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Working electrode for degrading petroleum hydrocarbons, device and application for degrading petroleum hydrocarbons

A technology for working electrodes and petroleum hydrocarbons, which is applied in the field of devices for degrading petroleum hydrocarbons and working electrodes for degrading petroleum hydrocarbons, and can solve problems such as the influence of electricity production performance, the limitation of the degradation process of petroleum hydrocarbons, and the limitation of repair scope.

Active Publication Date: 2022-04-01
NANKAI UNIV
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

[0004] However, in the current MET, the electroactive microorganisms are mainly enriched on the electrode, so the repair range is greatly limited, and only the petroleum hydrocarbon molecules within 1cm around the electrode enriched with electroactive microorganisms can be repaired, and the electroactive microorganisms are in the After being enriched on the electrode for a long time, due to the thickening of the electroactive microbial film, the mass transfer is affected, and its electricity production performance is also greatly affected, which further limits the degradation process of petroleum hydrocarbons.

Method used

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  • Working electrode for degrading petroleum hydrocarbons, device and application for degrading petroleum hydrocarbons
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  • Working electrode for degrading petroleum hydrocarbons, device and application for degrading petroleum hydrocarbons

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preparation example Construction

[0042] In the present invention, the preparation method of the working electrode of described degradation petroleum hydrocarbon preferably comprises the following steps:

[0043] providing a conductive substrate with a working surface including a conductive region and an etched region;

[0044] etching a groove in the etching region to obtain an electrode;

[0045] The electrode is used as the working electrode, and the platinum sheet or steel mesh is used as the counter electrode. In the suspension containing electroactive microorganisms, power is applied, and magnetite is laid in the groove behind the negative electroactive microorganisms in the conductive area. The working electrode for degrading petroleum hydrocarbons is obtained.

[0046] The present invention provides a conductive substrate whose working surface includes a conductive region and an etching region; the present invention does not have any special limitation on the source of the conductive substrate, and th...

Embodiment 1

[0071] as per figure 1 The structure shown:

[0072] Provide a conductive glass with a diameter of 5 cm containing a conductive area and an etched area, wherein the diameter of the conductive area is 2.5 cm;

[0073] Using a laser, etching 10 rows of grooves evenly distributed along the diameter direction in the etching area, the diameter of the grooves is 60nm, and the distance between two adjacent grooves is 0.5cm, to obtain electrodes;

[0074] With the electrode as the working electrode and the platinum sheet as the counter electrode, the working electrode and the counter electrode are placed in a suspension containing electroactive microorganisms (including 1 g / L of sodium acetate, OD600=0.4); wherein the The working surface of the working electrode and the counter electrode is parallel to the horizontal plane, connect the DC power supply, adjust the voltage to be 0.4V, and enrich in the conductive area for 7 days (in the enrichment process, the wireless current acquisit...

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Abstract

The invention relates to the technical field of microbial electrochemistry, in particular to a working electrode for degrading petroleum hydrocarbons, a device and application for degrading petroleum hydrocarbons. The working electrode for degrading petroleum hydrocarbons provided by the present invention includes a conductive substrate; the working surface of the conductive substrate is composed of a conductive region and an etching region; the conductive region and the conductive substrate are concentric circles, and the conductive substrate has a The diameter is greater than the diameter of the conductive region; the etched region is a ring; the sum of the diameter of the conductive region and the wall thickness of the etched region is the same as the diameter of the conductive substrate; the etched region includes Groove area and non-groove area; the grooves in the groove area are arranged at intervals along the diameter direction; electroactive microorganisms grow on the surface of the conductive region; the electroactive microorganisms include petroleum hydrocarbon degrading bacteria; the grooves The tank area is paved with magnetite. The working electrode expands the remediation range of electroactive microorganisms, and further enhances the degradation efficiency of degrading petroleum hydrocarbons.

Description

technical field [0001] The invention relates to the technical field of microbial electrochemistry, in particular to a working electrode for degrading petroleum hydrocarbons, a device and application for degrading petroleum hydrocarbons. Background technique [0002] At present, serious oil pollution problems will be brought about in the exploitation and utilization of oil fields. The erosion of ground oil and the leakage of oil transportation pipelines lead to the pollution of oil to the soil, and with the infiltration and migration in the soil, the oil will gradually pollute the surface water and groundwater, resulting in the decrease of dissolved oxygen in the water body, causing damage to the aquatic ecosystem. serious threat. Therefore, solving the problem of petroleum hydrocarbon pollution in water bodies has become a research hotspot of widespread concern in various countries. [0003] Due to the anaerobic characteristics of petroleum hydrocarbon-contaminated water b...

Claims

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Application Information

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Patent Type & Authority Patents(China)
IPC IPC(8): C02F3/00C02F3/34B09C1/08B09C1/10C02F101/32
CPCC02F3/005C02F3/34B09C1/085B09C1/10C02F2101/32C02F2001/46138C02F2201/46105C02F2305/08C02F2103/06C02F2103/007C02F3/341
Inventor 李田周启星张晓林李瑞祥
Owner NANKAI UNIV
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