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Enteric-coated pharmaceutical excipient polymethacrylate emulsion and preparation method thereof

A technology of polymethacrylate and methacrylic acid, applied in the field of medicine, can solve the problems of desorption, poor stability of emulsion polymerization, gelation, etc.

Active Publication Date: 2015-12-23
ENERGY RESOURCES INST HEBEI ACADEMY OF SCI
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

Conventional emulsifiers are adsorbed on the surface of latex particles by physical adsorption, and are easily desorbed by external influences, reducing the stability of the emulsion
In addition, due to the high water solubility of methacrylic acid, most of them are nucleated in the water phase, and oligomers are formed in the water phase to capture the emulsifier of the surrounding environment, resulting in poor polymerization stability of the emulsion, and gels appear during the reaction process. , and even demulsification

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0025] a. 68.5kg deionized water, 0.15kg potassium persulfate, 1.7kg emulsifier 2-allyl ether 3-hydroxypropane-1-sodium sulfonate, 1kg sodium lauryl sulfate and 0.6kg fatty alcohol polyoxyethylene ( 15) Add the ether into the pre-emulsification tank and stir to dissolve, add 21.3kg of methacrylic acid and 25.8kg of ethyl acrylate mixture at a temperature of 25°C and a stirring speed of 1200rad / min, and pre-emulsify for 3.5 hours to obtain a pre-emulsion for later use;

[0026] b. Add 68.5kg of deionized water and 0.12kg of potassium persulfate to the reactor, stir to raise the temperature to 82°C and keep it warm, and start to drop the pre-emulsion obtained in step a into the reactor, and the dropping time is 4h;

[0027] c. Heat at 82°C for 3 hours, cool naturally to 40°C, and filter through a 200-mesh filter to obtain an enteric-coated pharmaceutical excipient polymethacrylate emulsion with a solid content of 27%.

Embodiment 2

[0029] a. 90.8kg deionized water, 0.25kg ammonium persulfate, 2.85kg emulsifier 2-allyl ether 3-hydroxypropane-1-sodium sulfonate, 1.425kg sodium lauryl sulfate and 1.425kg fatty alcohol polyoxyethylene (7) Add the ether to the pre-emulsification tank and stir to dissolve. Add 46.5kg of methacrylic acid and 46.5kg of ethyl acrylate mixture at a temperature of 20°C and a stirring speed of 1200rad / min, and pre-emulsify for 4.5 hours to obtain a pre-emulsion for later use;

[0030] b. Add 136.2kg of deionized water and 0.08kg of ammonium persulfate into the reactor, stir and heat up to 85°C and keep it warm, then drop the pre-emulsion obtained in step a into the reactor, and the dropping time is 4.5h;

[0031] c. Heat at 85°C for 3 hours, cool naturally to 30°C, and filter through a 200-mesh filter to obtain an enteric-coated pharmaceutical excipient polymethacrylate emulsion with a solid content of 35%.

Embodiment 3

[0033] a. 234.37kg deionized water, 0.30kg potassium persulfate, 2.60kg emulsifier 2-allyl ether 3-hydroxypropane-1-sodium sulfonate, 2.80kg sodium lauryl sulfate and 1.2kg fatty alcohol polyoxyethylene (10) Ether is added here to the pre-emulsification tank and stirred to dissolve. At a temperature of 30°C and a stirring speed of 800rad / min, add 50kg of methacrylic acid and 55kg of ethyl acrylate mixture, and pre-emulsify for 0.5h to obtain a pre-emulsion for later use;

[0034] b. Then add 26.04kg of deionized water and 0.11kg of potassium persulfate to the reactor, raise the temperature to 50°C, and start to drop the pre-emulsion obtained in step a into the reactor, and the dropping time is 2h;

[0035] c. Reaction at 50°C for 2 hours, naturally cooled to 35°C, and filtered through a 200-mesh filter to obtain an enteric-coated pharmaceutical excipient polymethacrylate emulsion with a solid content of 30%.

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PUM

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Abstract

The invention relates to an enteric-coated pharmaceutic adjuvant polymethacrylate emulsion and a preparation method thereof. With methacrylic acid and ethyl acrylate as reaction monomers and potassium persulfate or ammonium persulfate as an initiating agent, the enteric-coated pharmaceutic adjuvant polymethacrylate emulsion is prepared by adopting a composite emulsification system composed of a reaction type emulsifier containing no APEO (alkylphenol ethoxylates) and a conventional emulsifier and adopting a pre-emulsification polymerization process. The average particle size of the prepared emulsion is 83nm, and the maximum particle size of the prepared emulsion does not exceed 110nm; and as the enteric-coated pharmaceutic adjuvant polymethacrylate emulsion does not contain APEO and an organic solution, environmental pollution is reduced, thus the enteric-coated pharmaceutic adjuvant polymethacrylate emulsion has wide application prospect in a pharmaceutical industry.

Description

technical field [0001] The invention relates to an emulsion and a preparation method thereof, in particular to an enteric-coated medicinally coated polymethacrylate emulsion and a preparation method thereof, belonging to the technical field of medicine. Background technique [0002] Enteric acrylic resin is a copolymer of methacrylic acid and acrylate monomers, which is mainly prepared by emulsion polymerization. In emulsion polymerization, the emulsifier plays a key role in the stability of the emulsion. Conventional emulsifiers are adsorbed on the surface of latex particles by physical adsorption, and are easily desorbed by external influences, reducing the stability of the emulsion. In addition, due to the high water solubility of methacrylic acid, most of them are nucleated in the water phase, and oligomers are formed in the water phase to capture the emulsifier of the surrounding environment, resulting in poor polymerization stability of the emulsion, and gels appear d...

Claims

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Application Information

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Patent Type & Authority Patents(China)
IPC IPC(8): A61K47/32C08F220/18C08F220/06C08F2/26C08F2/30
Inventor 李彦涛陈孝起周海军张晓蕾杨淑兰李富杰刘德居
Owner ENERGY RESOURCES INST HEBEI ACADEMY OF SCI