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Loaded type silver phosphate/polyphosphoric silver/silver chloride compound water treatment photo-catalyst and preparation method thereof

A technology of silver polyphosphate and photocatalyst, which is applied in the direction of physical/chemical process catalyst, light water/sewage treatment, energy wastewater treatment, etc. The effect of accelerating the decomposition

Active Publication Date: 2014-11-05
无锡米尔环保科技有限公司
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

However, due to the instability of silver phosphate itself, it is easy to self-erode in photocatalysis.

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0017] Weigh 1 mol of NaCl, grind it to a particle size of 100 μm, and add it into 3 L of H with a concentration of 1 mol / L under vigorous stirring (350 rpm). 3 PO 4 In the solution, keep stirring (200 rpm) for 30min; add dropwise AgNO with a concentration of 1mol / L to the above solution 3 A total of 2L, continue to stir during the dropwise addition, stir for another 60min after the dropwise addition, precipitate and age for 24h; wash the obtained precipitate with deionized water 4 times, and dry to obtain the loaded silver phosphate / silver polyphosphate / chlorine Silver compound water treatment photocatalyst.

[0018] Add 0.1 g of the obtained silver phosphate / silver polyphosphate / silver chloride photocatalyst into 500 mL of Orange II wastewater with a concentration of 30 mg / L, react for 20 min under the irradiation of a 500 w metal halide lamp, and the decolorization rate is 98.8%, repeat After 6 times of utilization, the decolorization rate of Orange II is 90.5%.

Embodiment 2

[0020] Weigh 2 mol of NaCl, grind it to a particle size of 300 μm, and add it into 4 L of H with a concentration of 2 mol / L under vigorous stirring (350 rpm). 3 PO 4 In the solution, keep stirring (200 rpm) for 40min; add dropwise AgNO with a concentration of 2mol / L to the above solution 3 A total of 4L, continue to stir during the dropwise addition, stir for another 70min after the dropwise addition is completed, precipitate and age for 24h; wash the obtained precipitate with deionized water 5 times, and dry to obtain the loaded silver phosphate / silver polyphosphate / chlorine Silver compound water treatment photocatalyst.

[0021] 0.1 g of the obtained silver phosphate / silver polyphosphate / silver chloride photocatalyst was added to 500 mL of methyl orange wastewater with a concentration of 20 mg / L, and reacted for 20 min under the irradiation of a 500 w metal halide lamp, and the decolorization rate was 97.6%. After repeated use for 6 times, the decolorization rate of methyl...

Embodiment 3

[0023] Weigh 2 mol of NaCl, grind it to a particle size of 300 μm, and add it into 3 L of H with a concentration of 2 mol / L under vigorous stirring (350 rpm). 3 PO 4 In the solution, keep stirring (200 rpm) for 40min; add dropwise AgNO with a concentration of 2mol / L to the above solution 3 A total of 3L, continue to stir during the dropwise addition, stir for another 70min after the dropwise addition, precipitate and age for 24h; wash the obtained precipitate with deionized water for 5 times, and dry to obtain the loaded silver phosphate / silver polyphosphate / chlorine Silver compound water treatment photocatalyst.

[0024] Add 0.1 g of the obtained silver phosphate / silver polyphosphate / silver chloride photocatalyst into 500 mL of acidic scarlet wastewater with a concentration of 20 mg / L, and react for 20 minutes under the irradiation of a 500 w metal halide lamp, and the decolorization rate is 99.8%. After being used for 6 times, the decolorization rate to acid scarlet is 91....

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Abstract

The invention discloses a loaded type silver phosphate / polyphosphoric silver / silver chloride compound water treatment photo-catalyst and a preparation method thereof. The preparation method comprises the following steps of: 1) weighting NaCl, grinding and then adding H3PO4 solution while severely stirring, and continuously stirring; 2) dropwise adding AgNO3 solution into the solution prepared in the step 1, continuously stirring while dropwise adding, stirring again after finishing dropwise adding, and then depositing and ageing; and 3) washing the obtained precipitate with deionized water, and drying, thereby obtaining the loaded type silver phosphate / polyphosphoric silver / silver chloride photo-catalyst. According to the preparation method provided by the invention, the strong complexing action of polyphosphates on metal is utilized to efficiently avoid the self-etching of silver phosphate; the visible photo-catalytic characteristic of the catalyst is efficiently utilized to prolong the service life of the catalyst and accelerate the decomposition on organic matters; and the silver phosphate, the silver chloride and the polyphosphoric silver are compounded together, thereby being beneficial to the synergistic effect and promoting the photo-degrading efficiency.

Description

technical field [0001] The invention relates to a loaded silver phosphate / silver polyphosphate / silver chloride water treatment photocatalyst and a preparation method thereof, belonging to the technical field of sewage treatment in environmental protection. Background technique [0002] Traditional water treatment methods have problems such as low efficiency, high cost, and secondary pollution, and sewage treatment has not been well resolved. The development and application of nanotechnology is likely to completely solve this problem. In 1972, A.Fujishima and K.Honda worked on n-type semiconductor TiO 2 Photocatalytic decomposition of water found on electrode, TiO 2 It has high oxidation activity, good chemical stability, non-toxicity to human body, low cost, no pollution, and wide application range, so it has received the most attention. It is currently the most widely used nano-photocatalytic material, and it is also a green and environmentally friendly catalyst with deve...

Claims

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Application Information

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Patent Type & Authority Patents(China)
IPC IPC(8): B01J27/18C02F1/30
CPCY02W10/37
Inventor 赵锦星马建锋
Owner 无锡米尔环保科技有限公司