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Preparation method of an electro-responsive three-dimensional carbon nanotube-enriched conductive double network polymer hydrogel

A technology of carbon nanotubes and hydrogels, applied in the field of electrically driven smart hydrogels, which can solve problems such as limited applications and poor mechanical properties of polymer hydrogels, and achieve low product costs, good application prospects, and simple preparation methods Effect

Active Publication Date: 2022-03-18
NANJING UNIV OF SCI & TECH
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

However, the poor mechanical properties of current polymer hydrogels severely limit their applications.

Method used

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Examples

Experimental program
Comparison scheme
Effect test

preparation example Construction

[0018] The preparation method of the electro-responsive three-dimensional carbon nanotube enriched conductive double network polymer hydrogel of the present invention comprises the following steps in sequence:

[0019] The first step is to immerse the foamed nickel in the carbon nanotube water-based slurry, and vacuumize the carbon nanotube water-based slurry to fill the foamed nickel. This process is repeated 1 to 5 times, and then dried to obtain the carbon nanotube-loaded foamed nickel;

[0020] In the second step, sodium montmorillonite, carbon nanotube aqueous slurry, acrylic acid, 2-acrylamido-2-methylpropanesulfonic acid, N, N'-methylenebisacrylamide and initiator are added to Mix evenly in deionized water to obtain hydrogel precursor mother liquid A;

[0021] The third step is to immerse the carbon nanotube-loaded nickel foam obtained in the first step into the hydrogel precursor mother liquid A obtained in the second step, and vacuumize the hydrogel precursor mother l...

Embodiment 1

[0031] Nickel foam is immersed in the carbon nanotube water-based slurry (carbon nanotube content 2.3wt%, slurry solid content 3.6%, dispersant content 1.26wt%, the same below), vacuumizes the carbon nanotube water-based slurry to be full of foam nickel and then dried. This process was repeated 5 times to obtain carbon nanotube-loaded nickel foam. 1.5 grams of sodium montmorillonite, 26 grams of carbon nanotube aqueous slurry, 3.1 grams of 2-acrylamido-2-methylpropanesulfonic acid, 9.7 grams of acrylic acid, 0.23 grams of N,N'-methylenebispropene Amide and 0.2 g of potassium persulfate were added to 25 g of deionized water and stirred to obtain a hydrogel precursor mother liquid A. Then, immerse the carbon nanotube-loaded nickel foam into the hydrogel precursor mother liquid A, vacuumize the hydrogel precursor mother liquid A to fill the carbon nanotube-loaded nickel foam, and then heat to 60 ° C for 8 hours of polymerization reaction to obtain Poly(2-acrylamido-2-methylpropa...

Embodiment 2

[0033] Nickel foam is immersed in the carbon nanotube water-based slurry (carbon nanotube content 2.3wt%, slurry solid content 3.6%, dispersant content 1.26wt%, the same below), vacuumizes the carbon nanotube water-based slurry to be full of foam nickel and then dried. This process was repeated three times to obtain carbon nanotube-loaded nickel foam. 2.1 grams of sodium montmorillonite, 20 grams of carbon nanotube aqueous slurry, 6.1 grams of 2-acrylamido-2-methylpropanesulfonic acid, 5.7 grams of acrylic acid, 0.23 grams of N,N'-methylenebispropene Amide and 0.2 g of ammonium persulfate were added to 25 g of deionized water and stirred to obtain a hydrogel precursor mother liquid A. Then, immerse the carbon nanotube-loaded nickel foam into the hydrogel precursor mother liquid A, vacuumize the hydrogel precursor mother liquid A to fill the carbon nanotube-loaded nickel foam, and then heat to 80 ° C for 5 hours of polymerization reaction to obtain Poly(2-acrylamido-2-methylpr...

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Abstract

The invention discloses a method for preparing an electric-responsive three-dimensional carbon nanotube-enriched conductive double-network polymer hydrogel. The preparation method of the present invention comprises the following steps in sequence: the first step is to obtain carbon nanotube-loaded nickel foam by using the carbon nanotube aqueous slurry; the second step is to prepare the hydrogel precursor mother liquid A of the sodium-containing carbon nanotube aqueous slurry; The third step is to make the hydrogel precursor mother liquid A filled with carbon nanotube-loaded nickel foam and then heat and polymerize; the fourth step is to etch the foamed nickel in inorganic acid; the fifth step is to prepare the sodium-containing carbon nanotube aqueous slurry The hydrogel precursor mother liquid B; the sixth step, the hydrogel precursor mother liquid B is filled with the hydrogel that has etched the foamed nickel, and then heated and polymerized to obtain an electro-responsive three-dimensional carbon nanotube enriched conductive double network polymer Hydrogels. The monomers used in the present invention are acrylic acid and 2-acrylamido-2-methylpropanesulfonic acid. The preparation method of the invention is simple, the electric response speed of the polymer hydrogel is fast, and the invention can be used as an artificial muscle.

Description

technical field [0001] The invention relates to an intelligent hydrogel and a preparation method thereof, in particular to a preparation method of an electric-responsive three-dimensional carbon nanotube-enriched conductive double-network polymer hydrogel, and belongs to the field of electric-driven intelligent hydrogel. Background technique [0002] Smart materials can respond to external signal stimuli such as external temperature, light, electric field and magnetic field, and become a hot spot in the research of functional materials today, among which polymer hydrogel is the most common and important one. Polymer hydrogel is a kind of intelligent polymer with hydrophilic three-dimensional polymer network structure, which can absorb water and swell in water. These characteristics make hydrogel widely used in tissue engineering, artificial muscle, separation membrane, chemical valve , sensors and other cutting-edge fields. [0003] Electroresponsive hydrogels that respond ...

Claims

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Application Information

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Patent Type & Authority Patents(China)
IPC IPC(8): C08J9/40C08J9/26C08J3/075C08F220/06C08F220/58C08F222/38C08K3/04C08K3/34C08L33/02C08L33/24
CPCC08J9/405C08J9/26C08J3/075C08F220/58C08F220/06C08J2201/0442C08J2333/02C08J2333/24C08K3/041C08K2201/011C08K3/346
Inventor 应宗荣王奇谢杰李博
Owner NANJING UNIV OF SCI & TECH