Heteroaromatic NMDA receptor modulators and uses thereof
An individual and carrier technology, applied in medical preparations containing active ingredients, drug combinations, organic chemistry, etc., can solve problems such as unclear functions
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[0050] Example 1-5-(3-chloro-4-fluorophenyl)-7-cyclopropyl-3-(2-(3-fluoro-3-methylazidine-1-yl)-2-oxo Preparation of ethyl)-3,7-dihydro-4H-pyrrole[2,3-d]pyrimidin-4-one (compound 1)
[0051]
[0052] Step-1: Preparation of 4,6-dichloro-5-(2,2-diethoxyethyl)pyrimidine (2):
[0053] Ammonium chloride was added to a solution of 2-(4,6-dichloropyrimidin-5-yl)acetaldehyde (1,5 g, 26.17 mmol) in ethanol (250 mL), and the reaction mixture was refluxed for 20 hours. The reaction mixture was concentrated; the residue was diluted with water (50 mL) and extracted with ethyl acetate (2 x 100 mL). The combined organic layers were dried over anhydrous sodium sulfate, filtered and concentrated to give the title compound 4,6-dichloro-5-(2,2-diethoxyethyl)pyrimidine (2 , 6.9 g, crude product). Calculated (M+H): 265.04; Found (M+H): 265.
[0054] Step-2: Preparation of 4-chloro-7-cyclopropyl-7H-pyrrole[2,3-d]pyrimidine (3):
[0055]Add cyclopropylamine (2 mL, 28.62 mmol) to 4,6-dichloro...
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