Composition containing a modified (poly)isocyanate and a solvent of the acetal or aliphatic ketone type, and use of said composition for producing coatings
A polyisocyanate and isocyanate technology, applied in polyurea/polyurethane coatings, coatings, organic chemistry, etc., can solve problems such as insoluble
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Embodiment 1
[0075] Other details or advantages of the present invention will become more apparent from the examples given below. Example Starting materials Jeffsol : Glycerol Carbonate, marketed by the company Huntsman and hereinafter indicated as GC; CAS No.: 931-40-8, MW=118.09 g / mol; Other names: Glycerol Carbonate (glycerol carbonate). HDT, marketed by Rhodia Corporation: Hexamethylene diisocyanate oligomer; CAS No.: 28182-81-2 Vialkyd AN 903 / 70EPAC, marketed by the company Cytec: 70% by weight polyester resin in ethoxypropyl acetate (70EPAC). % OH (by weight) on a dry solids basis: about 4.4%. Highsolv P , sold by the company Clariant: tetramethoxyethane, hereinafter denoted as solvent for HSP. stobicoat N873, marketed by the company Stockmeier: epoxy-amine system. Jeffamines , sold by Huntsman Company: Jeffamine XTJ 582, CAS No.: 9046-10-0; polyoxypropylene diamine 60-100% NH 2 -CH-(CH 3 )-CH 2 -[O-CH 2 -CH(-CH 3 )] n -O-CH 2 -CH(-CH 3 )-NH 2 Jeffa...
Embodiment 2
[0077] Add 50ppm of dibutyltin dilaurate (DBTL) catalyst, relative to HDT meter. The heating temperature was fixed at 90°C. After 5 minutes, the reaction was exothermic, reaching a temperature of 170°C. After cooling and maintaining the temperature of the medium at about 120° C. for 40 minutes, the product is analyzed by infrared spectroscopy. The NCO functions have disappeared and the product obtained is a polyisocyanate mainly having isocyanurate units, the NCO functions of which have been blocked to an extent of 100% by glycerol carbonate. It's labeled HDT-GC. Example 2 : With isocyanate functional groups masked by glycerol carbonate Study on Solubility of HDT
[0078] About 2.5 g of pure HDT GC from Example 1 was weighed into eleven 10 mL flasks.
[0079] About 0.83 g of solvent was then added to each flask in order to obtain a product with a solids content of 75%. The flask was closed. Each mixture was heated at about 100°C to melt the product, which was dissol...
Embodiment 3
[0084] Regardless of the solids content, it should be noted that Highsolv P allows the Good solubilization of the reaction product between HDT and glycerol carbonate, while the solvents usually used to solubilize polyisocyanates are not suitable. Example 3 : Synthesis of HDT-GC in Highsolv P at 75 wt%
[0085] A stream of argon was introduced into a 1-liter jacketed reactor, followed by successive introductions of: -402.5 g of HDT with an isocyanate (NCO) functional group content of 0.501 mol / 100 g, ie 21 wt% NCO functional groups / 100 g product; -237.9 g of glycerol carbonate (Jeffsol GC) (2.01 mol); and -213.4 g of HighSolv P.
[0086] The molar ratio of NCO functional groups / OH functional groups is 1. After heating at 110° C., it is then routinely checked by infrared whether the isocyanate functionality is still present in the medium. After 18 hours, all NCO functionalities had reacted (monitored by infrared) and the solids content of the final product was 75% solids.
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