A stable and efficient composite water-absorbing material and its preparation method
A water-absorbing material, high-efficiency technology, applied in chemical instruments and methods, alkali metal compounds, other chemical processes, etc., can solve the problems of poor degradability of highly cross-linked resins, limited production and industrial applications, increased toxicity, etc., to achieve stability. Good, rich pore channels, regular pore channels
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Embodiment 1
[0027] Under stirring conditions at room temperature, after dissolving 8g P123 and 50.15g concentrated hydrochloric acid (35%) in 195.16g aqueous solution, 19.80g ethyl orthosilicate (208.33g / mol) and 0.73g 3-aminopropyl trimethoxy Silane (179.29g / mol) was also added successively, the resulting white turbid liquid was continuously stirred at 40°C for 24h, and washed three times with 500mL, 2.6(v / v)% hydrochloric acid-ethanol mixed solution to remove the template After suction filtration and separation, low-temperature vacuum drying to obtain white powder-mesoporous molecular sieve introduced with long-chain alkylamine, the pore size of the mesoporous molecular sieve is 3-20nm, and the specific surface area is 500-1500m 2 / g, the pore volume is 0.8~1.5cm 3 / g.
[0028] After dissolving 2.00 g of polyethyleneimine (with an average molecular weight of 600) in 40 ml of methanol solution, add 2.00 g of the above white powder, continue stirring for 2 hours, evaporate the solvent in a fu...
Embodiment 2
[0030] Under the condition of stirring at room temperature, after dissolving 8g P123 and 50.15g concentrated hydrochloric acid (35%) in 195.16g aqueous solution, 15.86g ethyl orthosilicate (208.33g / mol) and 1.27g 3-aminopropyl triethyl Oxyoxysilane (221.37g / mol) was also added successively, and the resulting white turbid liquid was continuously stirred at 60°C for 12h, and washed three times with 300mL, 3.0(v / v)% hydrochloric acid-ethanol mixed solution to remove the template It is separated by suction and vacuum and dried at low temperature to obtain white powder-mesoporous molecular sieve introduced with long-chain alkylamine. The pore size of the mesoporous molecular sieve is 3-20nm and the specific surface area is 500-1500m. 2 / g, the pore volume is 0.8~1.5cm 3 / g.
[0031] After dissolving 0.80g of polyethyleneimine (average molecular weight of 10000) in 40ml of methanol solution, add 3.20g of the above white powder, continue stirring for 3h, evaporate the solvent in a fume h...
Embodiment 3
[0033] Under the condition of stirring at room temperature, dissolve 9.70g cetyltrimethylammonium bromide in 50ml water, adjust the solution pH=11 with 1:1 sulfuric acid, add 17.56g ethyl orthosilicate (208.33g / mol) And 1.17g of N-aminoethyl-γ-aminopropyltriethoxysilane (264.44g / mol) were also added successively, and the resulting white turbid liquid was continuously stirred at 60°C for 24h, and 500mL, 2.6( v / v)% hydrochloric acid-ethanol mixed solution was washed three times repeatedly to remove the template, separated by suction filtration and vacuum dried at low temperature to obtain a white powder-mesoporous molecular sieve introduced with long-chain alkylamine, the pore size of the mesoporous molecular sieve is 3~ 20nm, the specific surface area is 500~1500m 2 / g, the pore volume is 0.8~1.5cm 3 / g.
[0034] After dissolving 2.00 g of polyethyleneimine (with an average molecular weight of 600) in 40 ml of methanol solution, add 2.00 g of the above white powder, continue stirr...
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