Polyisocyanate curing agent for laminated adhensive and laminated adhensive using the same
A polyisocyanate and isocyanate-based technology, applied in the field of lamination adhesives and polyisocyanate curing agents for lamination adhesives, can solve the problems of difficult to obtain laminated films and the like
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Embodiment 1
[0091] In a reaction device with a capacity of 2 liters of a stirrer, a thermometer, an Arin cooling pipe, and a nitrogen inlet pipe, 1 gram of colonate (registered trademark) HX601 made by Nippon Polyurethane Industry Co., Ltd. and 399 grams of monohydric alcohol (1) were added at 70 °C for 3 hours. Then add coupling agent (1) 1 gram therein, prepare polyisocyanate curing agent A.
[0092] The polyisocyanate curing agent A had a viscosity of 2720 mPa·s at 25° C. and an isocyanate group content of 11.1%. The polyisocyanate curing agent A was stored in a dark place at 25°C for one month, and the stability over time was observed, but no special change in appearance was confirmed.
Embodiment 2-6、 comparative example 1、2
[0094] Using the raw materials in Table 1, the same reaction as in Example 1 was used to prepare polyisocyanate curing agents B-H. The obtained polyisocyanate curing agent was stored in a dark place at 25° C. for one month, and its stability over time was visually judged.
[0095] The results are summarized in Table 1.
[0096] Example
[0097] Note 1) In the measurement of the adhesive strength of the PET film / aluminum foil of Examples 7-12 and Comparative Examples 3 and 4, the PET film was broken.
Embodiment 1-6
[0098] In embodiment 1-6, comparative example 1,2 and table 1
[0099] colonateHX: Isocyanate-modified polyisocyanate derived from hexamethylene diisocyanate
[0100] Isocyanate group content = 21.3%
[0101] Viscosity = 1500mPa·s / 25°C
[0102] Monohydric alcohol (1): The number average molecular weight of the monohydric alcohol obtained by adding oxypropylene to methoxypolyethylene glycol with a number average molecular weight of 400 = 1100
[0103] Monohydric alcohol (2): the number average molecular weight of the monohydric alcohol obtained by adding oxypropylene to methoxypolyethylene glycol with a number average molecular weight of 400 = 1400
[0104] Monohydric alcohol (3): the number average molecular weight of the monohydric alcohol obtained by adding oxypropylene to methoxypolyethylene glycol with a number average molecular weight of 700 = 1700
[0105] Monohydric alcohol (4): methoxypolyethylene glycol number average molecular weight = 400
[0106] Monohydric alc...
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