Method for preparing biodiesel from waste animal fat under catalysis of imidazole hydrophobic ionic liquid

A technology of ionic liquid and animal fat, applied in the field of waste resource utilization, can solve the problems of raw material pollution, many reaction raw materials, complicated process flow, etc. Effect

Inactive Publication Date: 2019-06-21
KUNMING UNIV OF SCI & TECH
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

[0005] The patent application "A Method for Catalyzed Preparation of Biodiesel by Ionic Liquid" (publication number: CN102031202B) discloses a kind of ionic liquid or a composite catalyst composed of ionic liquid and transition metal chloride salt to catalyze the preparation of biodiesel. However, the hydrophilic ionic liquid used in this method reduces the catalytic performance of the ionic liquid, and it is difficult to separate the transition metal chloride salt from the ionic liquid, and the cost of the transition metal limits its large-scale application
[0006] The patent application "A method for preparing biodiesel by binuclear alkaline ionic liquid catalysis" (publication number: CN105368585A) introduces that the synthesis of binuclear ionic liquid catalyzes the preparation of biodiesel with high catalytic activity, but the synthesis of ionic liquid uses a three-step reaction method, the process flow Complicated, the introduction of a large number of reaction raw materials will cause raw material pollution, and this technology is difficult to be popularized and utilized

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0019] Example 1: Weigh the following bio-oil, methanol, 1-ethyl-3-methylimidazolium hexafluorophosphate ([Emim]PF 6 ), placed in a transesterification reaction device, at a reaction temperature of 30°C, a reaction time of 2h, and kept stirring until the end of the reaction, wherein the moles of bio-oil, methanol, 1-ethyl-3-methylimidazolium hexafluorophosphate The ratio is 2:5:0.2; the reaction solution is put into a separatory funnel, the reaction solution is left to stand for stratification, the upper layer is biodiesel, and the lower layer is a mixed solution of ionic liquid, methanol and by-product glycerol; the biodiesel is taken out and washed with water to obtain the purity For higher biodiesel, the lower methanol and glycerol are distilled under reduced pressure, the glycerol fraction is collected at 164-200 ℃, and the glycerol is further purified to obtain refined glycerol; the ionic liquid is distilled at 90 ℃ under reduced pressure to remove impurities and dried for...

Embodiment 2

[0021] Example 2: Weigh the following bio-oil ester, methanol, 1-hexyl-3-methylimidazolium tetrafluoroborate ([Hmim]BF 4 ) The ionic liquid was placed in the transesterification reaction device, and the reaction time was 1.5 h at a reaction temperature of 40 ° C, and the reaction was kept stirring until the end of the reaction. The molar ratio of the salt is 2:8:0.5; the reaction solution is put into a separatory funnel, the reaction solution is left to stand for stratification, the upper layer is biodiesel, and the lower layer is a mixed solution of ionic liquid, methanol and by-product glycerol; the biodiesel is taken out The biodiesel with higher purity is obtained by washing with water, the methanol and glycerol in the lower layer are distilled under reduced pressure, the glycerol fraction is collected at 164-200° C., and the glycerol is further purified to obtain refined glycerol. The ionic liquid was distilled at 90 °C under reduced pressure to remove impurities and then...

Embodiment 3

[0023] Example 3: Weigh the following biological oil, ethanol, 1-butyl-3-methylimidazole bis-trifluoromethanesulfonimide salt ([Bmim]Tf 2 N) The ionic liquid is placed in the transesterification reaction device, and the reaction time is 1 h at a reaction temperature of 45 ° C, and the reaction is kept stirring until the end of the reaction. The molar ratio of the methanesulfonimide salt is 2:10:0.3; the reaction solution is put into a separatory funnel, the reaction solution is left to stand for stratification, the upper layer is biodiesel, and the lower layer is a mixed solution of ionic liquid, ethanol and by-product glycerol The biodiesel is taken out and washed with water to obtain biodiesel with higher purity, the lower layer methanol and glycerol are distilled under reduced pressure, the glycerol fraction is collected at 164-200°C, and the glycerol is further purified to obtain refined glycerol. The ionic liquid was distilled at 90°C under reduced pressure to remove impu...

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Abstract

The invention discloses a method for preparing biodiesel from waste animal fat under catalysis of an imidazole hydrophobic ionic liquid. The method is characterized in that the biodiesel is prepared through a reaction of raw materials including waste animal fat and short-chain alcohol at 30-50 DEG C with the imidazole hydrophobic ionic liquid used as a catalyst. The catalyst used in the method hashigh stability for moisture in the raw materials and good catalytic effect, the high-yield and high-quality biodiesel can be obtained through the reaction, byproduct glycerin can be efficiently separated from the imidazole hydrophobic ionic liquid, and the catalyst can be recycled after being recovered.

Description

technical field [0001] The invention discloses a method for preparing biodiesel by catalyzing waste animal fats and oils by imidazole hydrophobic ionic liquid, and belongs to the technical field of waste resource utilization. Background technique [0002] Fossil fuels are non-renewable resources, which can no longer meet the needs of world development. In addition, the burning of fossil fuels will bring a series of environmental problems. Therefore, it is urgent to develop renewable and less polluting alternative energy sources to meet the normal development of society. Biodiesel is expected to become an environmentally friendly alternative energy because of its high cetane number, easy biodegradation, non-toxic and harmless, and complete combustion. Vigorously developing biodiesel can effectively alleviate the energy crisis and reduce environmental pollution. [0003] Human production and life produce a large amount of waste oil. According to statistics, the total annual di...

Claims

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Application Information

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Patent Type & AuthorityApplications(China)
IPC IPC(8): C10G3/00
CPCY02P30/20Y02E50/10
Inventor瞿广飞何艳华李晓芬李伟杰徐艺碧宁平
OwnerKUNMING UNIV OF SCI & TECH