Amphiphilic base conjugate nanoparticles for treating tumors and preparation method thereof
A nanoparticle and amphiphilic technology, applied in the field of biomedicine, can solve the problems of changing drug properties, affecting drug efficacy, increasing drug cost, etc., and achieving the effects of reducing toxic side effects, avoiding toxic side effects, and avoiding changes in the chemical structure of drugs
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Embodiment 1
[0035] Add raltitrexed (15 mg) and clofarabine (10 mg) into the sample bottle, then add 5 ml of dimethyl sulfoxide, and stir at room temperature for 12 hours to obtain the amphiphilic base conjugate. figure 1 is the chemical structural formula of the amphiphilic base conjugate (ratitrexed / clofarabine), and the amphiphilic base conjugate is formed by molecular recognition between raltitrexed and clofarabine . figure 2 One-dimensional NMR of the amphiphilic base conjugate (raltitrexed / clofarabine) 1 H NMR spectrum, test solvent is d 6 -DMSO. figure 2The assignment of the proton peaks in is as follows: δ(ppm from TMS), 8.14(1H, NCHCC), 7.84(1H, CONHCH), 7.59-7.61(2H, CCONHCNC, CCHCHCCCH), 7.36-7.40(3H, CCHCHCCCH, SCCHCHC) ,6.23(2H,NH 2 ), 5.91 (1H, SCCCHHC), 5.20 (1H, OCHCHCHCH), 5.11 (1H, OCHCHCHCH), 4.51 (2H, CCH 2 N), 4.33-4.36 (2H, OCHCHCHCH), 4.12, (1H, COHNCH), 4.0 (1H, CHCHOHCH), 3.74-3.81 (3H, CHCH 2 OH),2.98(3H,NCH 3 ),2.13(3H,CCH 3 ),1.84-1.98(4H,CHCH 2 CH 2...
Embodiment 2
[0038] Add doxifluridine (10 mg) and clofarabine (12 mg) into a sample bottle, then add 5 ml of dimethyl sulfoxide, stir at 40°C for 24 hours, and cool to room temperature to obtain the amphiphilic base base conjugates.
[0039] The chemical structural formula of the amphiphilic base conjugate synthesized in this embodiment is as follows Figure 4 shown. Doxifluridine and clofarabine form this amphiphilic base conjugate through molecular recognition between the bases.
[0040] The above-mentioned amphiphilic base conjugate (doxifluridine / clofarabine) was dissolved in dimethyl sulfoxide, dropped into water at room temperature, and then the dimethyl sulfoxide was removed to obtain two Aqueous solutions of nanoparticles of hydrophilic base conjugates. The transmission electron micrographs of the nanoparticles based on the amphiphilic base conjugate of doxifluridine and clofarabine prepared in this example are as follows: Figure 5 As shown, the average size of the nanoparticl...
Embodiment 3
[0042] Add bisfural fluorouracil (8 mg) and clofarabine (12 mg) into the sample bottle, then add 4 ml of dimethyl sulfoxide, stir at 60°C for 18 hours, cool to room temperature to obtain the amphiphilic base conjugate compound.
[0043] The chemical structural formula of the amphiphilic base conjugate synthesized in this embodiment is as follows Image 6 shown. The amphiphilic base conjugate is formed by the molecular recognition between bisfural fluorouracil and clofarabine.
[0044] Dissolve the prepared amphiphilic base conjugate (bisfururacil / clofarabine) in dimethyl sulfoxide, drop it into water at room temperature, and then remove the dimethyl sulfoxide to obtain amphiphilic Aqueous solutions of nanoparticles of sex base conjugates. The average size of the nanoparticles prepared in this example based on the amphiphilic base conjugate of bisfururacil / clofarabine is about 110 nanometers.
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