Ether oxygen bond-free type polymer anion-exchange membrane and preparation method thereof
An anion exchange membrane and polymer technology, applied in the field of ion exchange membrane without ether oxygen bond and its preparation, can solve the problem of inability to take into account the ion conductivity and stability of basic ion exchange membrane, achieve a wide range of solvent selection, Good solubility and fewer reaction steps
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Embodiment 1
[0040] Synthesis of polymers without ether oxygen bonds: under ice-water bath conditions, 1.0694g (4mmol) α,α-diphenyl-4-piperidinemethanol, 0.8240g (5.6mmol) indole-2,3-di Ketone, 7.43mL (84mmol) of trifluoromethanesulfonic acid were added to the three-necked flask of 50mL, and then 7.2mL of dichloromethane was added to make a mixed solution. After mechanical stirring for 30min, the temperature was gradually raised to room temperature, and kept at room temperature to react 4- 8 days. After the reaction, the product was crushed with tweezers and placed in ice water under mechanical stirring to obtain a white blocky polymer. The product was repeatedly washed and soaked with deionized water, and then dried to obtain a polymer, which was ready for use.
[0041] Preparation of functionalized ether-oxygen bond-free polymer anion exchange membrane: under nitrogen protection, weigh 0.15g of ether-oxygen bond-free aryl polymer into a 10mL three-necked flask, dissolve with 6mL DMSO, an...
Embodiment 2
[0046]Synthesis of polymer containing secondary amine group without ether oxygen bond: under ice-water bath conditions, 1.0694g (4mmol) α,α-diphenyl-4-piperidinemethanol, 0.8240g (5.6mmol) indole-2, 3-Dione and 7.43mL (84mmol) of trifluoromethanesulfonic acid were added to a 50mL three-necked flask, and then 7.2mL of dichloromethane was added to form a mixed solution. After mechanical stirring for 30min, the temperature was gradually raised to room temperature and kept at room temperature. React 4-8 days. After the reaction, the product was crushed with tweezers and placed in ice water under mechanical stirring to obtain a white blocky polymer. The product was repeatedly washed and soaked with deionized water, and then dried to obtain a polymer, which was ready for use.
[0047] Synthesis of 1-(6-bromohexyl)-1-methyl-4-piperidine bromide ionic liquid: Dissolve 5mL of 1,6-dibromohexane in 20mL of ethyl acetate with a 50mL single-necked flask, add 2.82 g N-methylpiperidine, rea...
Embodiment 3
[0053] Synthesis of polymer containing secondary amine group without ether oxygen bond: same as Example 2
[0054] Synthesis of 1-bromohexyl-1-methylpyrrolidine bromide ionic liquid: Dissolve 5mL of 1,6-dibromohexane in 15mL of ethyl acetate with a 50mL single-necked flask, add 1.754g of N-methylpyrrolidine , and reacted at 60 °C for 24 h to obtain the precipitated product in the form of milky white powder. The product was repeatedly washed with ethyl acetate for 3 to 5 times, and dried under vacuum at 60 °C for 12 h to obtain a milky white powdery ionic liquid.
[0055] Preparation of polyhexane branched-chain pyrrolidine functionalized ether-oxygen bond-free polymer anion exchange membrane: under nitrogen protection, weigh 0.15g of amine group-substituted ether-oxygen bond-free polymer into a 25mL three-neck flask, dissolve with 6mL DMSO, and wait for After the polymer is fully dissolved, add 0.2081g K 2 CO 3 and 6 mL, 0.3096 g of a DMSO solution of 1-bromohexyl-1-methylp...
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