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A kind of surface passivation treatment method of nickel base alloy

A nickel-based alloy and passivation treatment technology, which is applied in the direction of metal material coating process, coating, solid-state diffusion coating, etc., can solve problems such as nickel-based alloy corrosion, prolong service life, increase corrosion resistance, attach focus on good effect

Active Publication Date: 2020-07-03
SHANGHAI INST OF APPLIED PHYSICS - CHINESE ACAD OF SCI
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

[0005] The technical problem to be solved by the present invention is to provide a surface passivation treatment method for nickel-based alloys in order to overcome the defects of corrosion of existing nickel-based alloys in the environment of strong fluorinating agents

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0022] Use 0.5mol / L HNO in the nickel base alloy reactor 3 Pickling with -5% NaCl solution, and then washing with water, and then drying it in a blast drying oven at 90°C for 1 hour. Replace the gas in the reactor with high-purity argon, and finally carry out the passivation treatment of the nickel-based alloy reactor according to the following passivation treatment scheme 1.

[0023] Passivation treatment scheme 1 is as follows:

[0024] The first stage: Heating the nickel-based alloy reactor to 100°C, during which the fluorine gas fraction is 30% F 2 / Ar mixture;

[0025] The second stage: heating the nickel-based alloy reactor from 100°C to 350°C, during which the flow rate of 0.2L / min is 30% F 2 / Ar mixture;

[0026] The third stage: Keep the nickel-based alloy reactor at a constant temperature of 350°C for 3 hours, during which the flow rate is 0.1L / min and F with a fluorine gas fraction of 30% is introduced. 2 / Ar mixture;

[0027] The fourth stage: naturally cool ...

Embodiment 2

[0030] Use 1.0mol / L HNO in the nickel base alloy reactor 3 Pickling with -5% NaCl solution, then washing with water, and then drying it in a blast drying oven at 100°C for 5 hours. Replace the gas in the reactor with high-purity argon, and finally carry out the passivation treatment of the nickel-based alloy reactor according to the following passivation treatment scheme 2.

[0031] Passivation treatment scheme 2 is as follows:

[0032] The first stage: Heating the nickel-based alloy reactor to 130°C, during which the fluorine gas fraction is 20% F 2 / Ar mixture;

[0033] The second stage: Heating the nickel-based alloy reactor from 100°C to 400°C, during the period, according to the flow rate of 0.1L / min, F with a fluorine gas fraction of 20% 2 / Ar mixture;

[0034] The third stage: Keep the nickel-based alloy reactor at a constant temperature of 400 ° C for 6 hours, during which the flow rate is 0.2 L / min, and the fluorine gas fraction is 20% F 2 / Ar mixture;

[0035] ...

Embodiment 3

[0038] Use 1.5mol / L HNO in the nickel base alloy reactor 3 Pickling with -5% NaCl solution, and then washing with water, and drying in a vacuum oven at 110°C for 10 hours. Replace the gas in the reactor with high-purity argon, and finally carry out the passivation treatment of the nickel-based alloy reactor according to the following passivation treatment scheme 3.

[0039] Passivation treatment scheme 3 is as follows:

[0040] The first stage: Heating the nickel-based alloy reactor to 150°C, during which the flow rate of 0.1L / min is 0.1L / min. 2 / Ar mixture;

[0041] The second stage: Heating the nickel-based alloy reactor from 150°C to 500°C, during the period, according to the flow rate of 0.3L / min, F with a fluorine gas fraction of 5% 2 / Ar mixture;

[0042]The third stage: Keep the nickel-based alloy reactor at a constant temperature of 500°C for 5 hours, during which the flow rate is 0.2L / min and F with a fluorine gas fraction of 5% is introduced. 2 / Ar mixture;

[...

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PUM

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Abstract

The invention discloses a surface passivation treatment method of a nickel base alloy. The surface passivation treatment method of the nickel base alloy includes the following steps that after the nickel base alloy is pretreated and dried, a mixture of fluorine and argon is used for conducting surface passivation treatment; and the surface passivation treatment is divided into four phases. By adoption of the surface passivation treatment method of the nickel base alloy, a golden passivation layer is obtained from the surface of the nickel base alloy; the passivation layer has strong adhesion force, is homogeneous and compact, and can tolerate strong corrosive gas such as fluorine and hydrogen fluoride at a temperature from a room temperature to 600 degrees centigrade, and accordingly the corrosion resistance of nickel base alloy materials is improved, and the service life of the nickel base alloy materials are prolonged.

Description

technical field [0001] The invention relates to a metal surface treatment method, in particular to a nickel-based alloy surface passivation treatment method. Background technique [0002] Nickel-based alloy is a high-temperature alloy with nickel as the matrix (generally greater than 50%), and has high strength and good oxidation resistance and gas corrosion resistance in the range of 650-1000 ° C. Common nickel-based alloys include Monel Alloy, Inconel, Hastelloy, etc. Nickel-based alloys are often used in the manufacture of high-temperature components in aviation, nuclear reactors, and energy conversion equipment due to their excellent corrosion resistance. However, in some special industries, such as nuclear reactors and spent fuel reprocessing, when strong fluorinating agents (such as F 2 , HF), there will still be a certain corrosion of the nickel-based alloy, resulting in a decrease in the mechanical strength of the alloy and other issues. [0003] Nickel-based allo...

Claims

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Application Information

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Patent Type & Authority Patents(China)
IPC IPC(8): C23C8/08
CPCC23C8/08
Inventor 牛永生孙理鑫胡聪伟窦强李晴暖
Owner SHANGHAI INST OF APPLIED PHYSICS - CHINESE ACAD OF SCI