A class of gel emulsions stabilized by rosin-based amine oxide surfactants
A gel emulsion and amine oxide-based technology, applied in organic chemistry, chemical instruments and methods, chemical/physical processes, etc., can solve problems such as restricting the practical application of gel emulsion, achieve good emulsion stability, widen application scope, The effect of wide application prospects
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Embodiment 1
[0039] Example 1: Synthesis of 6-dehydroabietyl amido-N,N-dimethyl-hexyl amine oxide
[0040] The synthetic route of 6-dehydroabietyl amido-N,N-dimethyl-hexyl amine oxide is as follows:
[0041]
[0042] Add the dehydroabietic acid solid (30g, 0.1mol) into the there-necked flask equipped with tail gas absorption device and reflux condenser, add a small amount of 4-dimethylaminopyridine (DMAP) as catalyst, when the temperature rises to 50°C, start Thionyl chloride (17.94 g, 0.15 mol) was slowly added dropwise. During this process, a large amount of acid gas is generated, which is absorbed by the tail gas absorption device. After the dropwise addition, set the temperature to 72°C and continue the reaction for 3h. After the reaction was completed, excess thionyl chloride was removed by rotary evaporation under reduced pressure to obtain the crude compound 1.
[0043] Add 1,6-hexanediamine (58.1 g, 0.5 mol) and dichloromethane into a three-necked flask. Under full stirring,...
Embodiment 2
[0048] Embodiment 2: 6-dehydroabietyl amido-N, N-dimethyl-hexyl amine oxide gel property determination
[0049] Take 1 mL of deionized water, add 6-dehydroabietamido-N,N-dimethyl-hexylamine oxide (concentration is 4 mmol L -1 , 10mmol·L -1 , 15mmol·L -1 , 20mmol·L -1 , 25mmol·L -1 ), the solution was heated to 40°C to completely dissolve 6-dehydroabietamido-N,N-dimethyl-hexylamine oxide, and then stood at room temperature to observe the state of the solution.
[0050] From image 3 Appearance photographs of gels formed from 6-dehydroabietylamino-N,N-dimethyl-hexylamine oxide in medium (concentrations from left to right are 4mmol·L -1 , 10mmol·L -1 , 15mmol·L -1 , 20mmol·L -1 , 25mmol·L -1 ) It can be seen that when the concentration of 6-dehydroabietamido-N,N-dimethyl-hexylamine oxide is greater than 4mmol·L -1 It can support its own gravity when it is upside down, and has the characteristics of being inverted and not flowing, and the formed gel has good viscoelastic...
Embodiment 3
[0053] Determination of Surface Tension. A series of surfactant aqueous solutions with different concentrations were prepared, and the surface tension was measured by the suspension ring method at 25°C, and the relationship curve between the concentration of the sample aqueous solution and the surface tension was drawn.
[0054] From Figure 4 The surface tension γ of 6-dehydroabietyl amido-N, N-dimethyl-hexyl amine oxide in the medium varies with the concentration C. It can be seen that the surfactant 6-dehydroabietyl amido-N, N-dimethyl The critical micelle concentration of yl-hexylamine oxide is 0.56mmol·L -1 , gamma cmc 35mN·m -1 . It shows that 6-dehydroabietamido-N,N-dimethyl-hexyl amine oxide has good surface activity and can be used to stabilize the emulsion.
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