Trihydric alcohol hyperbranched monomer based on maleic anhydride and preparation method for trihydric alcohol hyperbranched monomer
A technology of hyperbranched monomer and maleic anhydride is applied in the preparation of carboxylate, chemical instruments and methods, preparation of organic compounds, etc., and can solve the problems of irritation, irritating odor of isocyanate, and large toxic and side effects, and achieves the The effect of good adhesion, few reaction steps and easy operation
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Embodiment 1
[0043] (1) Add 0.1mol (13.4g) trimethylolpropane and 0.3mol (29.4g) maleic anhydride into the reaction vessel, mix well, stir and heat up to 70°C, and add the catalyst p-toluenesulfonic acid (0.86g , 2wt% of the reaction system) and the polymerization inhibitor p-hydroxyanisole (0.21g, 5wt‰ of the reaction system), after the maleic anhydride melted, the temperature was raised to 80°C, and after stirring for 5h, the product was extracted with ethyl acetate , and then washed with water for 2 to 3 times, filtered, dried over anhydrous sodium sulfate, and evaporated under reduced pressure to remove the solvent to obtain the first generation product G0.5.
[0044] (2) Glycidyl methacrylate (GMA) of 0.3mol (42.66g), catalyst tetrabutylammonium chloride (1.61g, 2wt% of reaction system) and polymerization inhibitor p-hydroxyanisole (0.41g , 5wt‰ of the reaction system) was added to the reaction vessel, the temperature was raised to 70°C, and 1 part of G0.5 (0.1mol, 47.05g) was dropped...
Embodiment 2
[0048] (1) Add 0.1mol (13.4g) trimethylolpropane and 0.3mol (29.4g) maleic anhydride into the reaction vessel, mix well, stir and heat up to 60°C, and add the catalyst p-toluenesulfonic acid (0.86g , 2wt% of the reaction system) and the polymerization inhibitor p-hydroxyanisole (0.21g, 5wt‰ of the reaction system), after the maleic anhydride melts, the temperature is raised to 80°C, and after stirring for 5h, it is cooled to room temperature and washed with acetic acid The product was extracted with ethyl ester, washed with water 2-3 times, filtered, dried over anhydrous sodium sulfate, and the solvent was distilled off under reduced pressure to obtain the intermediate product G0.5.
[0049] (2) Glycidyl methacrylate (GMA) of 0.31mol (44.08g), catalyst tetrabutylammonium chloride (1.82g, 2wt% of the reaction system) and inhibitor p-hydroxyanisole (0.46g , 5wt‰ of the reaction system) was added to the reaction vessel, the temperature was raised to 70°C, and 1 part of the reacti...
Embodiment 3
[0053] (1) Add 0.1mol (13.4g) trimethylolpropane and 0.3mol (29.4g) maleic anhydride into the reaction vessel, mix well, stir and heat up to 60°C, and add the catalyst p-toluenesulfonic acid (0.86g , 2wt% of the reaction system) and the polymerization inhibitor p-hydroxyanisole (0.21g, 5wt‰ of the reaction system), after the maleic anhydride melts, the temperature is raised to 80°C, and after stirring for 5h, it is cooled to room temperature and washed with acetic acid The product was extracted with ethyl ester, washed with water 2-3 times, filtered, dried over anhydrous sodium sulfate, and the solvent was distilled off under reduced pressure to obtain the intermediate product G0.5.
[0054] (2) Glycidyl methacrylate (GMA) of 0.32mol (45.51g), catalyst tetrabutylammonium chloride (1.85g, 2wt% of reaction system) and polymerization inhibitor p-hydroxyanisole (0.46g , 5wt‰ of the reaction system) was added to the reaction vessel, the temperature was raised to 70°C, and 1 part of...
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