A method for preparing conductive microspheres suitable for conductive materials
A technology of conductive materials and microspheres, applied in the field of preparation of conductive metal-containing composite microspheres, can solve the problems of poor conductivity of gold layer, insignificant effect of surfactant, and unrepeatable dispersion effect.
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Embodiment 1
[0052] Step 1: Prepare 6.75μm matrix material microspheres, ie, polymer cores of composite microspheres
[0053] Take 13.1g 26.0% polystyrene seed suspension aqueous solution with a particle size of 2.1μm, 450g deionized water, 0.23g 10% sodium dodecylbenzene sulfonate aqueous solution into a 2000mL four-neck round bottom flask, pour nitrogen into it, and stir Then heat to 60°C. Take 18.8g divinylbenzene, 123.8g 1,6-hexanediol diacrylate, 7.5g allyl methacrylate, 10.7g 10% sodium dodecylbenzenesulfonate aqueous solution, 165g deionized water, and mix Stir with a homomixer and add to a four-neck round bottom flask. After stirring for 2 hours, the temperature was lowered to 40°C, and 0.2g of 30% hydrogen peroxide was added. Take 1.1g tert-butyl hydroperoxide, 0.3g 10% sodium dodecylbenzenesulfonate aqueous solution, 65g deionized water, mix with a homomixer, add it to a four-neck round bottom flask, and then add 56.3g 20% Polyvinylpyrrolidone aqueous solution, 25g deionized wate...
Embodiment 2
[0055] Step two, synthesize polymer microspheres with polymer exterior
[0056] Take 400.0 g of the microsphere suspension obtained in Example 1 with 15.4% removal of small particles, and 150 g of deionized water into a 2000 mL four-neck round bottom flask, pour in nitrogen, and stir and heat to 70°C. Take 0.08g of sodium formaldehyde sulfoxylate, 0.36g of 10% sodium dodecylbenzenesulfonate aqueous solution, mix 25.6g of deionized water into a homogeneous solution, and add 13.0g of the homogeneous solution into a round bottom flask. Take 0.11g tert-butyl hydroperoxide and mix it with 12.9g deionized water to form a homogeneous solution. Take 2.8g of methyl methacrylate, 11.5g of glycidyl methacrylate, and 0.03g of 1,6-hexanediol diacrylate and mix them into a uniform monomer solution. Add 1.0 g of the above two aqueous solutions every 15 minutes, for a total of 180 minutes. Add 1.3 g of the above monomer solution every 15 minutes, for a total of 150 minutes. After the aqueous ...
Embodiment 3
[0058] Step 3: Generate functional groups outside the polymer microspheres, namely the polymer microspheres obtained in functionalized embodiment 2
[0059] Take 100.0 g of the microsphere suspension obtained in Example 2, 200 mL of absolute ethanol, add it to a 500 mL round-bottomed flask, magnetically stir to disperse, and then take 50 mL of ethylenediamine and add it to the round-bottomed flask. Heat to 80°C for 12 hours. Cool the flask to 25° C., filter and separate to obtain functionalized microspheres, that is, form a functional part on the core, and the functional part is composed of high molecular polymer and has functional groups.
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