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A self-driven phenylboronic acid hydrogel driver and its preparation method

A technology of hydrogel driver and phenylboronic acid, which is applied in the field of self-driven phenylboronic acid hydrogel driver and its preparation, can solve the problems of difficult removal, complicated process, pollution and toxicity, etc., and achieve the goal of avoiding pollution and toxic organic solvents Use, increase the content of phenylboronic acid, the effect of high strength

Active Publication Date: 2021-03-30
SOUTH CHINA UNIV OF TECH
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

However, due to the low solubility of 3-acrylamidophenylboronic acid in water, to obtain a hydrogel with a higher content of phenylboronic acid, the organic gel is generally first synthesized in an organic solvent, and then the organic gel is soaked in water for further processing. Replacement to obtain hydrogel (such as: Macromol. Rapid Commun. 2013, 34, 63), this process is more complicated, and the organic solvent introduced is usually polluting or toxic, and it is difficult to remove completely, so the application of hydrogel will greatly increase restricted

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0015] Disperse 0.077 g of artificial hectorite in 7.765 mL of water at room temperature, then add 1.37 mL of acrylic acid and 2 μL N , N' -Aqueous solution of methylenebisacrylamide (20 mg / mL), mix uniformly to obtain solution 1, dissolve 0.573 g 3-acrylamidophenylboronic acid in 0.525 mL 2-hydroxyethyl methacrylic acid and mix uniformly to obtain solution 2, Add solution 2 to solution 1, stir rapidly to obtain uniform solution 3, pass argon gas into solution 3 to remove oxygen, then add 0.34 mL potassium persulfate aqueous solution (20 mg / mL), stir evenly to obtain reaction solution, the reaction solution was added to the mold and sealed, and placed at 60 ° C for 3 hours to obtain a phenylboronic acid hydrogel with a tensile breaking strength of about 100 kPa; the prepared phenylboronic acid hydrogel was twisted into a spiral shape and fixed In 0.1 mol / L sodium hydroxide solution for 1 minute, the hydrogel was set, and the phenylboronic acid hydrogel actuator was obtained; ...

Embodiment 2

[0017] Disperse 0.115 g of artificial hectorite in 7.765 mL of water at room temperature, then add 1.37 mL of acrylic acid and 2 μL N , N '-Methylenebisacrylamide aqueous solution (20 mg / mL), mix well to get solution 1, dissolve 0.573 g 3-acrylamidophenylboronic acid in 0.525 mL 2-hydroxyethyl methacrylic acid and mix evenly to get solution 2 , add solution 2 to solution 1, stir quickly to obtain uniform solution 3, pass nitrogen gas into solution 3 to remove oxygen, then add 0.34 mL potassium persulfate aqueous solution (20 mg / mL), stir well, and finally Add the reaction solution into the mold and seal it, and place it at 60 °C for 10 hours to obtain a phenylboronic acid hydrogel with a tensile breaking strength of about 110 kPa; twist the prepared phenylboronic acid hydrogel into a "Z" shape After being fixed in 0.2 mol / L sodium hydroxide solution for 5 minutes, the hydrogel was set to form a phenylboronic acid hydrogel actuator; the actuator was soaked in 0.5 mol / L hydroch...

Embodiment 3

[0019] Disperse 0.154 g of artificial hectorite in 7.765 mL of water at room temperature, then add 1.37 mL of acrylic acid and 2 μL N , N'-Methylenebisacrylamide aqueous solution (20 mg / mL), mix well to get solution 1, dissolve 0.573 g 3-acrylamidophenylboronic acid in 0.525 mL 2-hydroxyethyl methacrylic acid and mix evenly to get solution 2 , add solution 2 to solution 1, stir quickly to obtain uniform solution 3, pass nitrogen gas into solution 3 to remove oxygen, then add 0.34 mL potassium persulfate aqueous solution (20 mg / mL), stir well, and finally Add the reaction solution into the mold and seal it, and place it at 50 °C for 24 hours to obtain a phenylboronic acid hydrogel with a tensile breaking strength of about 120 kPa; twist the prepared phenylboronic acid hydrogel into an "M" shape After being fixed in 1 mol / L sodium hydroxide solution for 10 minutes, the hydrogel was set to form a phenylboronic acid hydrogel actuator; the actuator was soaked in 0.1 mol / L hydrochl...

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Abstract

The invention discloses a self-driven phenylboronic acid hydrogel driver and a preparation method thereof. The phenylboronic acid hydrogel is obtained by a 3-acrylamidophenylboronic acid monomer, an acrylic monomer, 2-hydroxyethyl methacrylate monomer and a chemical crosslinking agent N, N'-methylenediacrylamide, and an inorganic cross-linking agent artificial hectorite through free radical copolymerization; the hydrogel is fixed to a temporary shape in an alkaline solution by an external force to obtain the hydrogel driver, and the hydrogel driver can realize a driving function of spontaneousshape change in the solution by changing the pH of the solution. The method can synthesize phenylboronic acid hydrogel by a one-step method in aqueous solution without synthesizing in the organic solvent, the disadvantages of using the organic solvent in the synthesis process of the phenylboronic acid hydrogel can be overcome, and at the same time, the weakness of the low solubility of the 3-acrylamidophenylboronic acid monomer in water is eliminated. The method also increases the phenylboronic acid content while avoiding the usage of the organic solvent having pollution and toxicity performance.

Description

technical field [0001] The invention relates to the field of intelligent driver materials for functional hydrogels, in particular to a self-driving phenylboronic acid hydrogel driver and a preparation method thereof. Background technique [0002] Because hydrogel contains a large amount of water and has the characteristics of soft matter given by its perfect three-dimensional network structure, it has the advantages of weak stimulation-strong response, less addition-big effect, mild driving conditions, etc.; and soft matter drives especially hydrogels. The development of glue actuators in the field of smart devices has received increasing attention. In the study of gel actuators, shape memory gel actuators can return to the original shape from a temporary shape, which is a widely studied hydrogel actuator. However, each drive cycle of the currently reported shape memory hydrogel actuators requires an external force to fix the gel into a temporary shape (Chem. Sci., 2016, 7,...

Claims

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Application Information

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Patent Type & Authority Patents(China)
IPC IPC(8): C08F220/06C08F222/38C08F230/06C08F220/20C08K3/011
CPCC08F220/06C08K3/011C08F222/385C08F230/06C08F220/20
Inventor 王涛廖杰新杨述瑞张袁铖孙尉翔童真
Owner SOUTH CHINA UNIV OF TECH