Fluorescent monomers and labeling treatment polymers containing them for industrial water systems
A technology for labeling treatment and industrial water, which is applied in the field of fluorescent monomers, and can solve the problems of chemical combination of fluorescent parts and non-fluorescent polymers, and the difficulty of polymer labeling
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[0101] The preparation of high molecular weight water-in-oil emulsion polymers has been described in the following references: U.S. Patent 2,982,749 assigned to Dow Chemical Company; U.S. Patent 3,284,393 assigned to Dow Chemical Company; U.S. Patent 3,734,873 assigned to Nalco Chemical Company; Hundeler, D., Hamielec, A. and Baade, W. "Mechanism, Kinetics and Modeling of the Inverse-Microsuspension Homopolymerization of Acrylamide," polymer (1989), 30(1), 127-42; and "Mechanism, Kinetics and Modeling of Inverse-Microsuspension Polymerization: 2. Copolymerization of Acrylamide with Quaternary AmmoniumCationic Monomers," by D. Hunkeler and A.E. Hamielec polymer (1991), 32(14), 2626-40.
[0102] A general procedure for making water-in-oil emulsion marker treatment polymers is provided to exemplify the use of fluorescent monomers to prepare these marker treatment polymers. The type and amount of specific components in the formula (eg, monomers, initiators, chain transfer agent...
Embodiment 1
[0324]
[0325] Sulfonated-N-(3-N',N'-dimethylaminopropyl)benzo(k,l)xanthene-3,4-dicarboxylic acid imide, 2-hydroxy-3-allyl Preparation of oxypropyl quaternary salt (S-NDMAPBXA-DCI-HAPQ)
[0326] Benzoxanthenes were synthesized according to the method of A.T. Peters and Y.S.S. Behesti in Journal of the Society of Dyers and Colorists, 1989, 105, pp. 29-35, and were synthesized according to the procedure described in U.S. Patent No. 3,888,863 to H. Troster change.
[0327] first step:
[0328] Synthesis of sulfonated-N-(3-N',N'-dimethylaminopropyl)benzo(k,l)xanthene-3,4-dicarboxylic imide (I)
[0329] A 25 ml round bottom flask was charged with sulfonated benzo(k,l)xanthene-3,4-dicarboxylic acid imide (0.5 g, 0.714 mmol, 64%), 6.5 mL of water and 0.15 g of glacial acetic acid. 3-(Dimethylamino)-1-propanamine (0.131 g, 1.28 mmol) was added dropwise. The mixture was refluxed for 5 hours and cooled. The solution was concentrated to dryness to give the product.
[0330] Ste...
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