Bonding material and bonded body using same
A technology of bonding materials and bonding bodies, applied in nanotechnology for materials and surface science, printed circuits connected with non-printed electrical components, electrical solid devices, etc., can solve difficult problems such as lead-free
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Embodiment 1
[0032] 180.0 g of pure water was placed in a 300 mL beaker, and 33.6 g of silver nitrate (manufactured by Toyo Kagaku Co., Ltd.) was added and dissolved to prepare a silver nitrate aqueous solution as a raw material liquid.
[0033] Moreover, 3322.0 g of pure water was put into a 5L beaker, and it heated up to 40 degreeC, blowing nitrogen gas into this pure water for 30 minutes, and removing dissolved oxygen. After adding 44.8 g of sorbic acid (manufactured by Wako Pure Chemical Industry Co., Ltd. (Wako Pure Chemical Industry Co., Ltd.)) as an organic compound (for coating silver particles) to this pure water, add 28% ammonia water ( Wako Pure Chemical Industries, Ltd.) 7.1 g.
[0034] While stirring the aqueous solution after adding the ammonia water, 14.91 g of aqueous hydrazine (manufactured by Otsuka Chemical Co., Ltd.) with a purity of 80% was added as a reducing agent after 5 minutes from the time point of adding the ammonia water (when the reaction started), Prepare an...
Embodiment 2
[0046] 180.0 g of pure water was placed in a 300 mL beaker, and 33.6 g of silver nitrate (manufactured by Toyo Kagaku Co., Ltd.) was added and dissolved to prepare a silver nitrate aqueous solution as a raw material liquid.
[0047] Moreover, 3322.0 g of pure water was put into a 5 L beaker, and it heated up to 60 degreeC, blowing nitrogen gas into this pure water for 30 minutes, and removing dissolved oxygen. After adding 44.8 g of sorbic acid (manufactured by Wako Pure Chemical Industry Co., Ltd. (Wako Pure Chemical Industry Co., Ltd.)) as an organic compound (for coating silver particles) to this pure water, add 28% ammonia water ( Wako Pure Chemical Industries, Ltd.) 7.1 g.
[0048] While stirring the aqueous solution after adding the ammonia water, 14.91 g of aqueous hydrazine (manufactured by Otsuka Chemical Co., Ltd.) with a purity of 80% was added as a reducing agent after 5 minutes from the time point of adding the ammonia water (when the reaction started), Prepare a...
Embodiment 3
[0055] Except that the same (average primary particle diameter of 60nm) silver particle (silver particle 2) and (average primary particle diameter of 300nm) silver particle (silver particle 3) and the amount of the first solvent (ODO) are respectively 46.5 g, 46.5g and 6.25g, by the same method as in Example 2, the first solvent (ODO) containing 46.5% by mass of silver particles 2, 46.5% by mass of silver particles 3, 6.25% by mass, 0.5% by mass The bonding material 3 is composed of the silver paste of the second solvent (IPTL-A) and 0.25% by mass of the dispersant (BEA).
[0056] For this bonding material 3, the viscosity, Ti value, Ag concentration, and particle size were obtained by the same method as in Example 1. As a result, the viscosity measured at 5 rpm at 25°C was 40 (Pa·s), and the Ti value was 5.4, and the Ag concentration was 92.1% by mass. In addition, the first scratch is 1 μm or less, the fourth scratch is 1 μm or less, and the average particle diameter D 50 ...
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