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Novel treatment method for pentachlorophenol-containing wastewater

A treatment method, pentachlorophenol technology, applied in the direction of light water/sewage treatment, oxidized water/sewage treatment, mechanical oscillation water/sewage treatment, etc., can solve the problem of no PCP wastewater being retrieved, and achieve the promotion of photo-Fenton reaction Efficiency, wide range of sources, and simple process

Active Publication Date: 2014-09-03
SOUTH CHINA INST OF ENVIRONMENTAL SCI MEP
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

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Problems solved by technology

At present, the domestic patent search has not retrieved the research on the treatment of PCP wastewater by the light-assisted Fenton-like method

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0035] Under ultrasonic radiation conditions (ultrasonic power 200W, frequency 40kHz), 0.4g s-Fe 0 Particles (particle size: 3-5 mm), 10 μL H 2 o 2 Solution (30wt% aqueous solution) and RhB solution were added to the PCP solution (the final PCP concentration was 10ppm, the volume was 50mL, and the solution temperature was 30°C; at this time, the concentration of RhB was also 10ppm). Philae xenon lamp light source PLS-SXE300, the filter cut-off wavelength is λ>420nm) reaction, no RhB solution reaction system was used as the reaction control system, the sample was centrifuged and the concentration of RhB and PCP in the solution was monitored by HPLC. Sponge iron is magnetically separated and activated with 2% (v / v) dilute hydrochloric acid ultrasonic (200W, 1min) for recycling.

[0036] The experimental results showed that without adding RhB, the degradation rate of PCP in the wastewater solution was 12.63% after 60 minutes of reaction. In the case of adding RhB, the degradat...

Embodiment 2

[0038] Under ultrasonic radiation conditions (ultrasonic power 200W, frequency 40kHz), 0.4g s-Fe 0 Particles (particle size: 3-5 mm), 10 μL H 2 o 2 The solution (30wt% aqueous solution) was added to the PCP solution (50mL, 10ppm, the solution temperature was 30°C), and then RhB and crystal violet (CV) were added to the PCP solution (the final concentrations of RhB and CV were both 10ppm), The reaction was carried out under the condition of visible light radiation (Beijing Porphyra xenon lamp light source PLS-SXE300, the cut-off wavelength of the filter is λ>420nm). After the reaction, samples were centrifuged and HPLC was used to analyze the concentration of PCP, RhB and CV remaining in the solution, the sponge iron was magnetically separated, activated with 2% (v / v) dilute hydrochloric acid ultrasonic (200W, 1min), and recycled.

[0039]The experimental results show that: in the system of adding CV dye, the degradation rate of PCP in the wastewater solution after 60 minutes...

Embodiment 3

[0041] Under ultrasonic radiation conditions (ultrasonic power 200W, frequency 40kHz), 10μL H 2 o 2 Solution (30wt% aqueous solution) and RhB solution were added to PCP solution (final PCP concentration was 10ppm, volume was 50mL, solution temperature was 30°C; RhB concentration was 10ppm), and sponge iron (0.4g) and ferrous iron were added respectively Salt (Fe 2+ The final concentration is 2.3ppm), reacted under the condition of visible light radiation (Beijing Bofeilai xenon lamp light source PLS-SXE300, the cut-off wavelength of the filter is λ>420nm), the sample was centrifuged and the concentration of RhB and PCP in the solution was monitored by HPLC. Sponge iron is magnetically separated and activated with 2% (v / v) dilute hydrochloric acid ultrasonic (200W, 1min) for recycling.

[0042] The experimental results showed that the degradation rates of PCP and RhB were 51.03% and 54.09% after 10 minutes of reaction in the reaction system with ferrous ions added; after that...

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Abstract

The invention belongs to the field of environment friendly engineering for wastewater treatment and discloses a novel treatment method for pentachlorophenol-containing wastewater. The method comprises the following steps of: adding sponge iron, hydrogen peroxide and rhodamine B into a pentachlorophenol-containing wastewater solution under the condition of ultrasonic radiation, and reacting under visible radiation; and carrying out magnetic separation to recycle the sponge iron. The rhodamine B is sufficiently used as a photosensitizer in the reaction, visible radiation is caught to form an excited state, and a novel degradation reaction is triggered. The degradation rate of pentachlorophenols in wastewater which is treated by using the method is up to over 94%.

Description

technical field [0001] The invention belongs to the field of waste water treatment environmental protection engineering, and in particular relates to a treatment method for waste water containing pentachlorophenols. Background technique [0002] Pentachlorophenol (PCP) is one of the most toxic and refractory chlorophenol compounds. It has relatively stable chemical properties and has carcinogenic, teratogenic and mutagenic effects, so it is listed as one of the priority pollutants. At present, pentachlorophenol environmental pollution remediation technologies mainly include biological methods, physical methods, chemical methods (including photochemical methods) and so on. Due to the high biological toxicity of PCP, it is difficult to effectively remove high-concentration PCP pollutants by traditional biological methods. Adsorption processes such as activated carbon have achieved the migration of PCP in different media, but have not effectively degraded and eliminated PCP po...

Claims

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Application Information

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Patent Type & Authority Patents(China)
IPC IPC(8): C02F1/72C02F1/30C02F1/36
Inventor 鞠勇明岳建华李照勇李国华庞志华骆其金陈婵杨艳艳王晓燕方建德
Owner SOUTH CHINA INST OF ENVIRONMENTAL SCI MEP