Oxime Derivatives and Their Applications in Agriculture
A technology of pesticides and compounds, applied in the direction of application, chemicals for biological control, biocides, etc., can solve the problem of reduced control effect
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[0221] Example 1: (Z)-tert-butyl(6-(((((1-(4-fluorobenzyl)-1H-tetrazol-5-yl)(phenyl)methylene)amino)oxy )Methyl)pyridin-2-yl) carbamate synthesis
[0222]
[0223] Step 1: Synthesis of 1-(azidomethyl)-4-fluorophenyl
[0224] Add 4-fluorobenzyl bromide (3.00g, 15.87mmol) and sodium azide (1.55g, 23.81mmol) into a 100mL round bottom flask, then add N,N-dimethylformamide (50mL) at 60℃ React for 8 hours. Add ethyl acetate (50 mL), wash with saturated brine (50 mL x 3), dry with anhydrous sodium sulfate, filter, and concentrate the filtrate under reduced pressure to obtain 2.21 g of a pale yellow oily liquid, yield: 92%.
[0225] Step 2: Synthesis of (Z)-(1-(4-fluorobenzyl)-1H-tetrazol-5-yl)(phenyl)methanone oxime
[0226] Add 1-(azidomethyl)-4-fluorophenyl (1.00g, 6.62mmol) and benzoyl nitrile (1.50g, 10.38mmol) into a 120mL sealed tube, and react at 120℃ for 8 hours to obtain the intermediate (1-(4-fluorobenzyl)-1H-tetrazol-5-yl)(phenyl)methanone, hydroxylamine hydrochloride (1.75g, 2...
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