Synthesis and application of benzotriazole derivatives as rsk2 inhibitors
A kind of technology of use and compound, applied in the field of synthesis of benzotriazole derivatives
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[0074] synthetic part
[0075] Synthesis of N-((1H-benzo[d][1,2,3]triazole)-1-methyl)aniline (I-1)
[0076]
[0077] Weigh benzotriazole (5mmol, 596mg), aniline (5mmol, 466mg), 40% formaldehyde (5mmol, 375mg) into a 100mL round bottom bottle, add 60mL methanol, stir at room temperature for 2 hours, there are a lot of white solids Precipitate, filter with suction, wash the filter cake with cold methanol, and dry to obtain the target compound. White solid, mass: 1.009 g (yield: 90%). 1 HNMR (400MHz, DMSO-d 6 ): δ8.06(d, J=8.4Hz1H), δ8.01(d, J=8.4Hz1H), δ7.54(t, J=7.6Hz1H), δ7.38(t, J=7.6Hz1H), δ7.27(t, J=7.2Hz1H), δ7.07(t, J=7.6Hz2H), δ6.82(d, J=8Hz2H), δ6.595(t, J=7.2Hz1H), δ6.12 (d, J=7.2Hz2H).
[0078] Synthesis of N-((1H-benzo[d][1,2,3]triazole)-1-methyl)-4-nitroaniline (I-2)
[0079]
[0080] Weigh benzotriazole (5mmol, 596mg), p-nitroaniline (5mmol, 691mg), and 40% formaldehyde (5mmol, 375mg) into a 100mL round bottom bottle, add 60mL of methanol, stir at room ...
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