Polymer
A technology of polymers and copolymers, applied in the field of high-density polyethylene polymers
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Embodiment 1
[0110] The preparation of embodiment 1HDPE
[0111] In a volume of 500dm 3 Continuously introduce isobutane, ethylene and hydrogen into the loop reactor. Furthermore, a polymerization catalyst additionally prepared according to Example 3 in WO 95 / 35323 was introduced into the reactor together with triethylaluminum so that the molar ratio of aluminum in the activator to titanium in the solid component was 15. The loop reactor was operated at 96°C and 60 bar. In this slurry reactor, the content of ethylene in the liquid phase is 8.5 mol%, and the ratio of hydrogen to ethylene is 0.210 kg H 2 / t C2. The polymer produced in this loop reactor has an MFR of 0.9 g / 10 min 2 , MFR of 27g / 10min 21 and 958kg / m 3 Density. The feed rates of ethylene and catalyst were adjusted to give a polymer output rate of 30 kg / h.
[0112] The polymer powder was recovered and mixed with 1500 ppm of Irganox B215 and 3500 ppm of calcium stearate. The mixture was extruded and pelletized in a ZSK70...
Embodiment 2
[0113] The preparation of embodiment 2 film
[0114] Films of 30 μm were produced on a 3-layer coextrusion blown film line from Windmoller & Holscher (for all WVTR determinations above and below, tear resistance and other mechanical properties) with a 200 mm die. The die gap was 1.2mm. All three layers contain the same pure HDPE material.
[0115] The blow up ratio (BUR) was 3:1.
[0116] Cold line height (FLH): 70cm above the die head.
[0117] The temperature curve is a flat straight line at 200°C.
[0118] The output rate is 120kg / h.
[0119] Internal Bubble Cooling (IBC) is used.
Embodiment 3
[0121] The polymers and films of Examples 1 and 2 were compared to HDPE grades produced with commercially available catalysts as well as commercially available Ziegler-Natta HDPE grades. The results are shown in Table 1 below.
[0122] Table 1
[0123]
[0124]
[0125] It is evident that the polymers of the examples have higher crystallinity (density) and thus the higher WVTR of their films (example 2). At the same time, the HDPE has an improved strain at break. Oxygen permeability is also lower than products on the commercial market.
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Abstract
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