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Metal carrier type hydrogen-eliminating catalyst and preparation process thereof

A hydrogen elimination catalyst and catalyst technology, applied in the direction of metal/metal oxide/metal hydroxide catalyst, catalyst activation/preparation, physical/chemical process catalyst, etc. advanced questions

Active Publication Date: 2008-02-27
718TH RES INST OF CHINA SHIPBUILDING INDAL CORP
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

Such catalysts have high hydrogen elimination efficiency, but there are also some disadvantages in non-metallic carrier catalysts.
The strength of the non-metallic carrier catalyst is not high, it is easy to break, and the heat dissipation effect is not good. The surface of the catalyst is easy to form a local high temperature, which makes the catalyst high-temperature sintering. At the same time, if the hydrogen concentration is high, it is easy to ignite the air mixture containing hydrogen.

Method used

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Examples

Experimental program
Comparison scheme
Effect test

example 1

[0024] Take 5 pieces of 30×30mm spray Al 2 o 3 The stainless steel mesh is fully washed with detergent, baked in an oven at 100°C for 4 hours, and placed in a desiccator for later use.

[0025] Measure the concentration of 0.1gPd / ml of H 2 PdCl 4 Solution 5ml, 0.1gPt / ml of H 2 PtCl 6 Pour 10ml of the solution into an incubator, add 0.12gCe / ml of Ce(NO 3 ) 3 After 3ml of the solution, the metal support was put in for impregnation, stirred properly, and dried at 120°C for 2 hours. Then bake at 450°C for 3h, and then use hydrogen (space velocity 1000h -1 ) at 450° C. for 5 hours, cooled naturally to room temperature, and the finished catalyst was taken out to be uniform dark gray.

[0026] In the catalyst activity evaluation process, 5 pieces of catalyst samples were loaded, and the space velocity was 20,000 hours at normal temperature and pressure. -1 1. Under the condition that the hydrogen concentration is 2%, the hydrogen elimination activity is evaluated, and the hy...

example 2

[0028] Take 5 pieces of 30×30mm` sprayed Al 2 o 3 The stainless steel mesh is fully washed with detergent, baked in an oven at 100°C for 4 hours, and placed in a desiccator for later use.

[0029] Measure the concentration of 0.1gPd / ml of H 2 PdCl 4 Solution 5ml, concentration of 0.1gPt / ml of H 2 PtCl 6 Solution 6ml and 0.15gAg / ml AgNO 3 Pour 4ml of the solution into an incubator, add 0.12gCe / ml of La(NO 3 ) 3After 3ml of the solution, the metal support was put into for impregnation, stirred properly, and dried at 100°C for 2 hours. Then bake at 600°C for 2h, and then use hydrogen (space velocity 1000h -1 ) was reduced at 400°C for 5 hours, cooled naturally to room temperature, and the finished catalyst was light gray when taken out.

[0030] In the catalyst activity evaluation process, 5 pieces of catalyst samples were loaded, and the space velocity was 20,000 hours at normal temperature and pressure. -1 1. Under the condition that the hydrogen concentration is 2%, ...

example 3

[0032] Take 5 pieces of 30×30mm stainless steel mesh, wash them thoroughly with detergent, bake them in an oven at 100°C for 4 hours, and put them in a desiccator for later use.

[0033] Measure the concentration of 0.12gPd / ml H 2 PdCl 4 Solution 3ml, concentration of 0.07gPt / ml of H 2 PtCl 6 Solution 2ml and 0.19gAg / ml AgNO 3 Solution 1ml, mix well and stir evenly, then add a small amount of binder and 0.2gK 2 CO 3 , fully stirred evenly to make a coating solution.

[0034] Brush the coating solution onto the spare stainless steel mesh, place it in an oven to dry at 120°C for 15 minutes, then bake it at 580°C for 2 hours, and then use hydrogen (space velocity 1000 hours) -1 ) was reduced at 460°C for 5 hours, cooled naturally to room temperature, and the finished catalyst was dark gray when taken out.

[0035] In the catalyst activity evaluation process, 5 pieces of catalyst samples were loaded, and the space velocity was 20,000 hours at normal temperature and pressure...

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PUM

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Abstract

The invention relates to a catalyst which is use to eliminate hydrogen in nuclear power station, particularly in the closed space such as containing vessel in nuclear power station. The catalyst comprises a sheet metallic carrier, an active component of a plurality of noble metals, and an agent of Na, K, Cr element and rare-earth metal. The experiment expresses that the metallic carrier type catalyst has high dehydrogenation efficiency, long life time, and good moisture retardant property.

Description

(1) Technical field [0001] The invention relates to a catalyst for passive elimination of hydrogen in nuclear power plants, and is especially suitable for use in confined spaces such as containment shells of nuclear power plants. (two), background technology [0002] After a loss of water accident (LOCA) in a pressurized water reactor in a nuclear power plant, due to the loss of coolant and the failure of emergency backup coolant injection, the fuel temperature increased sharply, resulting in a high-temperature reaction between the residual steam in the main system and the zirconium in the fuel shell. Under severe accident conditions, the fuel casing may be completely oxidized, which is an exothermic reaction and produces large amounts of hydrogen gas. The hydrogen gas produced by this reaction enters the reactor containment environment from the main system damage along with the steam. In addition, the radiation decomposition of water and the reaction between core melt and ...

Claims

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Application Information

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Patent Type & Authority Patents(China)
IPC IPC(8): B01J23/54B01J37/02
Inventor 朱敏赵罗生赵新国王新喜金至嘉祝维燕陶好训沈耀雄
Owner 718TH RES INST OF CHINA SHIPBUILDING INDAL CORP