Propofol analogs, process for their preparation, and methods of use
a technology of propofol and analogs, applied in the field of substituted dialkylphenol propofol compounds, can solve the problems of pain upon injection, reduced blood pressure, and relative high incidence of apnea
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example 1
[0061] This example illustrates the preparation of (4-fluorophenyl)-(4-hydroxy-3,5-diisopropyl phenyl)methanone (CT7). To a solution of 2,6-diisopropylphenol (3.3 g, 18.5 mmol) in 98 mL of toluene were added dropwise 4-fluorobenzoyl chloride (4 mL, 37 mmol) and aluminum chloride (4.9 g, 37 mmol), while the temperature was maintained at room temperature. Stirring was continued for 7 hours and then the solvent was poured into ice-water. The mixture was extracted with ethyl acetate and hexane (1:9). The combined organic layers were washed with water and brine, dried (Na2SO4) and concentrated. The residue was purified by flash silica gel chromatography to generate the desired product as a yellowish solid. Yield 40%. 1H NMR (500 MHz, CDCl3) δ 1.28 (d, J=6.8 Hz, 12H), 3.18 (hept, J=6.8 Hz, 2H), 5.34 (br s. 1H), 7.55 (s, 2H), 7.16 (d, d, J=8.6 Hz, 1H), 7.15 (d, J=8.6 Hz, 1H), 7.79 (d, J=8.6 Hz, 1H), 7.81 (d, J=8.6 Hz, 1H); Anal. Calcd for (C19H21FO2+H)+ and (C19H21FO2+H)+: 301 and 323. Fou...
example 2
[0062] This example illustrates the preparation of (4-(trifluoromethyl)phenyl)-(4-hydroxy-3,5-diisopropylphenyl)methanone (CT8). The title compound was prepared essentially as described in Example 1. 1H NMR (500 MHz, CDCl3) δ 1.27 (d, J=6.6 Hz, 12H), 3.18 (hept, J=6.6 Hz, 2H), 5.40 (br s. 1H), 7.58 (s, 2H), 7.74 (d, J=8.0 Hz, 2H), 7.85 (d, J=8.0 Hz, 2H); Anal. Calcd for (C20H21F3O2+H)+ and (C20H21F3O2+Na)+: 351 and 373. Found: 351 and 373.
example 3
[0063] This example illustrates the preparation of (4-hydroxy-3,5-diisopropylphenyl)-(4-nitrophenyl)methanone (CY61). The title compound was prepared essentially as described in Example 1. 1H NMR (500 MHz, CDCl3) δ 1.27 (d, J=6.9 Hz, 12H), 3.20 (hept, J=6.9 Hz, 2H), 5.73 (br s. 1H), 7.57 (s, 2H), 7.89 (d, J=8.8 Hz, 2H), 8.33 (d, J=8.8 Hz, 2H); Anal. Calcd for (C19H21NO4+H)+ and (C19H21NO4+Na)+: 328 and 350. Found: 328 and 350.
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