Reduction of Nitro Groups to Primary Amines
[0119] Dissolve 40 mmol of the product from step A in 140 ml of ethyl acetate and incorporate 140 mmol of SnCl with stirring 2 2H 2 O and heated under reflux. The reaction progress was followed by DC (elution solvent: cyclohexane / ethyl acetate 1:1). After the end of the reaction (about 2-3h), dilute with 140ml eth...
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