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This invention belongs to the field of industrial solid waste resource utilization and inorganic material preparation technology, specifically relating to a coupled method and system for preparing jade core stone from gypsum waste residue and producing sulfuric acid as a byproduct. The coupled method includes: drying the gypsum waste residue in a first drying device to obtain semi-dry gypsum waste residue, then drying the semi-dry gypsum waste residue in a second drying device to obtain anhydrous gypsum raw material; mixing and grinding the anhydrous gypsum with pre-set auxiliary materials, and then processing it through a melting furnace roasting device, a calendering device, and a segmented crystallization annealing device to prepare jade core stone products, wherein the waste heat from the melting furnace roasting device, the calendering device, and the segmented crystallization annealing device is all returned to the second drying device; during the calcination of the anhydrous gypsum mixed and ground with pre-set auxiliary materials in the melting furnace roasting device, the sulfur-containing flue gas generated during the calcination process is collected and sequentially treated through a waste heat recovery device, a purification drying device, and a two-transfer two-absorption device to obtain industrial-grade sulfuric acid.